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Assembly of a core–shell MOF with stability into polyacrylamide hydrogel for boosting extraction of uranium from seawater

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Nano Research 2024年第4期17卷 3398-3406页

作者： Yucheng Song Huanhuan Tan Shiliang Qin Zhong Liu Chuntai Liu Changyu Shen Peipei Yang Songwei Li National Engineering Research Center for Advanced Polymer Processing Technology Key Laboratory of Materials Processing and Mold(Ministry of Education)Zhengzhou UniversityZhengzhou 450002China Key Laboratory of Comprehensive and Highly Efficient Utilization of Salt Lake Resources Qinghai Provincial Key Laboratory of Resources and Chemistry of Salt LakesQinghai Institute of Salt LakesChinese Academy of SciencesXining 810008China

Efficient and selective extraction of uranium(U(VI))from seawater is essential for sustainable nuclear power *** study reports a novel adsorbent zeolitic imidazolate framework(ZIF)-67@SiO_(2)-A/polyacrylamide(PAM)which was synthesized by grafting the core–shell metal–organic frameworks(MOFs)-based nanostructures coated with the 3-aminopropyl triethoxysilane(APTES)functionalized SiO_(2)(SiO_(2)-A)onto PAM *** SiO_(2) shell was grown on the surface of MOF,which improved the acid-base resistance of *** introduction of ZIF-67@SiO_(2)-A enhances the specific surface area and adsorption efficiency of the *** ZIF-67@SiO_(2)-A/PAM shows remarkable adsorption capacity,fast adsorption kinetics,and good reusability for *** has excellent adsorption property(6.33 mg·g^(-1),30 d)in natural *** X-ray photoelectron spectroscopy(XPS),Fourier transform infrared(FTIR),energy dispersive spectroscopy(EDS)mappings,and density functional theory reveal that the coordination by N and O in ZIF-67@SiO_(2)-A/PAM with uranium is the main mechanism of uranium ***,ZIF-67@SiO_(2)-A/PAM has great potential to capture uranium from natural seawater.

关键词： hydrogel metal–organic frameworks core–shelled nanostructures uranium extraction from seawater

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Regulating the electromagnetic balance of materials by electron transfer for enhanced electromagnetic wave absorption

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Journal of materials Science & technology 2024年第28期195卷 63-73页

作者： Kunyao Cao Weiping Ye Yue Zhang Lewei Shen Rui Zhao Weidong Xue Xiaoyu Yang School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 610054China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing&Shenzhen Research Institute&Joint Laboratory for Marine Advanced Materials Shenzhen 518063China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing and International School of Materials Science&Engineeringand School of Materials Science&EngineeringWuhan University of TechnologyWuhan 430070China School of Engineering and Applied Sciences Harvard UniversityCambridgeMassachusetts 02138United States

The fact that single dielectric loss materials have disadvantages of excessive conductivities and impedance mismatches has given rise to a large effort to develop effective strategies to fabricate electromagnetic wave(EMW)absorbing materials comprised of components that bring about a balance between dielectric loss and magnetic ***,little is known about the essential features that regulate EMW absorption *** study focused on the development of a new EMW absorbing material and gaining information about factors that govern EMW absorption *** materials at the center of the effort are light weight and porous cobalt sulfonated phthalocyanine-reduced graphene oxide(CoSPcrGO)aerogels that were synthesized by using a simple hydrothermal method followed by *** properties of these materials that contribute to the electromagnetic balance between dielectric and magnetic loss were elucidated by first formulating a reasonable hypothesis about how the relative orien-tation of the components in CoSPc-rGO govern p-conjugation and electron transfer from rGO to CoSPc,which is proposed to be a key factor contributing to the regulation of the electromagnetic *** relaxation process of materials was analyzed in detail using a variety of approaches including theoretical calculation,spectroscopic measurements,and experimental and simulation *** fabricated CoSPc-rGO aerogels that contain an ultra-low content of 4%were found to exhibit an extraordinary microwave absorption performance associated with a strong reflection loss of-53.23 dB and a broad effective absorption bandwidth of 8.04 *** results of this study should provide an effective guide for new designs of composite materials for EMW absorption.

关键词： Microwave absorption Polarization relaxation Electromagnetic balance Electrons transfer DFT calculation

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Yolk-shell FeSe_(2)@CoSe_(2)/FeSe_(2) heterojunction as anode materials for sodium-ion batteries with high rate capability and stability

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Journal of materials Science & technology 2024年第5期172卷 185-195页

作者： Liuyang Zhang Bicheng Zhu Difa Xu Zibao Qian Ping Xie Tao Liu Jiaguo Yu Laboratory of Solar Fuel Faculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430078China Hunan Key Laboratory of Applied Environmental Photocatalysis Changsha UniversityChangsha 410022China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

Sodium-ion batteries are promising candidates for large-scale grid storage systems and other *** foremost advantage derives from superior environmental credentials,enhanced safety as well as lower raw material costs than lithium-ion *** is still challenging to explore desirable anode *** this study,FeSe_(2)@CoSe_(2)/FeSe_(2),with a yolk-shell structure was prepared by ion exchange and *** FeSe_(2)@CoSe_(2)/FeSe_(2)prepared as anode material for sodiumion batteries exhibits excellent rate capability due to the synergistic effect of bimetallic selenides and the interfacial effect of the ***,it delivers high performance(510 mAh g^(-1)at 0.2 A g^(-1)),superior rate capa-bility(90%retention at 5 A g^(-1)),and good long-time cycling stability(78%capacity retention after 1800 cycles at a high current density of 2 A g^(-1)).The optimized sodiumion full cell with FeSe_(2)@CoSe_(2)/FeSe_(2)as the anode and Na 3 V 2(PO 4)3 as the cathode still demonstrates excellent ***,a ca-pacity of 272 mAh g^(-1)(at 1 A g^(-1))within the operating voltage from 1 to 3.8 V can be *** work illustrates the potential of bimetallic selenides with heterostructures for performance enhancement of sodium-ion batteries.

关键词： Cobalt-iron selenide Heterojunctions Sodium storage Anode material Full battery

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Proton acceleration from picosecond-laser interaction with a hydrocarbon target

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Plasma Science and technology 2023年第2期25卷 77-85页

作者：杨宇晨黄太武蒋轲郁明阳周沧涛 College of Applied Sciences Shenzhen UniversityShenzhen 518060People's Republic of China Shenzhen Key Laboratory of Ultraintense Laser and Advanced Material Technology Center for Advanced Material Diagnostic Technologyand College of Engineering PhysicsShenzhen Technology UniversityShenzhen 518118People's Republic of China

As an intense picosecond laser pulse irradiates a hydrocarbon target,the protons therein can be accelerated by the radiation pressure as well as the sheath field behind the *** investigate the effect of the laser and hydrocarbon target parameters on proton acceleration with two/threedimensional particle-in-cell *** is found that the resulting two-ion species plasma can generate a multiple peaked charge-separation field that accelerates the *** particular,a smaller carbon-to-hydrogen ratio,as well as the thinner and/or lower density of the target,leads to a larger sheath field and thus proton beams with a larger cutoff energy and smoother energy *** results may be useful in achieving high-flux quasi-monoenergetic proton beams by properly designing the hydrocarbon target.

关键词： picosecond laser pulse proton acceleration multiple peaked charge-separation field carbon-to-hydrogen ratio

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A model for fast electron-driven high-density plasma in the double-cone ignition scheme

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Chinese Physics B 2024年第11期33卷 322-330页

作者： Zhong-Yi Chen Kai-Ge Zhao Ying-Jun Li School of Science China University of Mining and TechnologyBeijing 100083China Shenzhen Key Laboratory of Ultraintense Laser and Advanced Material Technology Center for Intense Laser Application Technologyand College of Engineering PhysicsShenzhen Technology UniversityShenzhen 518118China State Key Laboratory for Tunnel Engineering China University of Mining and TechnologyBeijing 100083China

A model for fast electron-driven high-density plasma is proposed to describe the effect of injected fast electrons on the temperature and inner pressure of the plasma in the fast heating process of the double-cone ignition(DCI)*** to the collision of the two low-density plasmas,the density and volume of the high-density plasma ***,the ignition temperature and energy requirement of the high-density plasma vary at different moments,and the required energy for hot electrons to heat the plasma also *** practical experiments,the energy input of hot electrons needs to be *** reduce the energy input of hot electrons,the optimal moment and the shortest time for injecting hot electrons with minimum energy are *** this paper,it is proposed to inject hot electrons for a short time to heat the high-density plasma to a relatively high ***,the alpha particles with the high heating rate and PdV work heat the plasma to the ignition temperature,further reducing the energy required to inject hot *** study of the injection time of fast electrons can reduce the energy requirement of fast electrons for the high-density plasma and increase the probability of successful ignition of the high-density plasma.

关键词： fast electrons the high-density plasma alpha particles double-cone ignition scheme the optimal moment the shortest time

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Bioabsorbable fabrication of molybdenum nitride/carbon nanocomposites for supercapacitors and metal ion batteries with robust stability

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Rare Metals 2023年第12期42卷 4212-4225页

作者： Qiang-Hong Wu Huan-Zhong Zeng You-Zhi Wu Fen Ran State Key Laboratory of Advanced Processing and Recycling of Non-Ferrous Metals School of Materials Science and EngineeringLanzhou University of TechnologyLanzhou 730050China

Metal nitride is one of the best anode materials of the energy storage device;however,the low stability of the pure metal nitride limits its wide *** this work,a new method of bioabsorbable fabrication was developed for preparing molybdenum nitride that corporates into the porous carbon *** molybdenum ions in pollutions could be easily absorbed by Ligustrum quihoui,and the transportation,accumulation,and circulation of molybdenum ions in Ligustrum quihoui were *** obtained composite material of biochar and molybdenum nitride is employed as anode material of supercapacitors and batteries which exhibits good electrochemical performance,especially the rate and long lifespan ***,it is found that the specific capacity is344 F·g^(-1)at current density of 0.5 A·g^(-1)in 2 mol·L^(-1)KOH,and the capacitance retention and coulomb efficiency are above 90%after 10,000 *** should be noted that the novel approach combines fabricating anode materials with advanced nanostructure and suppressing the environmental problems with metal pollution at the same time.

关键词： Metal pollution Ligustrum quihoui Supercapacitors Metal ions batteries Anode materials

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Artificial Intelligence Meets Flexible Sensors:Emerging Smart Flexible Sensing Systems Driven by Machine Learning and Artificial Synapses

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Nano-Micro Letters 2024年第1期16卷 235-273页

作者： Tianming Sun Bin Feng Jinpeng Huo Yu Xiao Wengan Wang Jin Peng Zehua Li Chengjie Du Wenxian Wang Guisheng Zou Lei Liu Department of Mechanical Engineering State Key Laboratory of Tribology in Advanced EquipmentKey Laboratory for Advanced Manufacturing by Materials Processing TechnologyMinistry of Education of PR ChinaTsinghua UniversityBeijing 100084People’s Republic of China College of Materials Science and Engineering Shanxi ProvinceTaiyuan University of TechnologyTaiyuan 030024People’s Republic of China

The recent wave of the artificial intelligence(AI)revolution has aroused unprecedented interest in the intelligentialize of human *** an essential component that bridges the physical world and digital signals,flexible sensors are evolving from a single sensing element to a smarter system,which is capable of highly efficient acquisition,analysis,and even perception of vast,multifaceted *** challenging from a manual perspective,the development of intelligent flexible sensing has been remarkably facilitated owing to the rapid advances of brain-inspired AI innovations from both the algorithm(machine learning)and the framework(artificial synapses)*** review presents the recent progress of the emerging AI-driven,intelligent flexible sensing *** basic concept of machine learning and artificial synapses are *** new enabling features induced by the fusion of AI and flexible sensing are comprehensively reviewed,which significantly advances the applications such as flexible sensory systems,soft/humanoid robotics,and human activity *** two of the most profound innovations in the twenty-first century,the deep incorporation of flexible sensing and AI technology holds tremendous potential for creating a smarter world for human beings.

关键词： Flexible electronics Wearable electronics Neuromorphic Memristor Deep learning

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Simultaneous enhancement in mechanical and corrosion properties of Al-Mg-Si alloys using machine learning

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Journal of materials Science & technology 2023年第36期167卷 1-13页

作者： Xinming Feng Zhilei Wang Lei Jiang Fan Zhao Zhihao Zhang Institute for Advanced Materials and Technology University of Science and Technology BeijingBeijing 100083China Beijing Laboratory of Metallic Materials and Processing for Modern Transportation Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing 100083China Key Laboratory for Advanced Materials Processing(MOE) University of Science and Technology BeijingBeijing 100083China Beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing 100083China

Al-Mg-Si alloys with high strength and good corrosion resistance are regarded as desirable materials for all-aluminum ***,the traditional trial-and-error experimental methods are insufficient to address the trade-offbetween strength and corrosion *** this work,a non-dominated sorting genetic machine-learning algorithm(NSGA-II)was employed to optimize the chemical composition,so as to simultaneously improve the strength and corrosion *** high-performance Al-Mg-Si alloys with low Mg,Si,and Cu contents were successfully developed,where the yield strength(YS),ultimate tensile strength(UTS),and the elongation(δ)reached 375-380 MPa,410-416 MPa,and 13.7%-15.2%,*** with higher-Cu-content 6013 alloy,the YS and UTS of the present alloys increase by about 60 MPa,and the intergranular corrosion resistance is also significantly ***-ture characterization demonstrated thatβ’’and QP phases introduced a significant synergistic precipita-tion strengthening effect;the dispersoids formed by trace Mn,Cr,Fe,Zr,and Ti contributed dispersion strengthening effect;and the good pitting corrosion resistance is attributed to lower Mg and Si contents.

关键词： Aluminum alloy Machine learning High strength Corrosion resistance

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The impact of the coupling relationship between projectile size and yarn dimension on the ballistic performance of plain weave fabric

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Defence technology(防务技术) 2025年第1期43卷 288-303页

作者： Kaiying Wang Xuan Zhou Wenke Ren Yiding Wu Yilei Yu Yi Zhou Lizhi Xu Guangfa Gao School of Mechanical Engineering Nanjing University of Science and TechnologyNanjing210094China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan430079China

Aramid fibers,due to their relatively high inter-yarn friction,high strength,high modulus,and other characteristics,have become a typical representative of flexible anti-ballistic materials in modern *** research on the anti-penetration of aramid fabrics mostly focuses unilaterally on the structure and performance of aramid fabrics or the shape and size of projectiles,with fewer studies on the coupled effect of both on ballistic *** study analyzes how the coupling relationship(or size effect)between the projectile and fiber bundle dimensions affects the fabric ballistic performance from a mesoscopic scale *** plain weave aramid fabric as the research object,considering different diameter projectiles,through a large number of ballistic impact tests and numerical simulations,parameters such as ballistic limit velocity,average energy absorption of fabric,and specific energy absorption ratio(average energy absorption of fabric divided by projectile cross-sectional area)are obtained for ballistic performance *** influence law of projectile size on the ballistic performance of high-performance fabrics is as follows:The relative range of fitted ballistic limit velocity at different target positions gradually decreases and then stabilizes as the projectile diameter increases,indicating that the fabric structure effect gradually disappears at a projectile diameter of 12 mm;The average ballistic limit velocity at three impact positions,P1,P2,and P3,provides the corresponding ballistic limit velocity for 1000D aramid fabric,which increases with projectile diameter but the rate of increase slows down at an inflection point,which in this study occurs where the fabric structure effect nearly disappears at a projectile diameter of 12 mm;The energy absorption ratio increases and then decreases as the projectile diameter increases from 4 mm to 20 mm,reaching a peak at the diameter of 12 mm due to the gradual disappearance of the fabri

关键词： Plain weave fabric Ballistic performance Aramid fiber Projectile size Ballistic experiment

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Evidence of microstructural evolution linked to non-monotonic distribution of micromechanical properties induced by shot peening

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材料科学技术（英文版） 2025年第4期207卷 238-245页

作者： Guoxin Lu Qiang Wang Bonnie Attard Huhu Su Shijian Zheng Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials Ministry of EducationSchool of Materials Science and EngineeringShandong UniversityJinan250061China Aviation Key Laboratory of Science and Technology on Advanced Corrosion and Protection for Aviation Material AECC Beijing Institute of Aeronautical MaterialsBeijing100095China Department of Metallurgy and Materials Engineering University of MaltaMSD2080Malta Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology School of Materials Science and EngineeringHebei University of TechnologyTianjin300130China

The residual stress field induced by surface strengthening processes such as mechanical shot peening and other forms of plastic deformation does not generally exhibit a simple"monotonic"distribution *** researchers have analyzed this fact from a mechanical perspective based on Hertz ***,the micro/nano-scale microstructural changes corresponding to the distribution of residual stress fields still appear to be *** this study,we focused on a widely used material in aviation manufacturing,namely nickel-based superalloy GH4169,as our experimental *** subjected GH4169 alloy to me-chanical strengthening treatment using a shot peening intensity of 0.25 mmA,followed by quantitative testing of micromechanical performance indicators such as microhardness and residual *** thor-oughly investigate the relationship between micromechanical properties and microstructure changes,we utilized transmission electron microscopy(TEM)to observe and analyze shot-peened materials at differ-ent *** findings revealed that the most severe microstructural distortion induced by mechanical shot peening in GH4169 alloy was likely to occur within a depth range of 25 to 75 *** observation aligns with the actual phenomenon that the maximum microhardness and maximum residual compres-sive stress did not manifest on the outermost surface of the *** presenting a detailed analysis of deformation defects such as dislocations,stacking faults,and twinning in different depths of mechan-ically strengthened layers,our study contributes to a deeper understanding and practical application of post-processing technologies based on plastic deformation.

关键词： Mechanical shot peening Surface strengthening Residual stress Microstructure

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