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Vortex tuning magnetization configurations in porous Fe_(3)O_(4) nanotube with wide microwave absorption frequency

Nano Research 2022年第7期15卷 6743-6750页

作者： Ruixuan Zhang Lei Wang Chunyang Xu Chongyun Liang Xianhu Liu Xuefeng Zhang Renchao Che Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsDepartment of Materials ScienceFudan UniversityShanghai 200438China Joint-Research Center for Computational Materials Zhejiang LaboratoryHangzhou 311100China Department of Chemistry Fudan UniversityShanghai 200433China School of Materials Science and Engineering Shanghai Institute of TechnologyShanghai 201418China Key Laboratory of Materials Processing and Mold Ministry of EducationZhengzhou UniversityZhengzhou 450002China Institute of Advanced Magnetic Materials College of Materials and Environmental EngineeringHangzhou Dianzi UniversityHangzhou 310012China

The design and optimization of one-dimension(1D)magnetic material are of great importance for the energy conversion,storage and spin electron devices,which remain a huge ***,1D porous Fe_(3)O_(4) nanotubes(NTs)have been fabricated via a combined process of electrospinning and *** the electrospinning precursors,by regulating the content ratio between two types of polyvinyl pyrrolidone with different molecular weight,porous Fe_(3)O_(4) NTs with vortex-domain configuration have been *** on the unique 1D nanotube structure encapsulated with multi-domains,the composite Fe_(3)O_(4) NTs exhibit high complex permeability(μʹ,μʺ)values,and hold both strong magnetic storage and dissipation *** Fe_(3)O_(4) NTs exhibit excellent microwave absorption(MA)performance with the maximum reflection loss value of−57.1 dB and the efficient absorption bandwidth of 12.0 *** generated magnetic vortices make the crucial contribution to the spin-wave resonance which improves the MA dissipation under *** magnetic flux line distribution and magnetic domain moment were confirmed by the electron holography and micro-magnetic simulation,respectively,providing the deep insight to the microwave absorption mechanism.

关键词： microwave absorption vortex domain one-dimensional structure porous structure

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Machine learning in energy storage materials

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Interdisciplinary materials 2022年第2期1卷 175-195页

作者： Zhong-Hui Shen Han-Xing Liu Yang Shen Jia-Mian Hu Long-Qing Chen Ce-Wen Nan State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Center of Smart Materials and DevicesWuhan University of TechnologyWuhanChina International School of Materials Science and Engineering Wuhan University of TechnologyWuhanChina State Key Lab of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijingChina Department of Materials Science and Engineering University of Wisconsin-MadisonMadisonWisconsinUSA Department of Materials Science and Engineering The Pennsylvania State UniversityUniversity ParkPennsylvaniaUSA

With its extremely strong capability of data analysis,machine learning has shown versatile potential in the revolution of the materials research ***,taking dielectric capacitors and lithium‐ion batteries as two representa-tive examples,we review substantial advances of machine learning in the research and development of energy storage ***,a thorough discussion of the machine learning framework in materials science is ***,we summarize the applications of machine learning from three aspects,including discovering and designing novel materials,enriching theoretical simulations,and assisting experimentation and ***,a brief outlook is highlighted to spark more insights on the innovative implementation of machine learning in materials science.

关键词： dielectric capacitor energy storage lithiumion battery machine learning

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Novel Cellulosic Fiber Composites with Integrated Multi-Band Electromagnetic Interference Shielding and Energy Storage Functionalities

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Nano-Micro Letters 2025年第5期17卷 508-524页

作者： Xuewen Han Cheng Hao Yukang Peng Han Yu Tao Zhang Haonan Zhang Kaiwen Chen Heyu Chen Zhenxing Wang Ning Yan Junwen Pu Beijing Key Laboratory of Lignocellulosic Chemistry College of Materials Science and TechnologyBeijing Forestry UniversityBeijing 100083People’s Republic of China Department of Chemical Engineering and Applied Chemistry University of TorontoTorontoON M5S3E5Canada Key Laboratory of Advanced Marine Materials Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201People’s Republic of China College of Mechanical and Electronic Engineering Northwest A&F UniversityYangling 712100ShaanxiPeople’s Republic of China Jiangsu Provincial Key Lab of Sustainable Pulp and Paper Technology and Biomass Materials Nanjing Forestry UniversityNanjing 210037People’s Republic of China Co-Innovation Center of Efficient Processing and Utilization of Forest Resources Nanjing Forestry UniversityNanjing 210037People’s Republic of China

In an era where technological advancement and sustainability converge,developing renewable materials with multifunctional integration is increasingly in *** study filled a crucial gap by integrating energy storage,multi-band electromagnetic interference(EMI)shielding,and structural design into bio-based ***,conductive polymer layers were formed within the 2,2,6,6-tetramethylpiperidine-1-oxide(TEMPO)-oxidized cellulose fiber skeleton,where a mild TEMPO-mediated oxidation system was applied to endow it with abundant macropores that could be utilized as active sites(specific surface area of 105.6 m2 g-1).Benefiting from the special hierarchical porous structure of the material,the constructed cellulose fiber-derived composites can realize high areal-specific capacitance of 12.44 F cm^(-2)at 5 m A cm^(-2)and areal energy density of 3.99 m Wh cm^(-2)(2005 m W cm^(-2))with an excellent stability of maintaining 90.23%after 10,000 cycles at 50 m A cm^(-2).Meanwhile,the composites showed a high electrical conductivity of 877.19 S m-1 and excellent EMI efficiency(>99.99%)in multiple wavelength *** composite material’s EMI values exceed 100 d B across the L,S,C,and X bands,effectively shielding electromagnetic waves in daily *** proposed strategy paves the way for utilizing bio-based materials in applications like energy storage and EMI shielding,contributing to a more sustainable future.

关键词： Cellulose fiber skeleton TEMPO mediated oxidation In-situ polymerization Multi-band EMI shielding Energy storage

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MoC nanocrystals confined in N-doped carbon nanosheets toward highly selective electrocatalytic nitric oxide reduction to ammonia

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Nano Research 2022年第10期15卷 8890-8896页

作者： Ge Meng Mengmeng Jin Tianran Wei Qian Liu Shusheng Zhang Xianyun Peng Jun Luo Xijun Liu Key Laboratory of Carbon Materials of Zhejiang Province College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China Institute for New Energy Materials and Low-Carbon Technologies Tianjin Key Lab for Photoelectric Materials&DevicesSchool of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China MOE Key Laboratory of New Processing Technology for Non-Ferrous Metals and Materials and Guangxi Key Laboratory of Processing for NonFerrous Metals and Featured MaterialsSchool of ResourceEnvironments and MaterialsGuangxi UniversityNanning 530004China Institute for Advanced Study Chengdu UniversityChengdu 610106China College of Chemistry Zhengzhou UniversityZhengzhou 450000China Institute of Zhejiang University–Quzhou Quzhou 324000China

Electrochemical nitric oxide reduction reaction(NORR)to produce ammonia(NH3)under ambient conditions is a promising alternative to the energy and carbon-intensive Haber–Bosch approach,but its performance is still ***,molybdenum carbides(MoC)nanocrystals confined by nitrogen-doped carbon nanosheets are first designed as an efficient and durable electrocatalyst for catalyzing the reduction of NO to NH3 with maximal Faradaic efficiency of 89%±2%and a yield rate of 1,350±15μg·h^(−1)·cm^(−2) at the applied potential of−0.8 V *** hydrogen electrode(RHE)as well as high stable activity with negligible current density and NH3 yield rate decays over a 30 h continue the ***,as a proof-of-concept of Zn–NO battery,it achieves a peak power density of 1.8 mW·cm^(−2) and a large NH3 yield rate of 782±10μg·h^(−1)·cm^(−2),which are comparable to the best-reported *** calculations reveal that the MoC(111)has a strong electronic interaction with NO molecules and thus lowering the energy barrier of the potential-determining step and suppressing hydrogen evolution *** work suggests that Mo-based materials are a powerful platform providing great opportunities to explore highly selective and active catalysts for NH3 production.

关键词： ammonia electrosynthesis green route molybdenum carbides(MoC)nanocrystals nitric oxide reduction reaction high selectivity

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IRSEnet: Differentially Private Image Generation with Multi-Scale Feature Extraction and Residual Channel Attention 13

IRSEnet: Differentially Private Image Generation with Multi-...

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13th International Conference on Intelligent Control and Information processing, ICICIP 2025

作者： Li, Jiahao Wang, Zhongshuai Ghazali, Kamarul Hawari Bin Yan, Suqing Lan, Rushi Sun, Xiyan Luo, Xiaonan Guangxi Key Lab. of Image and Graphic Intelligent Processing Guilin University of Electronic Technology Guilin541004 China Centre for Advanced Industrial Technology University of Malaysia Pahang Al-Sultan Abdullah Pahang Pekan26600 Malaysia Int. Joint Research Lab. of Spatio-temporal Information and Intelligent Location Services Guilin University of Electronic Technology Guilin541004 China

ISBN: (纸本)9798331516147

Privacy-preserving image generation is particularly crucial in fields like healthcare, where data are both sensitive and limited. However, effective privacy preservation often compromises the visual quality and utility of the generated images due to privacy budget constraints. To address this issue, in this paper, We propose a novel network architecture, IRSEnet, which combines multi-scale feature extraction technology and residual channel attention mechanisms, aiming to enhance the visual quality of generated images and improve the performance of downstream classification tasks under differential privacy. The differential privacy mechanism ensures the security of sensitive data during training, while the multi-scale feature extraction module enhances feature extraction capabilities through parallel convolutional layers at multiple scales. Additionally, the channel attention module dynamically adjusts channel weights to focus on the most discriminative features. Experimental results demonstrate that this model significantly improves the utility of generated images and the accuracy of downstream classification tasks while preserving privacy. Future work will explore the application of this approach on larger datasets and across more diverse tasks. © 2025 IEEE.

关键词： Differential privacy

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3D Positioning and Robot Assembly Method for Multi-plane Workpiece

3D Positioning and Robot Assembly Method for Multi-plane Wor...

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2023 IEEE International Conference on Real-Time Computing and Robotics, RCAR 2023

作者： Jia, Ruoyu Zhong, Kai Huang, Jintao Li, Xi Li, Ruifeng Luo, Hua Li, Zhongwei Huazhong University of Science and Technology State Key Lab. of Materials Processing and Die and Mould School of Materials Science and Engineering Wuhan430074 China Xi'an Saineng Aerospace Automation Technology Co. Ltd. Xi'an710100 China

ISBN: (纸本)9798350327182

Aiming at the assembly of workpieces with multiple plane structures, this paper proposes a 3D visual positioning and robot assembly method. First, several planes are extracted by plane detection and outlier removal algorithms;then the poses of the plane point clouds are calculated by the oriented bounding box algorithm;finally, the target plane is found through the length and width constraints. Based on proper hand-eye calibration and motion planning, the method can achieve the workpieces' recognizing, positioning and assembly accurately, meanwhile has high computational efficiency and strong robustness. As shown in the experiment results, for the recognition and positioning accuracy, the translation error of the proposed method is less than 0.2mm, and the rotation error is less than 0.2°;for the robot assembly accuracy, the translation error of the proposed method is less than 0.8mm and the rotation error is less than 0.4°. Therefore, the proposed method can successfully satisfy the requirement of robot assembly tasks. © 2023 IEEE.

关键词： Robots

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Multi-functional layered double hydroxides supported by nanoporous gold toward overall hydrazine splitting

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Frontiers of Chemical Science and Engineering 2024年第1期18卷 61-69页

作者： Yongji Qin Huijie Cao Qian Liu Shaoqing Yang Xincai Feng Hao Wang Meiling Lian Dongxing Zhang Hua Wang Jun Luo Xijun Liu ShenSi Lab Shenzhen Institute for Advanced StudyUniversity of Electronic Science and Technology of ChinaShenzhen 518110China Institute for New Energy Materials and Low-Carbon Technologies School of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures Guangxi Key Laboratory of Processing for Non-ferrous Metals and Featured MaterialsSchool of ResourcesEnvironment and MaterialsGuangxi UniversityNanning 530004China Institute for Advanced Study Chengdu UniversityChengdu 610106China China National Coal Group Corporation Beijing 100120China Tianjin Engineering Research Center of Civil Aviation Energy Environment and Green Development School of Transportation Science and EngineeringCivil Aviation University of ChinaTianjin 300300China

Layered double hydroxides have demonstrated great potential for the oxygen evolution reaction,which is a crucial half-reaction of overall water ***,it remains challenging to apply layered double hydroxides in other electrochemical reactions with high efficiency and ***,we report two-dimensional multifunctional layered double hydroxides derived from metalorganic framework sheet precursors supported by nanoporous gold with high porosity,which exhibit appealing performances toward oxygen/hydrogen evolution reactions,hydrazine oxidation reaction,and overall hydrazine *** as-prepared catalyst only requires an overpotential of 233 mV to reach 10 mA·cm^(-2) toward oxygen evolution *** overall hydrazine splitting cell only needs a cell voltage of 0.984 V to deliver 10 mA·cm^(-2),which is far more superior than that of the overall water splitting system(1.849 V).The appealing performances of the catalyst can be contributed to the synergistic effect between the metal components of the layered double hydroxides and the supporting effect of the nanoporous gold substrate,which could endow the sample with high surface area and excellent conductivity,resulting in superior activity and stability.

关键词： layered double hydroxide oxygen evolution reaction hydrazine oxidation reaction overall hydrazine splitting hydrogen production

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Enhancement of in-plane thermal conductivity of flexible boron nitride heat spreaders by micro/nanovoid filling using deformable liquid metal nanoparticles

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Rare Metals 2023年第11期42卷 3662-3672页

作者： Pei-Di Tao Shao-Gang Wang Lu Chen Jun-Feng Ying Le Lv Li-Wen Sun Wu-Bo Chu Kazuhito Nishimura Li Fu Yue-Zhong Wang Jin-Hong Yu Nan Jiang Wen Dai Yao-Kang Lv Cheng-Te Lin Qing-Wei Yan College of Chemical Engineering Zhejiang University of TechnologyHangzhou310058China Qianwan Institute Ningbo Institute of Materials Technology and Engineering(NIMTE)Chinese Academy of SciencesNingbo315201China Key Laboratory of Marine Materials and Related Technologies Zhejiang Key Laboratory of Marine Materials and Protective TechnologiesNingboInstitute of Materials Technology and Engineering(NIMTE)Chinese Academy of SciencesNingbo315201China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang110016China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing100049China Advanced Nano-Processing Engineering Lab Mechanical Systems EngineeringKogakuin UniversityTokyo192-0015Japan College of Materials and Environmental Engineering Hangzhou Dianzi UniversityHangzhou310018China

With the fast development of integrated circuit devices as well as batteries with high energy densities,the thermal management of electronic components is becoming increasingly crucial to maintaining their reliable *** nitride nanosheets(BNNS),which have superhigh thermal conductivity along the in-plane direction while remaining electrically insulating,were widely regarded as an ideal filler for preparing high-performance polymer composites to address the‘‘thermal failure''***,due to the instinctive rigidity of BNNS,the nanosheets are unable to form a tightly interfacial contact between the adjoining fillers,resulting in some micro-and nanovoids within the heat transfer pathways and severely limiting further thermal conductivity enhancement for BNNS-based ***,soft and deformable liquid metal(eutectic gallium-indium,EGaIn)nanoparticles were employed to fill the gaps between the adjacent BNNS with a rational design of mass ratios of BNNS and EGaIn,leading to a strongly synergistic effect with BNNS on thermal conductivity *** a result,the composite film(BNNS:63 wt%and EGaIn:7 wt%)employing cellulose nanofibers(CNF:30 wt%)as the polymer matrix achieves superhigh thermal conductivity along the in-plane direction of up to(90.51±6.71)W·m^(-1)·K^(-1),showing the highest value among the BNNSbased composites with a bi-filler system as far as we ***,the film can work as a heat spreader for the heat dissipation of high-power light emitting diodes,outperforming tin foil in cooling efficiency.

关键词： Boron nitride nanosheet Liquid metal Eutectic gallium-indium In-plane thermal conductivity Heat spreader

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Preparation of meter-scale Cu foils with decimeter grains and the use for the synthesis of graphene films

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Journal of Materiomics 2024年第1期10卷 1-6页

作者： Ruitao Jia Fangzhu Qing Shurong Wang Yuting Hou Changqing Shen Feng Hao Yang Yang Hongwei Zhu Xuesong Li School of Integrated Circuit Science and Engineering(Exemplary School of Microelectronics) University of Electronic Science and Technology of ChinaChengdu610054China State Key Laboratory of Electronic Thin Films and Integrated Devices University of Electronic Science and Technology of ChinaChengdu610054China Shenzhen Institute for Advanced Study University of Electronic Science and Technology of ChinaShenzhen518110China School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu610054China PipeChina Southwest Pipeline Co. Ltd.Chengdu610041China State Key Lab of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing100084China

Chemical vapor deposition(CVD)is the most promising method for the preparation of high-quality and large-area graphene films,especially the epitaxial growth of graphene on large-area single-crystal Cu *** single-crystal Cu foils are normally achieved by thermally annealing the commercial poly-crystalline Cu foils,their size and therefore the size of graphene films grown on them are limited to the size of the reaction *** report a simple and feasible method to prepare large-area Cu foils with decimeter grains by thermally annealing the rolled-up Cu foils,where the Cu layers are separated by thin porous carbon fiber *** carbon fiber cloths prevent Cu layers from sticking to each other at high temperatures while do not block the gas *** such a way,the utilization efficiency of the reaction chamber is significantly improved,e.g.,0.2 m×(1e2)m Cu foils can be processed even in a 5 cm diameter quartz tube ***-quality graphene films grown on such Cu foils are then *** method may be suitable for the annealing of other metal foils to enlarge grain size and the synthesis of other two-dimensional materials on them such as h-BN.

关键词： Graphene Single-crystal Cu Chemical vapor deposition Synthesis

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Growth of magnetic metals on carbon microspheres with synergetic dissipation abilities to broaden microwave absorption

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Journal of materials Science & technology 2022年第12期107卷 100-110页

作者： Biao Zhao Yang Li Qingwen Zeng Bingbing Fan Lei Wang Rui Zhang Renchao Che Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsFudan UniversityShanghai 200438China Department of Materials Science Fudan UniversityShanghai 200438China Henan Key Laboratory of Aeronautical Materials and Application Technology School of Material Science and EngineeringZhengzhou University of AeronauticsZhengzhouHenan 450046China School of Material Science and Engineering Zhengzhou UniversityZhengzhouHenan 450001China State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an 710072China

Microwave absorption(MA) materials have been captured extensive attentions due to the serious electromagnetic(EM) pollution. Numerous interests focus on the MA performances of core-shell structural composites with magnetic constituents as cores and dielectric constituents as shells, which inevitably suppressed the magnetic coupling causing the decrease of magnetic loss to some extent. Herein, the coreshell structural carbon(C) microsphere/magnetic metal composites were fabricated through the combination of an electrostatic assembly approach and subsequent in-situ reduction reaction. The complex permittivity and permeability of core-shell C@magnetic metal composite system can be effective adjusted by the constituent and microstructure of shells. Thanks to the distinct magnetic coupling from the subtle designed structures and the promotion of the magnetic-dielectric synergy, the C@magnetic metal composite exhibited enhanced MA properties. The optimal reflection loss(RL) of C@Ni composite was-54.1 dB with a thickness of 3.4 mm, meanwhile the effective absorbing band could reach over 5.5 GHz at only a1.8 mm thickness. Broad absorption bandwidth with RL below-10 d B could achieve 6.0 GHz and 6.7 GHz for C@Co and C@Ni Co composites with a thin 2.1 mm thickness, respectively. Our exciting findings might lead a guide on the novel structure design for the functional core-shell structural composites used for microwave absorption.

关键词： Microwave absorption Core-shell structure C@magnetic metal composite Interfacial polarization Magnetic coupling

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