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Polarization-Induced Proton Adsorption and Charge Separation in Pyrene-Based Conjugated Microporous Polymers Via Substituent Regulation for Efficient Photocatalytic Hydrogen Evolution

SSRN

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SSRN 2023年

作者： Ren, Runtang Jiao, Zhengxu Li, Zhanfeng Tian, Yue Liu, Baoyou Yue, Gang Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province Taiyuan University of Technology Taiyuan030024 China Institute of Carbon Materials College of Materials Science and Engineering Taiyuan University of Technology Taiyuan030024 China Technology Innovation Center Ningxia Sinostar Display Material Co. Ltd. Yinchuan750003 China

Constructing photocatalysts with efficient light-harvesting abilities and charge separation properties is highly promising but still challenging for boosting photocatalytic hydrogen evolution from water. Herein, we report a simple and general polarization strategy through substituent regulation such as fluorination, chlorination and cyanation, to promote the photon capture and charge separation and unveil the latent structure–property–activity relationship in pyrene-based conjugated microporous polymers (CMPs). Notably, the introduction of fluorine, chlorine and cyano substituents onto the well-known full donor pyrene-benzene-based CMP network (Py-B) could induce a strong dipole along C–F/–Cl/–CN bonds and the backbone local polarization enhancement due to their strong electron-withdrawing ability, which afforded CMPs have a variety of superior effects such as narrowing band gaps, expanding optical absorption, improving interfacial wettability and solid-state morphology, and promoting charge separation inside organic photocatalysts. As a result, 1.73/2.50/4.69-fold increases of the hydrogen evolution rates of the –F/–Cl/–CN modified CMPs under visible light (λ > 420 nm) irradiation without Pt co-catalysts can be obtained in comparison with the counterpart Py-B (28.5/41.3/77.4 mmol g−1 h−1 vs 16.5 mmol g−1 h−1). Impressively, we find that the photocatalytic performance of this series of photocatalysts is linearly related to the dipole moment of polymers. Our studies reveal that the backbone local polarization enhancement induced by the substituent regulation could achieve high-performance organic photocatalysts toward solar-to-chemical energy conversion. © 2023, The Authors. All rights reserved.

关键词： Polarization

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Fabry-perot lasers as enablers for parallel reservoir computing

arXiv

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arXiv 2020年

作者： Bogris, Adonis Mesaritakis, Charis Deligiannidis, Stavros Li, Pu Department of Informatics and Computer Engineering University of West Attica Aghiou Spiridonos Egaleo Athens12243 Greece Department of Information & Communication Systems Engineering University of the Aegean 2 Palama & Gorgyras St. Karlovassi Samos83200 Greece Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China

We introduce the use of Fabry-Perot (FP) lasers as potential neuromorphic computing machines with parallel processing capabilities. With the use of optical injection between a master FP laser and a slave FP laser under feedback we demonstrate the potential for scaling up the processing power at longitudinal mode granularity and perform real-time processing for signal equalization in 25 Gbaud intensity modulation direct detection optical communication systems. We demonstrate the improvement of classification performance as the number of nodes increases and the capability of simultaneous processing of arbitrary data streams. Extensive numerical simulations show that up to 8 longitudinal modes in typical Fabry-Perot lasers can be leveraged so as to enhance classification performance. Copyright © 2020, The Authors. All rights reserved.

关键词： Recurrent neural networks

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Determination of weak squeezed vacuum state through photon statistics measurement

arXiv

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arXiv 2021年

作者： Zuo, Guanhua Zhang, Yuchi Li, Jing Zhu, Shiyao Guo, Yanqiang Zhang, Tiancai State Key Laboratory of Quantum Qptics and Quantum Optics Devices Collaborative Innovation Center of Extreme Optics Institute of Opto-Electronics Shanxi University Taiyuan030006 China College of Physics and Electronic Engineering Shanxi University Taiyuan030006 China Department of Physics Zhejiang University Hangzhou310027 China Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan030600 China

Weak squeezed vacuum light, especially resonant to the atomic transition, plays an important role in quantum storage and generation of various quantum sources. However, the general homodyne detection (HD) cannot determine weak squeezing due to the low signal to noise ratio and the limited resolution of the HD system. Here we provide an alternative method based on photon statistics measurement to determine the weak squeezing of the squeezed vacuum light generated from an optical parametric oscillator working far below the threshold. The approach is established the relationship between the squeezing parameter and the second-order degree of coherence. The theoretical analysis agrees well with the experiment results. The advantage of this method is that it provides a feasible and reliable experimental measure to determine the weak squeezing with high precision and the measurement is independent on the detection efficiency. This method can be used to measure other quantum features for various quantum states with extremely weak non-classicality. Copyright © 2021, The Authors. All rights reserved.

关键词： Optical parametric oscillators

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10-Hertz quantum light source generation on the cesium D2 line using single photon modulation

arXiv

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arXiv 2022年

作者： Zuo, Guan-Hua Zhang, Yu-Chi Li, Gang Zhang, Peng-Fei Yang, Peng-Fei Guo, Yan-Qiang Zhu, Shi-Yao Zhang, Tian-Cai State Key Laboratory of Quantum Optics and Quantum Optics Devices Collaborative Innovation Center of Extreme Optics Institute of Opto-Electronics Shanxi University Taiyuan030006 China College of Physics and Electronic Engineering Shanxi University Taiyuan030006 China Department of Physics Zhejiang University Hangzhou310027 China Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan030024 China

Generation of quantum light source is a promising technique to overcome the standard quantum limit in precision measurement. Here, we demonstrate an experimental generation of quadrature squeezing resonating on the cesium D2 line down to 10 Hz for the first time. The maximum squeezing in audio frequency band is 5.57 dB. Moreover, we have presented a single-photon modulation locking to control the squeezing angle, while effectively suppressing the influence of laser noise on low-frequency squeezing. The whole system operates steadily for hours. The generated low-frequency quantum light source can be applied in quantum metrology, light-matter interaction investigation and quantum memory in the audio frequency band and even below. Copyright © 2022, The Authors. All rights reserved.

关键词： Photons

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controllable Electrical Characteristic of Ti3c2t2/Mos2 (T=Oh, F, O) Interfaces for High Performance Electronics: Insights from First-Principles

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SSRN 2023年

作者： Zhang, Qiang Liu, Yan Zhang, Riguang Lv, Bohan Hao, Runfang Sang, Shengbo Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Electronic Information and Optical Engineering Taiyuan University of Technology Shanxi Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System of The Ministry of Education Taiyuan University of Technology Shanxi Taiyuan030024 China School of Software Taiyuan University of Technology Shanxi Taiyuan030024 China State Key Laboratory of Clean and Efficient Coal Utilization China Laboratory of Aerospace Servo Actuation and Transmission Beijing Institute of Precision Mechatronics and Controls Beijing100000 China

Two-dimensional (2D) semiconductors have shown competitive potential for applications into beyond-silicon electronics. However, the controllable electrical characteristic of metal-semiconductor interfaces is still a challenge for high performance electronics due to Fermi level pinning. To explore Ti3C2T2/MoS2 (T= OH, F, O) for high performance electronics, the vertical electric field and interlayer distance are adopted here to regulate the electrical characteristic of interfaces based on the first-principles calculations. Though this, the electrical characteristic of Ti3C2O2/MoS2 and Ti3C2F2/MoS2 are more sensitive to electric field or interlayer distance than that of Ti3C2(OH)2/MoS2. Especially, the negative electric field with larger than -0.2 V/Å makes Ti3C2O2/MoS2 interface change from p-type Schottky to n-type Schottky contact. Furthermore, the Ti3C2O2/MoS2 interface can not only switch from p-type Schottky to n-type Schottky contact, but also from p-type Schottky to n-type Ohmic contact by varying interlayer distance. Moreover, the tunneling barriers of all interfaces are more sensitive to interlayer distance than to electric field. This work provides vital insights for high-performance electronics of Ti3C2T2/MoS2 (T=OH, F, O) in experiments. © 2023, The Authors. All rights reserved.

关键词： Electric fields

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Study on Sensitization Mechanism of Novel Magnetorheological Composite Pdms Thin Film Based on Enhanced Magneto-Mechanical Effect

SSRN

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SSRN 2023年

作者： Sang, Shengbo Tan, Qiuyun Jiang, Jiaolin Wu, Kaile Xiao, Pengli Zhao, Dong Guo, Xing Yang, Zhuoqing Dong, Xiushan Ge, Yang Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Information and Computer Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China Shanghai200240 China Shanxi Academy of Medical Sciences China Shanxi Research Institute of 6D Artificial Intelligence Biomedical Science Taiyuan030024 China

High sensitivity is key to expand the range of bio-detection, especially in realizing biological detection on single molecular level. Herein, we introduce a novel magnetorheological membrane with enhanced magneto-mechanical effect into the biosensor. Specifically, we made the magnetorheological composite PDMS film (MREF) strengthened by magnetostrictive particles (MSP), and the anisotropic TbDyFe-PDMS can be magnetically deformed to 90 °with 5.8 emu/g, which possesses an initial tensile modulus 55% higher than isotropic. In particular, the modified MR effect equations were proposed considering magnetic dipole interaction and nonlinear magnetostrictive pre-strain of MSP. Such formulae indicate that the enhanced MR effect of MSP-MREF is greatly determined by Ms, remanence, and the flux linkage-like structure. In addition, finite element simulations were carried out to validate and complementarily demonstrate the nonlinear magneto-mechanical behaviors of MSP-MREF theoretically. Finally, the biosensor based on MSP-MREF was fabricated to detect the low concentrations of human serum albumin (HSA), and its sensitivity is around 4 times that of the conventional biosensor. Furthermore, it exhibits high reliability in detecting HSA in real human urine samples, making it the ideal candidate as a practical and effective way for the detection of biomolecules at low concentrations in the future. © 2023, The Authors. All rights reserved.

关键词： Finite element method

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Non-invasive optical focusing inside strongly scattering media with linear fluorescence

arXiv

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arXiv 2020年

作者： Li, Dayan Sahoo, Sujit Kumar Lam, Huy Quoc Wang, Dong Dang, Cuong Nanyang Technological University Singapore 50 Nanyang Avenue Singapore639798 Singapore School of Electrical Sciences Indian Institute of Technology Goa Goa403401 India Temasek Laboratories @ Nanyang Technological University 50 Nanyang Avenue 639798 Singapore Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan030024 China

Non-invasive optical focusing inside scattering media is still a big challenge because inhomogeneous media scatter both incoming photons for focusing and outgoing photons for observation. Various approaches, utilizing non-linear fluorescence or ultrasound, have been reported to address this difficulty. However, implementation of these methods is complicated and highly expensive, as ultrafast laser systems or photo-acoustic equipment must be employed. Here, we demonstrate a wavefront shaping technique to achieve non-invasive focusing (NiF) inside scattering media using only a linear fluorescent signal. Contrast and mean of incoherent speckles, produced by the linear fluorescence, are utilized as feedback signals to optimize the input wavefront. While increasing speckle contrast makes the focus tighter, and increasing the speckle mean enhances the intensity, fine-tuning the contribution of these two factors in our two-step optimization is essential. An optimal wavefront is found to achieve simultaneously both a micrometer focal spot size (down to 20 μm diameter) and high intensity (more than a 100-fold enhancement) inside the scattering media. Our method promises a new route in life science towards focusing, imaging or manipulating deep into biological tissues with linear fluorescent agents. Copyright © 2020, The Authors. All rights reserved.

关键词： Fluorescence

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Research on Highly Anti-Humidity and Selective NO2 Detection Based on GaN/MoO3 N-N Heterojunction

SSRN

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SSRN 2024年

作者： Hong, Yutao Han, Dan Li, Donghui He, Xiuli Zhao, Li Wang, Weidong Li, Hongwei Sang, Shengbo Liang, Hua Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China State Key Laboratory of Transducer Technology Aerospace Information Research Institute Chinese Academy of Sciences Beijing100190 China Bioengineering Research Center Medical Innovation Research Division Chinese PLA General Hospital Beijing China Shanxi Academy of Medical Sciences China

Effective and accuratedetection of NO2 gas is crucial for protecting the environment and public health. In this work, balsam pear-like GaN/MoO3 porous nanosheets (GaN/MoO3) composites were synthesized by the in situ assembling, the hydrothermal method, and the nitridation process to detect NO2. A series of characterization methods were used to manifest the successful synthesis and to analyze the morphology and elemental composition features of GaN/MoO3 composites. The results of the gas-sensing experiments show that at the operating temperature of 225 °C, the gas sensor based on the optimal ratio of GaN/MoO3 composites exhibits a low theoretical limit of detection (0.78 ppb) for NO2, which is significantly improved compared with the limit of detection of MoO3 (5 ppm). Further, the response value of the sensor based on GaN/MoO3 composites to 200 ppm NO2 (44.74) is 4.36 times higher than that of the sensor based on pure GaN, with an improvement in stability. Meanwhile, the sensor also possessed excellent repeatability, selectivity, stability, and splendid anti-humidity ability at 15-70 % RH. The improved gas-sensing performance is ascribed to the unique microstructure of both GaN and MoO3, and the heterojunction effect between them. This work provides a way to improve the efficiency and anti-humidity ability of real-time monitoring of NO2 for the sensors of MoO3-based composite. © 2024, The Authors. All rights reserved.

关键词： Gallium nitride

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AU Nanoparticles Decorated Gan Nanoflowers with Enhanced Nh3 Sensing Performance at Room Temperature

SSRN

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SSRN 2023年

作者： Han, Dan Chen, Yi Li, Donghui Shi, Jiexu Wang, Hongtao He, Xiuli Zhao, Li Wang, Weidong Sang, Shengbo Ji, Jianlong Shanxi Key Laboratory of Micro Nano Sensors and Artificial Intelligence Perception College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System The Ministry of Education Taiyuan University of Technology Taiyuan030024 China State Key Laboratory of Transducer Technology Aerospace Information Research Institute Chinese Academy of Sciences Beijing100190 China Bioengineering Research Center Medical Innovation Research Division Chinese PLA General Hospital Beijing China Shanxi Research Institute of 6D Artificial Intelligence Biomedical Science China

Surface modification with noble metal is considered as an effective strategy to enhance sensing performance of semiconductor gas sensors. In this work, gold nanoparticles (Au NPs) decorated Gallium Nitride nanoflowers (Au-GaN NFs) have been synthesized successfully by a feasible hydrothermal method combined with high temperature nitridation and followed by in-situ reduction process. The characterizations of the structure and morphology of as-obtained Au-GaN NFs indicated that the Au NPs were successfully loaded on the surface of GaN. The excellent gas sensing performance was observed for GaN of 2 mol% Au loaded, including the high response (86.8%) to 100 ppm NH3 with fast response/recovery time (41 s/169 s) at room temperature, low theoretical limit of detection (72 ppb), good stability and selectivity. Besides, the influence of humidity on the performance of sensors was explored, where the response can be reached 56.5% towards 100 ppm NH3 under 70% RH. The improvement of the sensing performance of Au-GaN NFs sensor can be attributed to the combined action of chemical and electronic sensitization of Au NPs. This work provides a candidate of Au-GaN NFs for the development of wireless sensing system in NH3 monitoring. © 2023, The Authors. All rights reserved.

关键词： Nanoflowers

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Fast all-optical random number generator

arXiv

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arXiv 2022年

作者： Zhao, Jiamin Li, Pu Zhang, Xing Gao, Zhensen Jia, Zhiwei Bogris, Adonis Alan Shore, K. Wang, Yuncai Key Laboratory of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China School of Information Engineering Guangdong University of Technology Guangzhou510006 China Guangdong Provincial Key Laboratory of Photonics Information Technology Guangzhou510006 China Key Laboratory of Specialty Fiber Optics and Optical Access Networks Shanghai University Shanghai200444 China Changchun Institute of Optics Fine Mechanics and Physics Chinese Academy of Sciences Changchun130033 China Department of Informatics and Computer Engineering University of West Attica Athens12243 Greece School of Electronic Engineering Bangor University WalesLL57 1UT United Kingdom

We propose a simple and all-optical method for fast random number generation based on the laser mode hopping. Through periodically restarting a two-mode laser operating in the bistable state, a random number stream can be generated due to the spontaneous emission noise. To validate the feasibility of this method, we perform a theoretical simulation using the common vertical-cavity surface-emitting laser (VCSEL) with two polarization modes. Numerical results demonstrate that fast 2.5 Gb/s random number streams can be continuously obtained with verified randomness. This scheme provide a fully monolithic solution for random number generator, due to its simple and all-optical structure. Copyright © 2022, The Authors. All rights reserved.

关键词： Random number generation

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