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Quantitatively investigating the self-attraction of nanowires

纳米研究（英文版） 2022年第4期15卷 3729-3736页

作者： Junfeng Cui Zhenyu Zhang Le Lv Kazuhito Nishimura Guoxin Chen Nan Jiang Key Laboratory for Precision and Non-Traditional Machining Technology of Ministry of Education Dalian University of TechnologyDalian 116024China Key Laboratory of Marine Materials and Related Technoloies Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China Key Laboratory for Precision and Non-Traditional Machining Technology of Ministry of Education Dalian University of TechnologyDalian 116024China Key Laboratory of Marine Materials and Related Technoloies Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China Advanced Nano-Processing Engineering Lab Mechanical EngineeringKogakuin UniversityTokyo 192-0015Japan

The self-attraction of nanowires(NWs)would lead to NWs bunching up together when fabricated in high density and the short circuit of NW-based devices during ***,the underlying mechanism of the self-attraction of NWs remains debatable due to the lack of in situ characterization of the *** this study,a versatile method of in situ investigating the self-attraction of NWs was *** attractive force between two NWs and their distance can be determined quantitatively in the process of attraction under an optical microscope,eliminating the influence of electron beam in electron *** this approach,the self-attraction of SiC NWs was investigated and a two-stage mechanism for the self-attraction was *** electrostatic force between two individual SiC NWs increased as their distance decreased,and acted as the initial driving force for the attraction of *** NWs remained in contact under van der Waals force until they separated when external force exceeded van der Waals *** charge density and the Hamaker constant of SiC NWs were determined to be 1.9×10-4 C·m-2 and 1.56×10-19 J,which played an important role in the attraction of *** results shed light on the mechanism of self-attraction among NWs and provide new insights into fabricating high-quality NWs and developing high-performance NW-based devices.

关键词： self-attraction nanowires in situ electrostatic force van der Waals force

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High-Throughput Production of Low-Cost Superhydrophobic and Oleophilic Mullite Fiber Sponges for High-Temperature Pm Filtration

SSRN

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SSRN 2024年

作者： Hu, Yuwen Zhu, Ruijian Zheng, Dazhi Liang, Shiou Wang, Zengmei School of Materials Science and Engineering Jiangsu Key lab. of Construction Materials Southeast University Nanjing211189 China School of Materials Science and Engineering Jiangsu Key Laboratory of Advanced Structural Materials and Application Technology Nanjing Institute of Technology Nanjing211167 China

Particulate matter (PM) from high-temperature emissions like chemical plants, coal stoves and vehicle exhausts poses a gravel challenge to human health. To address this issue, researchers have explored various fiber filters, yet the bulk struggle to withstand high temperatures. In this study, mullite fiber sponges were developed utilizing low-cost materials and Kármán vortex solution blow spinning. Optimized sponges demonstrate ultralight (18 mg cm−3), temperature-resistant reversible compressibility (50% strain) and a water contact angle of 135°. These sponges exhibited exceptional thermal insulation (thermal conductivity: 0.0269 W m−1 K−1) and performed well in high-temperature air filtration. At 800 °C, the mullite sponge with a base weight of 35 mg cm−2, achieved an average filtration efficiency of 98.18% and 99.57% for PM2.5 and PM2.5−10, respectively, with a quality value of 0.98 Pa-1 at a wind speed of 4 cm s−1. This low-cost mullite fiber sponge offers a promising avenue for designing high-performance filtration materials. © 2024, The Authors. All rights reserved.

关键词： Costs

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Solution-processed,flexible and broadband photodetector based on CsPbBr_(3)/PbSe quantum dot heterostructures

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Journal of materials Science & technology 2021年第9期68卷 216-226页

作者： Jinming Hu Shengyi Yang Zhenheng Zhang Hailong Li Chandrasekar Perumal Veeramalai Muhammad Sulaman Muhammad Imran Saleem Yi Tang Yurong Jiang Libin Tang Bingsuo Zou Beijing Key Laboratory of Nanophotonics and Ultrafine Optoelectronic Systems School of PhysicsBeijing Institute of TechnologyBeijing100081China Key Laboratory of Advanced Optoelectronic Quantum Design and Measurement.Ministry of Education Beijing Institute of Technology.Beijing100081China Kunming Institute of Physics Kunming650223China Beijing Key Laboratory for Precision Optoelectronic Measurement Instrument and Technology School of Optics and PhotonicsBeijing Institute of TechnologyBeijing100081China MOE Key Lab of New Processing Technology for Nonferrous Metals and Materials and Guangxi Key Lab of Processing for Nonferrous Metals and Featured Materials School of Physical Science and TechnologyGuangxi UniversityNanning530004China

Due to their promising applications in foldable displays,optical communication equipment and environmental monitoring systems,flexible and broadband optoelectronic devices have gained extensive attention in recent ***,a flexible and broadband photodetector based on CsPbBr_(3)/PbSe quantum dot(QD) heterostructures is firstly *** integrated QD heterostructures possess consecutive detection range from ultraviolet(UV) to long-wave length infrared(LW-IR) regions with efficient light absorption and chemical stability,in comparison with the pristine PbSe *** material characterizations reveal the improved exciton dissociation,carrier transport and carrier lifetime of the QD *** photodetector Ag/CsPbBr_(3)/PbSe/Ag demonstrate a high responsivity of 7.17 A/W with a specific detectivity of 8.97 × 10^(12) Jones under 25 μW/cm^(2) 365 nm illumination at 5 ***,it could maintain 91.2 %(or 94.9 %) of its initial performance even after bending for thousands of times(or exposing in ambient air for 4 weeks).More importantly,its re s ponse time is shortened more than three orders of magnitude as that of pristine PbSe QDs-based ***,it provides a feasible and promising method for the next-generation high-performance broadband photodetectors via constructing heterostructures of various QDs.

关键词： Quantum dots Broadband detection Flexible photodetectors Fast photoresponse speed Heterostructures

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Tris-based protic ionic liquids with multiple adsorption effects enabling excellent anti-wear and anti-corrosion performances

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Journal of Molecular Liquids 2025年 425卷

作者： Ge, Shanqin Chen, Long Li, Wei Cai, Qingzhao Gong, Genxiang Wu, Junhao Yu, Jinhong Nishimura, Kazuhito Jiang, Nan Cai, Tao School of Materials Science and Chemical Engineering Ningbo University Zhejiang Ningbo315211 China State Key Laboratory of Advanced Marine Materials Ningbo Institute of Materials Technology and Engineering Chinese Academy of Sciences Ningbo315201 China Advanced Nano-processing Engineering Lab Mechanical Engineering Kogakuin University Tokyo192-0015 Japan

Molecular additives have garnered widespread attention in the fields of lubrication and corrosion protection due to their designable interfacial film-forming efficiency. Herein, three protic ionic liquids (PILs) with the same cation but different anions have been designed and synthesized. Their physicochemical properties, tribological properties and anti-corrosion properties were systematically investigated. Results demonstrated that under dynamic steel-on-steel friction conditions, the PILs can maximally reduce the running-in period, friction coefficient, and wear rate by 90 %, 40 %, and 97 %, respectively, compared to the commercial ionic liquid, BMIMPF6. Under static copper corrosion conditions, the PILs efficiently adsorb onto the copper surface and formed a dense oxide layer on its surface, thus achieving excellent corrosion protection for the copper substrates. Molecular dynamics (MD) simulation results indicate that the exceptional lubricity of PILs is due to its ability to rapidly adsorb onto the metal surface through multiple interaction sites on both its anionic and cationic components, thereby reducing the running-in period and swiftly establishing a lubricating film. This study provides insights into the development of molecular additives featuring multiple adsorption sites, with potential applications in the fields of tribology and corrosion engineering. © 2025

关键词： Tribology

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ZnS nanolayer coated hollow carbon spheres with enhanced rate and cycling performance for Li-S batteries

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Science China(Technological Sciences) 2022年第2期65卷 272-281页

作者： MENG FanCheng XU Bin LONG Tao CHENG Sheng LI Yong ZHANG YongYi LIU JieHua School of Materials Science and Engineering Engineering Research Centre of High-Performance Copper Alloy Materials and ProcessingMinistry of EducationHefei University of TechnologyHefei 230009China Division of Nanomaterials and Jiangxi Key Lab of Carbonene Materials Suzhou Institute of Nano-Tech and Nano-BionicsNanchangChinese Academy of SciencesNanchang 330200China Instrumental Analysis Centre Hefei University of TechnologyHefei 230009China School of Instrument Science and Opto-electronics Engineering Hefei University of TechnologyHefei 230009China Key Laboratory of Multifunctional Nanomaterials and Smart Systems Advanced Materials DivisionSuzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China School of Nano-Tech and Nano-Bionics University of Science and Technology of ChinaHefei 230026China

Conductive carbon structure has been considered as a promising sulfur-hosting material as the cathode of lithium-sulfur ***, the issue of polysulfide shuttling requires an additional component to help restrict and convert sulfur ***, in this work, hollow and porous carbon nanospheres(HCS) are synthesized by a template method and a high-temperature carbonization treatment. A thin layer of ZnS coating is then deposited on the HCS-based sulfur(ZnS@HCS/S) cathode with controlled thickness, and the overall electrochemical properties are systematically evaluated. Results show that with 30 nm-thick ZnS coating, the cathode reveals an improved capacity of 1411 m A h g^(-1), and higher capacities from 0.2 to 3 C rate compared with bare HCS/S cathode. Moreover, the ZnS coating also enhances the cycling stability of ZnS@HCS/S cathode over 280 cycles at 0.5 C, with only 0.2% capacity decay per cycle. This work demonstrates potential applications for high-performance lithiumsulfur batteries.

关键词： lithium-sulfur battery ZnS nanolayer hollow carbon sphere rate performance cycling stability

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High-efficiency electrocatalytic NO reduction to NH_(3) by nanoporous VN

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Nano Research Energy 2022年第2期1卷 201-207页

作者： Defeng Qi Fang Lv Tianran Wei Mengmeng Jin Ge Meng Shusheng Zhang Qian Liu Wenxian Liu Dui Ma Mohamed SHamdy Jun Luo Xijun Liu MOE Key Laboratory of New Processing Technology for Non-Ferrous Metals and Materials and Guangxi Key Laboratory of Processing for Non-Ferrous Metals and Featured MaterialsSchool of ResourceEnvironments and MaterialsGuangxi UniversityNanning 530004China Institute for New Energy Materials and Low-Carbon Technologies Tianjin Key Lab for Photoelectric Materials&DevicesSchool of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China Key Laboratory of Carbon Materials of Zhejiang Province College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China College of Chemistry Zhengzhou UniversityZhengzhou 450000China Institute for Advanced Study Chengdu UniversityChengdu 610106China College of Materials Science and Engineering Zhejiang University of TechnologyHangzhou 310014China Catalysis Research Group(CRG) Department of ChemistryCollege of ScienceKing Khalid UniversityP.O.Box 900461413 AbhaSaudi Arabia

Electrocatalytic NO reduction reaction to generate NH_(3)under ambient conditions offers an attractive alternative to the energy-extensive Haber-Bosch route;however,the challenge still lies in the development of cost-effective and high-performance ***,nanoporous VN film is first designed as a highly selective and stable electrocatalyst for catalyzing reduction of NO to NH_(3)with a maximal Faradaic efficiency of 85%and a peak yield rate of 1.05×10^(-7)mol·cm^(-2)·s^(-1)(corresponding to 5,140.8mg·h^(-1)·mg_(cat).^(-1))at-0.6 V *** hydrogen electrode in acid ***,this catalyst maintains an excellent activity with negligible current density and NH_(3)yield rate decays over 40 ***,as a proof-of-concept of Zn-NO battery,it delivers a high power density of 2.0 mW·cm^(-2)and a large NH_(3)yield rate of 0.22×10^(-7)mol·cm^(-2)·s^(-1)(corresponding to 1,077.1mg·h^(-1)·mg_(cat).^(-1)),both of which are comparable to the best-reported *** analyses confirm that the VN surface favors the activation and hydrogenation of NO by suppressing the hydrogen *** work highlights that the electrochemical NO reduction is an eco-friendly and energy-efficient strategy to produce NH_(3).

关键词： NH_(3)electrosynthesis green route nanoporous VN NO reduction reaction high-performance

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Bio-based materials for sustainable energy harvesting: Applications in TENGs, PENGs, and solar-powered seawater desalination systems

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Chemical Engineering Journal 2025年 516卷

作者： Ding, Yutong Deng, Linbing Liu, Xiao-Xiao Wang, Lili Meng, Yanrong Ouyang, Mi Chen, Feng Huang, Zhao-Xia Kuang, Tairong Lab State Key Laboratory of Advanced Separation Membrane Materials Zhejiang Key Laboratory of Advanced Polymer Materials Modification and Application Technology College of Materials Science and Engineering Zhejiang University of Technology Hangzhou310014 China National Engineering Research Center of Novel Equipment for Polymer Processing Key Laboratory of Polymer Processing Engineering Ministry of Education Guangdong Provincial Key Laboratory of Technique and Equipment for Macromolecular Advanced Manufacturing Department of Mechanical and Automotive Engineering South China University of Technology Guangzhou510641 China School of Advanced Manufacturing Technology Guangdong Mechanical & Electrical Polytechnic Guangzhou510550 China Department of General Medicine First Medical Center of Chinese PLA General Hospital Beijing100039 China

The global energy crisis has intensified the need for sustainable energy solutions, yet conventional energy production still relies on non-renewable, environmentally damaging materials. Although significant advances have been made in green energy technologies, a critical gap remains in the development of materials that are both renewable and environmentally friendly. Bio-based materials, derived from renewable resources, offer a timely and sustainable alternative that can significantly improve the efficiency, functionality, and environmental compatibility of energy conversion devices. This review highlights the role of bio-based materials in addressing these challenges, focusing on their applications in emerging green energy technologies, particularly triboelectric nanogenerators (TENGs), piezoelectric nanogenerators (PENGs), and solar-powered seawater desalination systems. It provides a comprehensive overview of the latest advances in preparation methods, material properties, and their practical applications in energy conversion systems. By discussing the unique advantages and material selection challenges, this review underscores the importance of bio-based materials in the continued development of sustainable, high-performance energy harvesting devices. Furthermore, it emphasizes their potential to contribute to global sustainability goals, offering a critical pathway to more eco-friendly and cost-effective energy solutions. © 2025 Elsevier B.V.

关键词： Solar power generation

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Boosting carrier dynamics of BiVO_(4) photoanode via heterostructuring with ultrathin BiOI nanosheets for enhanced solar water splitting

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Journal of materials Science & technology 2021年第20期79卷 21-28页

作者： Can Li Fan Feng Jie Jian Youxun Xu Fan Li Hongqiang Wang Lichao Jia Key Laboratory of Applied Surface and Colloid Chemistry National Ministry of EducationShaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringShaanxi Normal University620 West Chang’an StreetXi’anShaanxi710119China State Key Laboratory of Solidification Processing Center for Nano Energy MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical University and Shaanxi Joint Labortary of GrapheneXi’an710072China

Bismuth vanadate(BiVO_(4))has been one of the most promising candidates for solar water splitting while still suffers from poor bulk charge transport that limits its solar to hydrogen conversion *** demonstrate in this work an efficient strategy for boosting bulk charge transport of BiVO_(4) through the facile impregnation of as-prepared BiVO_(4) photoanode in the precursor solution of ultrathin BiOI *** impregnation creates increased oxygen vacancies in the bulk of BiVO_(4) through the reduction of V^(5+)to V^(4+)by I^(-),which greatly improves bulk separation efficiency for BiVO_(4)-BiOI up to 65.9%at 1.23 V_(RHE) from the original 51.9%of pure BiVO_(4).Moreover,the decoration of the BiOI nanosheets on BiVO_(4) photoanode is also beneficial for addressing the carrier dynamics at surface due to the matched energy levels of BiOI nanosheets and BiVO_(4).The introduced plenty of oxygen vacancies in the bulk of BiVO_(4) and the built-in electric field in BiVO_(4)-BiOI synergistically improve the photocurrent density at 1.23 V_(RHE) up to 3.88 mA cm^(-2).We believe that such facile impregnation strategy will pave an alternative way to the development of highly efficient BiVO_(4) photoanode.

关键词： Bismuth vanadate BiOI nanosheets Heterojunction Solution impregnation Oxygen vacancy

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Single-atomic Mn sites coupled with Fe_(3)C nanoparticles encapsulated in carbon matrixes derived from bimetallic Mn/Fe polyphthalocyanine conjugated polymer networks for accelerating electrocatalytic oxygen reduction

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Nano Research 2022年第9期15卷 7976-7985页

作者： Yuan Pan Min Li Wanliang Mi Minmin Wang Junxi Li Yilin Zhao Xuelu Ma Bin Wang Wei Zhu Zhiming Cui Hailiang Yin Yunqi Liu State Key Laboratory of Heavy Oil Processing China University of Petroleum(East China)Qingdao 266580China Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) College of ChemistryNankai UniversityTianjin 300071China Research Institute of Petroleum Processing SinopecBeijing 100083China School of Chemical&Environmental Engineering China University of Mining&TechnologyBeijing 100083China School of Chemistry and Chemical Engineering Shaanxi Normal UniversityXi’an 710119China State Key Lab of Organic-Inorganic Composites Beijing University of Chemical TechnologyBeijing 100029China Key Laboratory of Fuel Cell Technology of Guangdong Province South China University of TechnologyGuangzhou 510641China Academy of Science&Technology China University of Petroleum(East China)Dongying 257061China

The construction of robust coupling catalysts for accelerating electrocatalytic oxygen reduction reaction(ORR)through the modulation of the electronic structure and local atomic configuration is critical but remains ***,we report a facile and effective isolation-polymerization-pyrolysis(IPP)strategy for high-precision synthesis of single-atomic Mn sites coupled with Fe_(3)C nanoparticles encapsulated in N-doped porous carbon matrixes(Mn SAs/Fe_(3)C NPs@NPC)catalyst derived from predesigned bimetallic Fe/Mn polyphthalocyanine(FeMn-BPPc)conjugated polymer networks by solid-phase reaction *** from the synergistic effects between the single-atomic Mn-N_(4)sites and Fe_(3)C NPs as well as the confinement effect of NPC,the Mn SAs/Fe_(3)C NPs@NPC catalyst exhibited excellent electrocatalytic activity and stability for *** assembled Znair battery displayed larger power density of 186 mW·cm^(−2)than that of Pt/C+Ir/C-based *** also exhibits excellent stability without obvious voltage change after 106 cycles with 36 *** in-situ Raman spectra with in-situ attenuated total reflectance surface-enhanced infrared absorption spectroscopy(ATR-SEIRAS)characterization results indicated that the Mn-N_(4)site as an active site for the O_(2)adsorption-activation process,which effectively facilitates the generation of key*OOH intermediates and*OH desorption to promote the multielectron reaction *** calculation reveals that the excellent electrocatalytic performance originates from the charge redistribution and the d orbital shift resulting from Mn-Fe bond,which buffers the activity of ORR through the electron reservoir capable of electron donation or *** work paves a novel IPP strategy for constructing high-performance coupling electrocatalyst towards the ORR for energy conversion devices.

关键词： single atom catalyst nanoparticles electrocatalyst oxygen reduction zinc-air battery

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New Insights into the Microstructure and Tribological Behaviors of the Boronized Layer on Inconel 718 Alloy Surface

SSRN

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SSRN 2024年

作者： Wu, Zhenjiang Chen, Shuqun Shao, Mengxue Liu, Yue Li, Yangzhong Peng, Jian Li, Hongyi Wang, Jinshu Key Laboratory of Advanced Functional Materials Education Ministry of China College of Materials and Engineering Beijing University of Technology Beijing100124 China Beijing University of Technology China High Performance Computing Department National Supercomputing Center in Shenzhen Guangdong Shenzhen518055 China State Key Lab of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China

Boronizing of nickel based superalloys is of great interests in aerospace industry due to the excellent wear resistance, however, little information has been known on its phase formation and load-dependent wear mechanism. In this work, high quality boronized layer was developed on the Inconel 718 alloy by powder pack-boriding process at 850 °C for 6 h under argon atmosphere. The microstructure characteristics and load-dependent tribological behaviors of the boronized layers were systematically investigate. It is found that the main boronized layer on Inconel 718 alloy consists of a ~11.3 um thick compound layer with nanocrystalline (Ni,Fe)23B6 and (Cr,Fe)B grains, and a ~10.9 um thick diffusion layer with dendritic Cr2B precipitation within the matrix. The phase evolution of the boronizing layer are explainable by thermodynamic modeling of Ni-Cr-B system and the phase stability for metastable Ni-B compounds is confirmed by DFT simulation. Due to the good interfacial bonding strength and high microhardness value, the boronized layer displays excellent wear resistance against Si3N4 ceramic balls at room temperature. In particular, the wear rates of the specimens under applied loads of 10-20 N are higher than those in the 50-100 N loads case. The latter is mainly facilitated by the formation of lubricating boron oxide tribolayer on friction ball surface. We believe the findings in present work will contribute to a deeper understanding of the boronizing treatment in nickel-based superalloys. © 2024, The Authors. All rights reserved.

关键词： Wear resistance

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