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Enhancing crystal integrity and structural rigidity of CsPbBr_(3) nanoplatelets to achieve a narrow colorsaturated blue emission

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Light(Science & Applications) 2024年第5期13卷 985-997页

作者： Qianqian Huang Wenxu Yin Bo Gao Qingsen Zeng Dong Yao Hao Zhang Yinghe Zhao Weijia Zheng Jiaqi Zhang Xuyong Yang Xiaoyu Zhang Andrey L.Rogach Key Laboratory of Automobile Materials MOE School of Materials Science&Engineeringand Jilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsJilin UniversityChangchunChina. State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchunChina. State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhanHubeiChina. Department of Chemistry University of VictoriaVictoriaBCCanada. Key Laboratory of Advanced Display and System Applications of Ministry of Education Shanghai UniversityShanghaiChina. Department of Materials Science and Engineering and Centre for Functional Photonics(CFP)City University of Hong KongHong Kong S.A.RChina

Quantum-confined CsPbBr_(3) perovskites are promising blue emitters for ultra-high-definition displays,but their soft lattice caused by highly ionic nature has a limited ***,we endow CsPbBr_(3) nanoplatelets(NPLs)with atomic crystal-like structural rigidity through proper surface engineering,by using strongly bound N-dodecylbenzene sulfonic acid(DBSA).A stable,rigid crystal structure,as well as uniform,orderly-arranged surface of these NPLs is achieved by optimizing intermediate reaction stage,by switching from molecular clusters to mono-octahedra,while interaction with DBSA resulted in formation of a Cs_(x)O monolayer shell capping the NPL *** a result,both structural and optical stability of the CsPbBr3 NPLs is enhanced by strong covalent bonding of DBSA,which inhibits undesired phase transitions and decomposition of the perovskite phase potentially caused by ligand ***,rather small amount of DBSA ligands at the NPL surface results in a short inter-NPL spacing in their closely-packed films,which facilitates efficient charge injection and *** photoluminescence of the produced CsPbBr_(3) NPLs is bright(nearly unity emission quantum yield)and peaks at 457 nm with an extremely narrow bandwidth of 3.7 nm at 80 K,while the bandwidth of the electroluminescence(peaked at 460 nm)also reaches a record-narrow value of 15 nm at room *** value corresponds to the CIE coordinates of(0.141,0.062),which meets Rec.2020 standards for ultra-high-definition displays.

关键词： temperature stability narrow

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The Influence of Ball Milling Time and Sintering Temperature on the Structural and Capabilities of FeCoCrNiMn High-Entropy Alloy 9

The Influence of Ball Milling Time and Sintering Temperature...

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2023 9th International Conference on Applied materials and Manufacturing technology, ICAMMT 2023

作者： Ma, Yutian Wang, Zhenming Tang, Xingchang Cheng, Ganghu Liu, Yajun Chen, Kexuan Zhang, Zhijian Lu, Sujun Sun, Yuanjun Liu, Junzhao State Key Laboratory of Nickel and Cobalt Resources Comprehensive Utilization Jinchang737100 China State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals Lanzhou University of Technology Lanzhou730050 China

This study reports the fabrication of FeCoCrNiMn high-entropy alloy using high-purity powders of Fe, Co, Cr, Ni, and Mn through the processes of mechanical alloying (MA) and spark plasma sintering (SPS). We systematically investigated the effects of different ball milling times (10 h, 20 h, 30 h, 40 h, 50 h) and sintering temperatures (700°C, 800°C, 900°C, 1000°C, 1100°C) on the structure and capabilities of the alloy. The findings indicate that the atomic proportion of Fe:Co:Cr:Ni:Mn approach 1:1:1:1:1. The distribution of all elements is basically uniform, but the Cr element is slightly biased in the structure after 40 h ball milling. The voids in the structure are gradually decreasing as temperatures rise. The matrix structure is mainly composed of a white FCC matrix phase and a gray Cr-rich σ phase. The alloy structure is the densest. It has the highest density of 7.060 g/cm3, the highest compressive strength of 1480 MPa, and a plastic deformation of 13% when the SPS temperature reaches 1000°C. The FeCoCrNiMn high-entropy alloy is prepared by a ball milling time of 40 h, and spark plasma sintering of 1000°C has the best comprehensive properties. © Published under licence by IOP Publishing Ltd.

关键词： Spark plasma sintering

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Prediction of intrusive gas pores caused by resin burning in sand core for iron castings

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China Foundry 2025年第1期22卷 23-32页

作者： Ji-wu Wang Xiao-long Wang Yu-cheng Sun Yu-hang Huang Xiu-ming Chen Xiong-zhi Wu Na Li Jin-wu Kang Tao Jing Tian-you Huang Hai-liang Yu School of Mechanical Electronic and Control EngineeringBeijing Jiaotong UniversityBeijing 100044China Weichai Power Co. Ltd.Weifang 261061ShandongChina School of Mechanical Engineering Central South UniversityChangsha 41000China School of Materials Science and Engineering Key Laboratory for Advanced Materials Processing TechnologyTsinghua UniversityBeijing 100084China

In the production of castings,intrusive gas pore represents a kind of common defects which can lead to leakage in high gas-tightness requirement castings,such as cylinder blocks and cylinder heads for *** occurs due to the intrusion of gases generated during the resin burning of the sand core into castings during the casting ***,a gas generation and flow constitution model was established,in which the gas generation rate is a function of temperature and time,and the flow of gas is controlled by the gas release,conservation,and Darcy's *** heat transfer and gas flow during casting process was numerically *** dangerous point of cores is firstly identified by a virtual heat transfer method based on the similarity between heat transfer and gas flow in the sand *** gas pores in castings are predicted by the gas pressure,the viscosity and state of the melt for these dangerous *** distinct sand core structures were designed and used for the production of iron castings,and the simulated gas pore results were validated by the obtained castings.

关键词： gas pore numerical simulation iron casting sand core resin

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Self-Cooling Hollow Mold With Containing Water and Its Effect on Microstructure and Mechanical Properties 75

Self-Cooling Hollow Mold With Containing Water and Its Effec...

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75th World Foundry Congress, WFC 2024

作者： Xu, Jingying Kang, Jinwu Mao, Weimin School of Materials Science and Engineering University of Science and Technology Beijing Beijing100083 China School of Materials Science and Engineering Key Laboratory for Advanced Materials Processing Technology Tsinghua University Beijing100084 China

The solidification process of castings directly determines the intrinsic quality and performance of castings, so controlling the cooling process during solidification of castings can eliminate or reduce defects such as shrinkage and porosity, cracks, deformation, etc., and then improve the performance of castings. 3D printing sand mold technology provides more options for the production of complex and high-quality castings, and improves the flexibility and innovation of the design of the sand structure. In order to control the sequential solidification of the castings, a new process of self-cooling hollow mold with containing water is proposed. The hollow mold is of a multi-shell structure which can contain water in the gaps between shells. Thus, it is convenient than the water dipping method or the bottom water cooling chill plate method. After pouring the molten metal, cooling water is pumped into the gaps between the shell layers, and the water level of the cooling water can be controlled to rise gradually to drive the solidification front per request, so as to realize the forced cooling of the castings from bottom to top, i.e., sequential solidification. By the casting experiment of barrels of aluminum alloy A357, it was found that the water cooling of the multi-layer shell hollow sand mold accelerates the cooling rate of the castings, the cooling rate increased by approximately 190% compared to natural cooling. The tensile strength of castings is 160 MPa, representing an increase of 14.3%, and the microhardness is 72.3 HV, showing an increase of about 43.5%. © 2024 75th World Foundry Congress, WFC 2024. All rights reserved.

关键词： Aluminum castings

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Effectiveness Evaluation Study of Self-made Zinc Alloy Sacrificial Anode under Chloride Salt Erosion Environment

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Journal of Wuhan University of technology(materials Science) 2023年第1期38卷 222-230页

作者：南雪丽 JI Jianrui LI Rongyang CHEN Hao WANG Yi TANG Weibin School of Materials Science and Engineering Lanzhou University of TechnologyLanzhou 730050China State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals Lanzhou University of TechnologyLanzhou 730050China Gansu Province Transportation Planning Survey&Design Institute Co.Ltd.Lanzhou 730000China

To investigate the effectiveness of self-made zinc alloy sacrificial anode material for the protection of reinforcement in concrete under chlorine salt erosion environment,salt solution immersion corrosion and electromigration accelerated corrosion tests were used to evaluate the effectiveness of self-made zinc alloy anode with the help of relevant cathodic protection guidelines and evaluation criteria for the corrosion of reinforcement in *** results showed that the protection was effective because the potential of the zinc alloy anode protection steel bar in the salt solution satis?ed the“-780 mV(SCE)”validity *** self-corrosion potential(E_(corr))of the sacri?cial anode protection steel in concrete was greater than-276 mV,and the protective current density of the zinc alloy anode was 1-3μA·cm^(-2),which met the standards of EN12696-2000,further indicating that the self-made zinc alloy sacri?cial anode had a good protection combining with the polarization resistance and the appearance of the corroded surface of the steel in *** microscopic morphology of the corroded surface and the composition of the corrosion products indicates that the mortar of the self-made zinc alloy anode has a lower pH than the imported anodes,so the long-term protection of the selfmade zinc alloy sacri?cial anode needs to be further improved.

关键词： zinc alloy anode cathodic protection steel corrosion concrete polarization curve

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异价离子取代构建高离子电导率的插层结构

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Science Bulletin 2023年第11期68卷 1134-1142,M0004页

作者：孙宗栋梁嘉宁刘开朗冯昕吴宇赵英鹤梁麒吴劲松李会巧翟天佑 State Key Laboratory of Materials Processing and Die&Mould Technology and School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Nanostructure Research CenterWuhan University of TechnologyWuhan 430070China

在纳米尺度通道内的离子传输是纳米流体学领域研究的重点.二维(2D)材料的本征层状结构为流体离子提供了稳健的纳米传输通道.为实现流体离子在2D材料薄膜内的高效传输,本文开发了一种新颖的异价离子取代插层策略,通过化学气相输运法直接... 详细信息

在纳米尺度通道内的离子传输是纳米流体学领域研究的重点.二维(2D)材料的本征层状结构为流体离子提供了稳健的纳米传输通道.为实现流体离子在2D材料薄膜内的高效传输,本文开发了一种新颖的异价离子取代插层策略,通过化学气相输运法直接合成多种具有高离子电导结构的单晶.将块体单晶置入水中通过手动摇晃即可获得二维纳米片分散液,组装后的薄膜展现出高的锂离子电导率,优于目前多数关于2D材料薄膜水相锂离子电导率的报道.这种在合成过程中直接构筑离子传输结构的策略与目前已有的先剥离2D材料后对纳米片修饰改性的方法完全不同.因此,这种普适性的异价离子取代插层策略将会为更多高离子电导率的2D材料薄膜的开发提供借鉴与参考.

关键词：离子电导率离子取代纳米片离子传输纳米流体材料薄膜传输通道插层结构

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Chemical cross-linking and mechanically reinforced carbon network constructed by graphene boosts potassium ion storage

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Nano Research 2022年第10期15卷 9019-9025页

作者： Chenxu Wang Ruohan Yu Wen Luo Wencong Feng Yuanhao Shen Nuo Xu Liqiang Mai Department of Physics School of ScienceWuhan University of TechnologyWuhan 430070China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology430070 WuhanChina Nanostructure Research Centre(NRC) Wuhan University of TechnologyWuhan 430070China

Carbon-based electrodes of potassium-ion batteries are of great research interest ascribed to their low cost and environmentally friendly ***,traditional carbon materials usually exhibit weak mechanical properties and incomplete crosslinking,resulting in poor stability and electrochemical ***,we report a new strategy for modifying reduced graphene oxide into a uniform few-layer structure through a sol–gel method combined with acid etching *** obtained chemical cross-linking and mechanically reinforced carbon network constructed by graphene(CNCG)demonstrates excellent electrochemical and mechanical *** as a free-standing anode(~7 mg·cm^(−2))for potassium ion battery,the asachieved CNCG delivers a high reversible specific capacity of 317.7 mAh·g^(−1) at a current density of 50 mA·g^(−1) and admirable cycle stability(208.4 mAh·g^(−1) at 50 mA·g^(−1) after 500 cycles).The highly reversible structural stability and fully cross-linked properties during potassiation are revealed by ex-situ *** work provides new ideas for the synthesis of new carbon materials and the development of high-performance electrodes.

关键词： potassium-ion battery graphene electrode chemical cross-linking mechanical property storage mechanism

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Efficiently coupled glucose oxidation for high-value D-glucaric acid with ultradurable hydrogen via Mn(III)in acidic solution

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Nano Research 2023年第8期16卷 10748-10755页

作者： Junhua Li Yi Jiang Xu Zhang Yidan Huo Fanglin Du Yongxiao Tuo Zhiyan Guo Dawei Chen Shenghua Chen College of Material Science and Engineering Qingdao University of Science and TechnologyQingdao 266042China National Innovation Platform(Center)for Industry-Education Integration of Energy Storage Technology Xi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of Heavy Oil Processing College of New EnergyChina University of Petroleum(East China)Qingdao 266580China

The electrooxidation of the alcohol and aldehyde molecules instead of water coupled with H2 production has been proven to be effective for producing high-value fine chemicals under alkaline *** is also noteworthy that under acidic conditions,the stability of non-noble metal water oxidation catalysts remains a great challenge due to the lattice oxygen ***,we coupled the biomass-derived glucose oxidation for high-value D-glucaric acid(GRA)with ultra-durable hydrogen in acid solution over a Yb-MnO_(2)*** Mn^(3+)regulated by Yb atoms doped in MnO_(2)can effectively optimize the adsorption and desorption processes of the alcohol and aldehyde group and improve the intrinsic activity but cannot for *** catalyst exhibited extremely high activity and stability after 50 h for glucose oxidation,inhibiting the lattice oxygen process and MnO4−formation,while the activity was quickly lost within 0.5 h for water *** functional theory(DFT)calculations further demonstrated that glucose oxidation reaction proceeds preferentially due to the oxidation of aldehyde group with lower adsorption-free energy(−0.4 eV)than water(ΔG>0 eV),avoiding the lattice oxygen *** work suggests that biomass-derived glucose oxidation not only provides a cost-effective approach for high-value chemicals,but also shows an extremely potential as an alternative to acidic oxygen evolution reaction(OER)for ultradurable H2 production.

关键词： acidic water oxidation lattice oxygen mechanism(LOM) non-noble metal catalyst stability D-glucaric acid(GRA)

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NASICONs-type solid-state electrolytes:The history,physicochemical properties,and challenges

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Interdisciplinary materials 2023年第1期2卷 91-110页

作者： Lixiao Zhang Yimeng Liu Ya You Ajayan Vinu Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhanChina International School of Materials Science and Engineering Wuhan University of TechnologyWuhanChina Global Innovative Center for Advanced Nanomaterials(GICAN) School of EngineeringCollege of EngineeringScienceand the EnvironmentThe University of NewcastleCallaghanNew South Wales 2308Australia

Solid-state electrolytes are critical for the development of next-generation high-energy and high-safety rechargeable *** all the candidates,sodium(Na)superionic conductors(NASICONs)are highly promising because of their evident advantages in high ionic conductivity and high chemical/electrochemical *** concept of NASICONs was proposed by Hong and Goodenough et *** 1976 by reporting the synthesis and characterization of Na1+xZr2(SixP3−x)O12(0≤x≤3),which has attracted tremendous attention on the NASICONs-type solid-state *** this review,we are committed to describing the development history of NASICONs-type solid-state electrolytes and elucidating the contribution of Goodenough as a tribute to *** summarize the correlations and differences between lithium-based and sodium-based NASICONs electrolytes,such as their preparation methods,structures,ionic conductivities,and the mechanisms of ion *** challenges of NASICONs-structured electrolytes are discussed,and several research directions are proposed to tackle the obstacles toward practical applications.

关键词： electrode/electrolyte interface grain boundary resistance high ionic conductivity NASICONs solid-state electrolyte

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Ultrafast Laser-Induced Excellent Thermoelectric Performance of PEDOT:PSS Films

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Energy & Environmental materials 2024年第3期7卷 425-431页

作者： Xuewen Wang Yuzhe Feng Kaili Sun Nianyao Chai Bo Mai Sheng Li Xiangyu Chen Wenyu Zhao Qingjie Zhang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing International School of Materials Science and EngineeringWuhan University of TechnologyNo.122Luoshi Rd.Wuhan 430070China Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory No.1Yangming Rd.Foshan 528200China

Because poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate)(PEDOT:PSS)is water processable,thermally stable,and highly conductive,PEDOT:PSS and its composites have been considered to be one of the most promising flexible thermoelectric ***,the PEDOT:PSS film prepared from its commercial aqueous dispersion usually has very low conductivity,thus cannot be directly utilized for TE ***,a simple environmental friendly strategy via femtosecond laser irradiation without any chemical dopants and treatments was *** optimal conditions,the electrical conductivity of the treated film is increased to 803.1 S cm^(-1)from 1.2 S cm^(-1)around three order of magnitude higher,and the power factor is improved to 19.0μW m^(-1)K^(-2),which is enhanced more than 200 *** mechanism for such remarkable enhancement was attributed to the transition of the PEDOT chains from a coil to a linear or expanded coil conformation,reduction of the interplanar stacking distance,and the removal of insulating PSS with increasing the oxidation level of PEDOT,facilitating the charge *** work presents an effective route for fabricating high-performance flexible conductive polymer films and wearable thermoelectric devices.

关键词： electrical conductivity PEDOT:PSS thermoelectric film ultrafast laser irradiation

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