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Hals-770 Interlayer Simultaneously Block Internal and External Degradation Paths of Perovskite for Stability and High Efficiency Perovskite Solar Cells

SSRN

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SSRN 2024年

作者： Hu, Lina Zhang, Chenxi Wu, Yukun Li, Shiqi Ren, Jingkun Hao, Yang Sun, Qinjun Wang, Yulin Hao, Yuying College of Electronic Information and Optical Engineering Key Lab of Advanced Transducers and Intelligent Control System Taiyuan University of Technology Taiyuan030024 China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan030000 China

Here, we proposed a feasible solution using bis(2,2,6,6-tetramethyl-4-piperidyl) sebacate (HALS-770) molecules as top protection layer of perovskite. The hindered amine groups of HALS-770 can form N-O· free radicals in oxygen environment and then react with superoxide (O2·-) to remove O2·- , hence improve the antioxidant ability of perovskite. Moreover, the water resistance of perovskite is improved by hydrophobic alkyl chains and hydrophilic groups adsorbing free water within perovskite, achieving double waterproof effect. HALS-770 not only suppress the external degradation path of perovskite but also block the channel of its internal degradation. The heterocyclic N atom and the carbonyl oxygen included in HALS-770 can coordinate with uncoordinated Pb2+ ions, block volatilization of organic cation and inhibit Ag+ and I- migration, thus improve thermal stability of perovskite and alleviate destruction of Ag electrode. As a result, the unencapsulated device maintains excellent stability over 95% of its initial efficiency after 30 days in ambient condition with about 25–50% humidity, and possesses remarkable continuous operation stability with projected T80 > 1400 h at maximum power point tracking in glove box, much higher than that the pristine device. Meanwhile, HALS-770 enable the achievement of efficiency of 21.89% , which is among the highest efficiencies for MAPbI3 based PSCs with p-i-n structure. Further, HALS-770 is used in FAMA-based devices with n-i-p structure, the efficiency of 23.03% and 20.73% are achieved for the devices with active area of 0.06 and 1.0 cm2, respectively. Also, HALS-770 devices show excellent stability. This work illustrates the key role of HALS-770 top interlayer in achieving high-performance photovoltaic devices. © 2024, The Authors. All rights reserved.

关键词： Perovskite

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Condition Monitoring of Railway Vehicle Suspension system Based on PCA-SVM Method

Condition Monitoring of Railway Vehicle Suspension System Ba...

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TEPEN International Workshop on Fault Diagnostics and Prognostics, TEPEN-IWFDP 2024

作者： Liu, Fulong Guo, Honglin Zhang, Xiaotao Chen, Wei Gu, Fengshou Tianjin Key Laboratory for Advanced Mechatronic System Design and Intelligent Control School of Mechanical Engineering Tianjin University of Technology Tianjin300384 China Tianjin300384 China Centre for Efficiency and Performance Engineering University of Huddersfield HuddersfieldHD1 3DH United Kingdom

ISBN: (纸本)9783031702341

The suspension system is critical to ensure the running safety and comfortability of railway vehicle. This paper employed conventional machine learning method of principal component analysis and support vector machine (PCA-SVM) to diagnose the damper fault, wheel surface fault, roller fault, damper fault coupled with wheel surface fault and damper fault coupled with wheel and roller surface faults. The effectiveness of this method was verified by data obtained from a 1/5th scaled roller rig. The results shown that the performance of PCA-SVM was acceptable for railway vehicle suspension system monitoring. © The Author(s), under exclusive license to Springer Nature Switzerland AG 2024.

关键词： Rollers (machine components)

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Real Time Surgical Instrument Object Detection Using YOLOv7 1

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6th EAI International Conference on Robotics and Networks, EAI ROSENET 2022

作者： Zheng, Laiwang Liu, Zhenzhong Tianjin Key Laboratory for Advanced Mechatronic System Design and Intelligent Control School of Mechanical Engineering Tianjin University of Technology Tianjin China National Demonstration Center for Experimental Mechanical and Electrical Engineering Education Tianjin University of Technology Tianjin China

ISBN: (数字)9783031338267

ISBN: (纸本)9783031338250

With the rapid development of minimally invasive surgery (MIS) in the medical field, surgical robot technology has developed rapidly. Human-machine combined assisted surgical technology has begun to bring good news to the majority of doctors and patients who need surgery. It has gradually become a common medical treatment. Minimally invasive surgery can overcome the shortcomings of traditional surgery. MIS has the advantages of less trauma, less impact on patients, faster recovery, less intraoperative blood loss, and so on. For surgical robots, surgical instruments are important execution components that have been widely concerned and studied in recent years. One of the core technologies of surgical robots is the detection of surgical equipment based on deep learning, which can effectively assist doctors to complete the surgery. Current surgical instrument detection methods need to be improved in real-time performance and accuracy. Therefore, this paper proposes a new real-time detection algorithm, which is based on the deep learning object detection system YOLOv7. The real dataset, which contained information on seven surgical instruments, was selected for training and validation. Experiments show that the method has good precision, recall rate, and mAP, which can be used to improve the ability of robot-assisted doctors to identify instruments during surgery. © 2023, The Author(s), under exclusive license to Springer Nature Switzerland AG.

关键词： Object recognition

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Slope-assisted Raman distributed optical fiber sensing

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Photonics Research 2022年第1期10卷 205-213页

作者： JIAN LI XINXIN ZHOU YANG XU LIJUN QIAO JIANZHONG ZHANG MINGJIANG ZHANG College of Physics and Optoelectronics Taiyuan University of TechnologyTaiyuan 030024China Key Laboratory of Advanced Transducers and Intelligent Control Systems(Ministry of Education and Shanxi Province) Taiyuan University of TechnologyTaiyuan 030024China

Raman distributed optical fiber sensing is required to achieve accurate temperature measurements in a micro-scale *** this study,we first analyze and demonstrate the pulse transmission feature in the temperature variation area and the superposition characteristics of Raman optical time-domain reflectometry(OTDR)signals by numerical *** equations of superimposed Raman anti-Stokes scattered signals at different stages are presented,providing a theoretical basis for the positioning and physical quantity demodulation of whole optical fiber systems based on the OTDR ***,we propose and experimentally demonstrate a slope-assisted sensing principle and scheme in a Raman distributed optical fiber *** the best our knowledge,this is the first experimental demonstration of Raman distributed optical fiber sensing in a centimeter-level spatial measurement region.

关键词： fiber optical OTDR

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An Approach for Predicting and Compensating the End Deformation of a Heavy Load Robot for Friction Stir Welding 16th

An Approach for Predicting and Compensating the End Deformat...

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16th International Federation of Theory of Machines and Mechanisms World Congress, IFToMM WC 2023

作者： Bai, Yujie Liu, Haitao Meng, Shaofei Ma, Yue Yue, Wei Li, Guangxi Xiao, Juliang Wang, Guofeng Ding, Yabin Key Laboratory of Mechanism Theory and Equipment Design of State Ministry of Education Tianjin University Tianjin300072 China Tianjin Key Laboratory for Advanced Mechatronic System Design and Intelligent Control School of Mechanical Engineering Tianjin University of Technology Tianjin300384 China Dongguan University of Technology Dongguan523808 China

ISBN: (纸本)9783031457043

Aiming at solving the problem of insufficient plunge depth by the deformation of friction stir welding robots, this paper presents a method for predicting and compensating for the end deformation of friction stir welding robots. Firstly, the numerical model of FSW is established using DEFORM-3D software, then the axial force on the welding tool is obtained. Subsequently, the robot stiffness model is established based on the screw theory to realize the prediction of robot deformation in the workspace. Finally, a deformation compensation method based on the mirror principle is proposed to realize the compensation of the welding trajectory. Taking the 10 mm AA6061 aluminium alloy FSW as an example, the compensation method proposed in this paper is verified by using computer simulation. The results show that the stiffness model established in this paper can accurately predict the end deformation of the robot. The maximum plunge depth deviation of the compensation method proposed in this paper is reduced by 95.17% compared with the uncompensated case, which proves the effectiveness of the proposed compensation method. © The Author(s), under exclusive license to Springer Nature Switzerland AG 2023.

关键词： Friction stir welding

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ESNet: Evolution and Succession Network for High-Resolution Salient Object Detection 41

ESNet: Evolution and Succession Network for High-Resolution ...

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41st International Conference on Machine Learning, ICML 2024

作者： Liu, Hongyu Cong, Runmin Li, Hua Xu, Qianqian Huang, Qingming Zhang, Wei Institute of Information Science Beijing Jiaotong University Beijing Key Laboratory of Advanced Information Science and Network Technology Beijing China School of Control Science and Engineering Shandong University Key Laboratory of Machine Intelligence and System Control Ministry of Education Jinan China School of Computer Science and Technology Hainan University Hainan China Key Laboratory of Intelligent Information Processing Institute of Computing Technology CAS Beijing China School of Computer Science and Technology University of Chinese Academy of Sciences Beijing China

Preserving details and avoiding high computational costs are the two main challenges for the High-Resolution Salient Object Detection (HRSOD) task. In this paper, we propose a two-stage HRSOD model from the perspective of evolution and succession, including an evolution stage with Low-resolution Location Model (LrLM) and a succession stage with High-resolution Refinement Model (HrRM). The evolution stage achieves detail-preserving salient objects localization on the low-resolution image through the evolution mechanisms on supervision and feature;the succession stage utilizes the shallow high-resolution features to complement and enhance the features inherited from the first stage in a lightweight manner and generate the final high-resolution saliency prediction. Besides, a new metric named Boundary-Detail-aware Mean Absolute Error (MAEBD) is designed to evaluate the ability to detect details in high-resolution scenes. Extensive experiments on five datasets demonstrate that our network achieves superior performance at real-time speed (49 FPS) compared to state-of-the-art methods. Our code is publicly available at: https://***/rmcong/ESNet_ICML24. Copyright 2024 by the author(s)

关键词： Miocene

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Temperature and strain sensitivities of surface and hybrid acoustic wave Brillouin scattering in optical microfibers

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Chinese Physics B 2022年第9期31卷 333-339页

作者： Yi Liu Yuanqi Gu Yu Ning Pengfei Chen Yao Yao Yajun You Wenjun He Xiujian Chou Taiyuan University of Technology Key Laboratory of Advanced Transducers and Intelligent Control SystemMinistry of Education and Shanxi ProvinceTaiyuan 030024China Taiyuan University of Technology Institute of Optoelectronic EngineeringCollege of Physics and OptoelectronicsTaiyuan 030024China Strong Digital Technology Co. Ltd.(Thinvent)Nanchang 410000China North University of China Key Laboratory of Instrumentation Science and Dynamic Measurement Ministry of EducationTaiyuan 030051China North University of China College of Mechatronics EngineeringTaiyuan 030051China North University of China Science and Technology on Electronic Test and Measurement LaboratorySchool of Instrument and ElectronicsTaiyuan 030051China

Temperature and strain sensitivities of surface acoustic wave(SAW)and hybrid acoustic wave(HAW)Brillouin scat-tering(BS)in 1μm-1.3μm diameter optical microfibers are *** contrast to stimulated Brillouin scattering(SBS)from bulk acoustic wave in standard optical fiber,SAW and HAW BS,due to SAWs and HAWs induced by the coupling of longitudinal and shear waves and propagating along the surface and core of microfiber respectively,facilitate innovative detection in optical microfibers *** highest temperature and strain sensitivities of the hybrid acoustic modes(HAMs)are 1.082 MHz/℃and 0.0289 MHz/με,respectively,which is suitable for microfiber sensing applica-tion of high temperature and strain ***,the temperature and strain sensitivities of the SAMs are less affected by fiber diameter changes,ranging from 0.05 MHz/℃/μm to 0.25 MHz/℃/μm and 1×10^(-4) MHz/με/μm to 5×10^(-4) MHz/με/μm,*** can be found that that SAW BS for temperature and strain sensing would put less stress on manufacturing constraints for optical ***,the simultaneous sensing of temperature and strain can be realized by SAW and HAW BS,with temperature and strain errors as low as 0.30℃-0.34℃and 14.47με-16.25με.

关键词： Brllouin scatering surface acoustic waves hybrid acoustic waves optical microfiber sensing

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Chlorine-Substituent Regulation in Dopant-Free Small-Molecule Hole-Transport Materials Improves the Effi ciency and Stability of Inverted Perovskite Solar Cells

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Transactions of Tianjin University 2024年第4期30卷 314-323页

作者： Xinyi Liu Xiaoye Zhang Zhanfeng Li Jinbo Chen Yanting Tian Baoyou Liu Changfeng Si Gang Yue Hua Dong Zhaoxin Wu Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi ProvinceTaiyuan University of TechnologyTaiyuan 030024China School of Electrical Engineering University of South ChinaHengyang 421001China College of Physics and Optoelectronics Taiyuan University of TechnologyTaiyuan 030024China Ningxia Hui Autonomous Region Screen Display Organic Materials Engineering Technology Research Center Ningxia Sinostar Display Material Co.Ltd.Yinchuan 750003China Organic Semiconductor Centre EaStCHEM School of ChemistryUniversity of St AndrewsFife KY169STUK Key Laboratory of Photonics Technology for Information School of Electronic and Information Engineering Xi’an Jiaotong UniversityXi’an 710049China

Although doped hole-transport materials(HTMs)off er an effi ciency benefi t for perovskite solar cells(PSCs),they inevi-tably diminish the ***,we describe the use of various chlorinated small molecules,specifi cally fl uorenone-triphenylamine(FO-TPA)-x-Cl[x=para,meta,and ortho(p,m,and o)],with diff erent chlorine-substituent positions,as dopant-free HTMs for *** chlorinated molecules feature a symmetrical donor-acceptor-donor structure and ideal intramolecular charge transfer properties,allowing for self-doping and the establishment of built-in potentials for improving charge *** effi cient hole-transfer interfaces are constructed between perovskites and these HTMs by strategi-cally modifying the chlorine ***,the chlorinated HTM-derived inverted PSCs exhibited superior effi ciencies and air ***,the dopant-free HTM FO-TPA-o-Cl not only attains a power conversion effi ciency of 20.82% but also demonstrates exceptional stability,retaining 93.8%of its initial effi ciency even after a 30-day aging test conducted under ambient air conditions in PSCs without *** fi ndings underscore the critical role of chlorine-substituent regulation in HTMs in ensuring the formation and maintenance of effi cient and stable PSCs.

关键词： Hole-transport materials Inverted perovskite solar cells Chlorinated small molecules Donor–acceptor–donor structure

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Experimental demonstration of a thermal-EM concentrator for enhancing EM signals and converging heat fluxes simultaneously

arXiv

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arXiv 2024年

作者： Chen,, Hanchuan Liu,, Yichao Sun,, Fei Sun, Qianhan Wu,, Xiaoxiao Sun, Ran Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Guangzhou510000 China

Simultaneously concentrating EM waves and heat fluxes to the same target region within an on-chip system carries substantial academic research importance and practical application value. Nevertheless, existing researches are primarily aimed at the design and experimentation of concentrators for individual EM waves or temperature fields. In this work, a thermal-EM concentrator, capable of simultaneously concentrating EM waves and heat fluxes, is designed using transformation optics/thermodynamics and fabricated with engineered EM-thermal metamaterials. The concentrating effects of the proposed thermal-EM concentrator on the thermal fluxes and EM waves are verified through numerical simulations and experimental measurements, respectively, which are in good agreement with each other. Both numerically simulated and experimentally measured results demonstrate the concentrating capability of the proposed thermal-EM concentrator, which can concentrate broadband TM-polarized EM waves ranging from 8-12 GHz and heat/cold flows to the same target region within an on-chip operating environment. The thermal-EM concentrator exhibits a thermal focusing efficiency close to 100% and more than three times enhancement of the magnetic field at the designed center frequency of 10 GHz. The proposed thermal-EM concentrator can be utilized for efficient cooling for the specified component and simultaneously enhancing the EM antenna's radiation/reception efficiency within an on-chip system. Copyright © 2024, The Authors. All rights reserved.

关键词： Heat flux

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0.75 Gbit/s high-speed classical key distribution with mode-shift keying chaos synchronization of Fabry–Perot lasers

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Light(Science & Applications) 2021年第9期10卷 1780-1788页

作者： Hua Gao Anbang Wang Longsheng Wang Zhiwei Jia Yuanyuan Guo Zhensen Gao Lianshan Yan Yuwen Qin Yuncai Wang Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi ProvinceTaiyuanChina College of Physics and Optoelectronics Taiyuan University of TechnologyTaiyuanChina School of Information Engineering Guangdong University of TechnologyGuangzhouChina Guangdong Provincial Key Laboratory of Photonics Information Technology GuangzhouChina Center for Information Photonics and Communications School of Information Science and TechnologySouthwest Jiaotong UniversityChengduChina

High-speed physical key distribution is diligently pursued for secure *** this paper,we propose and experimentally demonstrate a scheme of high-speed key distribution using mode-shift keying chaos synchronization between two multi-longitudinal-mode Fabry–Perot lasers commonly driven by a super-luminescent *** users dynamically select one of the longitudinal modes according to private control codes to achieve mode-shift keying chaos *** two remote chaotic light waveforms are quantized to generate two raw random bit streams,and then those bits corresponding to chaos synchronization are sifted as shared keys by comparing the control *** this method,the transition time,i.e.,the chaos synchronization recovery time is determined by the rising time of the control codes rather than the laser transition response time,so the key distribution rate is improved *** experiment achieved a 0.75-Gbit/s key distribution rate with a bit error rate of 3.8×10^(−3)over 160-km fiber transmission with dispersion *** entropy rate of the laser chaos is evaluated as 16 Gbit/s,which determines the ultimate final key rate together with the key generation *** is therefore believed that the method pays a way for Gbit/s physical key distribution.

关键词： Gbit/s synchronization chaos

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