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SSRN 2024年

作者： Tao, Youliang Nie, Zhongquan Zhang, Xuefeng Pan, Deng Wang, Han College of Aeronautics and Astronautics Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Institute of New Carbon Materials College of Materials Science and Engineering Taiyuan University of Technology Taiyuan030024 China Information Materials and Intelligent Sensing Laboratory of Anhui Province Anhui University 111 Jiu Long Road Hefei230601 China

Carbon-based nanomaterials with excellent electrical and optical properties are highly sought after for a plethora of hybrid applications ranging from advanced opto-electronic components to sustainable energy storage devices. In this contribution, we examine in detail the dependence of electrical conductivity and ultrafast optical nonlinearity of graphene oxide (GO) films on their degrees of reduction, as well as the link between the two properties. The GO films are first synthesized through the vacuum filtration method and then reduced partially controllab.y by the femtosecond laser direct writing with varying power doses. Subsequently, the 4-point probe measurements of the reduced GO (r-GO) films are demonstrated to exhibit superior resistivity and electrical conductivity compared with the pristine GO counterpart. It was found that the conductivity of the film increases and then decreases with increasing ablation laser power (P), GO was completely reduced at P = 100 mW with resistivity and electrical conductivity of 1.09 × 10-3Ω·m and 9.19 × 102s/m, respectively. GO was over reduced at P = 120 mW with resistivity and electrical conductivity being 3.72 × 10-3Ω·m and 2.69 × 102s/m, respectively. We further test the ultrafast optical nonlinearity (ONL) of the as-prepared pristine and reduced GO with the femtosecond Z-scan technique. The results show that the behavior of ONL is reversed whenever GO is reduced in a controlled manner. More interestingly, the higher the ablation laser power is, the stronger the optical nonlinearity of r-GO is. In particular, the nonlinear absorption and refraction coefficients of the r-GO films reach up to 3.26 × 10-8 m/W and -1.12 × 10-13 m2/W when P = 120 mW. The nonlinear absorption and refraction coefficients reach 1.9 × 10-8 m/W and -3 × 10-13 m2/W, respectively, for P = 70 mW. The GO/r-GO films endowing tunable electro-optical responses are potential building blocks for wide-ranging applications in microelectronic circuits, optoele

关键词： Femtosecond lasers

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controllab.e Electrical Characteristic of Ti3c2t2/Mos2 (T=Oh, F, O) Interfaces for High Performance Electronics: Insights from First-Principles

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SSRN 2023年

作者： Zhang, Qiang Liu, Yan Zhang, Riguang Lv, Bohan Hao, Runfang Sang, Shengbo Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Electronic Information and Optical Engineering Taiyuan University of Technology Shanxi Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System of The Ministry of Education Taiyuan University of Technology Shanxi Taiyuan030024 China School of Software Taiyuan University of Technology Shanxi Taiyuan030024 China State Key Laboratory of Clean and Efficient Coal Utilization China Laboratory of Aerospace Servo Actuation and Transmission Beijing Institute of Precision Mechatronics and Controls Beijing100000 China

Two-dimensional (2D) semiconductors have shown competitive potential for applications into beyond-silicon electronics. However, the controllab.e electrical characteristic of metal-semiconductor interfaces is still a challenge for high performance electronics due to Fermi level pinning. To explore Ti3C2T2/MoS2 (T= OH, F, O) for high performance electronics, the vertical electric field and interlayer distance are adopted here to regulate the electrical characteristic of interfaces based on the first-principles calculations. Though this, the electrical characteristic of Ti3C2O2/MoS2 and Ti3C2F2/MoS2 are more sensitive to electric field or interlayer distance than that of Ti3C2(OH)2/MoS2. Especially, the negative electric field with larger than -0.2 V/Å makes Ti3C2O2/MoS2 interface change from p-type Schottky to n-type Schottky contact. Furthermore, the Ti3C2O2/MoS2 interface can not only switch from p-type Schottky to n-type Schottky contact, but also from p-type Schottky to n-type Ohmic contact by varying interlayer distance. Moreover, the tunneling barriers of all interfaces are more sensitive to interlayer distance than to electric field. This work provides vital insights for high-performance electronics of Ti3C2T2/MoS2 (T=OH, F, O) in experiments. © 2023, The Authors. All rights reserved.

关键词： Electric fields

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Research on Highly Anti-Humidity and Selective NO2 Detection Based on GaN/MoO3 N-N Heterojunction

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SSRN 2024年

作者： Hong, Yutao Han, Dan Li, Donghui He, Xiuli Zhao, Li Wang, Weidong Li, Hongwei Sang, Shengbo Liang, Hua Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China State Key Laboratory of Transducer Technology Aerospace Information Research Institute Chinese Academy of Sciences Beijing100190 China Bioengineering Research Center Medical Innovation Research Division Chinese PLA General Hospital Beijing China Shanxi Academy of Medical Sciences China

Effective and accuratedetection of NO2 gas is crucial for protecting the environment and public health. In this work, balsam pear-like GaN/MoO3 porous nanosheets (GaN/MoO3) composites were synthesized by the in situ assembling, the hydrothermal method, and the nitridation process to detect NO2. A series of characterization methods were used to manifest the successful synthesis and to analyze the morphology and elemental composition features of GaN/MoO3 composites. The results of the gas-sensing experiments show that at the operating temperature of 225 °C, the gas sensor based on the optimal ratio of GaN/MoO3 composites exhibits a low theoretical limit of detection (0.78 ppb) for NO2, which is significantly improved compared with the limit of detection of MoO3 (5 ppm). Further, the response value of the sensor based on GaN/MoO3 composites to 200 ppm NO2 (44.74) is 4.36 times higher than that of the sensor based on pure GaN, with an improvement in stability. Meanwhile, the sensor also possessed excellent repeatability, selectivity, stability, and splendid anti-humidity ability at 15-70 % RH. The improved gas-sensing performance is ascribed to the unique microstructure of both GaN and MoO3, and the heterojunction effect between them. This work provides a way to improve the efficiency and anti-humidity ability of real-time monitoring of NO2 for the sensors of MoO3-based composite. © 2024, The Authors. All rights reserved.

关键词： Gallium nitride

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AU Nanoparticles Decorated Gan Nanoflowers with Enhanced Nh3 Sensing Performance at Room Temperature

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SSRN 2023年

作者： Han, Dan Chen, Yi Li, Donghui Shi, Jiexu Wang, Hongtao He, Xiuli Zhao, Li Wang, Weidong Sang, Shengbo Ji, Jianlong Shanxi Key Laboratory of Micro Nano Sensors and Artificial Intelligence Perception College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System The Ministry of Education Taiyuan University of Technology Taiyuan030024 China State Key Laboratory of Transducer Technology Aerospace Information Research Institute Chinese Academy of Sciences Beijing100190 China Bioengineering Research Center Medical Innovation Research Division Chinese PLA General Hospital Beijing China Shanxi Research Institute of 6D Artificial Intelligence Biomedical Science China

Surface modification with noble metal is considered as an effective strategy to enhance sensing performance of semiconductor gas sensors. In this work, gold nanoparticles (Au NPs) decorated Gallium Nitride nanoflowers (Au-GaN NFs) have been synthesized successfully by a feasible hydrothermal method combined with high temperature nitridation and followed by in-situ reduction process. The characterizations of the structure and morphology of as-obtained Au-GaN NFs indicated that the Au NPs were successfully loaded on the surface of GaN. The excellent gas sensing performance was observed for GaN of 2 mol% Au loaded, including the high response (86.8%) to 100 ppm NH3 with fast response/recovery time (41 s/169 s) at room temperature, low theoretical limit of detection (72 ppb), good stability and selectivity. Besides, the influence of humidity on the performance of sensors was explored, where the response can be reached 56.5% towards 100 ppm NH3 under 70% RH. The improvement of the sensing performance of Au-GaN NFs sensor can be attributed to the combined action of chemical and electronic sensitization of Au NPs. This work provides a candidate of Au-GaN NFs for the development of wireless sensing system in NH3 monitoring. © 2023, The Authors. All rights reserved.

关键词： Nanoflowers

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Self-Induced Backaction Optical Pulling Force

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Physical Review Letters 2018年第12期120卷 123901-123901页

作者： Tongtong Zhu Yongyin Cao Lin Wang Zhongquan Nie Tun Cao Fangkui Sun Zehui Jiang Manuel Nieto-Vesperinas Yongmin Liu Cheng-Wei Qiu Weiqiang Ding Department of Physics Harbin Institute of Technology Harbin 150001 China Department of Electrical and Computer Engineering National University of Singapore 4 Engineering Drive 3 Singapore 117583 Singapore Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan 030024 China Department of Biomedical Engineering Dalian University of Technology Dalian 116024 China Instituto de Ciencia de Materiales de Madrid Consejo Superior de Investigaciones Científicas Campus de Cantoblanco Madrid 28049 Spain Departments of Mechanical and Industrial Engineering and Electrical and Computer Engineering Northeastern University Boston Massachusetts 02115 USA

We achieve long-range and continuous optical pulling in a periodic photonic crystal background, which supports a unique Bloch mode with the self-collimation effect. Most interestingly, the pulling force reported here is mainly contributed by the intensity gradient force originating from the self-induced backaction of the object to the self-collimation mode. This force is sharply distinguished from the widely held conception of optical tractor beams based on the scattering force. Also, this pulling force is insensitive to the angle of incidence and can pull multiple objects simultaneously.

关键词： Electromagnetism Mechanical effects of light on material media Photonic crystals Optical microcavities Optical tweezers

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Gan/Moo3 N-N Heterojunction Based Anti-Humidity Gas Sensor for No2 Real-Time Monitoring

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SSRN 2024年

作者： Hong, Yutao Han, Dan Duan, Qi Li, Donghui He, Xiuli Li, Bing Liang, Hua Li, Hongwei Sang, Shengbo Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Integrated Circuits Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China State Key Laboratory of Transducer Technology Aerospace Information Research Institute Chinese Academy of Sciences Beijing100190 China Shanxi Province Key Laboratory of Oral Diseases Prevention and New Materials Shanxi Medical University School Hospital of Stomatology Shanxi Taiyuan030001 China Shanxi Province Cancer Hospital Shanxi Hospital Affiliated to Cancer Hospital Chinese Academy of Medical Sciences Cancer Hospital Affiliated to Shanxi Medical University Taiyuan030000 China University of Chicago United States

Effective and accurate detection of NO2 gas is crucial for protecting the environment and public health. In this work, balsam pear-like GaN/MoO3 porous nanosheets (GaN/MoO3) composites were synthesized by in situ assembling, the hydrothermal method, and the nitridation process to detect NO2. A series of characterization methods were used to manifest the successful synthesis and to analyze the morphology and elemental composition features of GaN/MoO3 composites. The results of the gas-sensing experiments show that, at the operating temperature of 225℃, the gas sensor based on the optimal ratio of GaN/MoO3 composites exhibits a 25-fold lower limit of detection for NO2 than that of MoO3, with a reduction of baseline resistance drift. Further, the response value of the sensor based on GaN/MoO3 composites to 200 ppm NO2 (44.74) is 4.36 times higher than that of the sensor based on pure GaN, with an improvement in stability. Meanwhile, the sensor possessed excellent repeatability, selectivity, stability, and splendid anti-humidity ability at 15-70% RH. The improved gas-sensing performance is ascribed to the unique microstructure of both GaN and MoO3 and the heterojunction effect between them. In addition, we constructed a real-time NO2 monitoring device based on the gas-sensing characteristic of GaN/MoO3, which realizes the alarm of excessive concentrations of NO2. Overall, this work provides a way to improve the ability of NO2 monitoring for the sensors of MoO3-based composites. © 2024, The Authors. All rights reserved.

关键词： III-V semiconductors

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Gan/Moo3 N-N Heterojunction Based Anti-Humidity Gas Sensor for No2 Real-Time Monitoring

SSRN

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SSRN 2024年

作者： Hong, Yutao Han, Dan Duan, Qi Li, Donghui He, Xiuli Li, Bing Liang, Hua Li, Hongwei Sang, Shengbo Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Integrated Circuits Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of Technology Taiyuan030024 China State Key Laboratory of Transducer Technology Aerospace Information Research Institute Chinese Academy of Sciences Beijing100190 China Shanxi Province Key Laboratory of Oral Diseases Prevention and New Materials Shanxi Medical University School and Hospital of Stomatology Shanxi Taiyuan030001 China Shanxi Province Cancer Hospital Shanxi Hospital Affiliated to Cancer Hospital Chinese Academy of Medical Sciences Cancer Hospital Affiliated to Shanxi Medical University Taiyuan030000 China University of Chicago United States

Effective and accurate detection of NO2 gas is crucial for protecting the environment and public health. In this work, balsam pear-like GaN/MoO3 porous nanosheets (GaN/MoO3) composites were synthesized by in situ assembling, the hydrothermal method, and the nitridation process to detect NO2. A series of characterization methods were used to manifest the successful synthesis and to analyze the morphology and elemental composition features of GaN/MoO3 composites. The results of the gas-sensing experiments show that, at the operating temperature of 225°C, the gas sensor based on the optimal ratio of GaN/MoO3 composites exhibits a 25-fold lower limit of detection for NO2 than that of MoO3, with a reduction of baseline resistance drift. Further, the response value of the sensor based on GaN/MoO3 composites to 200 ppm NO2 (44.74) is 4.36 times higher than that of the sensor based on pure GaN, with an improvement in stability. Meanwhile, the sensor possessed excellent repeatability, selectivity, stability, and splendid anti-humidity ability at 15-70% RH. The improved gas-sensing performance is ascribed to the unique microstructure of both GaN and MoO3 and the heterojunction effect between them. In addition, we constructed a real-time NO2 monitoring device based on the gas-sensing characteristic of GaN/MoO3, which realizes the alarm of excessive concentrations of NO2. Overall, this work provides a way to improve the ability of NO2 monitoring for the sensors of MoO3-based composites. © 2024, The Authors. All rights reserved.

关键词： Gallium nitride

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Antitumor Effects of Cds-Ppix Adducts for Nuclear-Targeted Sonodynamic Therapy

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SSRN 2023年

作者： Xue, Juanjuan Jia, Muyue Sang, Shengbo Li, Huaqian Wang, Xiaojuan Guo, Li Duan, Qianqian Xi, Yanfeng Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Information and Computer Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China Shanxi Research Institute of 6D Artificial Intelligence Biomedical Science Taiyuan030024 China Department of Pathology Shanxi Cancer Hospital Shanxi Hospital Affiliated to CancerHospital Chinese Academy of Medical Sciences Cancer Hospital Affiliated to Shanxi Medical University Shanxi Taiyuan030013 China Shanxi Key Laboratory of Bone and Soft Tissue Injury Repair Department of Orthopaedics Second Hospital of Shanxi Medical University Taiyuan030001 China Department of Pathology Shanxi Tumor Hospital Taiyuan030013 China

To achieve high-efficiency treatment to diseases, accurate delivery of drugs with a carrier into the specific organelles is of great importance. The nucleus is the ultimate target for a large number of drugs and direct delivery of drugs into nucleus can greatly improve the therapeutic treatment. Whereas, in sonodynamic therapy (SDT), the fact that most drug delivery systems can only deliver drugs to the cytoplasm of the cells and cannot act directly on the nucleus. In this paper, nucleolus-targeted carbondots (CDs) are prepared. Also, the conjugate of CDs and PpIX is synthesized by amide cross-linking and then release singlet oxygen to kill cancer cells under ultrasound radiation. The resulting CDs-PpIX nanoparticles showed significant nuclear targeting properties, and greatly improved the efficiency of acoustic dynamics treatment, as the nucleus exhibited poor tolerance to reactive oxygen species (ROS) generated during acoustic dynamics treatment. In addition, ROS as an extracellular signal can activate the p38MAPK protein pathway, which is the main mechanism of ultrasound killing of cancer cells. Our results demonstrate the great potential of CDs-PpIX in targeting cell nuclei for acoustic dynamics treatment. © 2023, The Authors. All rights reserved.

关键词： Cancer cells

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Ultra-wideband terahertz absorber based on graphene modulation: retraction

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Applied optics 2021年第30期60卷 9379页

作者： Xiaogang Li Guang Feng Suben Lin Lyncwell Innovation Intelligent System (Zhejiang) Co. Ltd. Ocean Science and Technology Innovation Park No. 19 Binhai 3rd Road Wenzhou 325024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optelectronics Taiyuan University of Technology Taiyuan 030024 China

The referenced paper [Appl. Opt.60, 3170 (2021)APOPAI0003-693510.1364/AO.420143] has been retracted by the authors.

关键词： Finite difference time domain Graphene Microwaves Modulation Ultrawideband signals

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Semidiscrete optical vortex droplets in quasi-phase-matched photonic crystals

arXiv

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arXiv 2023年

作者： Xu, Xiaoxi Zhao, Feiyan Huang, Jiayao He, Hexiang Zhang, Li Chen, Zhaopin Nie, Zhongquan Malomed, Boris A. Li, Yongyao School of Physics and Optoelectronic Engineering Foshan University Foshan528000 China School of Electronic and Computer Engineering Peking University Shenzhen518055 China Physics Department Solid-State Institute Technion Haifa32000 Israel Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Department of Physical Electronics School of Electrical Engineering Faculty of Engineering Tel Aviv University Tel Aviv69978 Israel Instituto de Alta Investigación Universidad de Tarapacá Casilla 7D Arica Chile Guangdong-Hong Kong-Macao Joint Laboratory for Intelligent Micro-Nano Optoelectronic Technology Foshan University Foshan528000 China

A new scheme for producing semidiscrete self-trapped vortices ("swirling photon droplets") in photonic crystals with competing quadratic (χ(2)) and self-defocusing cubic (χ(3)) nonlinearities is proposed. The photonic crystal is designed with a striped structure, in the form of spatially periodic modulation of the χ(2) susceptibility, which is imposed by the quasi-phase-matching technique. Unlike previous realizations of semidiscrete optical modes in composite media, built as combinations of continuous and arrayed discrete waveguides, the semidiscrete vortex "droplets" are produced here in the fully continuous medium. This work reveals that the system supports two types of semidiscrete vortex droplets, viz., onsite- and intersite-centered ones, which feature, respectively, odd and even numbers of stripes, N. Stability areas for the states with different values of N are identified in the system's parameter space. Some stability areas overlap with each other, giving rise to the multistability of states with different N. The coexisting states are mutually degenerate, featuring equal values of the Hamiltonian and propagation constant. An experimental scheme to realize the droplets is outlined, suggesting new possibilities for the long-distance transmission of nontrivial vortex beams in nonlinear media. © 2023, CC BY.

关键词： Photonic crystals

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