检索结果-内蒙古大学图书馆

Asymmetric impacts of natural and anthropogenic factors on wetland landscape evolution in Fenhe River Basin, China

Watershed Ecology and the environment 2024年第1期6卷 176-186页

作者： Xie, Chengjie Zeng, Yingzheng Hao, Xiaoyang Ning, Zhonghua Xie, Tian School of Environment and Resource Taiyuan University of Technology Taiyuan 030024 China Key Laboratory of Investigation Monitoring and Protection of Natural Resources in Mining Cities Coal Geological Geophysical Exploration Surveying & Mapping Institute of Shanxi Province Jinzhong 030600 China School of Ecology and Nature Conservation Beijing Forestry University Beijing 100083 China School of Environment State Key Joint Laboratory of Environmental Simulation and Pollution Control Beijing Normal University Beijing 100875 China

In recent years, Fenhe River Basin (FRB) wetlands have been facing severe challenges due to climate change and human activities. It was of great significance to understand the dynamic changes of FRB wetlands and their driving factors for ecological protection. Based on the land use data, runoff, rainfall and GDP data of FRB from 1980 to 2020, the evolution characteristics and driving factors of wetland pattern in FRB were analyzed. The results showed that the wetland types in FRB mainly included paddy, reservoir, river, beach and marsh. Among them, natural wetlands accounted for 72.46 %, and constructed wetlands accounted for 27.53 %. The main types of wetlands in FRB were river, reservoirs and beach, which account for 92.26 % of the whole wetland area. However, the dominant position of reservoir patch was more obvious than the others during 1980–2020. Landscape index showed that the shape of landscape tended to be regular and became more fragmentation. The transfer between wetlands and other land use types mainly occurred in the northern and southern parts of the FRB, and the main conversion types were occurred between dry land and wetlands, grassland and wetlands. Both natural and human factors drove the evolution pattern of wetlands, but the emphases were different. Runoff had a significant effect on wetland pattern at landscape level, while rainfall had a more significant effect on wetland evolution at class level. Urbanization rate and GDP had important effects on the evolution of wetland pattern at both class and landscape levels. © 2024 The Authors

关键词： Fenhe basin Land use types Landscape index Shanxi province Wetlands

来源：评论

学校读者我要写书评

暂无评论

Hydrothermal aging alleviates hydrocarbon poisoning effects on high-silica Cu-SSZ-16 catalysts for NH3-SCR

引用

Journal of environmental Sciences (China) 2025年 158卷 13-23页

作者： Zhou, Huan Liu, Jianqi Zhang, Yan Han, Shichao Du, Jinpeng Shan, Wenpo Fujian Key Laboratory of Atmospheric Ozone Pollution Prevention Institute of Urban Environment Chinese Academy of Sciences Xiamen361021 China Zhejiang Key Laboratory of Pollution Control for Port-Petrochemical Industry Ningbo Urban Environment Observation and Research Station Institute of Urban Environment Chinese Academy of Sciences Ningbo315800 China Shanghai Advanced Research Institute Chinese Academy of Sciences Shanghai201210 China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing100085 China

Hydrocarbons (HCs) exert toxic effects on the activity of Cu-based zeolite catalysts for NH3-SCR on diesel vehicles. This study investigated the hydrocarbon resistance of both fresh and hydrothermally aged high-silica Cu-SSZ-16 catalysts. It was found that low-temperature activity of Cu-SSZ-16 catalyst decreased after C3H6 poisoning, which was mainly due to the blockage of pore channels and the coverage of Cu active sites as well as acid sites by the formation of carbon deposits. Additionally, [Cu(OH)]+-Z was proposed to be more easily affected by C3H6 poisoning than Cu2+-2Z. Hydrothermally aged Cu-SSZ-16 presented better C3H6 resistance than the fresh catalyst since less carbon deposits were accumulated and [Cu(OH)]+-Z species were partially transformed to more-stable Cu2+-2Z in the aged sample. This was probably because of the reduction of acid sites and the formation of CuOx, which enhanced the oxidation of C3H6, thereby inhibiting the formation of carbon deposits. In addition, the coverage of the active Cu species also influenced the adsorption and oxidation of NO, causing a decrease in low-temperature activity. Thus, the low-temperature activity could be fully recovered by hydrothermal treatment at 500 °C due to the removal of carbon deposits and recovery of Cu active sites as well as acid sites. In summary, high-silica Cu-SSZ-16, with high resistance to HCs and excellent hydrothermal stability, is a competitive candidate as a catalyst for the NH3-SCR reaction in practical application. © 2024

关键词： Cu-SSZ-16 Diesel exhaust Hydrocarbon poisoning Hydrothermal aging NH3-SCR

来源：评论

学校读者我要写书评

暂无评论

Potential Effects of Cu2+ Stress on Nitrogen Removal Performance, Microbial Characteristics, and Metabolism Pathways of Biofilm Reactor

SSRN

引用

SSRN 2024年

作者： Zhang, Shuai Huang, Xiao Dong, Wenyi Wang, Hongjie Hu, Liangshan Zhou, Guorun Zheng, Zhihao Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control School of Environmental Science and Engineering Nanjing University of Information Science & Technology Nanjing210044 China Shenzhen518055 China State Key Laboratory of Urban Water Resource and Environment School of Environment Harbin Institute of Technology Harbin150090 China

Sequencing batch biofilm reactors (SBBR) were utilized to investigate the impact of Cu2+ on nitrogen (N) removal and microbial characteristics. The result indicated that the low concentration of Cu2+ facilitated the removal of ammonia nitrogen (NH4+-N), total nitrogen (TN). Compared with the control group of the average effluent concentration, the average effluent concentrations of NH4+-N, TN were found to decrease by 40.53%, 15.86%, respectively. Conversely, the high concentration of Cu2+ resulted in a increase of 94.27%, 14.23% in the aforementioned parameters, compared with the control group. The addition of low concentrations of Cu2+ significantly (P © 2024, The Authors. All rights reserved.

关键词： Nitrogen removal

来源：评论

学校读者我要写书评

暂无评论

Coordinated control of Fine-Particle and Ozone pollution by the Substantial Reduction of Nitrogen Oxides

引用

Engineering 2022年第8期8卷 13-16页

作者： Biwu Chu Yan Ding Xiang Gao Junhua Li Tingyu Zhu Yunbo Yu Hong He State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of the Chinese Academy of Sciences Beijing 100049China Chinese Research Academy of Environmental Sciences Beijing 100012China State Environmental Protection Engineering Center for Coal-Fired Air Pollution Control Zhejiang UniversityHangzhou 310027China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China National Engineering Laboratory for Hydrometallurgical Cleaner Production Technology Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

*** In recent years,the air quality in China has improved *** many cities,however,the concentration of fine particulate matter(PM_(2.5))remains higher than the secondary-level national ambient air quality standard(NAAQS level-2,35μg·m^(-3),GB3095-2012[1])and much higher than the first-level NAAQS(15μg·m^(-3),GB3095-2012[1])and the World Health Organization(WHO)air quality guidelines(5μg·m^(-3)).

关键词： pollution Ozone ambient

来源：评论

学校读者我要写书评

暂无评论

Development of a Method to Determine the environmental Burden of Diseases and an Application to Identify Factors Driving Changes in the Number of PM_(2.5)-Related Deaths in China between 2000 and 2010

引用

environment & Health 2024年第9期2卷 642-650页

作者： Ning Kang Pengfei Li Tao Xue Tong Zhu Institute of Reproductive and Child Health National Health Commission Key Laboratory of Reproductive Health/Department of Epidemiology and BiostatisticsMinistry of Education Key Laboratory of Epidemiology of Major Diseases(PKU)School of Public HealthPeking University Health Science CenterBeijing 100191China Institute of Medical Technology Peking University Health Science CenterBeijing 100191China Advanced Institute of Information Technology Peking UniversityHangzhou 311215China State Environmental Protection Key Laboratory of Atmospheric Exposure and Health Risk Management and Center for Environment and HealthPeking UniversityBeijing 100871China State Environmental Protection Key Laboratory of Atmospheric Exposure and Health Risk Management and Center for Environment and Health and State Key Joint Laboratory of Environment Simulation and Pollution ControlCollege of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China

The attributable burden is codetermined by the exposure level and nontarget ***,the conventional method of health impact assessment based on preestablished exposure−response functions includes only a few well-known characteristics and thus is insufficient to capture the comprehensive *** aimed to develop a method to fuse health impact assessment with epidemiological analysis and to identify factors driving baseline *** method was applied to identify the factors underlying the change in the number of fine particulate matter(PM_(2.5))related deaths in China between 2000 and *** the study period,the number of PM_(2.5)-related deaths across China's Mainland increased by 0.62(95%CI:0.57,0.69)million,with 0.65(95%CI:0.47,0.91)million,0.55(95%CI:0.39,0.79)million,and 0.11(95%CI:0.06,0.18)million deaths being associated with increased PM_(2.5)exposure,population aging,and growth in population size,***,economic growth,urbanization,improvement of welfare services,and improvement of hospital services resulted in 0.25(95%CI:0.15,0.40)million,0.16(95%CI:0.10,0.27)million,0.16(95%CI:0.09,0.26)million,and 0.09(95%CI:0.05,0.15)million fewer deaths,*** indicated that increased exposure was the major driver of the change in the number of PM_(2.5)-related deaths,and economic growth was the main driver of increased resilience to air pollution.

关键词： health burden decomposition analysis air pollution fine particulate matter premature deaths

来源：评论

学校读者我要写书评

暂无评论

Nano-sized Ag rather than single-atom Ag determines CO oxidation activity and stability

引用

Nano Research 2022年第1期15卷 452-456页

作者： Fei Wang Zhao Li Honghong Wang Min Chen Changbin Zhang Ping Ning Hong He State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Faculty of Environmental Science and Engineering Kunming University of Science and TechnologyKunming 650500China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China

Single-atom catalysis recently attracts great attentions,however,whether single atom or their nanoparticle(NP)has the advantage in its intrinsic activity remains under heated ***/Al_(2)O_(3) is a widely used catalyst for many catalytic reactions,while the effect of Ag particle size on the actity is seldom investigated due to the great difficulty in synthesizing single atom Ag and Ag clusters/particles with different ***,we firstly prepared an atomically dispersed Ag/Al_(2)O_(3) catalyst using a nano-sized y-Al_(2)O_(3) as the support,subsequently obtained a series of Ag/Al_(2)O_(3) catalysts with different Ag particle sizes by H_(2) reducing single-atom Ag/Al_(2)O_(3) catalyst at various *** Ag/Al_(2)O_(3) treated at 600℃demonstrated superior CO oxidation performance over single-atom Ag/Al_(2)O_(3) and the Ag/Al_(2)O_(3) treated at 400 and 800℃.Based on experimental data and dpnsity functional theory(DFT)calculation results,we reveal that the larger Ag°particle is beneficial to oxygen activation and improves the valence stability during oxidation reaction,while the aggregation of Ag°particle also accordingly decreases the concentration of surface active sites,hence,there is an optimum Ag0 particle *** findings clearly confirm that Ag0nanoparticle has the advantage over single-atom Ag species in its intrinsic activity for CO oxidation.

关键词： Reduction after anchoring Ag clusters single atom catalyst CO oxidation

来源：评论

学校读者我要写书评

暂无评论

Phosphorus removal from sediments by Potamogeton crispus:New high-resolution in-situ evidence for rhizosphere assimilation and oxidization-induced retention

引用

Journal of environmental Sciences 2021年第11期33卷 181-192页

作者： Hezhong Yuan Yiwei Cai Zhen Yang Qiang Li Enfeng Liu Hongbin Yin Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control and Collaborative Innovation Center of Atmospheric Environment and Equipment Technology(CICAEET) School of Environmental Science and EngineeringNanjing University of Information Science and TechnologyNanjing 210044China State Key Laboratory of Lake Science and Environment Nanjing Institute of Geography and LimnologyChinese Academy of SciencesNanjing 210008China Department of Soil Science University of Wisconsin-Madison53706 MadisonWIUnited States College of Geography and Environment Shandong Normal UniversityJi’nan 250359China

Macrophytes are usually chosen for phytoremediation tools to remove P in eutrophic aquatic ecosystems,but the lack of test methods hinders the understanding of removal mechanism and *** this study,we used the novel technologies combined of Diffusive gradients in thin films(DGT),Planar optode(PO),and Non-invasive micro-test technology(NMT)to explore P dynamics in water-sediment continuum and rhizosphere of Potamogeton crispus over *** of the high-resolution in situ measurement showed that labile P(LPDGT)fluxes at the surficial sediment significantly decreased from approximate 120,140,and 200 pg/(cm^(2)·sec)via 30 days incubation period to 17,40,and 56 pg/(cm2•sec)via that of 15 *** synchronous increase of LPDGT was not detected in overlying water,suggesting the intense assimilation of dissolve reactive P via root over *** measurement indicated that O_(2)concentration around the rhizosphere remarkably increased and radially diffused into deeper sediment until 100%saturation along with the root stretch *** detection of roots showed the obvious O_(2)inflow into root tissue with the uppermost flux of 30 pmol/(cm2•sec)from surroundings via aerenchyma on different treatment *** from previous reports,gradually saturating O_(2)concentrations around the rhizosphere was principally driven by O_(2)penetration through interspace attributing to root stretch downward rather than root O_(2)*** O_(2)concentrations in deep sediment over time finally induced the oxidization of labile Fe(II)into Fe(III)bound P and local P immobilization.

关键词： Phosphorus removal Potamogeton crispus Diffusive gradients in thin films (DGT) Planar optode(PO) Non-invasive Micro-test Technique (NMT) Rhizosphere

来源：评论

学校读者我要写书评

暂无评论

Rapid screening of acetylcholinesterase active contaminants in water: A solid phase microextraction-based ligand fishing approach

引用

Chemosphere 2024年 356卷 141976页

作者： Huang, Zhoubing He, Liwei Li, Huizhen Zhao, Junbo Chen, Tianyang Feng, Ziang Li, Yangyang You, Jing The Key Laboratory of Environmental Pollution Monitoring and Disease Control Ministry of Education School of Public Health Guizhou Medical University Guian New Area 561113 China Guangdong Key Laboratory of Environmental Pollution and Health School of Environment Jinan University Guangzhou511443 China

Effect-directed analysis (EDA) has been increasingly used for screening toxic contaminants in the environment, but conventional EDA procedures are often time-consuming and labor-extensive. This challenges the use of EDA for toxicant identification in the scenarios when quick answers are demanded. Herein, a solid phase microextraction ligand fishing (SPME-LF) strategy has been proposed as a rapid EDA approach for identifying acetylcholinesterase (AChE) active compounds in water. The feasibility of ligand fishing techniques for screening AChE active chemicals from environmental mixtures was first verified by a membrane separation method. Then, SPME fibers were prepared through self-assembly of boronic acid groups with AChE via co-bonding and applied for SPME-LF. As AChE coated SPME fibers selectively enriched AChE-active compounds from water, comparing sorbing compounds by the SPME fibers with and without AChE coating can quickly distinguish AChE toxicants in mixtures. Compared with conventional EDA, SPME-LF does not require repeating sample separations and bioassays, endowing SPME-LF with the merits of low-cost, labor-saving, and user-friendly. It is believed that cost-efficient and easy-to-use SPME-LF strategy can potentially be a rapid EDA method for screening receptor-specific toxicants in aquatic environment, especially applicable in time-sensitive screening. © 2024 Elsevier Ltd

关键词： Ligands

来源：评论

学校读者我要写书评

暂无评论

Microplastics in soils: Production, behavior process, impact on soil organisms, and related toxicity mechanisms

引用

Chemosphere 2024年 350卷 141060页

作者： Li, Kun Xiu, Xiaojia Hao, Wanqi School of Environmental Science and Engineering Nanjing University of Information Science and Technology Nanjing210044 China Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology China Changwang School of Honors Nanjing University of Information Science and Technology Nanjing210044 China

In recent years, microplastics (MPs) pollution has become a hot ecological issue of global concern and MP pollution in soil is becoming increasingly serious. Studies have shown that MPs have adverse effects on soil biology and ecological functions. Although MPs are evident in soils, identifying their source, abundance, and types is difficult because of the complexity and variability of soil components. In addition, the effects of MPs on soil physicochemical properties (PCP), including direct effects such as direct interaction with soil particles and indirect effects such as the impact on soil organisms, have not been reported in a differentiated manner. Furthermore, at present, the soil ecological effects of MPs are mostly based on biological toxicity reports of their exudate or size effects, whereas the impact of their surface-specific properties (such as environmentally persistent free radicals, surface functional groups, charge, and curvature) on soil ecological functions is not fully understood. Considering this, this paper reviews the latest research findings on the production and behavioral processes of MPs in soil, the effects on soil PCP, the impacts on different soil organisms, and the related toxic mechanisms. The above discussion will enhance further understanding of the behavioral characteristics and risks of MPs in soil ecosystems and provide some theoretical basis for further clarification of the molecular mechanisms of the effects of MPs on soil organisms. © 2023 Elsevier Ltd

关键词： Soils

来源：评论

学校读者我要写书评

暂无评论

An Ensemble Machine Learning Approach for Predicting Sources of Organic Aerosols Measured by Aerosol Mass Spectrometry

ACS ES&T Air

引用

ACS ES&T Air 2025年第3期2卷 378-385页

作者： Yunjiang Zhang Jie Fang Qingxiao Meng Xinlei Ge Hasna Chebaicheb Olivier Favez Jean-Eudes Petit Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control School of Environmental Science and Engineering Nanjing University of Information Science and Technology Nanjing 210044 China；Institut National de l’Environnement Industriel et des Risques Verneuil-en-Halatte 60550 France Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control School of Environmental Science and Engineering Nanjing University of Information Science and Technology Nanjing 210044 China Institut National de l’Environnement Industriel et des Risques Verneuil-en-Halatte 60550 France Laboratoire des Sciences du Climat et de l’Environnement CEA/Orme des Merisiers Gif sur Yvette 91191 France

Long-term source apportionment of atmospheric organic aerosols (OA) is essential for supporting air pollution management strategies. While aerosol mass spectrometry (AMS) combined with traditional source apportionment tools can accurately identify various OA sources, they face efficiency challenges when processing large volumes of long-term data. This study proposes an ensemble machine learning approach to efficiently apportion OA sources from long-term AMS measurements. Using six-year observation of a simplified version of AMS (i.e., ACSM) in the Paris region along with OA factor data derived from positive matrix factorization analysis, we developed an ensemble machine learning source apportionment model. Compared to individual machine learning algorithms, the ensemble model substantially reduced the root-mean-square error (RMSE) and increased the correlation coefficient in predicting OA sources by approximately 30% and 5%, respectively. Sensitivity analysis with five years of baseline data revealed that model performance relatively stabilizes when the training data exceeds two years, with RMSE values for primary and secondary OA factors at 0.31–0.45 μg/m3and 0.69–0.84 μg/m3, respectively. This ensemble model not only enhances the efficiency of long-term OA source apportionment but also holds potential for near-real-time online applications.

关键词：

来源：评论

学校读者我要写书评

暂无评论

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案：

请选择收藏分类：

通借通还

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：