Despite significant advances in image-to-image (I2I) translation with generative adversarial networks (GANs), it remains challenging to effectively translate an image to a set of diverse images in multiple target doma...
详细信息
Retaining the ultrathin structure of two-dimensional materials is very important for stabilizing their catalytic ***,aggregation and restacking are unavoidable,to some extent,due to the van der Waals interlayer intera...
详细信息
Retaining the ultrathin structure of two-dimensional materials is very important for stabilizing their catalytic ***,aggregation and restacking are unavoidable,to some extent,due to the van der Waals interlayer interaction of two-dimensional ***,we address this challenge by preparing an origami accordion structure of ultrathin twodimensional graphitized carbon nitride(oa-C_(3)N_(4))with rich *** novel structured oa-C_(3)N_(4) shows exceptional photocatalytic activity for the CO_(2) reduction reaction,which is 8.1 times that of the pristine C_(3)N_(4).The unique structure not only prevents restacking but also increases light harvesting and the density of vacancy defects,which leads to modification of the electronic structure,regulation of the CO_(2) adsorption energy,and a decrease in the energy barrier of the carbon dioxide to carboxylic acid intermediate *** study provides a new avenue for the development of stable highperformance two-dimensional catalytic materials.
The development of highly efficient energy conversion technologies to extract energy from wastewater is urgently needed,especially in facing of increasing energy and environment ***,we successfully fabricated a novel ...
详细信息
The development of highly efficient energy conversion technologies to extract energy from wastewater is urgently needed,especially in facing of increasing energy and environment ***,we successfully fabricated a novel hybrid fuel cell with BiOCl-NH_(4)PTA as *** polyoxometalate(NH_(4)PTA)act as the acceptor of photoelectrons and could retard the recombination of photogenerated electrons and holes,which lead to superior photocatalytic *** utilizing BiOCl-NH_(4)PTA as photocatalysts and Pt/C air-cathode,we successfully constructed an electron and mass transfer enhanced photocatalytic hybrid fuel cell with flow-through field(F-HFC).In this novel fuel cell,dyes and biomass could be directly degraded and stable power output could be *** 87%of dyes could be degraded in 30 min irradiation and nearly 100%removed within 90 *** current density could reach up to~267.1μA/cm^(2);with maximum power density(Pmax)of~16.2μW/cm^(2) with Rhodamine B as organic pollutant in *** power densities were 9.0μW/cm^(2),12.2μW/cm^(2),and 13.9μW/cm^(2) when using methyl orange(MO),glucose and starch as substrates,*** hybrid fuel cell with BiOCl-NH_(4)PTA composite fulfills the purpose of decontamination of aqueous organic pollutants and synchronous electricity ***,the novel design cell with separated photodegradation unit and the electricity generation unit could bring potential practical application in water purification and energy recovery from wastewater.
The random walk is one of the most basic dynamic properties of complex networks,which has gradually become a research hotspot in recent years due to its many applications in actual *** important characteristic of the ...
详细信息
The random walk is one of the most basic dynamic properties of complex networks,which has gradually become a research hotspot in recent years due to its many applications in actual *** important characteristic of the random walk is the mean time to absorption,which plays an extremely important role in the study of topology,dynamics and practical application of complex *** the mean time to absorption on the regular iterative self-similar network models is an important way to explore the influence of self-similarity on the properties of random walks on the *** existing literatures have proved that even local self-similar structures can greatly affect the properties of random walks on the global network,but they have failed to prove whether these effects are related to the scale of these self-similar *** this article,we construct and study a class of Horizontal Par-titioned Sierpinski Gasket network model based on the classic Sierpinski gasket net-work,which is composed of local self-similar structures,and the scale of these structures will be controlled by the partition coefficient ***,the analytical expressions and approximate expressions of the mean time to absorption on the network model are obtained,which prove that the size of the self-similar structure in the network will directly restrict the influence of the self-similar structure on the properties of random walks on the ***,we also analyzed the mean time to absorption of different absorption nodes on the network tofind the location of the node with the highest absorption efficiency.
Lead-free antiferroelectric ceramics with high energy storage performance show great potential in pulsed power ***,poor breakdown strength and antiferroelectric stability are the two main drawbacks that limit the ener...
详细信息
Lead-free antiferroelectric ceramics with high energy storage performance show great potential in pulsed power ***,poor breakdown strength and antiferroelectric stability are the two main drawbacks that limit the energy storage performance of antiferroelectric ***,highquality(Ag_(1-x)Na_(x))(Nb_(1-x)Ta_(x))O_(3)ceramics were prepared by the tape casting *** breakdown strength was greatly improved as a result of the high density and fine grains,while the antiferroelectric stability was enhanced owning to the M2 *** from the synergistic improvement in breakdown strength and antiferroelectric stability,(Ag_(0.80)Na_(0.20))(Nb_(0.80)Ta_(0.20))O_(3)ceramic reveals a benign energy storage performance of W_(rec)=5.8 J/cm^(3)and h=61.7%with good temperature stability,frequency stability and cycling *** is also found that the high applied electric field can promote the M2-M3 phase transition,which may provide ideas to improve the thermal stability of the energy storage performance in AgNbO_(3)-based ceramics.
The numerical stability of nonlinear equations has been a long-standing concern and there is no standard framework for analyzing long-term qualitative behavior. In the recent breakthrough work [XX23], a rigorous numer...
详细信息
The numerical stability of nonlinear equations has been a long-standing concern and there is no standard framework for analyzing long-term qualitative behavior. In the recent breakthrough work [XX23], a rigorous numerical analysis was conducted on the numerical solution of a scalar ODE containing a cubic polynomial derived from the Allen-Cahn equation. It was found that only the implicit Euler method converge to the correct steady state for any given initial value u0 under the unique solvability and energy stability. But all the other commonly used second-order numerical schemes exhibit sensitivity to initial conditions and may converge to an incorrect equilibrium state as tn → ∞. This indicates that energy stability may not be decisive for the long-term qualitative correctness of numerical solutions. We found that using another fundamental property of the solution, namely monotonicity instead of energy stability, is sufficient to ensure that many common numerical schemes converge to the correct equilibrium state. This leads us to introduce the critical step size constant h∗ = h∗(u0, ϵ) that ensures the monotonicity and unique solvability of the numerical solutions, where the scaling parameter ϵ ∈ (0, 1). For a given numerical method, if the initial value u0 is given, no matter how large it is, we prove that h∗ > 0. As long as the actual simulation step 0 ∗, the numerical solution preserves monotonicity and converges to the correct equilibrium state. On the other hand, we prove that the implicit Euler scheme h∗ = h∗(ϵ), which is independent of u0 and only depends on ϵ. Hence regardless of the initial value taken, the simulation can be guaranteed to be correct when h ∗. But for various other numerical methods, no mater how small the step size h is in advance, there will always be initial values that cause simulation errors. In fact, for these numerical methods, we prove that infu0∈R h∗(u0, ϵ) = 0. Various numerical experiments are used to confirm the theoretical anal
During August and September 2023,three giant icebergs,each bigger than Paris,successively grazed Clarence Island in the northeast of the Antarctic Peninsula,a home to a population of over 100000 *** incident may serve...
详细信息
During August and September 2023,three giant icebergs,each bigger than Paris,successively grazed Clarence Island in the northeast of the Antarctic Peninsula,a home to a population of over 100000 *** incident may serve as a clarion call for the increasing iceberg calving due to global warming and its subsequent impact on the Antarctic *** we investigate this unexpected event and employ historical records and probabilistic analyses of iceberg grounding to assess the degree of impact on penguin colonies of Clarence *** the eleven colonies,there is one with low impact,eight with medium impact,and two with high *** low-impact colony,Cape Lloyd,is located in the northern part of the island,while the high-impact colonies,False Ridge and Pink Pool,are in the *** eight medium-impact colonies are distributed along both the eastern and western coasts of the *** study provides essential support for evaluating the impact of iceberg activity on penguin *** argue that penguin colonies located in areas prone to iceberg drift,such as Clarence Island,may become more vulnerable to the heightened risk of iceberg collisions or groundings in the warming ***,we hope the public will become more aware of the grave impacts of climate change on penguins and underscore the urgent need for effective conservation strategies.
The single event effect of a silicon–germanium heterojunction bipolar transistor(SiGe HBT) was thoroughly investigated. By considering the worst bias condition, the sensitive area of the proposed device was scanned w...
详细信息
The single event effect of a silicon–germanium heterojunction bipolar transistor(SiGe HBT) was thoroughly investigated. By considering the worst bias condition, the sensitive area of the proposed device was scanned with a pulsed *** variation of the collector bias and pulsed laser incident energy, the single event transient of the SiGe HBT was ***, the single event transient produced by laser irradiation at a wavelength of 532 nm was more pronounced than at a wavelength of 1064 nm. Finally, the impact of the equivalent linear energy transfer of the 1064 nm pulsed laser on the single event transient was qualitatively examined by performing technology computer-aided design simulations, and a good consistency between the experimental data and the simulated outcomes was attained.
Clay mineral proxies have been widely used to reconstruct changes in provenance and the ***,high-altitude clay mineral indications and long-term and orbital variations have not been fully ***,we present an800-ka clay-...
详细信息
Clay mineral proxies have been widely used to reconstruct changes in provenance and the ***,high-altitude clay mineral indications and long-term and orbital variations have not been fully ***,we present an800-ka clay-mineral record from a lacustrine sediment core(ZB13-C2)from the Zoige Basin on the eastern Tibetan Plateau(TP).X-ray diffraction and scanning electron microscopy were used to identify the clay mineral assemblages and their micromorphological characteristics of core *** results revealed that the clay minerals in core ZB13-C2 are mainly illite,with small amounts of chlorite,kaolinite,and smectite(including irregular mixed-layers of illite-smectite(I/S)and chloritesmectite(C/S)).The clay mineral assemblages and proxies exhibit three stages of change,which are mainly controlled by the Zoige watershed range under different climate *** watershed was limited to the southeastern region with altitudes ranging from~3500 to~4200 meters above sea level(m a.s.l.),and glacial-interglacial hydraulic erosion controlled the input of bedrock debris during 800-621 ka *** expanded to higher altitudes(~4200 to~4700 m a.s.l.)due to stronger seasonal freezethaw weathering without significant glacial-interglacial variations under a cooling and drying climate during 621-100 ka ***,it expanded to its highest altitudes of~4700 to~5200 m *** of the watershed after 100 ka BP,and hydraulic erosion increased obviously under a warm climate of the interstadial MIS 3 on the *** watershed underwent two major expansions under different climatic conditions at~621 ka and 100 ka BP,with the wet/dry alternation became strong at~621 ka *** results reveal that long-term temperature changes and the wet/dry alternation at high altitudes controlled the watershed range and degree of the physical erosion,and that the indications of clay minerals should be carefully clarified before they are used as climate indicators,especi
Aimed at the demand of contingency return at any time during the near-moon phase in the manned lunar landing missions,a fast calculation method for three-impulse contingency return trajectories is ***,a three-impulse ...
详细信息
Aimed at the demand of contingency return at any time during the near-moon phase in the manned lunar landing missions,a fast calculation method for three-impulse contingency return trajectories is ***,a three-impulse contingency return trajectory scheme is presented by combining the Lambert transfer and maneuver at the special ***,a calculation model of three-impulse contingency return trajectories is ***,fast calculation methods are proposed by adopting the high-order Taylor expansion of differential algebra in the twobody trajectory dynamics model and perturbed trajectory dynamics ***,the performance of the proposed methods is verified by numerical *** results indicate that the fast calculation method of two-body trajectory has higher calculation efficiency compared to the semi-analytical calculation method under a certain accuracy *** to its high efficiency,the characteristics of the three-impulse contingency return trajectories under different contingency scenarios are further analyzed *** findings can be used for the design of contingency return trajectories in future manned lunar landing missions.
暂无评论