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High-strength aluminum alloys hollow billet prepared by two-phase zone continuous casting

China Foundry 2022年第3期19卷 253-262页

作者： Yao-hua Yang Xue-feng Liu Wang-zhang Chen Beijing Advanced Innovation Center for Materials Genome Engineering University of Science and Technology BeijingBeijing 100083China Beijing Laboratory of Metallic Materials and Processing for Modern Transportation University of Science and Technology BeijingBeijing 100083China Key Laboratory for Advanced Materials Processing of Ministry of Education University of Science and Technology BeijingBeijing 100083China Shunde Graduate School University of Science and Technology BeijingFoshan 528399GuangdongChina

The two-phase zone continuous casting(TZCC)technique was used to continuously cast high-strength aluminum alloy hollow billets,and a verified 3D model of TZCC was used to simulate the flow and temperature fields at casting speeds of 2-6 mm·min^(-1).Hollow billets under the same conditions were prepared,and their macro/microstructures were analyzed by an optical microscope and a scanning electron *** the TZCC process,a circular fluid flow appears in front of the mushy zone,and the induction heated stepped mold and convective heat transfer result in a curved solidification front with depressed region near the inner wall and a vertical temperature *** deflection of the solidification front decreases and the average cooling rate in the mushy zone increases with increasing casting *** results for a 2D12 alloy show that hot tearing periodically appears in the hollow billet accompanied by macrosegregation near the inner wall at casting speeds of 2 and 4 mm·min^(-1),while macroscopic defects of hot tearing and macrosegregation weaken and the average size of columnar crystals in the hollow billets decreases with further increasing casting speed.2D12 aluminum alloy hollow billets with no macroscopic defects,the finest columnar crystals,and excellent mechanical properties were prepared by TZCC at a casting speed of 6 mm·min^(-1),which is beneficial for the further plastic forming process.

关键词： two-phase zone continuous casting high-strength aluminum alloy hollow billet fluid flow heat transfer columnar crystals

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Wearable and interactive multicolored photochromic fiber display

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Light(Science & Applications) 2024年第3期13卷 454-465页

作者： Pan Li Yuwei Wang Xiaoxian He Yuyang Cui Jingyu Ouyang Ju Ouyang Zicheng He Jiayu Hu Xiaojuan Liu Hang Wei Yu Wang Xiaoling Lu Qian Ji Xinyuan Cai Li Liu Chong Hou Ning Zhou Shaowu Pan Xiangru Wang Huamin Zhou Cheng-Wei Qiu Yan-Qing Lu Guangming Tao State Key Laboratory of Material Processing and Die&Mould Technology School of Materials Science and Engineering and Wuhan National Laboratory for OptoelectronicsHuazhong University of Science and TechnologyWuhan 430074China Key Laboratory of Vascular Aging(HUST) Ministry of EducationWuhan 430030China School of Optoelectronic Science and Engineering University of Electronic Science and Technology of ChinaChengdu 611731China Department of Electrical and Computer Engineering National University of SingaporeSingapore 117583Singapore National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and ManipulationCollege of Engineering and Applied Sciencesand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210023China School of Performing Arts Wuhan Conservatory of MusicWuhan 430060China School of Mechanical Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China School of Architecture and Urban Planning Huazhong University of Science and TechnologyWuhan 430074China School of Fashion Beijing Institute of Fashion TechnologyBeijing 100029China School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074China Tongji Medical College Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai 201620China

Endowing flexible and adaptable fiber devices with light-emitting capabilities has the potential to revolutionize the current design philosophy of intelligent,wearable interactive ***,significant challenges remain in developing fiber devices when it comes to achieving uniform and customizable light effects while utilizing lightweight ***,we introduce a mass-produced,wearable,and interactive photochromic fiber that provides uniform multicolored light *** designed independent waveguides inside the fiber to maintain total internal reflection of light as it traverses the *** impact of excessive light leakage on the overall illuminance can be reduced by utilizing the saturable absorption effect of fluorescent materials to ensure light emission uniformity along the transmission *** addition,we coupled various fluorescent composite materials inside the fiber to achieve artificially controllable spectral radiation of multiple color systems in a single *** prepared fibers on mass-produced kilometer-long using the thermal drawing *** fibers can be directly integrated into daily wearable devices or clothing in various patterns and combined with other signal input components to control and display patterns as *** work provides a new perspective and inspiration to the existing field of fiber display interaction,paving the way for future human–machine integration.

关键词： fiber interactive colored

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Li3N film modified separator with homogenization effect of lithium ions for stable lithium metal battery

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Progress in Natural Science:materials International 2021年第6期31卷 845-851页

作者： Zhongyun Yan Cheng Zhou Cheng Li Yan Li Chunli Shen Kaijian Yan Xu Xu International School of Materials Science and Engineering State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology

Lithium metal anode with high theoretical capacity is considered to be one of the most potential anode materials of the next generation. However, the growth of lithium dendrite seriously affects the application of lithium metal anode and the development of lithium metal batteries（LMBs）. Herein, an ultrathin Li3N film modified separator to homogenize the lithium ions and protect the lithium metal anode was reported. Due to the intrinsic properties of Li3N, the functional separator possessed good thermal stability, mechanical properties and electrolyte wettability, and the homogenization of the lithium ion was realized without increasing the interface impedance. With this functional separator, the Li/Li symmetrical cell could achieve a long cycle with low overpotential for 1000 h at a current density of 1 m A cm-2. Furthermore, when the full battery was assembled with Li FePO4and the discharge capacity could be maintained at 151 m Ah g-1after 400 cycles at 1 C. In addition, the full battery also showed good rate performance, and provided a high discharge capacity of 114 m Ah g-1at 5 C.

关键词： Functional separator Solid electrolyte interface Physical vapor deposition Li metal anode

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Theoretical study of superradiant masing with solid-state spins at room temperature

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Science China(Physics,Mechanics & Astronomy) 2024年第6期67卷 38-47页

作者： Qilong Wu Yuan Zhang Hao Wu Shi-Lei Su Kai-Kai Liu Mark Oxborrow Chong-Xin Shan Klaus Mølmer Henan Key Laboratory of Diamond Optoelectronic Materials and Devices Key Laboratory of Material Physics Ministry of EducationSchool of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450052China Institute of Quantum Materials and Physics Henan Academy of SciencesZhengzhou 450046China Center for Quantum Technology Research and Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurements School of PhysicsBeijing Institute of TechnologyBeijing 100081China Beijing Academy of Quantum Information Sciences Beijing 100193China Department of Materials Imperial College LondonLondon SW72AZUK Niels Bohr Institute University of CopenhagenCopenhagen 2100Denmark

Steady-state superradiance and superradiant lasing attract significant attentions in the field of optical lattice clocks,but have not been achieved yet due to the technical challenges and atom loss *** this article,we propose that their counter-part may be observed in the microwave domain with solid-state spins,i.e.,nitrogen-vacancy center spins and pentacene molecular spins,coupled to microwave resonator at room temperature with realistic technical *** validate our proposal,we investigate systematically the system dynamics and steady-state by solving quantum master equations for the multi-level and multi-process dynamics of trillions of *** calculations show that the superradiant Rabi oscillations occur firstly due to transitions among different Dicke states,and the subsequent continuous-wave superradiant masing can achieve a linewidth well below *** work may guide further exploration of transient and steady-state superradiant masing with the mentioned and other solid-state spins *** ultra-narrow linewidth may find applications in deep-space communications,radio astronomy and high-precision metrology.

关键词： solid-state spins superradiance maser

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Research on temperature control system based on cheetah optimization fuzzy PID algorithm

Research on temperature control system based on cheetah opti...

引用

2024 China Automation Congress, CAC 2024

作者： Luo, Yuheng Hu, Wangyang Jin, Gang Xu, Qiang National Engineering Research Center of Novel Equipment for Polymer Processing Guangdong Provincial Key Laboratory of Technique and Equipment for Macromolecular Advanced Manufacturing South China University of Technology Guangzhou China Guangzhou Laboratory Guangzhou China

ISBN: (纸本)9798350368604

With the rapid development of industrial automation and intelligent control technology, temperature control systems have been deployed in many fields, such as process control, biomedical engineering and electric drives. However, the performance of traditional PID controllers is often far from acceptable when running in temperature control systems with high nonlinearity and complexity. To fix this problem, this paper first proposes a thermal network modeling and refinement method based on the Cauer model. Based on this model, this paper creates a fuzzy PID control method based on the Cheetah optimization algorithm to improve the robustness and response speed of the temperature control system. The simulation results show that the step response curve of the system with the CO-fuzzy PID controller reaches the stable state in 0.64 seconds, while the traditional PID controller takes 1.14 seconds. Moreover, the overshoot of the CO-fuzzy PID controller is far less than that of the traditional PID controller. Therefore, with such good dynamic and static characteristics, the CO-fuzzy PID controller in this paper is believed to have a wide range of applications and be particularly suitable for industrial areas requiring accurate temperature control. © 2024 IEEE.

关键词： Thermal variables control

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理论揭示锂硫电池第二放电平台的主要液固相转换机制

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Science China materials 2024年第8期67卷 2683-2693页

作者：张洪毅薛红涛魏承东孙杰许健汤富领 School of Materials Science and Engineering Lanzhou University of TechnologyLanzhou 730050China State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals Lanzhou University of TechnologyLanzhou 730050China

锂硫电池因其高理论能量密度、环境友好和低廉的成本而被认为是前景广阔的新型储能设备,但在放电后半程中缓慢的还原动力学严重阻碍其实际应用.虽然各种先进的正极材料改善了反应动力学,但硫还原反应(SRR)的复杂机理给提高锂硫电池性能... 详细信息

锂硫电池因其高理论能量密度、环境友好和低廉的成本而被认为是前景广阔的新型储能设备,但在放电后半程中缓慢的还原动力学严重阻碍其实际应用.虽然各种先进的正极材料改善了反应动力学,但硫还原反应(SRR)的复杂机理给提高锂硫电池性能设下许多障碍.深入研究其电催化机理是指导阴极材料设计和应用的重要环节.本文将揭示从Li_(2)S_(3);向Li_(2)_(S))(2)/Li_(2)_(S)的转化机制,即揭示从液相多硫化物到固相多硫化物的硫还原反应.以Ti、V、Fe、Co和Ni单原子催化剂为正极催化材料,建立基于密度泛函理论计算的电催化模型.中间产物^(*)LiS、^(*)LiS_(2)被用作预测反应路径、速率决定步骤和过电位的描述因子.这项工作解释了放电后期可溶多硫化物向不溶多硫化物的转化机理,为设计先进的高性能锂硫电池电催化剂提供了指导.

关键词：锂硫电池电催化剂阴极材料储能设备正极材料多硫化物电催化机理密度泛函理论计算

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Disordered Rocksalts with Lattice Oxygen Activation as Efficient Oxygen Evolution Electrocatalysts

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Transactions of Tianjin University 2023年第4期29卷 304-312页

作者： Zhengli Huan Haipeng Fu Xuerong Zheng Huiming Ji School of Materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin UniversityTianjin 300072China Key Laboratory of Electromagnetic Processing of Materials Ministry of EducationNortheastern UniversityShenyang 110819China State Key Laboratory of Marine Resource Utilization in South China Sea School of Materials Science and EngineeringHainan UniversityHaikou 570228China

The lattice oxygen oxidation mechanism(LOM)provides an efficient pathway for accelerating the oxygen evolution reaction(OER)in certain electrocatalysts by activating and involving lattice oxygen in the catalytic OER *** investigated the potential of disordered rocksalts as catalysts for accelerating the OER through the LOM process,leveraging their unique metastable Li-O-Li bond *** calculations were employed to predict the catalytic pathways and activities of disordered rocksalts(DRX),such as Li_(1.2)Co_(0.4)Ti_(0.5)O_(2)(LCTO).The results revealed that benefiting from the unhybridized Li-O electronic orbitals and the resulting metastable states of Li-O-Li bonds in DRX,LCTO exhibited a typical LOM pathway,and the lattice oxygen was easily activated and participated in the *** experimental results showed that LCTO exhibited a remarkable pH-dependent OER activity through the LOM pathway,with an overpotential of 241 mV at a current density of 10 mA/cm^(2),and excellent long-term *** work provides a novel chemical space for designing highly active and stable OER electrocatalysts by leveraging the LOM reaction pathway.

关键词： Lattice oxygen oxidation Disordered rocksalts Oxygen evolution reaction Electrocatalysts

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Fast preparation and thermoelectric performance of AgSTe based materials via plasma activated sintering

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materials Chemistry and Physics 2024年 323卷

作者： Melzi, Bachir Yang, Dongwang Zheng, Yu Zhang, Mingqi Jun, Li Cui, JingJing Jia, Yongzhong Pan, Zhicheng Zhong, Shenglong Yan, Yonggao State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China

AgSTe based materials have recently been identified as promising thermoelectric materials that have favorable properties at room temperature. They are usually obtained by conventional processes involving melting, annealing, and sintering, which incur significant energy and time expenditures. The present investigation involved the synthesis of Ag20S7Te3 compounds by a fast non-equilibrium methodology, i.e., plasma activated sintering from raw elemental powders. The monoclinic Ag20S7Te3 phase crystal was successfully formed at a temperature of 673 K, accompanied by the presence of a secondary monoclinic phase, Ag2S. The Ag20S7Te3 phase predominated in the monoclinic form, constituting a significant percentage at temperature of 873 K. Furthermore, the thermoelectric figure of merit (zT) of the AgSTe phase at 873 K was determined to be 0.42. The rapid sample synthesis described herein has the potential to significantly reduce the duration required for material synthesis, hence presenting a conspicuous advantage in the context of manufacturing on a wide scale. © 2024 Elsevier B.V.

关键词： Tellurium compounds

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Bi nanoparticles encapsulated in nitrogen-doped carbon as a long-life anode material for magnesium batteries

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Journal of Magnesium and Alloys 2023年第11期11卷 4181-4188页

作者： Junjun Wang Ruohan Yu Jianxiang Wang Juncai Long Fan Qiao Lei Zhang Guanjie He Qinyou An Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070China Christopher Ingold Laboratory Department of ChemistryUniversity College London20 Gordon StreetLondon WC1H 0AJUnited Kingdom of Great Britain and Northern IrelandUnited Kingdom Hubei Longzhong Laboratory Wuhan University of Technology(Xiangyang Demonstration Zone)Xiangyang 441000China

Bismuth has garnered significant interest as an anode material for magnesium batteries(MBs) because of its high volumetric specific capacity and low working potential. Nonetheless, the limited cycling performance(≤100 cycles) limits the practical application of Bi as anode for MBs. Therefore, the improvement of Bi cycling performance is of great significance to the development of MBs and is also full of challenges. Here, Bi nanoparticles encapsulated in nitrogen-doped carbon with single-atom Bi embedded(Bi@NC) are prepared and reported as an anode material for MBs. Bi@NC demonstrates impressive performance, with a high discharge capacity of 347.5 mAh g^(-1) and good rate capability(206.4 mAh g^(-1)@500 mA g^(-1)) in a fluoride alkyl magnesium salt electrolyte. In addition, Bi@NC exhibits exceptional long-term stability, enduring 400 cycles at 500 mA g^(-1). To the best of our knowledge, among reported Bi and Bi-based compounds for MBs, Bi@NC exhibits the longest cycle life in this work. The magnesium storage mechanism of Bi@NC is deeply studied through X-ray diffraction, transmission electron microscopy and X-ray photoelectron spectroscopy. This work provides some guidance for further improving the cycling performance of other alloy anodes in MBs.

关键词： Magnesium batteries Bismuth 3D tomography reconstruction Magnesium alloy Single-atom

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Electromagnetic Functions Modulation of Recycled By-Products by Heterodimensional Structure

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Nano-Micro Letters 2025年第6期17卷 264-278页

作者： Ze Nan Wei Wei Zhenhua Lin Ruimei Yuan Miao Zhang Jincheng Zhang Jianyong Ouyang Jingjing Chang Hejun Li Yue Hao State Key Laboratory of Wide-Bandgap Semiconductor Devices and Integrated Technology School of MicroelectronicsXidian UniversityXi’an 710071People’s Republic of China State Key Laboratory of Solidification Processing Shaanxi Province Key Laboratory of Fiber Reinforced Light Composite MaterialsCarbon/Carbon Composites Research CenterNorthwestern Polytechnical UniversityXi’an 710072People’s Republic of China Advanced Interdisciplinary Research Center for Flexible Electronics Xidian UniversityXi’an 710071People’s Republic of China Department of Materials Science and Engineering National University of Singapore7 Engineering Drive 1Singapore 117574Singapore

One of the significant technological challenges in safeguarding electronic devices pertains to the modulation of electromagnetic(EM)wave jamming and the recycling of defensive *** synergistic effect of heterodimensional materials can effectively enable the manipulation of EM waves by altering the *** we propose a novel approach for upcycling by-products of silver nanowires that can fabricate shape-tunable aerogels which enable the modulation of its interaction with microwaves by heterodimensional structure of ***-product heterodimensionality was used to design EM-wave-jamming-dissipation structures and therefore two typical tunable aerogel forms were *** first tunable form was aerogel film,which shielded EM interference(EMI shielding effectiveness(EMI SE)>89 dB)and the second tunable form was foam,which performed dual EM functions(SE>30 dB&reflective loss(RL)<-35 dB,effective absorption bandwidth(EAB)>6.7 GHz).We show that secondary recycled aerogels retain nearly all of their EM protection properties,making this type of closed-loop cycle an appealing *** findings pave the way for the development of adaptive EM functions with nanoscale regulation in a green and closed-loop cycle,and they shed light on the fundamental understanding of microwave interactions with heterodimensional structures.

关键词： Silver nanowires Electromagnetic shielding Microwave absorption Recycled aerogels

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