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Convenient folding-hot-pressing fabrication and enhanced piezoelectric properties of highβ-phasecontent poly(vinylidene fluoride)films

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Interdisciplinary materials 2024年第5期3卷 715-725页

作者： Jie Shen Yicheng Zeng Qiangzhi Li Jing Zhou Wen Chen State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Materials Science and EngineeringWuhan University of TechnologyWuhanChina Sanya Science and Education Innovation Park Wuhan University of TechnologySanyaChina Hubei Longzhong Laboratory Wuhan University of Technology Xiangyang Demonstration ZoneXiangyangChina

Poly(vinylidene fluoride)(PVDF)is the most attractive piezoelectric polymer for application in flexible *** attain excellent piezoelectric properties,a substantial amount of spontaneous polarβ-phase content is highly ***,the current reported manufacturing methods to increaseβ-phase contents are inconvenient and complex,hindering progress in PVDF's *** work proposes a folding-hot-pressing method to fabricate highβ-phase-content PVDF *** characterization indicates that the films haveαandβphases and the folding-hot-pressing process transforms theαphase into theβ*** to the 97.5%β-phase content and aligned structure,a piezoelectric constant of 20 pC/N is achieved in the three-times folded ***,the process method enhances the tensile strength(126.2 MPa)of the films,with a low Young's modulus(0.87 GPa)remaining,making the films applicable for flexible piezoelectric ***,sensors based on the achieved films were assembled and applied for human physiological activity *** work offers a scalable new melt-processing strategy for developing high-performance PVDF-based piezo-electric composite films for wearable electronic devices.

关键词： flexible sensors highβ-phase content piezoelectric properties PVDF film

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Targeted inhibition NCOA4-mediated ferritinophagy limits ferroptosis to ameliorate alcohol-induced liver injury in vivo and in vitro

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Food Science and Human Wellness 2024年

作者： Yanan Zhao Bin Li Jiang Liu Fei Yu Lei Chen Hui Teng College of Food Science and Technology， Guangdong Ocean University Guangdong Provincial Key Laboratory of Aquatic Product Processing and Safety Guangdong Province Engineering Laboratory for Marine Biological Products Guangdong Provincial Engineering Technology Research Center of Seafood Key Laboratory of Advanced Processing of Aquatic Product of Guangdong Higher Education Institution

Alcoholic liver injury (ALD) is a serious liver disease resulting from prolonged and excessive alcohol consumption， with significant morbidity and mortality and closely relate to iron accumulation and ferroptosis. Ferritinophagy is the process of autophagic degradation of ferritin and results in labile iron accumulation and ferroptosis. However， whether ferritinophagy involves in alcohol-induced liver injury and ferroptosis remains unexplored. Here， we demonstrated the involvement of ferroptosis in alcohol-induced liver injury by modulating nuclear receptor coactivator 4 (NCOA4)-mediated ferritinophagy. Utilizing both in vivo and in vitro models， we observed activation of autophagy and ferroptosis following alcohol administration. Intriguingly， we found that alcohol-induced ferroptosis is autophagy-dependent， because autophagy inhibitor 3-MA (30 mg/kg bw. in vivo， 1 mM in vitro， respectively) profoundly mitigated alcohol-induced ferroptosis. We further demonstrated that alcohol-induced ferritinophagy was derived by iron overload， by showing that iron chelator DFO (100 mg/kg bw. in vivo， 10 μM in vitro， respectively) can abolish alcohol-induced ferritinophagy and ferroptosis. Moreover， we observed an upregulation of NCOA4 expression， and knockdown of NCOA4 significantly reversed alcohol-induced disturbances in iron metabolism and subsequently blocking ferroptosis. Our findings suggest a connection between ferritinophagy and alcohol-induced ferroptosis in mouse liver and HepG2 cells， highlighting NCOA4-mediated ferritinophagy as a novel mechanism of alcohol-induced liver injury. This study enhances our understanding of the molecular mechanisms underlying alcohol-induced liver injury， and targeting ferritinophagy may provide new strategies for preventing or treating ALD.

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Unprecedented strong and reversible atomic orbital hybridization enables a highly stable Li-S battery

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国家科学评论（英文版） 2022年第7期9卷 109-119页

作者： Min Yan Wenda Dong Fu Liu Lihua Chen Tawfique Hasan Yu Li Bao-Lian Su State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Hubei Engineering Technology Research Center of Optoelectronic and New Energy MaterialsSchool of Materials Science and EngineeringWuhan Institute of TechnologyWuhan 430205China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China School of Materials Science and Engineering Zhejiang UniversityHangzhou 310027China Cambridge Graphene Centre University of CambridgeCambridge CB3 OFAUK State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Laboratory of Inorganic Materials Chemistry(CMI) University of NamurNamur B-50000 Belgium

The shuttle effect and excessive volume change of the sulfur cathode severely impede the industrial implementation of Li-S *** is still highly challenging to find an efficient way to suppress the shuttle effect and volume ***,we report,for the first time,an innovative atomic orbital hybridization concept to construct the hierarchical hollow sandwiched sulfur nanospheres with double-polyaniline layers as the cathode material for large-scale high-performance Li-S *** hierarchically 3D,cross-linked and stable sulfur-polyaniline backbone with interconnected disulfide bonds provides a new type and strong intrinsic chemical confinement of sulfur owing to the atomic orbital hybridization of Li 2s,S 3p,C 2p and N ***,such atomic orbital hybridization of sulfur sandwiched in the double sulfur-polyaniline network is highly reversible during the discharge/charge process and can very efficiently suppress the shuttle effect and volume expansion,contributing to a very high capacity of 1142 mAh g-1 and an excellent stabilized capacity of 886 mAh g-1 at 0.2 C after 500 cycles with a suppressed volume expansion and an unprecedented electrode *** innovative atomic orbital hybridization concept can be extended to the preparation of other electrode materials to eliminate the shuttle effect and volume expansion in battery *** present work also provides a commercially viable and up-scalable cathode material based on this strong and highly reversible atomic orbital hybridation for large-scale high-performance Li-S batteries.

关键词： atomic orbital hybridization double sulfur–polyaniline networks hierarachical hollow sandwiched sulfur nanosphere insitu vulcanization lithium–sulfur batteries

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Epitaxial growth of Cu_(2-x)Se on Cu(220)crystal plane as high property anode for sodium storage

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Chinese Chemical Letters 2024年第7期35卷 519-523页

作者： Zhijia Zhang Shihao Sun Yuefang Chen Yanhao Wei Mengmeng Zhang Chunsheng Li Yan Sun Shaofei Zhang Yong Jiang School of Materials Science and Engineering Institute of Quantum Materials and DevicesState Key Laboratory of Separation Membrane and Membrane ProcessesTiangong UniversityTianjin 300387China School of Chemistry and Life Sciences Suzhou University of Science and TechnologySuzhou 215009China Key Laboratory of Advanced Electrode Materials for Novel Solar Cells for Petroleum and Chemical Industry of China Suzhou University of Science and TechnologySuzhou 215009China Hebei Key Laboratory of Flexible Functional Materials/Hebei Key Laboratory of Material Near-Net Forming Technology School of Materials Science and EngineeringHebei University of Science and TechnologyShijiazhuang 050018China

Three-dimentional(3D)transition metal selenides with sufficient channels could produce significant superiority on enhancing reaction kinetics for sodium-ion ***,the thorough exploration of 3D architecture with a facile strategy is still *** we report that a polycrystalline Cu_(2-x)Se film was epitaxial grown on(220)facets-exposed Cu by direct selenization of a nanoporous Cu skeleton,which is obtained by dealloying rolled Cu Mn@Cu alloy *** functional theory calculation result shows strong adsorption energy for Se atoms on Cu(220)planes during selenization reaction,rendering a low energy *** virtue of this core-shell 3D nanoporous architecture to offer abundant active sites and endow fast electron/ion transportation,the nanoporous Cu_(2-x)Se@Cu-0.15 composite electrode exhibits remarkable sodium-ion storage properties with high reversible capacity of 950.6μAh/cm^(2)at 50μA/cm^(2),suprior rate capability of 457.6μAh/cm^(2)at 500μA/cm^(2),as well as an ultra-long stability at a high current *** investigation reveals that the electrochemical reaction is a typical conversion-type reaction with different *** novel electrode synthetic strategy provides useful instructions to design the high-performance anode material for sodium-ion batteries.

关键词： Cu_(2)se 3D architecture Anode materials Density functional theory calculation Sodium-ion battery

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Simulation of inclined dendrites under natural convection by KKS phase field model based on CUDA

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China Foundry 2023年第5期20卷 432-442页

作者： Chang-sheng Zhu Tian-yu Li Bo-rui Zhao Cang-long Wang Zi-hao Gao College of Computer and Communication Lanzhou University of TechnologyLanzhou 730050China State Key Laboratory of Gansu Advanced Processing and Recycling of Non-Ferrous Metal Lanzhou University of TechnologyLanzhou 730050China Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China Advanced Energy Science and Technology Guangdong Laboratory Huizhou 516000GuangdongChina

In this work,Al-4.5wt.%Cu was selected as the research object,and a phase field-lattice Boltzmann method(PF-LBM)model based on compute unified device architecture(CUDA)was established to solve the problem of low serial computing efficiency of a traditional CPU and achieve significant *** model was used to explore the evolution of dendrite growth under natural *** the study of the tip velocities,it is found that the growth of the dendrite arms at the bottom is inhibited while the growth of the dendrite arms at the top is promoted by natural *** addition,research on the inclined dendrite under natural convection was *** is observed that there is a deviation between the actual growth direction and the preferred angle of the inclined *** the increase of the preferred angle of the seed,the difference between the actual growth direction and the initial preferred angle of the inclined dendrite shows a trend of increasing at first and then *** the simulation area,the relative deflection directions of the primary dendrite arms in the top right corner and the bottom left corner of the same dendrite are almost counterclockwise,while the relative deflection directions of the other two primary dendrite arms are clockwise.

关键词： PF-LBM natural convection inclined dendrites CUDA

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GPU parallel computation of dendrite growth competition in forced convection using the multi-phase-field-lattice Boltzmann model

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Chinese Physics B 2023年第7期32卷 530-547页

作者：高梓豪朱昶胜王苍龙 College of Computer and Communication Lanzhou University of TechnologyLanzhou 730050China State Key Laboratory of Gansu Advanced Processing and Recycling of Non-Ferrous Metal Lanzhou University of TechnologyLanzhou 730050China Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China Advanced Energy Science and Technology Guangdong Laboratory Huizhou 516000China

A graphics-processing-unit(GPU)-parallel-based computational scheme is developed to realize the competitive growth process of converging bi-crystal in two-dimensional states in the presence of forced convection conditions by coupling a multi-phase field model and a lattice Boltzmann *** elimination mechanism in the evolution process is analyzed for the three conformational schemes constituting converging bi-crystals under pure diffusion and forced convection conditions,respectively,expanding the research of the competitive growth of columnar dendrites under melt convection *** results show that the elimination mechanism for the competitive growth of converging bi-crystals of all three configurations under pure diffusion conditions follows the conventional Walton-Chalmers *** there is forced convection with lateral flow in the liquid phase,the anomalous elimination phenomenon of unfavorable dendrites eliminating favorable dendrites occurs in the grain *** particular,the anomalous elimination phenomenon is relatively strong in conformation 1 and conformation 2 when the orientation angle of unfavorable dendrites is small,and relatively weak in conformation ***,the presence of convection increases the tip growth rate of both favorable and unfavorable dendrites in the grain *** addition,the parallelization of the multi-phase-field-lattice Boltzmann model is achieved by designing the parallel computation of the model on the GPU platform concerning the computerunified-device-architecture parallel technique,and the results show that the parallel computation of this model based on the GPU has absolute advantages,and the parallel acceleration is more obvious as the computation area increases.

关键词： multi-phase field model GPU grain competition growth lattice Boltzmann model

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Effect of electrolyte cation-mediated mechanism on electrocatalytic carbon dioxide reduction

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Chinese Chemical Letters 2024年第7期35卷 139-146页

作者： Yuan Dong Mutian Ma Zhenyang Jiao Sheng Han Likun Xiong Zhao Deng Yang Peng Soochow Institute of Energy and Material Innovations College of EnergyJiangsu Key Laboratory of Advanced Carbon Materials and Wearable Energy TechnologiesSoochow UniversitySoochow 215006China Jiangsu Key Laboratory of Advanced Negative Carbon Technologies Soochow UniversitySoochow 215123China School of Chemistry and Chemical Engineering Shihezi UniversityShihezi 832003China School of Chemical and Environmental Engineering Shanghai Institute of TechnologyShanghai 201418China

The steep reduction in costs and systematic optimization of renewable electricity has ignited an intensifying interest in harnessing electroreduction of carbon dioxide(CO_(2)RR)for the generation of chemicals and *** focus of research over the past few decades has been on the optimization of the electrode and the electrolyte ***,cation species in the latter have recently been found to dramatically alter the selectivity of CO_(2)RR and even their catalytic activity by multiple orders of *** a result,the selection of cations is a critical factor in designing catalytic interfaces with high selectivity and efficiency for targeted *** decision-making regarding cation selection relies on a comprehensive understanding of prevailing electrolyte effect models that have been used to elucidate observed experimental *** this perspective,we review the hypotheses that explain how electrolyte cations influence CO_(2)RR by mechanisms such as through tuning of the interfacial electric field,buffering of the local pH,stabilization of the key intermediates and regulation of the interfacial *** endeavor is to elucidate the molecular mechanisms underpinning cation effects,thus fostering the evolution of more holistic and universally applicable predictive *** this regard,we highlight the current challenges in this area of research,while also identifying potential avenues for future investigations.

关键词： CO_(2)electrocatalytic reduction Cation effects Catalytic mechanisms Catalytic interfaces Electric double layer

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Enhanced polysulfide redox kinetics by niobium oxynitrides via insitu adsorptive and catalytic effect in wide temperature range

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Nano Research 2022年第7期15卷 6200-6207页

作者： Benben Wei Chaoqun Shang Qiao Cu Le Hu Xuelian Fu Guofu Zhou Xin Wang School of Materials Science and Engineering&Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Wuhan Institute of TechnologyWuhan 430205China Faculty of Materials Science and Chemistry China University of GeosciencesWuhan 430074China Guangdong Provincial Key Laboratory of Optical Information Materials and Technology&South China Academy of Advanced Optoelectronics South China Normal UniversityGuangzhou 510006China School of Materials Science and Engineering&State Key Laboratory of Material Processing and Die and Mold Technology Huazhong University of Science and TechnologyWuhan 430074China

The development of Li-S batteries(LSBs)is hindered by the low utilization of S species and sluggish redox reaction *** metal oxides always possess high adsorption to polar S species,while conductive metal nitrides show fast electron transport and ensure fast redox reaction of S *** combination merits of metal oxides and metal nitrides in one provide an effective strategy to improve the electrochemical performance of *** this work,defect design of niobium oxynitrides highly dispersed on graphene(NbON-G)is evaluated as effective trapper and catalyst for S *** to the effective structural merits including enriched active sites,alleviated volume variation,defect modulated electronic property,and in-situ chemisorption and catalytic conversion of soluble lithium polysulfides(LiPSs),the LSBs with NbON-G modified separator show remarkably enhanced performance compared to NbN-G and Nb_(2)O_(5)-***,even at low temperature of−40°C,the LSBs with NbON-G can operate for 1,000 cycles with 0.04%capacity decay per cycle(Rate:2 C).

关键词： lithium polysulfides Li-S batteries niobium oxynitrides catalyst low temperature

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Recent progress in inhibition of hydrogen evolution reaction in alkaline Al-air batteries

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National Science Open 2024年第6期3卷 42-67页

作者： Yingjie Liu Zhong Wu Zhenbo Qin Yichun Liu Wenbin Hu Tianjin Key Laboratory of Composite and Functional Material Key Laboratory of Advanced Ceramics and Machining Technology(Ministry of Education)School of Materials Science and EngineeringTianjin UniversityTianjin 300350China School of Materials Science and Engineering Kunming University of Science and TechnologyKunming 650093China

Alkaline Al-air batteries(AABs)have attracted considerate attention due to their high theoretical capacity density and energy density with intrinsic safety and low ***,severe hydrogen evolution reaction(HER)decreases the discharge performance and increases usage risk,which restricts the development of *** this comprehensive review,a systematic overview of progress in inhibition methods of HER is provided,including anodic alloying,structural treatment,surface modification,additives and non-aqueous *** them,the most efficient method is additives,which was simple and provided the highest inhibition ***,suggestions and perspectives for future research are offered on improving the commercial application potential of AABs,providing guidance for aqueous metal-air batteries.

关键词： Al-air battery hydrogen evolution reaction anode electrolyte additive capacity density

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Pore structure of porous Mg-1Mn-xZn alloy fabricated by metal–gas eutectic unidirectional solidification

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Journal of Magnesium and Alloys 2022年第8期10卷 2137-2146页

作者： Canxu Zhou Gangqiang Liang Yuan Liu Huawei Zhang Xiang Chen Yanxiang Li School of Materials Science and Engineering Tsinghua UniversityBeijing 100084China Key Laboratory for Advanced Materials Processing Technology Ministry of EducationTsinghua UniversityBeijing 100084China

Lotus-type porous Mg-1 wt.% Mn-xZn(x = 0 wt.%, 1 wt.% and 2 wt.%) alloys were fabricated by metal–gas eutectic unidirectional solidification(the Gasar method). Effects of Zn addition and the fabrication process on the porosity, pore diameter and microstructure of the porous Mg alloys were investigated. Zn addition from 0 wt.% to 1 wt.% and 2 wt.% to the Mg-1 wt.% Mn alloy decreased the porosity from41.2% to 36.9% and 35.8%, respectively, with the same preparation processing. In the lotus-type porous Mg-1 wt.%Mn-1 wt.%Zn alloy, the porosities and average pore diameters changed with hydrogen pressures from 0.1 to 0.6 MPa. Conical areas that were rich in elemental Zn existed below the directional pores, and precipitates were also found in conical areas. Homogeneous directional pores existed in the lower portion of the ingot, and coarser directional pores and finer non-directional pores formed in the upper part. A theoretical model of the change in porosity with hydrogen pressure agreed well with the calculated porosities in the steady bubble growing area. The compressive strength of Mg-1 ***-Zn alloys can be increased by around 20 MPa through rising Zinc content from 1 wt.% to 2 wt.%, which basically linearly decline with the increasing of porosity. This work provides the basis for Gasar Mg-Zn-Mn alloy synthesis in biological applications and shows that the Gasar process is a promising method to fabricate Mg-Zn-Mn alloys with directional pores and a controllable pore structure.

关键词： Porous material Mg-Mn-Zn alloy Porosity Gasar Directional solidification

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