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CC@BCN@PANI core-shell nanoarrays as ultra-high cycle stability cathode for Zn-ion hybrid supercapacitors

Frontiers in Energy 2023年第4期17卷 555-566页

作者： Shixian XIONG Hongcheng KE Lei CAO Yu WANG Qian ZHU Liqin ZHONG Lanlan FAN Feng GU Nanchang Key Laboratory for Advanced Manufacturing of Electronic Information Materials and Devices/Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems International Institute for InnovationJiangxi University of Science and TechnologyNanchang330013China

Exploring cathode materials that combine excellent cycling stability and high energy density poses a challenge to aqueous Zn-ion hybrid supercapacitors(ZHSCs).Herein,polyaniline(PANI)coated boron-carbon-nitrogen(BCN)nanoarray on carbon cloth surface is prepared as advanced cathode materials via simple high-temperature calcination and electrochemical deposition *** of the excellent specific capacity and conductivity of PANI,the CC@BCN@PANI core-shell nanoarrays cathode shows an excellent ion storage ***,the 3D nanoarray structure can provide enough space for the volume expansion and contraction of PANI in the charging/discharging cycles,which effectively avoids the collapse of the microstructure and greatly improves the electrochemical stability of ***,the CC@BCN@PANI-based ZHSCs exhibit superior electrochemical performances showing a specific capacity of 145.8 mAh/g,a high energy density of 116.78 Wh/kg,an excellent power density of 12 kW/kg,and a capacity retention rate of 86.2%after 8000 charge/discharge cycles at a current density of 2 A/*** addition,the flexible ZHSCs(FZHSCs)also show a capacity retention rate of 87.7%at the current density of 2 A/g after 450 cycles.

关键词： CC@BCN@PANI cathode Zn-ion hybrid supercapacitor core-shell nanoarrays high energy density ultra-high cycle stability

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A novel method for modeling the phase change of iron ore particles in the cohesive zone of a blast furnace

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Particuology 2024年第3期86卷 252-261页

作者： Dianyu E Yingming Wen Jiayun Dan Youyuan Jiang Guangchao Wei Jiaxin Cui Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science and TechnologyNanchang330013China International Institute for Innovation Jiangxi University of Science and TechnologyNanchang330013China Ironmaking Plant Xiangtan Iron and Steel Corporation of Hunan HualingXiangtan411101China Schoolof Transportation and Vehicle Enginering Shandong University of TechnologyZibo255000China

Cohesive zone plays a vital role in the stable operation of a blast furnace(BF),yet the complex phase change process of iron ore particles in this zone is still not well *** this study,a novel one-dimensional(1D)unsteady phase change model was developed to elucidate the heat transfer and melting mechanisms of iron ore *** model validation,the effects of several key operating parameters(e.g.,particle diameter,gas velocity,initial temperature)on the phase change behavior of iron ore particles were analyzed,and the joint effect of multiple parameters was *** results show that larger-sized iron ore particles possess lower specific surface areas,which in turn reduces their convective heat absorption ***,the distance from the solid-liquid phase interface to the particle surface increases,thereby slowing down the movement of the phase interface and pro-longing the melting duration of the *** the gas velocity and the initial temperature does not have a significant impact on reducing the duration of the complete melting *** the specified conditions,it is observed that increasing the gas velocity by 3-fold and 9-fold results in a reduction of the melting duration by 2.4%and 8.3%,*** the initial temperature of iron ore particles results in a decrease in the core-to-surface temperature difference,a slower heating rate,and a shorter duration to achieve *** the factors affecting the melting process,the particle diameter is found to be the most significant in terms of the liquid phase precipitation,mushy zone thickness,and core-to-surface temperature difference of iron ore particles.

关键词： Blast furnace Iron ore melting Cohesive zone Heat transfer Phase change

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Numerical study of effects of hydrogen addition on methane combustion behaviors

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Journal of Iron and Steel Research International 2023年第11期30卷 2173-2185页

作者： Dian-yu E Ling-yi Weng Guang-wu Tang Jing Li Guang-chao Wei Jia-xin Cui Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science and TechnologyNanchang330013JiangxiChina International Institute for Innovation Jiangxi University of Science and TechnologyNanchang330013JiangxiChina Shenzhen Smoore Technology Limited Shenzhen518102GuangdongChina ARC Research Hub for Computational Particle Technology Department of Chemical and Biological EngineeringMonash UniversityClaytonVIC3800Australia School of Transportation and Vehicle Engineering Shandong University of TechnologyZibo255000ShandongChina

The methane combustion with hydrogen addition can effectively reduce carbon emissions in the iron and steel making industry,while the combustion mechanism is still poorly *** oxy-fuel combustion of methane with hydrogen addition in a 0.8 MW oxy-natural gas combustion experimental furnace was numerically studied to investigate six different combustion *** results show that the 28-step chemical reaction mechanism is the optimal recommendation for the simulation balancing the numerical accuracy and computational *** the hydrogen enrichment increases in fuel,the highest flame temperature ***,the chemical reaction accelerates with enlarging the peak of the highest flame temperature and intermediate OH *** the hydrogen enrichment reaches 75 vol.%,the flame front is the farthest,and the flame high-temperature zone occupies the largest proportion corresponding to the most vigorous chemical reactions in the same oxygen supply.

关键词： Oxy-fuel combustion Hydrogen Combustion mechanism Flame temperature simulation Modeling

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Discrete Particle simulation of Gas-Solid Flow in Air-Blowing Seed Metering Device

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Computer Modeling in Engineering & Sciences 2021年第6期127卷 1119-1132页

作者： Zhengquan Li Pei Zhang Yongchang Sun Chenglin Zheng Liang Xu Dianyu E Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science&TechnologyGanzhou341000China Energy Materials Computing Center Jiangxi University of Science&TechnologyNanchang330013China

In this paper,the gas and seed flow characters in the air-blowing seed metering device are investigated by using the coupled computational fluid dynamics and discrete element method(CFD-DEM)in three dimensions(3D).The method of establishing boundary model based on the computer-aided design(CAD)drawing,has been used to build the boundary model of seed metering *** 3D laser scanning technique and multi-element method are adopted to establish the particle *** a combined numerical and experimental effort,using 3D CFD-DEM software,which is based on the in-house codes,the mechanisms governing the gas and solid dynamic behaviors in the seed metering device have been *** gas velocity field and the effect of different rotational speeds and air pressures on the seeding performance and particle velocity have been studied,similar agreements between numerical and experimental results are *** reveals that the 3D CFD-DEM model established is able to predict the performance of the air-blowing seed metering *** can be used to design and optimize the air-blowing seed metering device and other similar agriculture devices.

关键词： Seed metering device CFD-DEM CAD simulation gas-solid flow

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Particle shape effect on hydrodynamics and heat transfer in spouted bed:A CFD-DEM study

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Particuology 2022年第10期20卷 10-21页

作者： Dianyu E Peng Zhou Suya Guo Jia Zeng Jiaxin Cui Youyuan Jiang Yuanxiang Lu Zeyi Jiang Zhengquan Li Shibo Kuang Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science and TechnologyGanzhou 341000China Ironmaking Plant Xiangtan Iron and Steel Corporation of Hunan HualingXiangtan 411101China School of Energy and Environmental Engineering University of Science and Technology BeijingBeijing 100083China ARC Research Hub for Computational Particle Technology Department of Chemical EngineeringMonash UniversityClaytonVIC 3800Australia

Spouted bed has drawn much attention due to its good heat and mass transfer efficiency in many chemical *** the flow patterns and heat and mass transfer inside a spouted bed can help optimize the spouting ***,in this study,the effects of particle shape on the hydrodynamics and heat transfer in a spouted bed are *** is done by using a validated computational fluid dynamics-discrete element method(CFD-DEM)model,considering volume-equivalent spheres and oblate and prolate *** results are analysed in detail in terms of the flow pattern,microstruc-ture,and heat transfer *** numerical results show that the prolate spheroids(Ar=2.4)form the largest bubble from the beginning of the spouting process and rise the highest because the fluid drag forces can overcome the interlocking and particle-particle frictional *** with spherical particles,ellipsoidal spheroids have better mobility because of the stronger rotational kinetic energy resulting from the rough surfaces and nonuniform *** addition,the oblate spheroid system exhibits better heat transfer performance benefiting from the larger surface area,while prolate spheroids have poor heat transfer efficiency because of their orientation *** findings can serve as a reference for optimizing the design and operation of complex spouted beds.

关键词： Spouted bed Gas-solid flow Particle shape CFD-DEM Heat transfer

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Cc@Bcn@Pani Core-Shell Nanoarrays as Ultra-High Cycle Stability Cathode for Zn-Ion Hybrid Supercapacitors

SSRN

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SSRN 2023年

作者： Xiong, Shixian Ke, Hongcheng Cao, Lei Wang, Yu Zhu, Qian Zhong, Liqin Fan, Lanlan Gu, Feng Nanchang Key Laboratory for Advanced Manufacturing of Electronic Information Materials and Devices Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems International Institute for Innovation Jiangxi University of Science and Technology Nanchang330013 China

Exploring cathode materials that combine excellent cycling stability and high energy density remains challenging for aqueous zinc ion hybrid supercapacitors (ZHSCs). Herein, polyaniline (PANI) coated BCN nanoarray on carbon cloth surface is prepared as advanced cathode materials via simple high-temperature calcination and electrochemical deposition methods. Due to the high specific capacity and conductivity of PANI, the CC@BCN@PANI core-shell nanoarrays cathode shows excellent ion storage capability. Furthermore, the 3D nanoarray structure can provide enough space for the volume expansion and contraction of PANI during the charging and discharging process, which effectively avoids the collapse of the microstructure and greatly improves the electrochemical stability of PANI. Therefore, the CC@BCN@PANI based ZHSCs exhibit the superior electrochemical performances with a high capacity of 145.8 mAh g-1 (0.5 A g-1), a high energy and power density of 116.78 Wh kg-1 and 12 W kg-1, and a high-capacity retention rate of 86.2% at 2 A g-1 after 8000 cycles. In addition, the flexible Zn-ion hybrid supercapacitors (FZHSCs) are also investigated, and show a high capacity of 160 mAh g-1 (0.1 A g-1), and a capacity retention rate of 87.7% at 2 A g-1 after 450 cycles. © 2023, The Authors. All rights reserved.

关键词： Cathodes

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Improved Ductility by Reducing Powder Size in Laser Powder Bed Fusion of AlSi10Mg

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Additive Manufacturing Frontiers 2024年第1期3卷 160-172页

作者： Fuzhong Chu Haopeng Shen Jianwen Li Juan Hou Kai Zhang Zongyan Zhou Yuman Zhu Xinhua Wu Aijun Huang ARC Research Hub for Computational Particle Technology Department of Chemical and Biological EngineeringMonash UniversityClaytonVIC 3800Australia Monash Centre for Additive Manufacturing Monash UniversityNotting HillVIC 3168Australia Department of Materials Science and Engineering Monash UniversityClaytonVIC 3800Australia School of Materials and Chemistry University of Shanghai for Science and TechnologyShanghai200093China Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science and TechnologyNanchang330013China

Strict control of powder properties,especially particle size distribution(PSD),is critical in the laser powder bed fusion(LPBF)process to ensure the quality of the fabricated *** work shows that reducing the powder size could improve the ductility of LPBF fabricated *** tensile elongation increased from 4.1%to 8.8%when AlSi10Mg powder sizes(D50 value)decreased from 76μm to 16μm in the as-fabricated *** results showed that fine powder size stimulates epitaxial grain growth due to excessive *** presence of epitaxial columnar grains makes the crack path across inner melt pools more frequent and travels from the coarse melt pool zones to the fine melt pool *** work suggests that powder size is a crucial factor to be considered in maintaining repeatable mechanical properties in LPBF processes,particularly when ductility and ductility-dominated properties are critical.

关键词： Particle size distribution Laser powder bed fusion Ductility Epitaxial columnar grain

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Lightweight and Covalent-Crosslinked Polybenzoxazine Aerogels for Fire Resistance and Thermal Insulation

SSRN

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SSRN 2024年

作者： Li, Liangjun Zhou, Jinlong Xiao, Yunyun Zeyu, Li Liu, Saihui Zhang, Sizhao Feng, Jian Science and Technology on Advanced Ceramic Fibers and Composites Laboratory College of Aerospace Science and Technology National University of Defense Technology Changsha410073 China International Institute for Innovation Jiangxi University of Science and Technology Jiangxi Nanchang330013 China Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi Nanchang330013 China

The rapid advancement of modern industry and aerospace has imposed demands on thermal insulators to possess not only efficient isolation but also multifunctionality. Polybenzoxazine (PBz) aerogels with several advantages have garnered considerable research interests in recent years. Nevertheless, PBz aerogels acquired from ambient pressure drying still confront the challenge of exhibiting relatively high densities and thermal conductivities. Herein, to enrich the category and provide ideas for overcoming the above plight, hexamethylene diisocyanate (HDI) was chosen as an additive to achieve the chemical modification of the PBz aerogels. The chemical structure characterization shown that a successful reaction was occurred between the isocyanates and the hydroxyl groups, forming a urethane-bridged structure between two PBz molecular chains. In this paper, the effect of introducing HDI on the physical and thermal insulation properties of the aerogels was investigated. The HDI-modified PBz (PBz-HDI) aerogels demonstrated lower densities (0.237–0.256 g·cm−3) and thermal conductivities (0.0354−0.0370 W·m−1·K−1) in comparison with the pristine aerogel. In addition, despite an observed reduction in the residual char yields in the PBz-HDI groups, the introduction of HDI has been demonstrated to not impact their superior intrinsic flame retardancy. Given such commendable properties, PBz-HDI aerogel is expected to be a promising candidate for thermal insulation and fire resistance applications in various domains. © 2024, The Authors. All rights reserved.

关键词： Thermal insulation

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Boric Acid-Regulated Gelation and Ethanol-Assisted Preparation within Polybenzoxazine Aerogels Toward Excellent Flame Resistance, Alterable Wettability, and Effective Thermal Insulation

SSRN

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SSRN 2023年

作者： Zhou, Jinlong Xiao, Yunyun Liu, Saihui Li, Zeyu Liu, Xinyi Zhang, Sizhao Li, Zhengquan International Institute for Innovation Jiangxi University of Science and Technology Jiangxi Nanchang330013 China Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi Nanchang330013 China School of Energy and Mechanics Jiangxi University of Science and Technology Jiangxi Nanchang330013 China

Polybenzoxazine aerogels have gained widespread attention in recent years, but the prevalent use of hazardous solvents in the preparation process has severely impeded their further development and promotion for practical applications. Herein, using ethanol as a solvent, a strategy of boric acid-induced microstructure regulation is proposed to construct boron-doped polybenzoxazine (BPBz) aerogels, which provides a feasible approach to overcome the above situation. The introduction of boric acid enhances the backbone strength by forming intermolecular bridging structures between PBz chains and allows the use of ambient pressure drying. The resulting BPBz aerogel demonstrates high stiffness (specific modulus up to 266.02 kN·m·kg−1), low bulk density (0.203 g·cm−3), and low thermal conductivity (0.043 W·m−1·K−1), exhibiting excellent fire resistance when exposed to a 1200 °C flame (the self-extinguishing interval less than 1 s). More interestingly, the aerogel demonstrates intrinsic and tunable wettability that correlates with the morphology. Combining the environmentally friendly preparation strategy and these advantages, BPBz aerogels hold promise for thermal management and fire protection applications in energy-saving construction and other harsh conditions. © 2023, The Authors. All rights reserved.

关键词： Boric acid

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粉末床熔融的多材料铺粉过程中粉末扩散的数值研究

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Acta Mechanica Sinica 2023年第1期39卷 23-29页

作者：王林李二垒周宗彦张百成余艾冰 ARC Hub for Computational Particle Technology Department of Chemical & Biological Engineering Monash University Clayton VIC 3800 Australia Delft University of Technology Stevinweg 1 2628 CN Delft The Netherlands Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science and Technology Nanchang 330013 China Beijing Advanced Innovation Center Materials Genome Engineering Advanced Material & Technology Institute University of Science and Technology Beijing Beijing 100083 China

粉末床熔融增材制造技术已应用于功能梯度材料的制造.文献中报道了一种材料成分沿垂直于粉末铺粉方向变化的新设计.基于此设计,本工作采用离散单元数值模拟研究了两种密度差异较大的金属粉末在铺粉过程中颗粒的偏析情况.结果发现,在铺... 详细信息

粉末床熔融增材制造技术已应用于功能梯度材料的制造.文献中报道了一种材料成分沿垂直于粉末铺粉方向变化的新设计.基于此设计,本工作采用离散单元数值模拟研究了两种密度差异较大的金属粉末在铺粉过程中颗粒的偏析情况.结果发现,在铺粉过程中,较大密度粉末(重颗粒)一侧的铺粉量小于较小密度粉末(轻颗粒)的一侧的铺粉量.这种现象表明重颗粒从粉末密度大的一侧向粉末密度较小的一侧扩散.这种扩散受铺粉速度影响较大,铺粉速度越快,扩散越明显.但粉末层厚度对扩散影响不大.结果还表明,重颗粒与轻颗粒间的粒径差异影响扩散较大,减小重颗粒的粒径可能是控制颗粒偏析的一种方案.

关键词：材料成分颗粒偏析功能梯度材料离散单元金属粉末密度差异增材制造技术扩散影响

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