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Detection of Picric Acid by Terpy-Based Metallo- Supramolecular Fluorescent Coordination Polymers in Aqueous Media

Chinese Journal of Chemistry 2017年第4期35卷 447-456页

作者： Zhongyu Ding Hongqing Li Wanqing Gao Yiquan Zhang Chunhua Liu Yuanyuan Zhu School of Chemistry and Chemical Engineering Hefei University of Technology and Anhui Key Laboratory of Advanced Functional Materials and Devices Hefei Anhui 230009 China Jiangsu Provincial Key Laboratory for Numerical Simulation of Large Scale Complex Systems (NSLSCS) School of Physical Science and Technology Nanjing Normal University Nanjing Jiangsu 210023 China

The synthesis of two linear terpy-based metallo-supramolecular fluorescent coordination polymers through 1 ： 1 complexation of Zn^2＋ and Cd^2＋ ions with ditopic terpyridine ligand was reported. The dispersibility of P1 and P2 was significantly improved in organic solvent and water through the introduction of hydrophilic oligo-ethyoxy side chain. Two polymers displayed yellow light emission both in solution and the solid state due to the intra-ligand charge transfer （ILCT） between the d^10 metal ions and the conjugated spacer unit. These coordination polymers were explored as fluorescent chemosensors for detecting picric acid in aqueous media, displaying high sensitivity and good selectivity. In addition, test strips were prepared from these polymers and exhibited the practical potential of detecting the NACs pollutants in the outdoor water for public safety and security.

关键词： coordination polymer fluorescent chemosensors nitroaromatic explosives picric acid aqueous media

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A New Analytical Solution for Tide-Induced Groundwater Fluctuations in An Unconfined Aquifer with A Sloping Beach

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China Ocean Engineering 2011年第3期25卷 479-494页

作者：孔俊宋志尧辛沛沈城吉 College of Harbor Coastal and Offshore Engineering Hohai University Key Laboratory of Virtual Geographic Environment under Ministry of Education and Jiangsu Key Laboratory for Numerical Simulation of Large-Scale Complex SystemNanjing Normal University National Centre for Groundwater Research and Training The University of Queensland

Deriving analytical solutions for tide-induced groundwater fluctuations in unconfined aquifers confronts two problems：（1） As the Boussinesq equation itself contains nonlinear terms, the ＂secular term＂ would be generated in derivation, thus making perturbation solution unable to be deduced to higher order; （2） for aquifers with sloping beaches, the perturbation parameter in existing analytical solution integrating the beach slope and hydrogeological property would be sometimes larger than 1. So the application of perturbation solutions is relatively limited. Furthermore, as the beach slope decreases, the error of analytical solution would gradually increase. Given that water table over-height would increase the aquifer thickness and speed up wave propagation, this paper integrates over-height into the perturbation parameter and adjusts boundary conditions to settle the problem of ＂secular term＂ and to derive a new high-order analytical solution for nonlinear Boussinesq equation in terms of sloping beaches. Results show that the new analytical solution is more reasonable, and the analytical accuracy is obviously improved in comparison with the existing analytical solution for a gentle slope. The new analytical solution provides a theoretical basis for analyzing the propagation characteristics （e.g., wave length and over-height variation） of tide-induced groundwater wave in unconfined aquifers, particularly those with sloping beaches.

关键词： tide groundwater analytical solution over-height perturbation method

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Comparison and Modification: TVD Schemes for Scalar Transport on An Unstructured Grid

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China Ocean Engineering 2016年第4期30卷 615-626页

作者：张卓宋志尧郭飞张东温永宁胡迪 Key Lab of Virtual Geographic Environment under Ministry of Education Nanjing Normal University Jiangsu Center for Collaborative Innovation in Geographical Information Resource Development and Application Nanjing Normal University Jiangsu Key Lab for Numerical Simulation of Large-Scale Complex System Nanjing Normal University

In most TVD schemes, the r-factors were proposed according to the cell-centered（CC） finite volume method（FVM） framework for the numerical approximation to the convective term. However, it is questionable whether those r-factors would be appropriate and effective for the vertex-centered（VC） FVM. In the paper, we collected five kinds of r-factor formulae and found out that only three of those, respectively by Bruner（1996）, Darwish and Moukalled（2003） and Cassuli and Zanolli（2005） can be formally extended to a context of the VC FVM. numerical tests indicate that the TVD schemes and r-factors, after being extended and introduced to a context of the VC FVM, maintained their similar characteristics as in a context of the CC FVM. However, when the gradient-based r-factors and the SUPERBEE scheme were applied simultaneously, non-physical oscillations near the sharp step would appear. In the transient case, the oscillations were weaker in a context of the VC FVM than those in a context of the CC FVM, while the effect was reversed in the steady case. To eliminate disadvantages in the gradient-based r-factor formula, a new modification method by limiting values on the virtual node, namely Фu in the paper, was validated by the tests to effectively dissipate spurious oscillations.

关键词： TVD scheme unstructured grid vertex-centered FVM flux limiter, r-factor

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Lattice thermal conductivity switching via structural phase transition in ferromagnetic VI_(3)

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Chinese Physics B 2023年第5期32卷 20-26页

作者：吴超刘晨晗 Laboratory of Solid State Microstructures Nanjing UniversityNanjing 210093China Micro-and Nano-scale Thermal Measurement and Thermal Management Laboratory School of Energy and Mechanical EngineeringNanjing Normal UniversityNanjing 210023China Jiangsu Key Laboratory for Numerical Simulation of Large-Scale Complex Systems Nanjing Normal UniversityNanjing 210023China Jiangsu Key Laboratory for Design and Manufacture of Micro-Nano Biomedical Instruments School of Mechanical EngineeringSoutheast UniversityNanjing 211100China

The realization of reversible thermal conductivity through ferromagnetic ordering can improve the heat management and energy efficiency in magnetic materials-based ***_(3),as a new layered ferromagnetic semiconductor,exhibits a structural phase transition from monoclinic(C2/m)to rhombohedral(R3^(-))phase as temperature decreases,making it a suitable platform to investigate thermal switching in magnetic phase transition *** work reveals that the thermal switching ratio of VI_(3)can reach 3.9 along the *** properties analysis indicates that the C2/m structure is stiffer than the R^(-)one,causing the larger phonon velocity in C2/m ***,due to the fewer phonon branches in C2/m phase,the number of phonon–phonon scattering channels in C2/m phase is smaller compared to that of R^(-)*** the larger phonon velocity and the longer phonon lifetime lead to larger lattice thermal conductivity in C2/m *** study uncovers the mechanical and thermal properties of VI_(3),which provides useful guides for designing magnetic materials-based devices such as thermal switch.

关键词： thermal switching ferromagnetic ordering phonons

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Effects of phonon bandgap on phonon-phonon scattering in ultrahigh thermal conductivityθ-phase TaN

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Chinese Physics B 2023年第4期32卷 543-548页

Phonon bandgap typically has a significant effect on phonon-phonon scattering *** this work,the effects of mass modified phonon bandgap inθ-phase Ta N are systemically investigated by the means of first-principles calculations with linearized Boltzmann transport *** detailed calculations,we find that phonon bandgap has a significant effect on three-phonon process while exhibits a much weaker effect on four-phonon *** reason for the ultrahigh thermal conductivity ofθ-phase Ta N is the long lifetime of phonons including both three-phonon and four-phonon processes,which originates from the weak phonon anharmonicity and large phonon bandgap-induced small phonon-phonon scattering phase *** work advances the understanding of phonon bandgap effects on phonon transport.

关键词： ultrahigh thermal conductivity phonon-phonon scattering phase space first-principles calculation phonon bandgap

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Resonance contributions fromχ_(c0)in charmless three-body hadronic B meson decays

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Chinese Physics C 2023年第4期47卷 148-154页

作者：张亚兰王超林毅肖振军 Faculty of Mathematics and Physics Huaiyin Institute of TechnologyHuaian 223200China Department of Physics and Institute of Theoretical Physics Nanjing Normal UniversityNanjing 210023China Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems Nanjing Normal UniversityNanjing 210023China

Within the framework of perturbative QCD factorization,we investigate the nonfactorizable contributions to the factorization-forbidden quasi-two-body decays B_((s))→h_((χ)_(c0))→hπ^(+)π^(-)(K^(+)K^(-))with h=π,*** compare our predicted branching ratios for the B_(()(s))→K_(χc0)→Kπ^(+)π-(K^(+)K^(-))decay with available experiment data as well as predictions by other theoretical *** branching ratios of these decays are consistent with data and other theoretical ***,in the Cabibbo-suppressed decays B_((s))→h_((χ)_(c0))→hπ^(+)π^(-)(K^(+)K^(-))with h=K^(0),π,the values of the branching ratios are of the order of 10^(-7)and 10^(-8).The ratio R_((χ)_(c0))between the decays B^(+)→π^(+)χ_(c0)→π^(+)π^(+)π^(-)and B^(+)→K^(+)χc0→K^(+)π^(+)π^(-)and the distribution of branching ratios for different decay modes in invariant mass are considered in this study.

关键词： three-body B meson decays resonance contributions perturbative QCD factorization approach

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The semileptonic decays of B/B_s meson in the perturbative QCD approach:a short review

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Chinese Science Bulletin 2014年第29期59卷 3787-3800页

作者： Zhen-Jun Xiao Ying-Ying Fan Wen-Fei Wang Shan Cheng Department of Physics and Institute of Theoretical Physics Nanjing Normal University Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems Nanjing Normal University Institute of High Energy Physics and Theoretical Physics Center for Science Facilities Chinese Academy of Sciences

In this short review,we present the current status about the theoretical and experimental studies for some important semileptonic decays of B=*** firstly gave a brief introduction for the experimental measurements for B=Bs!Peltl;l ml;m mT decays,the BaBar’s ReDT and ReD T anomaly,the P05deviation for B0!K 0ltl *** then made a careful discussion about the evaluations for the relevant form factors in the light-cone QCD sum rule,the heavy quark effective theory,and the perturbative QCD factorization *** using the form factors calculated in the perturbative(pQCD)approach,we then calculate and show the pQCD predictions for the decay rates of many semileptonic decays of B=*** also made careful phenomenological analysis for these pQCD predictions and found,in general,the following points:(a)For all the considered B=Bssemileptonic decays,the next-to-leading order pQCD predictions for their decay rates agree well with the data and those from other different theoretical methods;(b)For ReDT and ReD T,the pQCD predictions agree very well with the data,the BaBar’s anomaly of ReDe TT are therefore explained successfully in the standard model by employing the pQCD approach;and(c)We defined several new ratios Rl;s Dand Rl;s Ds,they may be more sensitive to the QCD dynamics which controls the B=Bs!eDe T;De T sT transitions than the old ratios,we therefore strongly suggest LHCb and the forthcoming Super-B experiments to measure these new ratios.

关键词：微扰QCD 衰变率 BS 介子光锥QCD求和规则实验测量评论 QCD因子化

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S-wave resonance contributions to B(s)^0→ηc(2S)π^+π^-in the perturbative QCD factorization approach

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Chinese Physics C 2017年第8期41卷 47-52页

作者： Ai-Jun Ma Ya Li Wen-Fei Wang Zhen-Jun Xiao Department of Physics and Institute of Theoretical Physics Nanjing Normal UniversityNanjing 210023China Institute of Theoretical Physics Shanxi UniversityTaiyuanShanxi 030006China Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems Nanjing Normal UniversityNanjing 210023China

By employing the perturbative QCD（PQCD） factorization approach, we study the quasi-two-body B（s）^0→ηc（2S）π^＋π^- decays, where the pion pair comes from the S-wave resonance f0（X）. The Breit-Wigner formula for the f0（500） and f0（1500） resonances and the Flatt′e model for the f0（980） resonance are adopted to parameterize the time-like scalar form factors in the two-pion distribution amplitudes. As a comparison, Bugg＇s model is also used for the wide f0（500） in this work. For decay rates, we found the following PQCD predictions：（a）-B（Bs^0 →ηc（2S）f0（X）[π^＋π^-]s）= 2.67-1.08^＋1.78 ×10^-5 when the contributions from f0（980） and f0（1500） are all taken into account;（b）B（B0→η-c（2S）f0（500）[π^＋π^-]s） = 1.40（-0.56）（＋0.92） ×10^-6 in the Breit-Wigner model and 1.53（-0.61）^（＋0.97） ×10^-6 in Bugg＇s model.

关键词： PQCD factorization approach two-pion distribution amplitudes quasi-two-body decay

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The Effect of Quantum Coins on the Spreading of Binary Disordered Quantum Walk

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Chinese Physics Letters 2015年第6期32卷 20-23页

作者：赵静胡亚运童培庆 Department of Physics and Institute of Theoretical Physics Nanjing Normal University Nanjing 210023 Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems Nanjing Normal University Nanjing 210023 Kavli Institute for Theoretical Physics China Chinese Academy of Sciences Beijing 100190

The dynamical and static disordered quantum walks were extensively studied recently. It is found that, for the dynamicM disorder case, the transport behavior of particles is diffusive, and for the static disorder ease the transport behavior is localized. In this work, we study the effect of quantum coins on the transport behaviors of the binary disordered quantum walks. We lind that once the coins satisfy certain conditions, the sub-ballistic spreading could be found in binary dynamical disorder quantum walks, and the sub-ballistic, diffusive and sub- diffusive spreadings could be found in binary static disorder quantum walks. We obtain the necessary conditions for those abnormal diffusive behaviors.

关键词： The Effect of Quantum Coins on the Spreading of Binary Disordered Quantum Walk

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Arbitrarily High-Order Energy-Preserving Schemes for the Camassa-Holm Equation Based on the Quadratic Auxiliary Variable Approach

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Advances in Applied Mathematics and Mechanics 2023年第5期15卷 1233-1255页

作者： Yuezheng Gong Qi Hong Chunwu Wang Yushun Wang School of Mathematics Nanjing University of Aeronautics and AstronauticsNanjingJiangsu 211106China Key Laboratory of Mathematical Modelling and High Performance Computing of Air Vehicles(NUAA) MIITNanjingJiangsu 211106China Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems School of Mathematical SciencesNanjing Normal UniversityNanjingJiangsu 210023China

In this paper,we present a quadratic auxiliary variable(QAV)technique to develop a novel class of arbitrarily high-order energy-preserving algorithms for the Camassa-Holm *** QAV approach is first utilized to transform the original equation into a reformulated QAV system with a consistent initial *** the reformulated QAV system is discretized by applying the Fourier pseudo-spectral method in space and the symplectic Runge-Kutta methods in time,which arrives at a class of fully discrete *** the consistent initial condition,they can be rewritten as a new fully discrete system by eliminating the introduced auxiliary variable,which is rigorously proved to be energy-preserving and *** numerical experiments are conducted to confirm the expected order of accuracy,conservative property and efficiency of the proposed *** presented numerical strategy makes it possible to directly apply a special class of Runge-Kutta methods to develop energy-preserving algorithms for a general conservative system with any polynomial energy.

关键词： Camassa-Holm equation quadratic auxiliary variable high-order energy-preserving schemes symplectic Runge-Kutta methods

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