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Single-Component Color-Tunable Smart Organic Emitters with Simultaneous Multistage Stimuli-Responsiveness and Multimode Emissions

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Research 2024年第2期2023卷 719-728页

作者： Yu Yan Chengfang Liu Jianzhong Fan Yusheng Li Huanling Liu Qian Wang Xiangchun Lil Junfeng Li Wen-Yong Lai State Key Laboratory of Organic Electronics and Information Displays(SKLOEID) Institute of Advanced Materials(IAM)School of Chemistry and Life SciencesNanjing University of Posts&Telecommunications9 Wenyuan RoadNanjng 210023China Shandong Province Key Laboratory of Medical Physics and Image Processing Technology School of Physics and ElectronicsShandong Normal UniversityJinan 250358China

Achieving color-tunable emission in single-component organic emitters with multistage stimuli-responsiveness is of vital significance for intelligent optoelectronic applications,but remains enormously ***,we present an unprecedented example of a color-tunable single-component smart organic emitter(DDOP)that simultaneously exhibits multistage stimuli-responsiveness and multimode *** based on a highly twisted amide-bridged donor-tcceptor-donor structure has been found to facilitate intersystem crossing,form multimode emissions,and generate multiple emissive species with multistage *** pristine crystalline powders exhibit abnormal excitation-dependent emissions from a monomer-dominated blue emission centered at 470 nm to a dimer-dominated yellow emission centered at 550 nm through decreasing the ultraviolet(UV)excitation wavelengths,whereas DDOP single crystals show a wide emission band with a main emission peak at 585 nm when excited at different *** emission behaviors of pristine crystalline powders and single crystals are different,demonstrating emission features that are closely related to the aggregation *** work has developed color-tunable single-component organic emitters with simultaneous multistage stimuli-responsiveness and multimode emissions,which is vital for expanding intelligent optoelectronic applications,including multilevel information encryption,multicolor emissive patterns,and visual monitoring of UV wavelengths.

关键词： donor excitation Smart

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Effect of La on microstructure,mechanical properties and fracture behavior of Al/Mg bimetallic interface manufactured by compound casting

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Journal of materials Science & technology 2022年第10期105卷 214-225页

作者： Zheng Zhang Wenming Jiang Guangyu Li Junlong Wang Feng Guan Guoliang Jie Zitian Fan State Key Laboratory of Materials Processing and Die and Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China State Key Laboratory for Advanced Metals and Materials University of Science and Technology BeijingBeijing 100083China

To improve the Al/Mg bimetallic interface,La was added into the Al/Mg bimetallic interface manufactured by a compound casting *** effect of La addition on the microstructure,mechanical properties and fracture behavior of the Al/Mg bimetallic interface and the formation mechanism of the interface were studied in ***_(11)La_(3),Al_(8)Mn_(4)La,Al_(20)Ti_(2)La,and other rare earth precipitates(RE precipitates)preferentially precipitated at the interface with La addition,while the number of the Al_(11)La_(3)and Al_(8)Mn_(4)La located in eutectic structure area(E area)gradually increased and aggregated in the interface with the increase of the La ***,the matrix structure in different areas of the Al/Mg interface changed in different degrees,and the eutectic structure and primaryγ(Mg_(17)Al_(12))dendrites in the E area were refned,but the intermetallic compounds area(IMC area)had no obvious *** the addition of the La,the interface was strengthened under the comprehensive effect of refnement strengthening and precipitation strengthening from the E *** the La content increased to 1.0%,the shear strength of the Al/Mg bimetal reached the maximum of 51.54 MPa,which was 30.95%higher than the group without La ***,with the further increase of the La content,the large area aggregation of the Al_(11)La_(3)and Al_(8)Mn_(4)La occurred in the interface,leading to the separation of the matrix structure of the E area and the decrease of the shear strength of the Al/Mg interface.

关键词： Compound casting Al-Mg intermetallic compounds Rare earth La Al/Mg interface Microstructure Mechanical properties

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Cobalt-Free BaFe_(0.6)Zr_(0.1)Y_(0.3)O_(3−δ)Oxygen Electrode for Reversible Protonic Ceramic Electrochemical Cells

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Transactions of Tianjin University 2023年第6期29卷 444-452页

作者： Chenghao Yang Jin Li Ao Hu Jian Pu Bo Chi State Key Laboratory of Materials Processing and Die and Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials MOE Key Laboratory for the Green Preparation and Application of Functional MaterialsFaculty of Materials Science and EngineeringHubei UniversityWuhan 430062China MOE Key Laboratory of Material Chemistry for Energy Conversion and Storage Huazhong University of Science and TechnologyWuhan 430074China

Reversible protonic ceramic electrochemical cells(R-PCECs)are ideal,high-effi ciency devices that are environmentally friendly and have a modular *** paper studies BaFe_(0.6)Zr_(0.1)Y_(0.3)O_(3−δ)(BFZY3)as a cobalt-free perovskite oxygen electrode for high-performance R-PCECs where Y ions doping can increase the concentration of oxygen vacancies with a remarkable increase in catalytic *** cell with confi guration of Ni-BZCYYb/BZCYYb/BFZY3 demonstrated promising performance in dual modes of fuel cells(FCs)and electrolysis cells(ECs)at 650℃with low polarization resistance of 0.13Ωcm^(2),peak power density of 546.59 mW/cm^(2)in FC mode,and current density of−1.03 A/cm^(2)at 1.3 V in EC *** alternative operation between FC and EC modes for up to eight cycles with a total of 80 h suggests that the cell with BFZY3 is exceptionally stable and reversible over the long *** results indicated that BFZY3 has considerable potential as an air electrode material for R-PCECs,permitting effi cient oxygen reduction and water splitting.

关键词： Protonic ceramic cells Oxygen electrode Perovskite oxides Cobalt-free Oxygen vacancies

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Advancing the pressure sensing performance of conductive CNT/PDMS composite film by constructing a hierarchical-structured surface

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Nano materials Science 2023年第4期5卷 343-350页

作者： Ye Zhao Taoyu Shen Minyue Zhang Rui Yin Yanjun Zheng Hu Liu Hongling Sun Chuntai Liu Changyu Shen Key Laboratory of Materials Processing and Mold(Zhengzhou University) Ministry of EducationNational Engineering Research Center for Advanced Polymer Processing TechnologyZhengzhou UniversityZhengzhouHenan450002China China Astronaut Research and Training Center Beijing100094China

Flexible pressure sensors have attracted wide attention due to their applications to electronic skin,health monitoring,and human-machine ***,the tradeoff between their high sensitivity and wide response range remains a *** by human skin,we select commercial silicon carbide sandpaper as a template to fabricate carbon nanotube(CNT)/polydimethylsiloxane(PDMS)composite film with a hierarchical structured surface(h-CNT/PDMS)through solution blending and blade coating and then assemble the h-CNT/PDMS composite film with interdigitated electrodes and polyurethane(PU)scotch tape to obtain an h-CNT/PDMS-based flexible pressure *** on in-situ optical images and finite element analysis,the significant compressive contact effect between the hierarchical structured surface of h-CNT/PDMS and the interdigitated electrode leads to enhanced pressure sensitivity and a wider response range(0.1661 kPa^(-1),0.4574 kPa^(-1)and 0.0989 kPa^(-1)in the pressure range of 0–18 kPa,18–133 kPa and 133–300 kPa)compared with planar CNT/PDMS composite film(0.0066 kPa^(-1)in the pressure range of 0–240 kPa).The prepared pressure sensor displays rapid response/recovery time,excellent stability,durability,and stable response to different loading modes(bending and torsion).In addition,our pressure sensor can be utilized to accurately monitor and discriminate various stimuli ranging from human motions to pressure magnitude and spatial *** study supplies important guidance for the fabrication of flexible pressure sensors with superior sensing performance in next-generation wearable electronic devices.

关键词： Flexible pressure sensor Hierarchical structure Polydimethylsiloxane Carbon nanotubes Electronic skin

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Fractal Geometry-based Porosity Analysis of Cementitious Composite material Using Wollastonite Under Freeze-thaw Condition

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Journal of Wuhan University of technology(materials Science) 2025年第3期40卷 769-779页

作者： Aziza Kuldasheva HUANG Bin Kholjigit Kuldashev LI Beixing Bakhtiyor Saidmuratov College of Civil Engineering and Architecture Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Ad-vanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Department of Tech-nology of Building Material and Products Samarkand State Architectural and Civil Engineering UniversitySamarkand-140100Uzbeki-stan State Key Laboratory of Silicate Materials for Architecture Wuhan University of TechnologyWuhan 430070China Samarkand International University of Technology School of EngineeringSamarkand-140100Uzbekistan

Low porosity is very significant for cementitious composite materials(CCM)under freeze-thaw *** reduce the porosity of CCM,we used wollastonite mineral fibers as a partial replacement for cement and *** five combinations,in which 10%,32%,and 48%Wollastonite were added,were made for scanning using both scanning electron microscopy(SEM)and computed tomography scan technology(CT).Then,the 2D SEM pictures and the 3D pore distribution curves are obtained before and after the freezing and thawing processes,where the micro-pores in the CCM materials are *** fractal dimension is used to quantify the topography image in two dimensions,as well as the pore distribution in three *** method allows for the determination of both surface porosity and volume porosity,both of which show an increase in response to an escalation of freeze-thaw *** is also found that the micro-damage in the concrete is of self-similarity,and in the context of the fractal dimension,the pore evolution can be quantitatively characterized across different sizes,ranging from local to global levels,before and after freezing and thawing.

关键词： wollastonite recycled-enriched aggregates fractal dimension freeze-thaw cycle CCM SEM CT

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Microwave sintering of TiCN-based cermets prepared from electroless Co-coated(Ti,W,Mo,V)CN powders

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Rare Metals 2022年第12期41卷 4209-4216页

作者： Jia Pang Ying Liu Jin-Wen Ye Zheng-Hua Tang Jie Wang School of Materials Science and Engineering Sichuan UniversityChengdu 610065China Key Laboratory of Advanced Special Material and Technology Ministry of EducationChengdu 610065China

In this study,the densification and microstructure evolution of microwave sintered(Ti,W,Mo,V)CN-30 wt%Co cermets,which was prepared from electroless cobalt-coated submicron(Ti,W,Mo,V)CN powders,were *** microwave sintering of mechanical milled powders as well as the conventional sintering of mechanical milled powders and Co-coated(Ti,M)CN powders was conducted as a *** results indicate that a slight densification is observed at sintering temperature of≤1100℃followed by a sharp shrinkage at the temperature range of 1200-1350℃due to the substantial formation of liquid phase at 1200℃.The 98.5%densification is obtained at 1375℃.Moreover,the samples sintered at 1375℃for 10 min have the micro structure with fine and homogeneous grains of about 700 *** to mechanical milling,electroless cobalt plating suppresses coalescence of neighboring grain at the solid-state sintering stage,thereby inhibiting grain *** mechanical properties of samples sintered at different temperatures for varied holding time were also discussed.

关键词： Microwave sintering Electroless plating TiCN-based cermets Microstructure

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Robustα-Fe_(2)O_(3)/Epoxy Resin Superhydrophobic Coatings for Anti-icing Property

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Journal of Wuhan University of technology(materials Science) 2024年第3期39卷 621-626页

作者：乔燕明 TAO Xuan LI Lei 阮敏鲁礼林 College of Chemistry and Chemical Engineering Wuhan University of Science and TechnologyWuhan 430081China Hubei Key Laboratory of Mine Environmental Pollution Control&Remediation and Hubei Engineering Research Center for Collaborative Technology of Advanced Material Manufacturing and Solid Waste Recycling Hubei Polytechnic UniversityHuangshi 435003China

α-Fe_(2)O_(3)/epoxy resin composite superhydrophobic coating was prepared withα-Fe_(2)O_(3) nanoparticles and epoxy resin by spin coating *** coating without epoxy resin has higher contact angle(CA)and lower ice adhesion strength(IAS),but the mechanical properties are ***α-Fe_(2)O_(3)/epoxy resin composite superhydrophobic coating exhibits good mechanical *** addition,compared with the bare aluminum substrate,the Ecorr of the composite coating is positive and the Jcorr is *** inhibition efficiency of the composite coating is as high as 99.98%in 3.5 wt%NaCl *** difference in the microstructure caused by the two preparation methods leads to the changes in mechanical properties and corrosion resistance of composite superhydrophobic coating.

关键词： superhydrophobic anti-corrosion anti-icing robust

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Mobile energy storage technologies for boosting carbon neutrality

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The Innovation 2023年第6期4卷 132-151页

作者： Chenyang Zhang Ying Yang Xuan Liu Minglei Mao Kanghua Li Qing Li Guangzu Zhang Chengliang Wang School of Integrated Circuits Wuhan National Laboratory for Optoelectronics(WNL 0)Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Material Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China Wenzhou Advanced Manufacturing Institute Huazhong University of Science and TechnologyWenzhou 325035China

Carbon neutrality calls for renewable energies,and the efficient use of renewable energies requires energy storage mediums that enable the storage of excess energy and reuse after spatiotemporal *** with traditional energy storage technologies,mobile energy storage technologies have the merits of low cost and high energy conversion efficiency,can be flexibly located,and cover a largerange from miniature to large systems and from high energy density to high power density,although most of them still face challenges or technical *** this review,we provide an overview of the opportunities and challenges of these emerging energy storagetechnologies(induding rechargeable batteries,fuel cells,and electrochemical and dielectric capacitors).Innovative materials,strategies,and technologies are ***,the future directions are *** hope this review will advance the development of mobile energy storage technologies and boost carbon neutrality.

关键词： neutral boosting energy

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Swarming magnetic photonic-crystal microrobots withon-the-fly visual pH detection and self-regulated drug delivery

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InfoMat 2023年第10期5卷 64-79页

作者： Zheng Yu Luolin Li Fangzhi Mou Shimin Yu Di Zhang Manyi Yang Qing Zhao Huiru Ma Wei Luo Tianlong Li Jianguo Guan State Key Laboratory of Advanced Technology for Materials Synthesis and Processing International School of Materials Science and Engineering Wuhan University of TechnologyWuhanthe People's Republic of China State Key Laboratory of Robotics and System Harbin Institute of TechnologyHarbinthe People's Republic of China Wuhan Institute of Photochemistry and Technology Wuhanthe People's Republic of China

Swarming magnetic micro/nanorobots hold great promise for biomedical applications,but at present suffer from inferior capabilities to perceive and respond to chemical signals in local *** we demonstrate swarming magnetic photonic crystal microrobots(PC-bots)capable of sponta-neously performing on-the-fly visual pH detection and self regulated drug delivery by perceiving local pH *** magnetic PC-bots consist of pH-responsive hydrogel microspheres with encapsulated one-dimensional periodic assemblies of Fe3O4 *** programming extemnal rotating magnetic fields,they can self-organize into large swarms with much-enhanced collective velocity to actively find targets while shining bright“blinking”structural *** approaching the target with abnormal pH conditions(*** ulcerated superficial tumor lesion),the PC-bots can visualize local pH changes on the fly via pH-responsive structural colors,and realize self-regulated release of the loaded drugs by recognizing local *** work facilita tes the develop-ment of intelligent micro/nanorobots for active“motile-targeting”tumor diag-nosis and treatment.

关键词： collective behaviors drug delivery micro/nanorobots on-the-fly sensing responsivephotonic crystals

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Sol-gel-based porous Ti-doped tungsten oxide films for high-performance dual-band electrochromic smart windows

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Journal of Energy Chemistry 2023年第2期77卷 137-143,I0004页

作者： Qiancheng Meng Sheng Cao Juquan Guo Qingke Wang Ke Wang Tao Yang Ruosheng Zeng Jialong Zhao Bingsuo Zou School of Physical Science and Technology MOE Key Laboratory of New Processing Technology for Non-ferrous Metals and MaterialsGuangxi UniversityNanning 530004GuangxiChina Beijing Advanced Innovation Center for Materials Genome Engineering University of Science and Technology BeijingBeijing 100083China

Dual-band electrochromic smart windows(DESWs)with independent control of the transmittance of near-infrared and visible light show great potential in the application of smart and energy-saving *** current strategy for building DESWs is to screen materials for composite or prepare plasmonic nanocrystal *** rigorous preparation processes seriously limit the further development of ***,we report a facile and effective sol-gel strategy using a foaming agent to achieve porous Ti-doped tungsten oxide film for the high performance of *** introduction of foaming agent polyvinylpyrrolidone during the film preparation can increase the specific surface area and free carrier concentration of the films and enhance their independent regulation ability of near-infrared *** a result,the optimal film shows excellent dual-band electrochromic properties,including high optical modulation(84.9%at 633 nm and 90.3%at 1200 nm),high coloration efficiency(114.9 cm^(2) C^(-1) at 633 nm and 420.3 cm^(2) C^(-1) at 1200 nm),quick switching time,excellent bistability,and good cycle stability(the transmittance modulation losses at 633 and 1200 nm were 11%and 3.5%respectively after 1000 cycles).A demonstrated DESW fabricated by the sol-gel film showed effective management of heat and light of *** study represents a significant advance in the preparation of dual-band electrochromic films,which will shed new light on advancing electrochromic technology for future energy-saving smart buildings.

关键词： Electrochromism Tungsten oxide Smart windows Sol-gel method Dual-band absorption

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