Off-axis-rotating elliptical Gaussian beams(Oare GB)oblique incidence in strong nonlocal medium exhibit novel propagation *** analytical expressions of semi-axial beam widths,and center-of-mass trajectory equations fo...
详细信息
Off-axis-rotating elliptical Gaussian beams(Oare GB)oblique incidence in strong nonlocal medium exhibit novel propagation *** analytical expressions of semi-axial beam widths,and center-of-mass trajectory equations for transmitting off-axis-rotating elliptical Gaussian beams in strong nonlocal media are obtained using the ABCD transfer matrix *** study revealed that the trajectory of the mass's center in the cross-section can be controlled by changing the sizes of the Oare GB parameters c,d,ζ,and *** gradient force of the light field causes the spot region to form a spatial potential well in the media,and this spatial potential well can effectively capture *** particles captured by the light field can move along with the beam,realizing the effective manipulation of the particle *** laws may be applied to modulating the propagation path of light beams and optical tweezer technology.
Acoustic wave isolation and noise reduction are significant challenges in the fields of physics and various *** noise-control devices are often hampered by substantial size limitations,and their operational efficacy i...
详细信息
Acoustic wave isolation and noise reduction are significant challenges in the fields of physics and various *** noise-control devices are often hampered by substantial size limitations,and their operational efficacy is generally restricted to planar *** this study,we demonstrate perfect confinement of acoustic vortex waves using an acoustic metacage consisting of phase-gradient *** leveraging the parity-reversed diffraction rule of phase-gradient metasurfaces,the designed metacage exhibited remarkable capabilities for the perfect confinement of acoustic vortex waves,showing robust performance even in the presence of source *** findings present a promising strategy for developing precise and adaptable acoustic confinement technologies.
The Einstein-de Haas(EdH)effect,which establishes that changes in magnetization induce mechanical rotation,was experimentally demonstrated in 1915[1],independently of Richardson’s[2]earlier conceptual prediction rela...
详细信息
The Einstein-de Haas(EdH)effect,which establishes that changes in magnetization induce mechanical rotation,was experimentally demonstrated in 1915[1],independently of Richardson’s[2]earlier conceptual prediction related to this aspect.
We introduce a novel method for precise control of quantum dot (QD) charge states using a bipolar junction transistor (BJT). By adjusting the base-emitter and collector-base voltages, we can switch the QD between diff...
详细信息
The volcano plot is widely used to elucidate the activity trends among different catalysts,thereby effectively screening and guiding catalyst ***,the inherent linear scaling relationship(LSR)constrains the breakthroug...
详细信息
The volcano plot is widely used to elucidate the activity trends among different catalysts,thereby effectively screening and guiding catalyst ***,the inherent linear scaling relationship(LSR)constrains the breakthrough in the activity of catalysts,and the understanding of the activity limit in volcano plot is still *** this work,by employing first-principles calculations and microkinetic modeling,we proposed coordination engineering(CE)and dual-site(DS)strategies to surpass the Sabatier’s limitation of WS_(2)-supported TM(TM@WS_(2))single-atom catalysts(SACs)for electrocatalytic nitrogen reduction reaction(eNRR).We found that the LSR betweenΔG(^(*)N_(2)→^(*)N_(2)H)andΔG(^(*)NH_(2)→^(*)NH_(3))was optimized to be closer to the ideal space of eNRR activity after modulating TM@WS_(2)SACs by these two design *** combining the reaction selectivity trend plot,we picked out N-Os@WS_(2),C-Ir@WS_(2),Fe_(2)@WS_(2),and Ru_(2)@WS_(2)as optimal eNRR catalysts with low limiting potential(UL),and N-Os@WS_(2)SAC(UL:-0.28 V)outperforms the best eNRR catalyst among TM@WS_(2)*** constructing explicit solvent models,we conducted a detailed study on the reaction kinetics of proton transfer over these four *** propose that the activity enhancement in TM@WS_(2)SACs for eNRR can be attributed to the ligand effect and geometric effect brought about by CE and DS strategies,improving the donation-backdonation process of electron transfer between N_(2)and the active *** designed catalyst has certain resistance to demetallization and agglomeration under simulated solvent *** work provides a feasible design strategy for the activity enhancement of SACs and brings a new perspective to deeply understanding the volcano plot in heterogeneous catalysis.
The discharge and plasma characteristics of Ag magnetron sputtering discharge operated near the electron series resonance(ESR)oscillation,which was excited using the driving frequency of 27.12 MHz,was *** imaginary pa...
详细信息
The discharge and plasma characteristics of Ag magnetron sputtering discharge operated near the electron series resonance(ESR)oscillation,which was excited using the driving frequency of 27.12 MHz,was *** imaginary part of impedance was found to undergo a transition from capacitive to inductive on varying radio-frequency(RF)power,and the conditions for the ESR excitation were *** current–voltage(I–V)characteristic of discharge showed that the lower discharge voltage with higher current was an important feature of RF magnetron sputtering operated near the ESR oscillation,which was caused by the small impedance Z originated from the mutual compensation between the sheath capacitive reactance and the plasma inductive *** higher electron temperature,ion flux density and ion energy as well as the moderate electron density were *** interaction of higher energy ions on substrate surface improved the crystallographic quality of Ag ***,the 27.12 MHz magnetron sputtering operated near the ESR oscillation has better deposition characteristics than that of commercial 13.56 MHz RF magnetron sputtering.
A control method of electromagnetic feedback is proposed for adjusting frequency response characteristics of fiber optic accelerometers, which could expand the flat working bandwidth and enhance performance consistenc...
详细信息
High-energy-density(HED)fuel(*** used JP-10 and RJ-4),featuring compact 3D polycyclic structure with high strain,is of critical importance for volume-limited military aircraft,since their high density and combustion h...
详细信息
High-energy-density(HED)fuel(*** used JP-10 and RJ-4),featuring compact 3D polycyclic structure with high strain,is of critical importance for volume-limited military aircraft,since their high density and combustion heat can provide more propulsion *** reduce the reliance on petroleum source,it is highly desirable to develop renewable alternatives for the production of strained polycyclic HED fuel,but which remains a big challenge because of the inaccessibility caused by the high strain,We herein demonstrate a three-step catalytic route towards highly strained C_(17)and C_(18)spirofuel with biomass *** process includes catalytic aldol condensation of renewable cyclohexanone/cyclopentanone with benzaldehyde,catalytic spiro Diels-Alder(D-A)reaction of aldol adduct with isoprene,and catalytic *** key spiro D-A reaction is enabled by the catalysis of heterogeneous Lewis acidic ionic *** chloroaluminate IL,formed by benign urea and AICl3,exhibits good catalytic performance and reusability for this *** eventual hydrodeoxygenation(HDO)over Pd/C and H-Y produces strained tricyclic spirofuel with density>0.93 g/mL,combustion heat>41 MJ/L and freezing point<-40℃,which are better than the properties of tactical fuel ***,it is anticipated that the as-prepared renewable fuels have the potential to replace traditional petroleum-derived HED fuels.
The recent transport measurements of La_(3)Ni_(2)O_(7)uncovered a“right-triangle”shape of the superconducting dome in the pressure-temperature(P-T)phase *** by this,we perform theoretical first-principles studies of...
详细信息
The recent transport measurements of La_(3)Ni_(2)O_(7)uncovered a“right-triangle”shape of the superconducting dome in the pressure-temperature(P-T)phase *** by this,we perform theoretical first-principles studies of La_(3)Ni_(2)O_(7)with the pressure ranging from 0 to 100 ***,we reveal a pressure dependence of the Ni-d_(z^(2))electron density at the Fermi energy(n_(z)^(E_(F)))that highly coincides with such *** this basis,we further explore the electronic structure under uniaxial *** tracking the stress response of n_(z)^(E_(F)),we propose that superconductivity can be achieved by applying only ~2GPa of compression along the c *** idea is further exemplified from the perspectives of lattice distortion,band structure,Fermi surface and superconducting phase *** also discuss the possible charge modulation under the stress and provide an insight into the relation between nz E Fand the superconducting T_(c)in La_(3)Ni_(2)O_(7)*** study provides new routes to the search of high-T_(c)superconductors in future experiments.
Shaping the waveform of attosecond pulses is crucial for controlling electron dynamics and is typically achieved using a high-order harmonic generation (HHG) spectrum containing a minimum. Here, we propose a novel met...
详细信息
暂无评论