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Polarization-Induced Proton Adsorption and Charge Separation in Pyrene-Based Conjugated Microporous Polymers Via Substituent Regulation for Efficient Photocatalytic Hydrogen Evolution

SSRN

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SSRN 2023年

作者： Ren, Runtang Jiao, Zhengxu Li, Zhanfeng Tian, Yue Liu, Baoyou Yue, Gang Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province Taiyuan University of Technology Taiyuan030024 China Institute of Carbon Materials College of Materials Science and Engineering Taiyuan University of Technology Taiyuan030024 China Technology Innovation Center Ningxia Sinostar Display Material Co. Ltd. Yinchuan750003 China

Constructing photocatalysts with efficient light-harvesting abilities and charge separation properties is highly promising but still challenging for boosting photocatalytic hydrogen evolution from water. Herein, we report a simple and general polarization strategy through substituent regulation such as fluorination, chlorination and cyanation, to promote the photon capture and charge separation and unveil the latent structure–property–activity relationship in pyrene-based conjugated microporous polymers (CMPs). Notably, the introduction of fluorine, chlorine and cyano substituents onto the well-known full donor pyrene-benzene-based CMP network (Py-B) could induce a strong dipole along C–F/–Cl/–CN bonds and the backbone local polarization enhancement due to their strong electron-withdrawing ability, which afforded CMPs have a variety of superior effects such as narrowing band gaps, expanding optical absorption, improving interfacial wettability and solid-state morphology, and promoting charge separation inside organic photocatalysts. As a result, 1.73/2.50/4.69-fold increases of the hydrogen evolution rates of the –F/–Cl/–CN modified CMPs under visible light (λ > 420 nm) irradiation without Pt co-catalysts can be obtained in comparison with the counterpart Py-B (28.5/41.3/77.4 mmol g−1 h−1 vs 16.5 mmol g−1 h−1). Impressively, we find that the photocatalytic performance of this series of photocatalysts is linearly related to the dipole moment of polymers. Our studies reveal that the backbone local polarization enhancement induced by the substituent regulation could achieve high-performance organic photocatalysts toward solar-to-chemical energy conversion. © 2023, The Authors. All rights reserved.

关键词： Polarization

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Cavitation of a Submerged Jet at the Spherical Valve Plate/Cylinder Block Interface for Axial Piston Pump

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Chinese Journal of Mechanical Engineering 2020年第5期33卷 197-211页

作者： Bin Zhao Weiwei Guo Long Quan College of Mechanical and Vehicle Engineering Taiyuan University of TechnologyTaiyuan 030024China Transducers and Intelligent Control System of Ministry of Education and Shanxi Province Taiyuan University of TechnologyTaiyuan 030024China The State Key Laboratory of Fluid Power&Mechatronic Systems Zhejiang UniversityHangzhou 310027China

The spherical valve plate/cylinder block pair has the advantages of strong overturning resistance and large bearing ***,the configurations of the unloading and pre-boosting triangular grooves on the spherical valve plate are different from those in the planar valve plate,resulting in special cavitation phenomenon on the spherical port plate *** order to study cavitation characteristics of spherical port plate pair,a dynamic CFD model of the piston pump including turbulence model,cavitation model and fluid compressibility is established.A detailed UDF compilation scheme is provided for modelling of the micron-sized spherical oil film mesh,which makes up for the lack of research on the meshing of the spherical oil *** this paper,using CFD simulation tools,from the perspectives of pressure field,velocity field and gas volume fraction change,a detailed analysis of the transient evolution of the submerged cavitation jet in a axial piston pump with spherical valve plate is carried *** study indicates the movement direction of the cavitation cloud cluster through the cloud image and the velocity vector direction of the observation *** sharp decrease of velocity and gas volume fraction indicates the collapse phenomenon of bubbles on the part wall *** discoveries verify the special erosion effect in case of the spherical valve plate/cylinder block *** submerged cavitation jet generated by the unloading triangular grooves distributed on the spherical valve plate not only cause denudation of the inner wall surface of the valve plate,but also cause strong impact and denudation on the lower surface of the cylinder ***,the direction of the unloading triangular groove was modified to extend the distance between it and the wall surface which can effectively alleviate the erosion effect.

关键词： Cavitation submerged jet Spherical valve plate/cylinder block pair Axial piston pump

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A Graphical Pressure Sensor Array With Multilayered Structure: Written Through Graphene Ink on Cellulose Paper Substrate

Research Square

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Research Square 2021年

作者： Ji, Chao Zhang, Qiang Li, Qiang Pei, Zhen Zhao, Dong Yuan, Zhongyun Wang, Jie Zhang, Wendong Sang, Shengbo MicroNano System Research Center Key Laboratory of Advanced Transducers and Intelligent Control System of the Ministry of Education and Shanxi Province College of Information and Computer Taiyuan University of Technology Shanxi Taiyuan030024 China

Paper based flexible pressure sensors have received extensive attention due to their recoverability and accessibility. In this paper, we proposed graphical pressure sensors array with multilayered structure. A simple writing method was adopted to achieve the adsorption of sensitive materials on the fiber structure of cellulose paper. Pressure sensors with 1, 3, 5 and 7 stacked layers were fabricated and compared, respectively. The results show that the 7-layers sensor combined high sensitivity (44 kPa-1) and fast time response (150 ms). The highly sensitive stacked paper-based sensor array realizes the pressure detection of objects and special-shaped surfaces. A pressure sensor base on commercial corrugated box was also fabricated to compare. The corrugated carton array was made to switch reminder devices for its convenience and accessibility. Since there are many scenarios that require a safe distance, especially under the influence of the COVID-19, the writable paper-based sensor array was used to realize graphical distance perception and warning. © 2021, CC BY.

关键词： Pressure sensors

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Study on Sensitization Mechanism of Novel Magnetorheological Composite Pdms Thin Film Based on Enhanced Magneto-Mechanical Effect

SSRN

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SSRN 2023年

作者： Sang, Shengbo Tan, Qiuyun Jiang, Jiaolin Wu, Kaile Xiao, Pengli Zhao, Dong Guo, Xing Yang, Zhuoqing Dong, Xiushan Ge, Yang Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Information and Computer Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China Shanghai200240 China Shanxi Academy of Medical Sciences China Shanxi Research Institute of 6D Artificial Intelligence Biomedical Science Taiyuan030024 China

High sensitivity is key to expand the range of bio-detection, especially in realizing biological detection on single molecular level. Herein, we introduce a novel magnetorheological membrane with enhanced magneto-mechanical effect into the biosensor. Specifically, we made the magnetorheological composite PDMS film (MREF) strengthened by magnetostrictive particles (MSP), and the anisotropic TbDyFe-PDMS can be magnetically deformed to 90 °with 5.8 emu/g, which possesses an initial tensile modulus 55% higher than isotropic. In particular, the modified MR effect equations were proposed considering magnetic dipole interaction and nonlinear magnetostrictive pre-strain of MSP. Such formulae indicate that the enhanced MR effect of MSP-MREF is greatly determined by Ms, remanence, and the flux linkage-like structure. In addition, finite element simulations were carried out to validate and complementarily demonstrate the nonlinear magneto-mechanical behaviors of MSP-MREF theoretically. Finally, the biosensor based on MSP-MREF was fabricated to detect the low concentrations of human serum albumin (HSA), and its sensitivity is around 4 times that of the conventional biosensor. Furthermore, it exhibits high reliability in detecting HSA in real human urine samples, making it the ideal candidate as a practical and effective way for the detection of biomolecules at low concentrations in the future. © 2023, The Authors. All rights reserved.

关键词： Finite element method

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Biocompatible chitosan/polyethylene glycol/multi-walled carbon nanotube composite scaffolds for neural tissue engineering

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2022年第1期23卷 58-73页

作者： Shengbo SANG Rong CHENG Yanyan CAO Yayun YAN Zhizhong SHEN Yajing ZHAO Yanqing HAN Shanxi Key Laboratory of Micro Nano Sensors&Artificial Intelligence Perception College of Information and ComputerTaiyuan University of TechnologyTaiyuan030024China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of TechnologyTaiyuan030024China College of Information Science and Engineering Hebei North UniversityZhangjiakou075000China Shanxi Six-Dimensional Artificial Intelligence Biomedical Research Institute Taiyuan030031China Department of Neurology Shanxi Provincial Cardiovascular HospitalTaiyuan030024China

Carbon nanotube(CNT)composite materials are very attractive for use in neural tissue engineering and biosensor *** scaffolds are excellent mimics of extracellular matrix due to their hydrophilicity,viscosity,and *** can also impart conductivity to other insulating materials improve mechanical stability guide neuronal cell behavior and trigger axon *** performance of chitosan(CS)/polyethylene glycol(PEG)composite scaffolds could be optimized by introducing multi-walled CNTs(MWCNTs).CS/PEG/CNT composite scaffolds with CNT content of 1%,3%,and 5%(1%=0.01 g/mL)were prepared by *** physical and chemical properties and biocompatibility were *** electron microscopy(SEM)showed that the composite scaffolds had a highly connected porous *** electron microscope(TEM)and Raman spectroscopy proved that the CNTs were well dispersed in the CS/PEG matrix and combined with the CS/PEG nanofiber *** enhanced the elastic modulus of the *** porosity of the scaffolds ranged from 83%to 96%.They reached a stable water swelling state within 24 h,and swelling decreased with increasing MWCNT *** electrical conductivity and cell adhesion rate of the scaffolds increased with increasing MWCNT *** showed that rat pheochromocytoma(PC12)cells grown in the scaffolds had characteristics similar to nerve *** measured changes in the expression of nerve cell markers by quantitative real-time polymerase chain reaction(qRT-PCR),and found that PC12 cells cultured in the scaffolds expressed growth-associated protein 43(GAP43),nerve growth factor receptor(NGFR),and class IIIβ-tubulin(TUBB3)*** research showed that the prepared CS/PEG/CNT scaffold has good biocompatibility and can be further applied to neural tissue engineering research.

关键词： Multi-walled carbon nanotube(MWCNT) Cell-scaffold PC12 cells Biocompatibility

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What Matters for 3D Scene Flow Network

arXiv

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arXiv 2022年

作者： Wang, Guangming Hu, Yunzhe Liu, Zhe Zhou, Yiyang Tomizuka, Masayoshi Zhan, Wei Wang, Hesheng Department of Automation Key Laboratory of System Control and Information Processing of Ministry of Education Key Laboratory of Marine Intelligent Equipment and System of Ministry of Education Shanghai Jiao Tong University China MoE Key Lab of Artificial Intelligence Shanghai Jiao Tong University China Mechanical Systems Control Laboratory University of California Berkeley United States

3D scene flow estimation from point clouds is a low-level 3D motion perception task in computer vision. Flow embedding is a commonly used technique in scene flow estimation, and it encodes the point motion between two consecutive frames. Thus, it is critical for the flow embeddings to capture the correct overall direction of the motion. However, previous works only search locally to determine a soft correspondence, ignoring the distant points that turn out to be the actual matching ones. In addition, the estimated correspondence is usually from the forward direction of the adjacent point clouds, and may not be consistent with the estimated correspondence acquired from the backward direction. To tackle these problems, we propose a novel all-to-all flow embedding layer with backward reliability validation during the initial scene flow estimation. Besides, we investigate and compare several design choices in key components of the 3D scene flow network, including the point similarity calculation, input elements of predictor, and predictor & refinement level design. After carefully choosing the most effective designs, we are able to present a model that achieves the state-of-the-art performance on FlyingThings3D and KITTI Scene Flow datasets. Our proposed model surpasses all existing methods by at least 38.2% on FlyingThings3D dataset and 24.7% on KITTI Scene Flow dataset for EPE3D metric. We release our codes at https://***/IRMVlab/3DFlow. Copyright © 2022, The Authors. All rights reserved.

关键词： Embeddings

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Super-twisting Finite Time control for Third Order Nonlinear systems

Super-twisting Finite Time Control for Third Order Nonlinear...

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第40届中国控制会议

作者： Xinjian Liu Jianxiong Li Zhi Li Yiming Fang Research Center of the Ministry of Education for Intelligent Control System and Intelligent Equipment The Key Lab of Industrial Computer Control Engineering of Hebei Province

A novel super-twisting control method is proposed for a class of third-order systems with matched Lipschitz disturbance in this paper. The proposed method ensures finite-time convergence to the fourth-order sliding set, by using a homogeneous, continuously differentiable and strict Lyapunov function. Finally, numerical simulation results are shown to illustrate the effectiveness of the proposed method.

关键词： Third-order sliding mode Super-twisting algorithm Finite time control

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Research on Highly Anti-Humidity and Selective NO2 Detection Based on GaN/MoO3 N-N Heterojunction

SSRN

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SSRN 2024年

作者： Hong, Yutao Han, Dan Li, Donghui He, Xiuli Zhao, Li Wang, Weidong Li, Hongwei Sang, Shengbo Liang, Hua Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China State Key Laboratory of Transducer Technology Aerospace Information Research Institute Chinese Academy of Sciences Beijing100190 China Bioengineering Research Center Medical Innovation Research Division Chinese PLA General Hospital Beijing China Shanxi Academy of Medical Sciences China

Effective and accuratedetection of NO2 gas is crucial for protecting the environment and public health. In this work, balsam pear-like GaN/MoO3 porous nanosheets (GaN/MoO3) composites were synthesized by the in situ assembling, the hydrothermal method, and the nitridation process to detect NO2. A series of characterization methods were used to manifest the successful synthesis and to analyze the morphology and elemental composition features of GaN/MoO3 composites. The results of the gas-sensing experiments show that at the operating temperature of 225 °C, the gas sensor based on the optimal ratio of GaN/MoO3 composites exhibits a low theoretical limit of detection (0.78 ppb) for NO2, which is significantly improved compared with the limit of detection of MoO3 (5 ppm). Further, the response value of the sensor based on GaN/MoO3 composites to 200 ppm NO2 (44.74) is 4.36 times higher than that of the sensor based on pure GaN, with an improvement in stability. Meanwhile, the sensor also possessed excellent repeatability, selectivity, stability, and splendid anti-humidity ability at 15-70 % RH. The improved gas-sensing performance is ascribed to the unique microstructure of both GaN and MoO3, and the heterojunction effect between them. This work provides a way to improve the efficiency and anti-humidity ability of real-time monitoring of NO2 for the sensors of MoO3-based composite. © 2024, The Authors. All rights reserved.

关键词： Gallium nitride

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High-accuracy disposable micro-optical anti-counterfeiting labels based on single-molecule quantum coherence

arXiv

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arXiv 2025年

作者： Han, Shuangping Song, Kai Zan, Pengyu Yu, Changzhi Li, Ao Zhou, Haitao Qin, Chengbing Xiao, Liantuan College of Physics and Optoelectronics Engineering Taiyuan University of Technology Shanxi Taiyuan030024 China Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education Taiyuan University of Technology Taiyuan030024 China Department of Nuclear Medicine The First Hospital of Shanxi Medical University Collaborative Innovation Center of Molecular Imaging Precision Medical Shanxi Medical University Taiyuan030001 China State Key Laboratory of Quantum Optics and Quantum Optics Devices Institute of Laser Spectroscopy Shanxi University Shanxi Taiyuan030006 China

In this work we introduce an innovative approach to single-molecule quantum coherence (SMQC)-based disposable micro-optical anti-counterfeiting labels. This method facilitates the editing and reading of anti-counterfeiting with single molecules used as the anti-counterfeiting information labels. The label is meticulously crafted through inkjet printing technology, while its authentication is achieved via frequency domain imaging. Through a validation process including experimental demonstration, numerical simulation, and neural network analysis, we demonstrate the feasibility of this approach, further validate the integrity of the miniature anti-counterfeiting information storage, and verify the signal extraction accuracy with the recognition accuracy of the labels is consistently above 99.995%. The combination of SMQC-based disposable micro-optical anti-counterfeiting technology is expected to enable more precise preparation of single-molecule-array chips, thus providing a crucial foundation for the advancement of high-tech and smart manufacturing industries. Copyright © 2025, The Authors. All rights reserved.

关键词： Ink jet printing

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On-chip ultra-compact hexagonal boron nitride topological ring-resonator in visible region

arXiv

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arXiv 2022年

作者： Wu, Min Yang, Yibiao Fei, Hongming Lin, Han Zhao, Xiaodan Kang, Lijuan College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan030024 China Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China Centre for Translational Atomaterials Faculty of Science Engineering and Technology Swinburne University of Technology HawthornVIC3122 Australia

Ultra-compact topological ring-resonators with chirality are important devices for quantum optics. However, there are limited demonstrations of chiral resonators, especially in the visible region. We proposed a topological photonic ring-resonator based on hexagonal boron nitride (hBN) valley photonic crystal (VPC). The spin-valley locking effect in VPC allows achieving robust unidirectional transmission of edge states in the visible region (600 nm-650 nm). As a result, a high quality factor (679.3) with a free spectral range of 15.2 nm in the visible region can be achieved in a hBN all-pass filter with a compact size (2.1 μm∗1.8 μm). In addition, we investigated the transmission properties of hBN ring-resonators with different shapes and combinations, confirming the flexibility of designing topological ring-resonators based on this principle. This design can be readily integrated with quantum photonic chips for broad applications. Copyright © 2022, The Authors. All rights reserved.

关键词： Photonic crystals

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