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Synthesis of chitosan-based grafting magnetic flocculants for flocculation of kaolin suspensions

Journal of Environmental Sciences 2024年第5期139卷 193-205页

作者： Chuang Liu Xiaoyu Wang Sicong Du Wenyan Liang Beijing Key Lab for Source Control Technology of Water Pollution/Engineering Research Center for Water Pollution Source Control&Eco-remediation/College of Environmental Science and Engineering Beijing Forestry UniversityBeijing 100083China

A series of novel chitosan-based magnetic flocculants FS@CTS-P(AM-DMC)was prepared by molecular structure *** characterization results showed that FS@CTS-P(AM-DMC)had a uniform size of about 21.46 nm,featuring a typical core-shell structure,and the average coating layer thickness of CTS-P(AM-DMC)was about 5.03 ***@CTS-P(AM-DMC)exhibited excellent flocculation performance for kaolin suspension,achieved 92.54% turbidity removal efficiency under dosage of 150 mg/L,pH 7.0,even at high turbidity(2000 NTU)with a removal efficiency of 96.96%.The flocculation mechanism was revealed to be dominated by charge neutralization under acidic and neutral conditions,while adsorption and bridging effects play an important role in alkaline *** properties of magnetic aggregates during flocculation,breakage,and regeneration were studied at different pH levels and *** the process of magnetophoretic,magnetic particles collide and adsorb with kaolin particles continuously due to magnetic and electrostatic attraction,transform into magnetic chain clusters,and then further form three-dimensional network magnetic aggregates that can capture free kaolin particles and other chain *** image velocimetry confirmed the formation of eddy current of magnetic flocs and experienced three stages:acceleration,stabilization,and deceleration.

关键词： Magnetic flocculation Chitosan Fe_(3)O_(4) Graft copolymerization PIV

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Catalytic applications of amorphous alloys in wastewater treatment: A review on mechanisms, recent trends, challenges and future directions

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Chinese Chemical Letters 2024年第10期35卷 73-81页

作者： Yulong Liu Haoran Lu Tong Yang Peng Cheng Xu Han Wenyan Liang Engineering Research Center for Water Pollution Source Control&Eco-remediation Beijing Key Lab for Source Control Technology of Water PollutionCollege of Environmental Science and EngineeringBejing Forestry UniversityBeijing 100083China

Amorphous alloys,with unique atomic structures and metastable nature,are treated as superior candi-dates for environmental wastewater remediation due to their superior catalytic *** the strong demand for environmental protection,the field of amorphous alloys in wastewater treatment has great development prospects,and numerous research results have been published in recent *** a promising catalyst,it was demonstrated that amorphous alloys could exhibit many excellent proper-ties in wastewater treatment,such as high catalytic efficiency,easily adjustable parameters and reliable *** paper aims to summarize recent research trends regarding amorphous alloys in the field of catalysis,focusing on the preparation methods,physical performance,catalytic mechanisms and environmental ***,this review also investigates the challenges encountered and fu-ture perspectives of amorphous alloys,offering new research opportunities to enlarge their applicability spectra.

关键词： Amorphous alloys Wastewater treatment Advanced oxidation processes Catalyst Catalytic mechanism

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Boosting oxygen vacancies by modulating the morphology of Au decorated In_(2)O_(3)with enhanced CO_(2)hydrogenation activity to CH_(3)OH

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Journal of Environmental Sciences 2024年第6期140卷 91-102页

作者： Ruxian Hou Jiewen Xiao Qian Wu Tianyu Zhang Qiang Wang Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China Engineering Research Center for Water Pollution Source Control&Eco-remediation College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China

CO_(2)hydrogenation to methanol has become one of the most promising ways for CO_(2)utilization,however,the CO_(2)conversion rate and methanol selectivity of this reaction still need to be improved for industrial *** we investigated the structure-activity relationship for CO_(2)conversion to methanol of In_(2)O_(3)-based catalysts by modulating morphology and decorating *** different Au/In_(2)O_(3)catalysts were prepared,their activity follow the sequence of Au/In_(2)O_(3)-nanosphere(Au/In_(2)O_(3)-NS)>Au/In_(2)O_(3)-nanoplate(Au/In_(2)O_(3)-NP)>Au/In_(2)O_(3)-hollow microsphere(Au/In_(2)O_(3)-HM).Au/In_(2)O_(3)-NS exhibited the best performance with good CO_(2)conversion of 12.7%,high methanol selectivity of 59.8%,and large space time yield of 0.32 g CH_(3)OH/(hr·gcat)at 300℃.The high performance of Au/In_(2)O_(3)-NS was considered as the presence of *** contributes to the creation of more surface oxygen vacancies,which further promoted the CO_(2)adsorption and facilitated CO_(2)activation to form the formate intermediates towards *** work clearly suggests that the activity of In_(2)O_(3)catalyst can be effective enhanced by structure engineering and Au decorating.

关键词： CO_(2)hydrogenation Methanol Au/In_(2)O_(3) Morphology Oxygen vacancies

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Effect of allelochemicals sustained-release microspheres on the ingestion, incorporation, and digestion abilities of Daphnia magna Straus

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Journal of Environmental Sciences 2023年第2期124卷 205-214页

作者： Benhang Li Yijun Yin Xiaohong Zhou Li Feng Yongze Liu Ziwen Du Yajun Tian Liqiu Zhang Beijing Key Laboratory for Source Control Technology of Water Pollution Engineering Research Center for Water Pollution Source Control and EcoremediationBeijing Forestry UniversityBeijing 100083China College of Environment Zhejiang University of TechnologyHangzhou 310014China

Allelochemicals sustained-release microspheres(ACs-SMs)exhibited great inhibition effect on algae,however,few studies have focused on ACs-SMs toxicity on *** this study,the effects of single high-concentration ACs(15 mg/L,SH-ACs),repeated lowconcentration ACs(3×5 mg/L,RL-ACs)and ACs-SMs containing 15 mg/L ACs exposure on the ingestion,incorporation,and digestion of Daphniamagna Straus(DS)were investigated by stable isotope 15N labeling ***,the diversity and abundance of microflora in DS guts were determined by 16S rRNA genes and cloning *** results showed that SH-ACs exposure caused 50%and 33.3%death rates for newborn and adult DS,while RL-ACs exposure caused 10%death rate for newborn DS and no obvious effect on the activity of adult *** ACs-SMs exposure did not diminish the motility of both newborn and adult DS,indicating the lower acute toxicity of ***,SH-ACs inhibited the ingestion(-6.45%),incorporation(-47.1%)and digestion(-53.8%)abilities of DS and reduced the microbial abundance(-27.7%)in DS *** with SH-ACs,RL-ACs showed relatively low impact on the ingestion(-3.23%),incorporation(-5.89%)and digestion(-23.9%)abilities of ***,ACs-SMs enhanced the ingestion(+9.68%),incorporation(+52.9%)and digestion(+51.3%)abilities of DS and increased the microbial abundance(+10.7%)in DS *** ACs and ACs-SMs reduced the diversity of microflora in DS *** conclusion,ACs-SMs can release ACs sustainably and prolong the sustained release time,which not only effectively reduce the toxicity of ACs,but also had positive effects on DS.

关键词： Allelochemicals(ACs) Sustained-release microspheres (SMs) Daphnia magna Straus(DS)

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Enhanced hydrolytic removal of tylosin in wastewater using polymer-based solid acid catalysts converted from polystyrene

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Journal of Environmental Sciences 2023年第4期126卷 287-296页

作者： Shiling Li Shuhan Sun Fei Qi Xiaomin Dou Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China Engineering Research Center for Water Pollution Source Control and Eco-remediation College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China

Antibiotic production wastewater usually contains high concentrations of antibiotic residues,which can cause instability and deterioration of biological wastewater treatment units and also domestication and proliferation of antibiotic-resistance *** effective pretreatment on antibiotics production wastewater is expected to selectively reduce the concentration of antibiotics and decrease the toxicity,rather than mitigate organic and other contaminants before further *** this work,two polymer-based solid acids,PS-S and CPS-S bearing high concentrations of-SOH_(3)groups (up to 4.57 mmol/g),were prepared and successfully used for hydrolytic mitigation of 100 mg/L tylosin within 20 *** co-existence of high concentrations of COD and humic substances did not affect the mitigation of tylosin obviously,while more than 500 mg/L of nitrogenous compounds suppressed the hydrolytic *** and reuse experiments showed that the solid acids performed well in five cycles after *** transformation products (P1,P2 and P3)were identified using UPLC-QTOF-MS/*** moieties including mycarse,mycaminose,and mycinose detached and released simultaneously or in order from the 16-member lactone ring through desugarization,which led to a dramatic decrease in antibacterial activity as revealed by cytotoxicity evaluations using *** estimation indicated the acute toxicities of the hydrolyzed products to model species (e.g.,fish,daphnid and green algae) were classified as“not harmful”.This work suggested an effective and selective method to pretreat tylosin-contained production wastewater by using polymer-based solid *** results will shed light on effective elimination of antibiotics pollution from pharmaceutical industries through strengthening the pretreatments.

关键词： Polymer Sulfonation Solid acid catalysts Tylosin hydrolysis Antibiotic

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Removal efficiencies of natural and synthetic progesterones in hospital wastewater treated by different disinfection processes

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Frontiers of Environmental Science & Engineering 2022年第10期16卷 11-22页

作者： Jinhui Liang Yuchen Luo Benhang Li Shiqi Liu Liansheng Yang Peng Gao Li Feng Yongze Liu Ziwen Du Liqiu Zhang Beijing Key Laboratory for Source Control Technology of Water Pollution Engineering Research Center for Water Pollution Source Control and Eco-remediationBeijing Forestry UniversityBeijing 100083China

Progesterones are ubiquitous in hospital wastewater(HWW)with concentrations much higher than those of estrogens and *** ensure that these water systems are safe to use,disinfection is crucial during HWW treatment by providing"front line"defense against biological ***,five disinfection processes,namely,chlorine(Cl_(2)),chlorine dioxide(ClO_(2)),ozone(O_(3)),ultraviolet(UV)),and UV/chlorine(UV/Cl_(2)),were selected to investigate their removal efficiencies for progesterones in primary filtration and secondary biological treatment *** were 61 natural and synthetic progesterones detected in HWW,with the natural progesterones being the main components with a concentration of 845.51 ng/L and contributing to 75.08%of the total *** primary filtration treatment presented insignificant removal effects on the progesterones,while the secondary biological treatment significantly reduced the progesterone content by *** order of removal efficiencies of total progesterones by different disinfection processes was UV/Cl_(2)>Cl_(2)>O_(3)>ClO_(2)>***/Cl_(2)showed the highest removal efficiency against progesterones mainly due to the activation of Cl_(2)by ultraviolet(UV)photolysis,which helps open the heterocyclic,aromatic,and phenolic rings,thus accelerating progesterone *** addition,the removal efficiencies of natural progesterones in the five disinfection processes were higher than those of synthetic progesterones(progesterone derivatives,19-nortestosterone derivatives,and 17α-hydroxyprogesterone derivatives).

关键词： Progesterones Hospital wastewater Primary filtration treatment effluent Secondary biological treatment effluent Disinfection process

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Occurrence and migration of microplastics and plasticizers in different wastewater and sludge treatment units in municipal wastewater treatment plant

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Frontiers of Environmental Science & Engineering 2022年第11期16卷 203-212页

作者： Sen Dong Peng Gao Benhang Li Li Feng Yongze Liu Ziwen Du Liqiu Zhang Beijing Key Laboratory for Source Control Technology of Water Pollution Engineering Research Center for Water Pollution Source Control and Eco-remediationBeijing Forestry UniversityBeijing 100083China

Microplastics(MPs)and plasticizers,such as phthalate esters(PAEs),were frequently detected in municipal wastewater treatment plants(MWTP).Previous research mainly studied the removal of MPs and PAEs in ***,the occurrence of MPs and PAEs in the sludge was generally *** comprehensively investigate the occurrence and the migration behaviors of MPs and PAEs in MWTP,a series of representative parameters including the number,size,color,shape of MPs,and the concentrations of PAEs in wastewater and sludge were systematically *** this study,the concentrations of MPs in the influent and effluent were 15.46±0.37 and 0.30±0.14 particles/*** MP removal efficiency of 98.1%was achieved and about 73.8%of MPs were accumulated in the sludge in the *** numbers of MPs in the sludge before and after digestion were 4.40±0.14 and 0.31±0.01 particles/g(dry sludge),*** Transform Infrared Spectroscopy(ATR FT-IR)analysis showed that the main types of MPs were polyethylene terephthalate(PET),polypropylene(PP),polyethylene(PE),and polystyrene(PS).Six PAEs,including phthalate(DMP),diethyl phthalate(DEP),diisobutyl phthalate(DIBP),ortho dibutyl phthalate(DBP),butyl benzyl phthalate(BBP),and bis(2-ethyl)hexyl phthalate(DEHP),were detected in the *** concentrations of total PAEs(ΣPAEs)in the influent and effluent were 76.66 and 6.28μg/L,*** concentrations ofΣPAEs in the sludge before and after digestion were 152.64 and 31.70μg/g,*** the process of thermal hydrolysis,the number and size of MPs decreased accompanied by the increase of the plasticizer concentration.

关键词： Microplastics Municipal wastewater treatment plant Phthalate esters Thermal hydrolysis

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Characteristics of typical dissolved black carbons and their influence on the formation of disinfection by-products in chlor(am)ination

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Frontiers of Environmental Science & Engineering 2022年第12期16卷 1-14页

作者： Jinhui Liang Peng Gao Benhang Li Longfei Kang Li Feng Qi Han Yongze Liu Liqiu Zhang Beijing Key Laboratory for Source Control Technology of Water Pollution Engineering Research Center for Water Pollution Source Control and Eco-remediationBeijing Forestry UniversityBeijing100083China

Dissolved black carbon(DBC)released from biochar can be one of the potential disinfection by-products(DBPs)precursors in the dissolved organic matter ***,the physiochemical and structural properties of DBC and the effects on the development of DBPs and DBP formation potential(DBPFP)during the disinfection process remain *** this study,the characteristics of two kinds of DBC,namely,animal-derived DBC(poultry litter DBC,PL-DBC)and plant-derived DBC(wheat straw DBC,WS-DBC),were *** effects of different kinds of DBC on the evolution of DBPs and DBPFP in chlorine and chloramine disinfection processes were compared with natural organic matter(NOM).The results showed that the total DBPs concentrations derived from PL-DBC,WS-DBC and NOM were similar during chlorination(i.e.,61.23µg/L,64.59µg/L and 64.66µg/L,respectively)and chloramination(i.e.,44.63µg/L,44.42µg/L and 45.58µg/L,respectively).The lower total DBPs and DBPFP concentrations in chloramination could be attributed to the fact that the introduction of ammonia in chloramine inhibited the breaking of the bond between the disinfectant and the active group of the ***,DBC presented much lower total DBPFP concentrations than NOM in both chlorination and ***,both kinds of DBC tended to form more monochloroacetic acids and haloacetamides than NOM,which could result from the higher organic strength,higher protein matter,and nitrogen-rich soluble microbial products of DBC.

关键词： Dissolved black carbon(DBC) Chlorine Chloramine Disinfection by-products(DBPs) Disinfection by-products formation potential(DBPFP)

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Surface modification of Cu_(2)O with stabilized Cu^(+) for highly efficient and stable CO_(2) electroreduction to C_(2+) chemicals

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Journal of Energy Chemistry 2023年第9期84卷 277-285页

作者： Ziyu Zhou Shuyu Liang Jiewen Xiao Tianyu Zhang Min Li Wenfu Xie Qiang Wang Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China Engineering Research Center for Water Pollution Source Control&Eco-remediation College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China

Copper(Cu)-based materials are known as the most attractive catalysts for electrochemical carbon dioxide reduction reaction(CO_(2)RR),especially the Cu^(+) species(e.g.,Cu_(2)O),which show excellent capability for catalyzing CO_(2) to C_(2+) chemicals because of their unique electronic ***,the active Cu^(+) species are prone to be reduced to metallic Cu under an electroreduction environment,thus resulting in fast deactivation and poor ***,we developed an advanced surface modification strategy to maintain the active Cu^(+) species via assembling a protective layer of metal-organic framework(copper benzenetricarboxylate,CuBTC) on the surface of Cu_(2)O octahedron(Cu_(2)O@CuBTC).It's encouraging to see that the Cu_(2)O@CuBTC heterostructure outperforms the bare Cu_(2)O octahedron in catalyzing CO_(2) to C_(2+) chemicals and dramatically enhances the ratio of C_(2)H_(4)/CH_(4) products.A systematic study reveals that the introduced CuBTC shell plays a critical role in maintaining the active Cu^(+) species in Cu_(2)O@CuBTC heterostructure under reductive *** work offers a practical strategy for improving the catalytic performance of CO_(2)RR over copper oxides and also establishes a route to maintain the state of valence-sensitive catalysts.

关键词： CO_(2)RR Copper Oxide Metal-organic Framework Core-shell Structure C_(2+)Chemicals

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Dimension-controlled synthesis of BiOI for efficient visible light photodegradation of tetracycline: role of pore structure

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Environmental Science and pollution Research 2024年第20期31卷 29101-29112页

作者： Gao, Peng Qiu, Nanting Feng, Li Zhang, Liqiu Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and Engineering Beijing Forestry University Beijing100083 China Engineering Research Center for Water Pollution Source Control & amp Eco-Remediation College of Environmental Science and Engineering Beijing Forestry University Beijing100083 China

The transformation of photogenerated charge carriers (PC) in variable dimensional photocatalyst plays a pivotal role in unraveling the generation of reactive species (RS). However, the dimensional structure–activity relationship in photocatalysis remains elusive, with limited insights into its intricacies. Herein, we report a controlled synthesis strategy by using polyvinyl pyrrolidone (PVP)-assisted precipitation method for BiOI photocatalyst. Due to the steric hindrance of PVP, the 3D microsphere (3D-PVP0.5) and porous structure (3D-PVP1) of BiOI catalysts have been successfully prepared at room temperature. The 3D-PVP1 photocatalyst contains abundant mesopores and larger pores, which significantly shorten the diffusion distance of PC. Also, these PC in porous structure is beneficial for transferring from the inner phase to the surface of materials. Combined with optical property and radicals trapping experiments, the recombination rate of PC in porous structure performs a significant decrease, leading to the generation of more dominated ROS (•O2− and h+). The •O2− played a dominated role (86.98% of contribution rate) in photodegradation of tetracycline (TC) in 3D-PVP1 photocatalytic process. Compared with 2D nanosheet of BiOI (16.7% removal rate of TC), the as-prepared 3D porous structure of BiOI catalyst exhibits unique stable and high removal capacities (90.5%) for TC photodegradation under visible light irradiation. The kobs of 3D-PVP1 photocatalyst increased by 5.1 times than that of 2D nanosheet. To investigate its practical application, the effects of inorganic anions and pH have been systematically studied. This work sheds light on the design of variable dimension BiOI catalyst and provides more insight into the transfer mechanism of PC. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.

关键词： Bismuth compounds

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