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Emerging Organic Contaminants in Chinese Surface Water:Identification of Priority Pollutants

Engineering 2022年第4期8卷 111-125页

作者： Mengmeng Zhong Tielong Wang Wenxing Zhao Jun Huang Bin Wang Lee Blaney Qingwei Bu Gang Yu Beijing Key Laboratory for Emerging Organic Contaminants Control State Key Joint Laboratory of Environment Simulation and Pollution Control(SKLESPC)School of EnvironmentTsinghua UniversityBeijing 100084China Department of Chemical Biochemicaland Environmental EngineeringUniversity of Maryland Baltimore CountyBaltimoreMD 21250USA School of Chemical and Environmental Engineering China University of Mining and Technology-BeijingBeijing 100083China

The occurrence and impacts of emerging organic contaminants(EOCs)in the aquatic environment have gained widespread attention over the past two *** to large number of potential contaminants,monitoring campaigns,treatment plants,and proposed regulations should preferentially focus on specific pollutants with the highest potential for ecological and human health *** the present study,a multi-criteria screening approach based on hazard and exposure potentials was developed for prioritization of 405 unregulated EOCs already present in Chinese surface *** potential,exposure potential,and risk quotients for ecological and human health effects were quantitatively analyzed and used to screen *** hazard potential was defined by contaminant persistence,bioaccumulation,ecotoxicity,and human health effects;similarly,the exposure potential was a function of contaminant concentration and detection *** total,123 compounds passed the preselection process,which involved a priority index equal to the normalized hazard potential multiplied by the normalized exposure *** on the prioritization scheme,11 compounds were identified as top-priority,and 37 chemicals were defined as *** results obtained by the priority index were compared with four other prioritization schemes based on exposure potential,hazard potential,or risk quotients for ecological effects or human *** priority index effectively captured and integrated the results from the more simplistic prioritization *** on identified data gaps,four uncertainty categories were classified to recommend:①regular monitoring,derivation of environmental quality standards,and development of control strategies;②increased monitoring;③fortified hazard assessment;and④increased efforts to collect occurrence and toxicity ***,20 pollutants were recommended as priority *** prioritized list of contaminants provides the necessary information for autho

关键词： Prioritization Emerging organic contaminants Hazard potential Ecotoxicity Risk assessment

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CeO_(2)-supported Fe,Co and Ni toward CO_(2) hydrogenation:Tuning catalytic performance via metal-support interaction

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Journal of Rare Earths 2023年第6期41卷 926-932,I0005页

作者： Bolang Li Fei Wang Kai Li Ping Ning Min Chen Changbin Zhang Faculty of Environmental Science and Engineering Kunming University of Science and TechnologyKunming 650500China National-Regional Engineering Center for Recovery of Waste Gases from Metallurgical and Chemical Industries Kunming University of Science and TechnologyKunming 650500China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environment SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China

The chemical transformation of CO_(2) produces carbon compounds that can be used as precursors for the production of chemicals and ***,we investigated the activity and selectivity of the transition metals(Fe,Co,and Ni)supported on CeO_(2) catalyst for CO_(2) hydrogenation at atmospheric *** found that Ni/CeO_(2) shows the highest CO_(2)conversion compared with Fe/CeO_(2) and Co/CeO_(2).Besides,Co/CeO_(2)and Ni/CeO_(2) exhibit nearly 100%CH_(4)selectivity while Fe/CeO_(2) inclines to produce *** characterization results show that the metal-support interaction order is Fe/CeO_(2)>Co/CeO_(2)>Ni/CeO_(2),the weak metal-support inte raction over Ni/CeO_(2)benefits the activation of H_(2) and then promotes the activity of CO_(2) ***,in situ DRIFTS results demonstrate that monodentate formate species rather than bidentate formate are the active *** main route of CO_(2) hydrogenation to CH_(4) is that CO_(2) is firstly transformed to m-HCOO*and then direct hydrogenation of the m-HCOO*to CH_(4).This study provides insights into the understanding of the mechanisms of CO_(2) hydrogenation on CeO_(2)based catalysts.

关键词： Ni CeO_(2) Metal-support interaction CO_(2)hydrogenation Rare earths

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Vehicle emissions of primary air pollutants from 2009 to 2019 and projection for the 14th Five-Year Plan period in Beijing, China

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Journal of environmental Sciences 2023年第2期124卷 513-521页

作者： Tongran Wu Yangyang Cui Aiping Lian Ye Tian Renfei Li Xinyu Liu Jing Yan Yifeng Xue Huan Liu Bobo Wu National Engineering Research Center of Urban Environmental Pollution Control Beijing Municipal Research Institute of Environmental ProtectionBeijing 100037China Beijing Municipal Ecology and Environment Bureau Beijing 100048China State Key Joint Laboratory of ESPC School of EnvironmentTsinghua UniversityBeijing 100084China School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China

Over the past decade,the emission standards and fuel standards in Beijing have been upgraded twice,and the vehicle structure has been improved by accelerating the elimination of 2.95 million old *** the formulation and implementation of these policies,the emissions of carbon monoxide(CO),volatile organic compounds(VOCs),nitrogen oxides(NO_(x)),and fine particulate matter(PM_(2.5))in 2019 were 147.9,25.3,43.4,and 0.91 kton in Beijing,*** emission factor method was adopted to better understand the emissions characteristics of primary air pollutants from combustion engine vehicles and to improve pollution *** combination with the air quality improvement goals and the status of social and economic development during the 14th Five-Year Plan period in Beijing,different vehicle pollution control scenarios were established,and emissions reductions were *** results show that the emissions of four air pollutants(CO,VOCs,NO_(x),and PM_(2.5))fromvehicles in Beijing decreased by an average of 68% in 2019,compared to their levels in *** contribution of NOx emissions from diesel vehicles increased from 35% in 2009 to 56% in 2019,which indicated that clean and energy-saving diesel vehicle fleets should be further *** vehicle adoption could be an important measure to reduce pollutant *** the further upgrading of vehicle structure and the adoption of electric vehicles,it is expected that the total emissions of the four vehicle pollutants can be reduced by 20%-41% by the end of the 14th Five-Year Plan period.

关键词： Emission variations Vehicle structure Electric vehicle 14th Five-Year Plan Air pollution

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Secondary organic aerosol formation from straw burning using an oxidation flow reactor

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Journal of environmental Sciences 2022年第4期34卷 249-258页

作者： Hui Wang Song Guo Zhijun Wu Kai Qiao Rongzhi Tang Ying Yu Weizhao Xu Wenfei Zhu Liwu Zeng Xiaofeng Huang Lingyan He Mattias Hallquist State Key Joint Laboratory of Environmental Simulation and Pollution Control International Joint Laboratory for Regional Pollution ControlMinistry of Education(IJRC)College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Nanjing University of Information Science&TechnologyNanjing 10044China Key Laboratory for Urban Habitat Environmental Science and Technology College of Environment and EnergyPeking University Shenzhen Graduate SchoolShenzhen 518055China Department of Chemistry and Molecular Biology Atmospheric ScienceUniversity of GothenburgSE-41296 GothenburgSweden

Herein,we use an oxidation flow reactor,Gothenburg:Potential Aerosol Mass(Go:PAM)reactor,to investigate the secondary organic aerosol(SOA)formation from wheat straw *** burning emissions are exposed to high concentrations of hydroxyl radicals(OH)to simulate processes equivalent to atmospheric oxidation of 0-2.55 *** volatile organic compounds(VOCs)were investigated,and particles were measured before and after the Go:PAM *** influence of water content(i.e.5%and 11%)in wheat straw was also *** burning stages,the flaming stage,and non-flaming stages,were *** particle emission factors(EFs)at a water content of 11%(~3.89 g/kg-fuel)are significantly higher than those at a water content of 5%(~2.26 g/kg-fuel)during the flaming ***,the water content showed no significant influence at the non-flaming *** of aromatics at a non-flaming stage(321.8±46.2 mg/kg-fuel)are larger than that at a flaming stage(130.9±37.1 mg/kg-fuel).The OA enhancement ratios increased with the increase in OH exposure at first and decreased with the additional increment of OH *** maximum OA enhancement ratio is~12 during the non-flaming stages,which is much higher than~1.7 during the flaming *** mass spectrum of the primary wheat burning organic aerosols closely resembles that of resolved biomass burning organic aerosols(BBOA)based on measurements in ambient *** results show that large gap(0%-90%)still remains to estimate biomass burning SOA if only the oxidation of VOCs were included.

关键词： Gothenburg:Potential Aerosol Mass(Go:PAM)reactor Wheat straw burning Flaming Non-flaming Secondary organic aerosol formation

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Perspectives on the impacts of climate change and their adaptation

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National Science Open 2024年第1期3卷 4-5页

作者： Guohe Huang Jiapei Chen State Key Joint Laboratory of Environmental Simulation and Pollution Control China-Canada Center for EnergyEnvironment and Ecology ResearchUR-BNUSchool of EnvironmentBeijing Normal UniversityBeijing 100875China Environmental Systems Engineering Program University of ReginaReginaSaskatchewan S4S 0A2Canada

The pressing impacts of climate change and the imperative for adaptation strategies emphasize the immediate necessity for proactive global *** challenges encompass the enhancement of climate modeling,the development of sector-tailored strategies,and the implementation of adaptation *** these issues necessitates worldwide collaborations,sustainable practices,technological innovations.

关键词： climate adaptation collaboration

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Direct Current Driven Persulfate Delivery and Activation for Heterogeneous Porous Media Remediation: Coupling Effects of Electric-Thermal-Chemical-Flow Fields

SSRN

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SSRN 2024年

作者： Geng, Zhuning Zheng, Di Qi, Zhen Xie, Qianli Li, Guanghe Zhang, Fang School of Environment State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua University Beijing100084 China Beijing100015 China

Direct current (DC) has promising potential for persulfate delivery and activation in heterogeneous site remediation, yet requires deeper understanding. Here, we investigated the efficiency of DC for persulfate delivery and activation and compared with alternating current (AC). While AC electric field only influenced persulfate fate by Joule heating effect, DC electric field induced electrokinetic migration of persulfate and contaminants, as well as promoted persulfate activation with Joule heating and electrochemical reactions. DC system achieved 95% MCB removal which was 3.1 times of that in AC system using the same voltage input (60 V) with a velocity of 0.5 m/d. When the applied DC voltage increased from 20 V to 60 V (0.5-1.5 V/cm), persulfate activation pathway changed from electrode reactions to the coupled activation pathways of electrode, chemical and heat reactions, thus resulting in increasing MCB removal efficiency from 57% (20 V) to 95% (40 V and 60 V). The energy consumption with 40 V (11.6 kWh/g) was 2.6 times of that using 20 V (4.4 kWh/g), and dramatically increased to 11.7 times with 60 V (50.2 kWh/g). This study provides a new perspective on improving the efficiency of persulfate delivery and activation in heterogeneous sites remediation using DC-driven system. © 2024, The Authors. All rights reserved.

关键词： Chemical activation

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Comparing the costs and benefits of virgin and urban mining

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Journal of Management Science and Engineering 2022年第1期7卷 98-106页

作者： Xianlai Zeng Tongxin Xiao Guochang Xu Eva Albalghiti Guijuan Shan Jinhui Li State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China School of Forestry and Environmental Studies Yale UniversityNew HavenCT06511USA

Resource and environmental management are shaping our society and *** mining is rapidly becoming unsustainable as primary resources are in increasingly short supply and energy consumption continues to *** mining through a circular economy has emerged as a promising option for securing copper and aluminum ***,the sustainability and viability of this circular economy industry are heavily dependent on its ***,we demonstrate the economic benefits of urban mining for anthropogenic minerals:e-waste,end-of-life vehicles,waste wiring and *** material and cost flows associated with urban mining are deeply *** life cycle cost and cost-benefit analysis,the cost of obtaining one ton of copper or aluminum is found to be,on average,3,000 US$or 1,660 US$,which is significantly lower than the cost of virgin ***,in terms of the costs and benefits,copper may differ tremendously from aluminum depending on the type of anthropogenic *** additional regulations or policies enactment need to reinforce the urban mining and circular economy.

关键词： Circular economy Resource sustainability Cost-benefit analysis Urban mining Virgin mining

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Microbial responses to the use of NaClO in sediment treatment

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Frontiers of environmental Science & Engineering 2022年第2期16卷 25-38页

作者： Kun Li Tingming Ye Wang Zhang Jianfeng Peng Yaohui Bai Weixiao Qi Huijuan Liu Key Laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China University of Chinese Academy of Sciences Beijing 100049China China University of Mining&Technology Beijing 100083China

Chlorine is often used in algal removal and deodorization of landscape waters,and occasionally used as an emergency treatment of heavily polluted ***,the ecological impact of this practice has not been fully studied and *** this study,NaClO at 0.1 mmol/g based on dry weight sediment was evenly mixed into the polluted sediment,and then the sediment was incubated for 150 days to evaluate its microbial *** showed that NaClO addition enhanced the release of TOC,TN,Cr and Cu from the *** microbial richness in the examined sediment decreased continuously,and the Chao1 index declined from 4241 to 2731,in 150 *** microbial community composition was also *** abundance of Proteobacteria and Bacteroidetes increased to 54.8%and 4.2%within 7 days compared to the control,and linear discriminant analysis(LDA)showed gram-negative bacteria and aerobic bacteria enriched after *** functional prediction with PICRUSt2 showed the functions of the microbial community underwent major adjustments,and the metabolic-related functions such as carbon metabolism,including pyruvate and methane metabolisms were significantly inhibited;besides,15 out of 22 analyzed key enzymes involved in C cycling and 6 out of 12 key enzymes or genes involved in N cycling were strongly impacted,and the enzymes and genes involved in carbon degradation and denitrification showed remarkable *** can be concluded that chlorination posed a seriously adverse effect on microbial community structure and *** study deepens the understanding of the ecological effects of applying chlorine for environmental remediation.

关键词： Sediment chlorination Substance mobility Microbial response Community composition Function

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Identification of resistant pharmaceuticals in ozonation using QSAR modeling and their fate in electro-peroxone process

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Frontiers of environmental Science & Engineering 2021年第5期15卷 325-338页

作者： Majid Mustafa Huijiao Wang Richard H.Lindberg Jerker Fick Yujue Wang Mats Tysklind Department of Chemistry UmeåUniversityUmeåS-90187Sweden School of Environment Beijing Key Laboratory for Emerging Organic Contaminants ControlState Key Joint Laboratory of Environmental Simulation and Pollution Control(Ministry of Education)Tsinghua UniversityBeijing100084China

The abatements of 89 pharmaceuticals in secondary effluent by ozonation and the electro-peroxone(E-peroxone)process were *** on the results,a quantitative structure-activity relationship(QSAR)model was developed to explore relationship between chemical structure of pharmaceuticals and their oxidation rates by *** orthogonal projection to latent structure(OPLS)method was used to identify relevant chemical descriptors of the pharmaceuticals,from large number of descriptors,for model *** resulting QSAR model,based on 44 molecular descriptors related to the ozone reactivity of the pharmaceuticals,showed high goodness of fit(R^(2)=0.963)and predictive power(Q^(2)=0.84).After validation,the model was used to predict second-order rate constants of 491 pharmaceuticals of special concern(k_(O_(3)))including the 89 studied *** predicted k_(O_(3))values and experimentally determined pseudo-first order rate constants of the pharmaceuticals’abatement during ozonation(k_(OZ))and the E-peroxone process(k_(EP))were then used to assess effects of switching from ozonation to the E-peroxone process on removal of these *** results indicate that the E-peroxone process could accelerate the abatement of pharmaceuticals with relatively low ozone reactivity(k_(O_(3))<∼10^(2)M^(−1)⋅s^(−1))than ozonation(3–10 min versus 5–20 min).The validated QSAR model predicted 66 pharmaceuticals to be highly O_(3)-*** developed QSAR model may be used to estimate the ozone reactivity of pharmaceuticals of diverse chemistry and thus predict their fate in ozone-based processes.

关键词： Ozone Electro-peroxone Wastewater Quantitative structure activity relationship Advanced oxidation processes

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Impacts of Comorbidity and Mental Shock on Organic Micropollutants in Surface Water During and After the First Wave of COVID-19 Pandemic in Wuhan (2019–2021), China

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Engineering 2024年第6期37卷 40-48页

作者： Jian Zhao Jin Kang Xiaofeng Cao Rui Bian Gang Liu Shengchao Hu Xinghua Wu Chong Li Dianchang Wang Weixiao Qi Cunrui Huang Huijuan Liu Jiuhui Qu Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China Hubei Provincial Research Institute of Environmental Science Wuhan 430072China Key Laboratory of Drinking Water Science and Technology Research Centre for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Sanitary Engineering Department of Water ManagementFaculty of Civil Engineering and GeosciencesDelft University of TechnologyDelft 2600 GAThe Netherlands China Three Gorges Corporation Wuhan 430010China Vanke School of Public Health Tsinghua UniversityBeijing 100084China

The first pandemic wave of coronavirus disease 2019(COVID-19)induced a considerable increase in several antivirals and antibiotics in surface *** common symptoms of COVID-19 are viral and bacterial infections,while comorbidities(e.g.,hypertension and diabetes)and mental shock(e.g.,insomnia and anxiety)are ***,little is known about the long-term impacts of comorbidities and mental shock on organic micropollutants(OMPs)in surface ***,we monitored 114 OMPs in surface water and wastewater treatment plants(WWTPs)in Wuhan,China,between 2019 and *** pandemic-induced OMP pollution in surface water was confirmed by significant increases in 26 OMP *** increases in four antihypertensives and one diabetic drug suggest that the treatment of comorbidities may induce OMP ***,cotinine(a metabolite of nicotine)increased 155 times to 187 ngL1,which might be associated with increased ***,the increases in zolpidem and sulpiride might be the result of worsened insomnia and ***,it is reasonable to note that mental-health protecting drugs/behavior also contributed to OMP *** the observed OMPs,telmisartan,lopinavir,and ritonavir were associated with significantly higher ecological risks because of their limited WWTP-removal rate and high *** study provides new insights into the effects of comorbidities and mental shock on OMPs in surface water during a pandemic and highlights the need to monitor the fate of related pharmaceuticals in the aquatic environment and to improve their removal efficiencies in WWTPs。

关键词： Coronavirus disease 2019 Comorbidities Mental shock Micropollutant Surface water

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