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Research Square 2021年

作者： Sun, Zhuangzhi Li, Zhaoxin Han, Changlong Jing, Mingxing Yu, Haipeng Wang, Zuankai Province Key Laboratory of Forestry Intelligent Equipment Engineering College of Mechanical and Electrical Engineering Northeast Forestry University Harbin150000 China Key Laboratory of Bio-based Material Science & Technology Ministry of Education Northeast Forestry University Harbin150000 China Department of Mechanical and Biomedical Engineering City University of Hong Kong Hong Kong

In nature, liquid evaporation occurs everywhere all the time. This low-grade energy absorption to drive liquid evaporation is greatly potential for sustainable spontaneously power generation. Here, a natural liquid evaporation strategy of interfacial evaporation driven nanogenerator (IENG) is developed in this work. Coupled by the phonon wind and a fluctuating Coulomb field, an induced direct current is generated. Simultaneously, inspired by the light-trapping properties of moth eye, a simple and efficient BLT-IENG including a hierarchical surface of bionic light-trapping and electrospinning perovskite conductivity with an enhanced thermally insulating and water storage capability is designed. This enhancement of the output performance is greatly attributed to the improvement of the interfacial evaporation characteristics driven by natural solar and wind energies. Hence, our BLT-IENG achieves a breakthrough in the unit area open-circuit voltage in the marine environment, which is improved by a factor of 7.6 over the currently reported average value. This work provides an unexplored strategy for multi-energies inspired natural interfacial evaporation driven power generation. © 2021, CC BY.

关键词： Nanogenerators

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biomimetic construction of oxygen vacancy-rich In 2 O 3 /In 2 S 3 @C heterostructures with built-in electric field for boosting bidirectional regulation of polysulfides in lithium-sulfur batteries

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Chemical Engineering Journal 2025年 516卷

作者： Peixuan Lei Xudong Zhou Xiangxian Wu Hongjian Fu Hongpeng Li Haibo Huang Key Laboratory of Bio-Based Material Science and Technology (Ministry of Education) Northeast Forestry University Harbin 150040 PR China State Key Laboratory of Utilization of Woody Oil Resource Northeast Forestry University Harbin 150040 PR China School of Automotive Engineering Nantong Institute of Technology Nantong 226001 PR China College of Mechanical Engineering Yangzhou University Yangzhou 225127 PR China

Lithium-sulfur (Li-S) batteries are plagued by polysulfide shuttling and sluggish sulfur redox kinetics, while previously reported heterojunction-based cathodes often suffer from ill-defined interfaces, inadequate active sites, and insufficient mechanistic understanding of interfacial charge modulation. Herein, we report a bio-templated In 2 O 3 /In 2 S 3 @C heterojunction cathode engineered with a built-in electric field (BIEF) to address these challenges. The BIEF, arising from Fermi-level alignment between In 2 S 3 and In 2 O 3 , drives directional electron transfer, reducing polysulfide conversion barriers by 1.2 eV. The bacterial cellulose derived carbon framework synergizes strong lithium polysulfides chemisorption ( via In 2 O 3 oxygen vacancies), metallic conductivity ( via In 2 S 3 ), and mechanical resilience against sulfur volume expansion. The optimized cathode delivers a high initial capacity of 1325.5 mAh g −1 at 0.1 C and retains 753.1 mAh g −1 at 2 C with ultralow decay (0.074% per cycle over 200 cycles). Density functional theory calculations validate a record Li 2 S 6 binding energy (−3.08 eV) and BIEF-enhanced charge transfer kinetics. This work resolves critical heterojunction design challenges, offering a scalable bioinspired blueprint for high-energy–density batteries.

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Environmental load of solid wood floor production from larch grown at different planting densities based on a life cycle assessment

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Journal of Forestry Research 2018年第5期29卷 1443-1448页

作者： Siying Hu Xin Guan Minghui Guo Jinman Wang Key Laboratory of Bio-Based Material Science and Technology of the Ministry of Education Northeast Forestry University College of Material Engineering Fujian Agriculture and Forestry University

As one of the main structural units in a building,a solid wood floor has significant strategic research value for low-carbon energy *** the production line of a solid larch wood floor as a case study,we assessed the environmental load during production based upon a life cycle *** GaBi 6.0 software,we analyzed the associated carbon sequestration during floor production,with the initial planting density serving as the disturbance factor in a modular *** results indicated that the cutting and finishing steps have relatively intense,negative influences on the environment,whereas transportation,ripping,and trimming do ***,recycling biomass waste has the potential to reduce greenhouse gas *** the initial planting density was 3.0×3.0 m,carbon sequestration was relatively *** the emissions of freshwater pollutants,volatile organic compounds,and fine particulate matter（matter with a 2.5-μm diameter） were comparatively high,the reduction of greenhouse gas emissions was still excellent at this planting density.

关键词： Environmental effect Larch Life cycle assessment Planting density Solid wood floor

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Unraveling the Atomic-Level Vacancy Modulation in Cu9S5 for NIR-Driven Efficient Inhibition of Drug-Resistant Bacteria: key Role of Cu Vacancy Position

SSRN

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SSRN 2022年

作者： Sun, Jingyu Wen, Jinghong Mo, Shudi Wang, Jianling Zhang, Ze Yang, Yang Wang, Guichang Liu, Jiandang Yu, Qilin Liu, Mingyang Tianjin Key Laboratory of Environmental Remediation and Pollution Control College of Environmental Science and Engineering Nankai University Tianjin300350 China College of Chemistry and Chemical Engineering Liaocheng University Liaocheng252059 China Key Laboratory of Advanced Energy Materials Chemistry Ministry of Education The Tianjin key Lab and Molecule-based Material Chemistry College of Chemistry Nankai University Tianjin300071 China Anhui Hefei230026 China Key Laboratory of Molecular Microbiology and Technology Ministry of Education College of Life Sciences Nankai University Tianjin300071 China

Cu9S5 possesses high hole concentration and potential superior electrical conductivity as a novel p-type semiconductor, whose biological applications remain largely unexploited. Encouraged by our recent work that Cu9S5 has enzyme-like antibacterial activity in the absence of light, which may further enhance the near infrared (NIR) antibacterial performance. Moreover, vacancy engineering can modulate the electronic structure of the nanomaterials and thus optimize their photocatalytic antibacterial activities. Here, we designed two different atomic arrangements with same VCuSCu vacancies of Cu9S5 nanomaterials (CSC-4 and CSC-3) determined by positron annihilation lifetime spectroscopy (PALS). Aiming at CSC-4 and CSC-3 as a model system, for the first time, we investigated the key role of different copper (Cu) vacancies positions in vacancy engineering toward optimizing the photocatalytic antibacterial properties of the nanomaterials. Combined with the experimental and theoretical approach, CSC-3 exhibited stronger absorption of surface adsorbate, higher separation of photogenerated charge carriers, and lower reaction active energy than those of CSC-4, leading to the generation of abundant ·OH for attaining rapid drug-resistant bacteria killed and wound healed under NIR light irradiation. This work provided a novel insight for the effective inhibition of drug-resistant bacteria infection via vacancy engineering at the atomic-level modulation. © 2022, The Authors. All rights reserved.

关键词： Electronic structure

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Performance optimization of microbial electrolysis cell (MEC) for palm oil mill effluent (POME) wastewater treatment and sustainable bio-H2 production using response surface methodology (RSM)

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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 2022年第34期47卷 15464-15479页

作者： Chandrasekhar, Abudukeremu Kadier ab Junying Wang ab K. Wang, Junying Chandrasekhar, K. Abdeshahian, Peyman Islam, M. Amirul Ghanbari, Farshid Bajpai, Mukul Katoch, Surjit Singh Bhagawati, Prashant Basavaraj Li, Hui Kalil, Mohd Sahaid Hamid, Aidil Abdul Abu Hasan, Hassimi Ma, Peng-Cheng [a]Laboratory of Environmental Science and Technology The Xinjiang Technical Institute of Physics and Chemistry Key Laboratory of Functional Materials and Devices for Special Environments Chinese Academy of Sciences Urumqi 830011 China [b]Center of Material and Opto-electronic Research University of Chinese Academy of Sciences Beijing 100049 China [c]School of Civil and Environmental Engineering Yonsei University Seoul 03722 Republic of Korea [d]Department of Biotechnology Engineering School of Lorena University of São Paulo São Paulo 12602-810 Brazil [e]Laboratory for Quantum Semiconductors and Photon-based BioNanotechnology Department of Electrical and Computer Engineering Faculty of Engineering Université de Sherbrooke Sherbrooke Québec J1K 2R1 Canada [f]Research Center for Environmental Contaminants (RCEC) Abadan University of Medical Sciences Abadan Iran [g]Environmental Engineering Lab Civil Engineering Department National Institute of Technology Hamirpur Hamirpur Himachal Pradesh 177005 India [h]Faculty of Engineering Department of Civil Engineering Annasaheb Dange College of Engineering and Technology Ashta Maharashtra 416301 India [i]Department of Chemical and Process Engineering Faculty of Engineering and Built Environment National University of Malaysia (UKM) UKM Bangi 43600 Selangor Malaysia [j]School of Biosciences and Biotechnology Faculty of Science and Technology National University of Malaysia (UKM) UKM Bangi 43600 Selangor Malaysia [k]Research Centre for Sustainable Process Technology Faculty of Engineering and Built Environment National University of Malaysia (UKM) UKM Bangi 43600 Selangor Malaysia

Microbial electrolysis cells (MECs) are a new bio-electrochemical method for converting organic matter to hydrogen gas (H-2). Palm oil mill effluent (POME) is hazardous wastewater that is mostly formed during the crude oil extraction process in the palm oil industry. In the present study, POME was used in the MEC system for hydrogen generation as a feasible treatment technology. To enhance biohydrogen generation from POME in the MEC, an empirical model was generated using response surface methodology (RSM). A central composite design (CCD) was utilized to perform twenty experimental runs of MEC given three important variables, namely incubation temperature, initial pH, and influent dilution rate. Experimental results from CCD showed that an average value of 1.16 m(3) H-2/m(3) d for maximum hydrogen production rate (HPR) was produced. A second-order polynomial model was adjusted to the experimental results from CCD. The regression model showed that the quadratic term of all variables tested had a highly significant effect (P < 0.01) on maximum HPR as a defined response. The analysis of the empirical model revealed that the optimal conditions for maximum HPR were incubation temperature, initial pH, and influent dilution rate of 30.23 ?, 6.63, and 50.71%, respectively. Generated regression model predicted a maximum HPR of 1.1659 m(3) H-2/m(3) d could be generated under optimum conditions. Confirmation experimentation was conducted in the optimal conditions determined. Experimental results of the validation test showed that a maximum HPR of 1.1747 m(3) H-2/m(3) d was produced. (c) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

关键词： Microbial electrolysis cell (MEC) Hydrogen production Palm oil mill effluent (POME) Wastewater Optimization Response surface methodology (RSM)

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Effect of the atomic mass mismatch in nanopillars on surface localization

Thermal Advances

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Thermal Advances 2024年 1卷

作者： Zhuo Zhao Haobo Fan Yiyi Li Meng Yuan Daxin Liang Jian Zhang Key Laboratory of Bio-Based Material Science & Technology Ministry of Education Northeast Forestry University Harbin 150040 China Yangtze Delta Region Academy of Beijing Institute of Technology (Jiaxing) Jiaxing 314019 China School of Astronautics Harbin Institute of Technology Harbin 150001 China ChinaState Key Laboratory of Advanced Nuclear Energy Technology Nuclear Power Institute of China Chengdu 610213 China CNNC Key Laboratory of Nuclear Reactor Thermal and Hydraulic Engineering Nuclear Power Institute of China Chengdu 610213 China

In recent years, nanophononic metamaterials (NPMs) have attracted great interest from researchers. Theoretical calculations and experimental studies have revealed the mechanism of reducing thermal conductivity through localized resonant hybridization. In addition, researchers have studied the effects of nanopillar height, spacing, and atomic mass in nanopillars on surface localization. The atomic mass mismatch in nanopillars has important application in practice. Taking the silicon-based nanopillar structure as an example, this paper studies the effects of atomic mass mismatch in nanopillars on surface localization effect and heat flux. The results show that atomic mass mismatch in nanopillars can enhance the surface localization effect, and the greater the difference in atomic mass in nanopillars, the stronger the surface localization. Finally, the effect of atomic mass mismatch in nanopillars on heat flux was calculated by nonequilibrium molecular dynamics. The results of this study can provide useful guidance for the design of nanoscale heat flux regulation devices.

关键词： Crystalline silicon Phononic metamaterials Atomic mass mismatch Phonon localization Molecular dynamics

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Nanocellulose-Derived Hierarchical Carbon Framework-Supported P-Doped MoO2Nanoparticles for Optimizing Redox Kinetics in Lithium–Sulfur Batteries (Adv. Mater. 22/2025)

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Advanced materials 2025年第22期37卷

作者： Mengjiao Shi Xue Han Wen Qu Meihui Jiang Qing Li Feng Jiang Xiang Xu Shinsuke Ifuku Chunlei Zhang Chao Wang Junfeng Hu Liansheng Yang Yuanjun Lin Haipeng Yu Shouxin Liu Jian Li Yiqiang Wu Wenshuai Chen Key Laboratory of Bio-Based Material Science and Technology of the Ministry of Education Northeast Forestry University Harbin 150040 P. R. China Sustainable Functional Biomaterials Lab Department of Wood Science University of British Columbia Vancouver BC V6T 1Z4 Canada Key Lab of Smart Prevention and Mitigation of Civil Engineering Disasters of the Ministry of Industry and Information Technology and Key Lab of Structures Dynamic Behavior and Control of the Ministry of Education Harbin Institute of Technology Harbin 150090 P. R. China Research Institute for Sustainable Humanosphere Kyoto University Uji 611-0011 Japan College of Materials Science and Technology Central South University of Forestry and Technology Changsha 410004 P. R. China

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technology Roadmap for Flexible Sensors

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ACS NANO 2023年第6期17卷 5211-5295页

作者： Luo, Yifei Abidian, Mohammad Reza Ahn, Jong-Hyun Akinwande, Deji Andrews, Anne M. Antonietti, Markus Bao, Zhenan Berggren, Magnus Berkey, Christopher A. Bettinger, Christopher John Chen, Jun Chen, Peng Cheng, Wenlong Cheng, Xu Choi, Seon-Jin Chortos, Alex Dagdeviren, Canan Dauskardt, Reinhold H. Di, Chong-an Dickey, Michael D. Duan, Xiangfeng Facchetti, Antonio Fan, Zhiyong Fang, Yin Feng, Jianyou Feng, Xue Gao, Huajian Gao, Wei Gong, Xiwen Guo, Chuan Fei Guo, Xiaojun Hartel, Martin C. He, Zihan Ho, John S. Hu, Youfan Huang, Qiyao Huang, Yu Huo, Fengwei Hussain, Muhammad M. Javey, Ali Jeong, Unyong Jiang, Chen Jiang, Xingyu Kang, Jiheong Karnaushenko, Daniil Khademhosseini, Ali Kim, Dae-Hyeong Kim, Il-Doo Kireev, Dmitry Kong, Lingxuan Lee, Chengkuo Lee, Nae-Eung Lee, Pooi See Lee, Tae-Woo Li, Fengyu Li, Jinxing Liang, Cuiyuan Lim, Chwee Teck Lin, Yuanjing Lipomi, Darren J. Liu, Jia Liu, Kai Liu, Nan Liu, Ren Liu, Yuxin Liu, Yuxuan Liu, Zhiyuan Liu, Zhuangjian Loh, Xian Jun Lu, Nanshu Lv, Zhisheng Magdassi, Shlomo Malliaras, George G. Matsuhisa, Naoji Nathan, Arokia Niu, Simiao Pan, Jieming Pang, Changhyun Pei, Qibing Peng, Huisheng Qi, Dianpeng Ren, Huaying Rogers, John A. Rowe, Aaron Schmidt, Oliver G. Sekitani, Tsuyoshi Seo, Dae-Gyo Shen, Guozhen Sheng, Xing Shi, Qiongfeng Someya, Takao Song, Yanlin Stavrinidou, Eleni Su, Meng Sun, Xuemei Takei, Kuniharu Tao, Xiao-Ming Tee, Benjamin C. K. Thean, Aaron Voon-Yew Trung, Tran Quang Wan, Changjin Wang, Huiliang Wang, Joseph Wang, Ming Wang, Sihong Wang, Ting Wang, Zhong Lin Weiss, Paul S. Wen, Hanqi Xu, Sheng Xu, Tailin Yan, Hongping Yan, Xuzhou Yang, Hui Yang, Le Yang, Shuaijian Yin, Lan Yu, Cunjiang Yu, Guihua Yu, Jing Yu, Shu-Hong Yu, Xinge Zamburg, Evgeny Zhang, Haixia Zhang, Xiangyu Zhang, Xiaosheng Zhang, Xueji Zhang, Yihui Zhang, Yu Zhao, Siyuan Zhao, Xuanhe Zheng, Yuanjin Zheng, Yu-Qing Zheng, Zijian Zhou, Tao Zhu, Bowen Zhu, Ming Zhu, Rong Zhu, Yangzhi Zhu, Yong Zou, Guijin Chen, Xiaodong 08-03 Innovis Singapore 138634 Republic of Singapore Innovative Centre for Flexible Devices (iFLEX) School of Materials Science and Engineering Nanyang Technological University Singapore 639798 Singapore Department of Biomedical Engineering University of Houston Houston Texas 77024 United States School of Electrical and Electronic Engineering Yonsei University Seoul 03722 Republic of Korea Department of Electrical and Computer Engineering The University of Texas at Austin Austin Texas 78712 United States Microelectronics Research Center The University of Texas at Austin Austin Texas 78758 United States Department of Chemistry and Biochemistry California NanoSystems Institute and Department of Psychiatry and Biobehavioral Sciences Semel Institute for Neuroscience and Human Behavior and Hatos Center for Neuropharmacology University of California Los Angeles Los Angeles California 90095 United States Colloid Chemistry Department Max Planck Institute of Colloids and Interfaces 14476 Potsdam Germany Department of Chemical Engineering Stanford University Stanford California 94305 United States Laboratory of Organic Electronics Department of Science and Technology Campus Norrköping Linköping University 83 Linköping Sweden Wallenberg Initiative Materials Science for Sustainability (WISE) and Wallenberg Wood Science Center (WWSC) SE-100 44 Stockholm Sweden Department of Materials Science and Engineering Stanford University Stanford California 94301 United States Department of Biomedical Engineering and Department of Materials Science and Engineering Carnegie Mellon University Pittsburgh Pennsylvania 15213 United States Department of Bioengineering University of California Los Angeles Los Angeles California 90095 United States School of Chemistry Chemical Engineering and Biotechnology Nanyang Technological University Singapore 637457 Singapore Nanobionics Group Department of Chemical and Biological Engineering Monash University Clayton Australia 3800 Monash

Humans rely increasingly on sensors to address grand challenges and to improve quality of life in the era of digitalization and big data. For ubiquitous sensing, flexible sensors are developed to overcome the limitations of conventional rigid counterparts. Despite rapid advancement in bench-side research over the last decade, the market adoption of flexible sensors remains limited. To ease and to expedite their deployment, here, we identify bottlenecks hindering the maturation of flexible sensors and propose promising solutions. We first analyze continued...challenges in achieving satisfactory sensing performance for real-world applications and then summarize issues in compatible sensor-biology interfaces, followed by brief discussions on powering and connecting sensor networks. Issues en route to commercialization and for sustainable growth of the sector are also analyzed, highlighting environmental concerns and emphasizing nontechnical issues such as business, regulatory, and ethical considerations. Additionally, we look at future intelligent flexible sensors. In proposing a comprehensive roadmap, we hope to steer research efforts towards common goals and to guide coordinated development strategies from disparate communities. Through such collaborative

关键词： soft materials mechanics engineering flexible electronics conformable sensors bioelectronics human-machine interfaces body area sensor networks technology translation sustainable electronics

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The properties of flax fiber reinforced wood flour/high density polyethylene composites

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Journal of Forestry Research 2018年第2期29卷 524-531页

作者： Jingfa Zhang Haigang Wang Rongxian Ou Qingwen Wang Key Laboratory of Bio-Based Material Science and Technology (Ministry of Education) Northeast Forestry University College of Materials and Energy South China Agricultural University

Flax fiber(FF) was used to reinforce wood flour/high density polyethylene composites(WF/PE).WF/PE particles were uniformly mixed with FF via high-speed mixing and then extruded with a single screw extruder to prepare FF reinforced WF/PE composites(FF/WF/PE).Mechanical testing,dynamic mechanical analysis,scanning electron microscopy(SEM),creep measurement and Torque rheology were used to characterize the resulting *** results indicate that the mechanical performance of the composites could be remarkably improved by adding a limited amount of *** flexural strength and modulus increased by 14.6 and 51.4%,respectively(FF content of 9 wt%),while the unnotched impact strength could be increased by 26.5%(FF content of12 wt%).The creep resistance and toughness of thecomposite was markedly improved without changing the plastic content of the composite material.

关键词： Wood-plastic composites Flax fiber Reinforcement Processing Mechanical property Creep resistance

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[email protected] @SnO 2-x sandwich structure with electrostatic repulsion effect and oxygen deficiency: enhanced photocatalytic hydrogen evolution activity and inhibited photo-corrosion

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Chemical Engineering Journal 2022年 434卷

作者： Xing Liu Tingting Zhang Yudong Li Jian Zhang Yunchen Du Yulin Yang Yanqiu Jiang Kaifeng Lin MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage School of Chemistry and Chemical Engineering Harbin Institute of Technology Harbin 150001 PR China Key Laboratory of Bio-based Material Science & Technology Ministry of Education Northeast Forestry University Harbin 150040 China

The activity and stability of photocatalysts are usually restricted to photo-corrosion issues. Here, an efficient electrostatic repulsion and anchor strategy via constructing a [email protected] @SnO 2-x sandwich structure with numerous oxygen vacancies through a simple chemical bath deposition approach. During the formation process, the CdS nanorods are wrapped by the catechol fragments from polydopamine (PDA) and display an electronegative surface. This strong electrostatic repulsion can effectively repel S 2- , thereby effectively preventing S 2- from being separated from CdS and being oxidized by holes or oxygen. Furthermore, the PDA employed as an interlayer of the heterojunction sandwich structure can fix the multivalent metal ions, such as Cd 2+ and Sn 4+ ions on CdS and SnO 2-x, which can be used as a bridge for electronic transmission. More importantly, the as-prepared SnO 2-x nanocrystals are found to possess a large amount of oxygen vacancies, which can effectively control the electronic structure of the catalyst, enhance the electron enrichment effect, promote the absorption of visible light and change the charge transfer ability. More importantly, the accumulation of [email protected] @SnO 2-x (411.37 mmol) photocatalytic hydrogen evolution is 34.3 times than pristine CdS (12.0 mmol) within 5 h, and the catalytic activity remains stable after 10 cycles. Photoelectrochemical characterization, Scanning Kelvin Probe (SKP), Finite Difference Time Domain (FDTD) simulations verified the mechanism of enhanced photocatalytic activity. Herein, this work displays a novel structure and mechanism to enhance the stability of sulfide semiconductors, which may further open a new path in the structural control strategy of photocatalysts.

关键词： Hydrogen evolution Oxygen vacancies Photocatalysis FDTD simulations Corrosion resistant

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