Exploring low-cost,high-performance,and stable electrocatalysts toward the oxygen evolution reaction(OER)is highly desired but remains *** metal hydroxide has been wildly utilized as a promising candidate,but practica...
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Exploring low-cost,high-performance,and stable electrocatalysts toward the oxygen evolution reaction(OER)is highly desired but remains *** metal hydroxide has been wildly utilized as a promising candidate,but practical implementation is impeded by insufficient catalytic activity,easy agglomeration,and poor ***,we report that both phosphorization and combination with MXnene can improve the catalysts’intrinsic activity and ***,MXene also prevents the agglomeration of the nanoparticles,resulting in the enhanced exposure of active *** char-acterizing and density functional theory simulations revealed that P species can attract electrons to pro-mote the formation of high-valence states of adjacent metal atoms,and coupling MXene support can effectively modulate the electronic structure and optimize the d-band center,which boosts the OER ***,the optimized NiFeCoP/Mxene catalyst exhibits a low overpotential of 240 mV at a current density of 10 mA cm^(−2),a small Tafel slope of 55 mV dec^(−1),and superior long-term stability of 40 h in 1 M KOH electrolyte,which is superior to other counterparts.
Osteoporotic Vertebral Fracture(OVFs)is a common lumbar spine disorder that severely affects the health of *** a clear bone blocks boundary,CT images have gained obvious advantages in OVFs *** with CT images,X-rays ar...
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Osteoporotic Vertebral Fracture(OVFs)is a common lumbar spine disorder that severely affects the health of *** a clear bone blocks boundary,CT images have gained obvious advantages in OVFs *** with CT images,X-rays are faster and more inexpensive but often leads to misdiagnosis and miss-diagnosis because of the overlapping *** how to transfer CT imaging advantages to achieve OVFs classification in X-rays is *** this purpose,we propose a multi-modal semantic consistency network which could do well X-ray OVFs classification by transferring CT semantic consistency *** from existing methods,we introduce a feature-level mix-up module to get the domain soft labels which helps the network reduce the domain offsets between CT and *** the meanwhile,the network uses a self-rotation pretext task on both CT and X-ray domains to enhance learning the high-level semantic invariant *** employ five evaluation metrics to compare the proposed method with the state-of-the-art *** final results show that our method improves the best value of AUC from 86.32 to 92.16%.The results indicate that multi-modal semantic consistency method could use CT imaging features to improve osteoporotic vertebral fracture classification in X-rays effectively.
This paper presents both a priori and a posteriori error analyses for a really pressure-robust virtual element method to approximate the incompressible Brinkman problem. We construct a divergence-preserving reconstruc...
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Ni-Fe-based catalysts are considered to be among the most active catalysts for the oxygen evolution reaction(OER)under alkaline conditions,with Fe playing a crucial ***,Fe leaching occurs during the reaction due to th...
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Ni-Fe-based catalysts are considered to be among the most active catalysts for the oxygen evolution reaction(OER)under alkaline conditions,with Fe playing a crucial ***,Fe leaching occurs during the reaction due to thermodynamic instability,which has resulted in conflicting reports within the literature regarding its *** clarify this point,we propose a strategy consisting of modulating the electronic orbital occupancy to suppress the extensive loss of Fe atoms during the OER *** calculations,in-situ X-ray photoelectron spectroscopy,molecular dynamics simulations,and a series of characterization showed that the stable presence of Fe not only accelerates the electron transfer process but also optimizes the reaction barriers of the oxygen evolution intermediates,promoting the phase transition of Fe_(5)Ni_(4)S_(8)to highly active catalytic *** modulated Fe_(5)Ni_(4)S_(8)-based pre-catalysts exhibit improved OER activity and long-term *** study provides a novel perspective for understanding the role of Fe in the OER process.
In terms of the requirement of contingency return during the circumlunar flight phase in manned lunar missions, this article presents a contingency point return trajectory design approach. In consideration of the poin...
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Procedurally generating cities in Minecraft provides players more diverse scenarios and could help understand and improve the design of cities in other digital worlds and the real world. This paper presents a city gen...
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This paper presents a novel framework aimed at quantifying uncertainties associated with the 3D reconstruction of smoke *** approach reconstructs color and density fields from 2D images using Neural Radiance Field(NeR...
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This paper presents a novel framework aimed at quantifying uncertainties associated with the 3D reconstruction of smoke *** approach reconstructs color and density fields from 2D images using Neural Radiance Field(NeRF)and improves image quality using frequency *** NeRF model is obtained via joint training ofmultiple artificial neural networks,whereby the expectation and standard deviation of density fields and RGB values can be evaluated for each *** addition,customized physics-informed neural network(PINN)with residual blocks and two-layer activation functions are utilized to input the density fields of the NeRF into Navier-Stokes equations and convection-diffusion equations to reconstruct the velocity *** velocity uncertainties are also evaluated through ensemble *** effectiveness of the proposed algorithm is demonstrated through numerical *** presentmethod is an important step towards downstream tasks such as reliability analysis and robust optimization in engineering design.
This paper presents an effective low-rank generalized alternating direction implicit iteration (R-GADI) method for solving large-scale sparse and stable Lyapunov matrix equations and continuous-time algebraic Riccati ...
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The demand for indoor synthesis has increased significantly in recent years because of the emergence of computational design. This work designs and develops MyRoom, a Unity plugin that can import layout datasets for i...
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Implicit-explicit Runge-Kutta-Rosenbrock methods are proposed to solve nonlinear sti ordinary di erential equations by combining linearly implicit Rosenbrock methods with explicit Runge-Kutta ***,the general order con...
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Implicit-explicit Runge-Kutta-Rosenbrock methods are proposed to solve nonlinear sti ordinary di erential equations by combining linearly implicit Rosenbrock methods with explicit Runge-Kutta ***,the general order conditions up to order 3 are ***,for the nonlinear sti initial-value problems satisfying the one-sided Lipschitz condition and a class of singularly perturbed initial-value problems,the corresponding errors of the implicit-explicit methods are *** last,some numerical examples are given to verify the validity of the obtained theoretical results and the e ectiveness of the methods.
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