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Ultrarobust, Stretchable, and Highly Elastic Supramolecular Elastomer with Hydrogen-Bond Interactions via sp2Hybridized Boron-Urethane Bonds

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Angewandte Chemie 2025年

作者： Yuehan Qian Fuhao Dong Shanshan Wang Yunmeng Jiang Xu Xu He Liu College of Chemical Engineering Jiangsu Provincial Key Lab for the Chemistry and Utilization of Agro-Forest Biomass Jiangsu Key Lab of Biomass-Based Green Fuels and Chemicals Co-Innovation Center of Efficient Processing and Utilization of Forest Resources International Innovation Center for Forest Chemicals and Materials Nanjing Forestry University Nanjing 210037 China Institute of Chemical Industry of Forestry Products Key Laboratory of Biomass Energy and Material National Engineering Laboratory for Biomass Chemical Utilization Key and Open Laboratory of Forest Chemical Engineering State Forestry Administration Chinese Academy of Forestry Nanjing 210042 China

Elastomers are omnipresent in everyday life and industry, yet the development of an elastomer with both superb stress and toughness presents a prodigious challenge. In this report, a high-strength, tough, and high-elastic elastomer derived from sp 2 hybrid orbitals of phenylboronic acid was designed. The spatial conformation of network becomes significantly more compact due to the sp 2 hybridization of boron. This enhances supramolecular hydrogen bonding interactions, resulting in a marked improvement in the material's mechanical properties. Notably, the hydrogen bonding energy in the polyurethane chain segments enhanced by 37%. The robust hydrogen bonding imparts the elastomer with super high true stress (1.30 GPa), superior toughness (442.2 MJ·m −3 ), and super puncture resistance strength of 167.8·N·mm −1 . The material exhibited excellent fatigue resistance during continuous tensile cycles, while the irreversible deformation disappeared after standing at room temperature. Moreover, the elastomer bespeaks extraordinary elastic restorability, swiftly reverting to its primitive length after being extended to 16 times. This work provides a strategy that the mechanical properties of materials can be enhanced and toughened by utilizing spatial conformational changes in intermolecular interactions.

关键词： Elastomer High mechanical properties Hydrogen bond sp2 Hybrid orbitals Spatial conformation

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A new method for semi-automatic image annotation

A new method for semi-automatic image annotation

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2007 8th International Conference on Electronic Measurement and Instruments, ICEMI

作者： Xuelong, Hu Yuhui, Zhang Li, Yang School of Information Engineering Yangzhou University Yangzhou 225009 China Jiangsu Province Key Lab. of Image Processing and Communication Nanjing University of Post and Telecommunications Nanjing 215006 China Jiangsu Province Key Lab. of Computer Information Processing Technology Suzhou University Suzhou 215006 China

ISBN: (纸本)1424411351

Semantic-based image retrieval bridges the gap between visual features and human understanding of image in the field of image retrieval. image annotation is one important technology of image retrieval based on the semantic. This paper proposed one method to realize semi-automatic image annotation with the tool Support Vector Machine (SVM). The image collection was divided into two parts, one for manual annotation and the other for testing. After being classified by SVM, the output was changed into a probability, and K-NN algorithm was applied to get the keywords for unlabeled images. The experiments show that the approach is feasible. © 2007 IEEE.

关键词： Support vector machines

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Stereo matching using aggregated likelihood and multi-scale prior

Stereo matching using aggregated likelihood and multi-scale ...

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International Conference on Audio, Language and image processing, ICALIP

作者： Liang Wang Tianliang Liu Xiuchang Zhu Jiangsu Provincial Key Laboratory of Image Processing and Image Communication Nanjing University of Posts and Telecommunications Nanjing China

ISBN: (纸本)9781467301732

This paper proposes a novel global stereo matching method using aggregated likelihoods and multi-scale priors. The likelihoods of dense stereo correspondences as data term can be robustly expressed by aggregated matching costs based on Weber feature descriptors in an asymmetrical linear filtering model. The multi-scale priors on disparity surface are designed to capture scene smooth term from larger neighborhood besides 4-connected neighborhood. The presented stereo approach being relatively simple does not rely on image segmentation and any scene semantic analysis. Experiments demonstrate that the proposed stereo matching algorithm can produce the dense smooth disparity results comparable to those of excellent stereo matching techniques.

关键词： Stereo vision Visualization Robustness image segmentation Algorithm design and analysis Computer vision image color analysis

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image retrieval based on character-matching technology

Image retrieval based on character-matching technology

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5th International Conference on Information Assurance and Security, IAS 2009

作者： Shan, Zhao Jing, Liu School of Computer Science and Technology Henan Polytechnic University Jiaozuo 454003 China Jiangsu Province Key Lab. on Image Processing and Image Communication Nanjing University of Posts and Communication Nanjing 210003 China

ISBN: (纸本)9780769537443

In order to introduce effective text-retrieval technologies into content-based image retrieval, a novel method based on string-matching technology was presented incorporating the different sensitivity along variant directions of human visual system. The image is firstly divided into non-overlapped blocks and sub-feature is extracted according to the human visual feature. Then, a novel descriptor is defined. Based on which, the sub-features is mapping into characters and the image into the text. Finally, the technology of the character string matching is adopted as the similarity measurement. Meantime, the situation information of character is considered, an adjusted method is proposed. Experimental results show that the proposed method has sound and robust retrieval performance. © 2009 IEEE.

关键词： Content based retrieval

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Robust piecewise planar stereo with modified segmentation cues in urban scenes

Robust piecewise planar stereo with modified segmentation cu...

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International Conference on Multimedia Technology

作者： Zengtao Jiao Tianliang Liu Xiuchang Zhu Jiangsu Provincial Key Laboratory of Image Processing and Image Communication Nanjing University of Posts and Telecommunications Nanjing China

This paper proposes a robust piecewise planar multi view stereo (MVS) approach specifically designed for urban scenes. These architectural scenes are problematic for traditional computer vision methods. In our work, we focus on exploiting some useful constraints of artificial structures such as piecewise coplanarity and boundaries of superpixels. Firstly, we reconstruct quasi-dense 3D point clouds of urban scenes using patches-based MVS (PMVS) method. Secondly, a set of 3D candidate planes are generated by the obtained point clouds without any assumption on the normals of planes, unlike famous Manhattan-world assumption. Then, we segment multi-view images with watershed algorithm and modify the contours of superpixels by the classical Douglas-Peucker approximation algorithm to fit the contours to the boundaries of objects in urban scenes as much as possible. Finally, we use the candidate planes as labels and superpixels as nodes to formulate our Markov Random Field (MRF) optimization problem, then a piecewise planar depth map for each view is recovered by solving the optimization problem using graph-cuts. Experiments show that our method outperforms previous approaches in terms of accuracy.

关键词： Three dimensional displays image segmentation Computer vision Stereo vision Approximation methods image reconstruction Optimization

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Classification rules mining based on SOFM networks

Classification rules mining based on SOFM networks

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MIPPR 2005: Geospatial Information, Data Mining, and Applications

作者： Yao, Min Jiang, Zhiwei Shen, Bin College of Computer Zhejiang University Hangzhou 310027 China Provincial Key Lab. for Computer Information Processing Technology in Jiangsu Suzhou University Suzhou 215006 China

Self-organization feature mapping (SOFM) networks have strong ability for self-learning and self-adaptive. According to the characteristics of human thought, this paper constructed a kind of combined criterion, which may be used to guide the learning of self-organization feature mapping network. Then this paper presents subsection algorithm, amalgamation algorithm and dynamical adaptive algorithm for SOFM networks so as to solve a kind of problems of classification rule mining. Finally, a practical example shows its flexibility and practicability.

关键词： Self organizing maps

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Exploiting constituent dependencies for tree kernel-based semantic relation extraction

Exploiting constituent dependencies for tree kernel-based se...

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22nd International Conference on Computational Linguistics, Coling 2008

作者： Qian, Longhua Zhou, Guodong Kong, Fang Zhu, Qiaoming Qian, Peide Jiangsu Provincial Key Lab. for Computer Information Processing Technology School of Computer Science and Technology Soochow University 1 Shizi Street Suzhou 215006 China

ISBN: (纸本)9781905593446

This paper proposes a new approach to dynamically determine the tree span for tree kernel-based semantic relation extraction. It exploits constituent dependencies to keep the nodes and their head children along the path connecting the two entities, while removing the noisy information from the syntactic parse tree, eventually leading to a dynamic syntactic parse tree. This paper also explores entity features and their combined features in a unified parse and semantic tree, which integrates both structured syntactic parse information and entity-related semantic information. Evaluation on the ACE RDC 2004 corpus shows that our dynamic syntactic parse tree outperforms all previous tree spans, and the composite kernel combining this tree kernel with a linear state-of-the-art feature-based kernel, achieves the so far best performance. © 2008. Licensed under the Creative Commons.

关键词： Semantics

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Research of event pronoun resolution

Research of event pronoun resolution

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2011 International Conference on Asian Language processing, IALP 2011

作者： Zhang, Ning Kong, Fang Li, Peifeng JiangSu Provincial Key Lab. for Computer Information Processing Technology Soochow University Suzhou China School of Computer Science and Technology Soochow University Suzhou China

ISBN: (纸本)9780769545547

Event anaphora resolution plays an important role in discourse analysis. In comparison with general noun phrases, pronouns carry little information of themselves, resolving the event pronouns is a more difficult task. This paper proposes a machine learning-based framework for event pronoun resolution. All kinds of features, including both flat and structural features, are explored for event pronoun resolution. Experiments on OntoNotes corpus show that both flat and structural features are very effective for this task. © 2011 IEEE.

关键词： Learning systems

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Research of noun phrase coreference resolution

Research of noun phrase coreference resolution

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2011 International Conference on Asian Language processing, IALP 2011

作者： Gao, Junwei Kong, Fang Li, Peifeng Zhu, Qiaoming JiangSu Provincial Key Lab. for Computer Information Processing Technology Soochow University Suzhou China School of Computer Science and Technology Soochow University Suzhou China

ISBN: (纸本)9780769545547

Coreference resolution is an important subtask in natural language processing systems. The process of it is to find whether two expressions in natural language refer to the same entity in the world. Machine learning approaches to this problem have been reasonably successful, operating primarily by recasting the problem as a classification task. A great deal of research has been done on this task in English, using approaches ranging from those based on linguistics to those based on machine learning. In Chinese, however, much less work has been done in this area. The lack of public resources is a big problem in the research of Chinese NLP. The other problem is that some features are more difficult to get than those features of English. In this paper, We present a noun phrase coreference system that refers to the work of Soon et al. (2001). We also explore the impact of various features on our system's performance. Experiments on the Chinese portion of OntoNotes 3.0 show that the platform achieves a good performance. © 2011 IEEE.

关键词： Natural language processing systems

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Research on cross-document coreference of Chinese person name

Research on cross-document coreference of Chinese person nam...

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2011 International Conference on Asian Language processing, IALP 2011

作者： Ni, Ji Kong, Fang Li, Peifeng Zhu, Qiaoming JiangSu Provincial Key Lab. for Computer Information Processing Technology Soochow University Suzhou China School of Computer Science and Technology Soochow University Suzhou China

ISBN: (纸本)9780769545547

In reality, different persons often have the same person name. The Person Cross Document Co-reference Resolution is a task, which requires that all and only the textual mentions of an entity of type Person be individuated in a collection of text documents. In this paper, we implement a Chinese Person Name Cross Document Co-reference Resolution System. First, we utilize name identification module to recognize all person names of the texts, and then classify the document collection of same person name by rules preliminarily, and at last, we compute similarities of each classification based on VSM, according to the prior similarities, the system get the final classification results. We test the system on 30 usual Chinese names of the corpus provided by CLP, and average F measure is 85.9%. © 2011 IEEE.

关键词： Information retrieval systems

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