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Particle number size distributions and formation and growth rates of different new particle formation types of a megacity in China

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Journal of environmental Sciences 2023年第9期131卷 11-25页

作者： Liang Dai Yu Zhao Lei Zhang Dong Chen Rongrong Wu State Key Laboratory of Pollution Control and Resource Reuse and School of the Environment Nanjing UniversityJiangsu 210023China Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology(CICAEET) Nanjing University of Information Science and TechnologyJiangsu 210044China

To understand the contribution of new particle formation(NPF)events to ambient fine particle pollution,measurements of particle size distributions,trace gases and meteorological conditions,were conducted at a suburban site(NJU)from October to December 2016 and at an industrial site(NUIST)from September to November 2015 in *** to the temporal evolution of the particle size distributions,three types NPF events were observed:typical NPF(Type A),moderate NPF events(Type B)and strong NPF(Type C)*** favorable conditions for Type A events included low relative humidity,low concentration of pre-existing particles,and high solar *** favorable conditions of Type B events were similar to Type A,except for a higher concentration of pre-existing *** C events were more likely to happen with the higher relative humidity,lower solar radiation and continuous growth of pre-existing particle *** formation rate of 3 nm(J3)was the lowest for Type A events and highest for Type C *** contrast,the growth rates of 10 nm and 40 nm particles were the highest for Type A,and lowest for Type *** show that NPF events with only higher J3 would lead to the accumulation of nucleation mode *** acid was important for the formation of particles but had little effect on the growth of particle size.

关键词： New particle formation Size distribution Formation and growth rate Aerosol pollution

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Ultralong-life lithium metal batteries enabled by decorating robust hybrid interphases on 3D layered framworks

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Chinese Chemical Letters 2023年第5期34卷 610-615页

作者： Qiongjie Ke Qingshuai Xu Xuejun Lai Xianfeng Yang Huichun Gao Zaisheng Wang Yongcai Qiu School of Environment and Energy State Key Laboratory of Luminescent Materials and DeviceGuangdong Provincial Key Laboratory of Atmospheric Environment and Pollution ControlSouth China University of TechnologyGuangzhou 510000China EVE Energy Co. Ltd.Huizhou 516000China

Stable solid-electrolyte interphase(SEI)is crucial for advanced development of lithium metal ***,the continuous collapse and reconstruction of SEI will deplete fresh Li and electrolytes upon cycling,leading to irreversible capacity ***,we addressed this issue by pre-formation of artificial robust hybrid interphase on a 3D layered graphene/lithium metal framework,in which is constructed by LiF associated with Li2TiF 6generated by the in-situ reaction between the surfacial lithium and titanium fluoride contained *** as-obtained interphase can maintain the structure integrality and avoid continuous consumption of the fresh Li and *** a consequence,the Li symmetric cells achieve high-efficiency Li deposition and stable cycling over 3600 *** paired with LiFePO_(4)cathodes,the coin cells exhibit long lifespan(>800 cycles)with almost 88.3%retention of the initial capacity.

关键词： Lithium metal battery TiF_4 Artificial SEI Dendrite free 3D frameworks

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Chemical characterization of volatile organic compounds (VOCs) emitted from multiple cooking cuisines and purification efficiency assessments

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Journal of environmental Sciences 2023年第8期130卷 163-173页

作者： Hanyu Zhang XuejunWang Xianbao Shen Xin Li BoboWu Guohao Li Huahua Bai Xinyue Cao Xuewei Hao Qi Zhou Zhiliang Yao School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China State Environmental Protection Key Laboratory of Food Chain Pollution Control Beijing Technology and Business UniversityBeijing 100048China Beijing Municipal Research Institute of Environmental Protection Beijing Key Laboratory of Urban Atmospheric Volatile Organic Compounds Pollution Control and ApplicationNational Urban Environmental Pollution Control Engineering Research CenterBeijing 100037China

Cooking process can produce abundant volatile organic compounds(VOCs),which are harmful to environment and human ***,we conducted a comprehensive analysis in which VOCs emissions from multiple cuisines have been sampled based on the simulation and acquisition platform,involving concentration characteristics,ozone formation potential(OFP)and purification efficiency *** emissions varied from 1828.5 to 14,355.1μg/m^(3),with the maximumand minimumvalues fromBarbecue and Family cuisine,*** and alcohol had higher contributions to VOCs from Sichuan and Hunan cuisine(64.1%),Family cuisine(66.3%),Shandong cuisine(69.1%)and Cantonese cuisine(69.8%),with the dominant VOCs species of ethanol,isobutane and *** comparison,alcohols(79.5%)were abundant for Huaiyang cuisine,while alkanes(19.7%),alkenes(35.9%)and haloalkanes(22.9%)accounted for higher proportions from ***,carbon tetrachloride,n-hexylene and 1-butene were the most abundant VOCs species for Barbecue,ranging from 8.8%to 14.6%.The highest OFP occurred in *** sensitive species of OFP for Huaiyang cuisine were alcohols,while other cuisines were *** efficiency assessments shed light on the removal differences of individual and synergistic control *** emissions exhibited a strong dependence on the photocatalytic oxidation,with the removal efficiencies of 29.0%–54.4%.However,the high voltage electrostatic,wet purification and mechanical separation techniques played a mediocre or even counterproductive role in the VOCs reduction,meanwhile collaborative control technologies could not significantly improve the removal *** results identifiedmore effective control technologies,which were conductive to alleviating air pollution from cooking emissions.

关键词： Cooking emissions Volatile organic compounds(VOCs) VOCs categories Ozone formation potential(OFP) Purification efficiency

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Acute Effects of Exposure to Fine Particulate Matter and Its Constituents on Sex Hormone Among Postmenopausal Women — Beijing, Tianjin, and Hebei PLADs, China, 2018–2019

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China CDC weekly 2024年第13期6卷 249-253,I0001-I0004页

作者： Yanlin Tian Jiaonan Wang Jianlong Fang Chen Chen Feng Zhao Yi Zhang Peng Du Yawei Li Wanying Shi Yuanyuan Liu Enmin Ding Song Tang Xu Yue Xiaoming Shi Chinese Research Academy of Environmental Sciences BeijingChina Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control(AEMPC)Nanjing University of Information Science&TechnologyNanjing CityJiangsu ProvinceChina China CDC Key Laboratory of Environment and Population Health National Institute of Environmental HealthChinese Center for Disease Control and PreventionBeijingChina Department of Epidemiology and Health Statistics School of Public HealthCapital Medical Universityand Beijing Municipal Key Laboratory of Clinical EpidemiologyBeijingChina National Key Laboratory of Intelligent Tracking and Forecasting for Infectious Diseases National Institute of Environmental HealthChinese Center for Disease Control and PreventionBeijingChina

What is already known on this topic?Exposure to fine particulate matter(PM_(2.5))was linked to endocrine hormone disruption in the reproductive ***,it was unclear which specific components of PM_(2.5) were primarily responsible for these *** is added by this report?The study presented the initial epidemiological evidence that brief exposure to PM_(2.5) can elevate estradiol levels in postmenopausal *** particle components had unique effects,with watersoluble ions and specific inorganic elements like Ag,As,Cd,Hg,Ni,Sb,Se,Sn,and Tl potentially playing significant roles in increasing estradiol *** are the implications for public health practice?The study established that the prevalence of air pollution,along with its specific components,has been recognized as a novel risk factor affecting the balance of sex hormones.

关键词： pollution Particulate primarily

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Formaldehyde oxidation on Pd/USY catalysts at room temperature: The effect of acid pretreatment on supports

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Journal of environmental Sciences 2023年第3期125卷 811-822页

作者： Xiaofeng Liu Chunying Wang Yumin Chen Qi Qin Yaobin Li Hong He Center for Excellence in Regional Atmospheric Environment Key Laboratory of Urban Pollutant ConversionChinese Academy of SciencesInstitute of Urban EnvironmentXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China Zhejiang Key Laboratory of Urban Environmental Processes and Pollution Control Chinese Academy of SciencesNingbo Urban Environment Observation and Research Station-NUEORSNingbo 315800China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-environmental SciencesChinese Academy of SciencesBeijing 100085China Xiamen Key Laboratory of Materials for Gaseous Pollutant Control Chinese Academy of SciencesInstitute of Urban EnvironmentXiamen 361021China

The complete catalytic oxidation of formaldehyde (HCHO) to CO_(2)and H_(2)O at room temperature is a green route for indoor HCHO *** is an excellent carrier material for HCHO oxidation due to its large surface area,intricate pores and high adsorption ***,the zeolite-supported noble metal catalysts have currently shown relatively low activity especially at room *** this work,we present a facile acid treatment strategy for zeolite catalysts to improve the hydroxyl concentration and further enhance their catalytic activity for HCHO *** tests illustrated that HCHO could be completely oxidized to CO_(2)and H_(2)O at a nearly 100%conversion rate with a weight hourly space velocity (WHSV) of 150,000 mL/(g·hr) at 25℃,when the support of Pd/USY catalysts was pretreated by hydrochloric acid with a concentration of 0.20 mol/*** characterization results revealed that the active hydroxyl groups originated from the dealumination in the acid treatment play a key role in the HCHO oxidation *** deduced reaction mechanism suggests that bridging hydroxyl groups may oxidize HCHO to dioxymethylene(DOM) species and terminal hydroxyl groups are responsible for the transformation of DOM groups to formate (HCOO) species.

关键词： Formaldehyde oxidation USY zeolite Acid treatment Hydroxyl groups

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Mechanism for the promotional formation of NH_(4)^(+) by SO_(2) on different mineral dust surfaces

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Particuology 2023年第4期75卷 109-118页

作者： Hao Li Qingxin Ma Biwu Chu Hong He State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-environmental SciencesChinese Academy of SciencesBeijing100085China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen361021China Institute of Atmospheric Physics Chinese Academy of SciencesBeijing100029China

Ammonium is an important atmospheric particulate component that dictates many environmental *** promotion of the heterogeneous conversion of NH_(3) to NH_(4)^(+) by SO_(2) on different mineral dust surfaces displays remarkable discrepancies,especially on MgO and α-Fe2O3 surfaces,however,the underlying mechanisms are not well ***,using periodic density functional theory(DFT)calculation and Born-Oppenheimer molecular dynamics(BOMD)simulation,we explored the hetero-geneous adsorption of NH_(3) on MgO(110)and α--Fe2O3(001)surfaces in the presence and absence of SO_(2).The results show that on MgO(110)surface,hydrogen-bonding interactions of NH_(3) on both adsorbed hydroxyl or bisulfite/bisulfate sites are observed no matter whether SO_(2) is present or ***,on theα-Fe2O3(001)surface,significant conversion of NH_(3) to NH_(4)^(+)occurs with the coexistence of SO_(2),which is due to the hydrogen transfer reaction from surface HSO4 to N in NH_(3).The fundamental reason may be that the stronger electron affinity of Fe3+than Mg2+results in adsorbed bisulfate and/or bisulfite with greater acidity on α-Fe2O3 surface than MgO *** results give a molecular-level explanation for the heterogeneous conversion of NH_(3) to NH_(4)^(+)on different mineral dust surfaces under complex air pollution *** the fact that ammonium is abundant in secondary particulates,this work would help in understanding the rapid conversion of ammonia to ammonium and in developing classification governance policies for the key precursor pollutants in China.

关键词： Mineral dust Heterogeneous reaction Theoretical calculation Ammonium SO_(2)

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A review of whole-process control of industrial volatile organic compounds in China

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Journal of environmental Sciences 2023年第1期123卷 127-139页

作者： Hailin Wang Shumei Sun Lei Nie Zhongshen Zhang Wenpeng Li Zhengping Hao Beijing Key Laboratory for Urban Atmospheric VOCs Pollution Control and Technology Application Beijing Municipal Research Institute of Environmental ProtectionBeijing 100037China College of Resources Environment and Tourism Capital Normal UniversityBeijing 100048China National Engineering Laboratory for VOCs Pollution Control Material&Technology Research Center for Environmental Material and Pollution Control TechnologyUniversity of Chinese Academy of SciencesBeijing 101408China

Volatile organic compounds(VOCs)play an important role in the formation of ground-level ozone and secondary organic aerosol(SOA),and they have been key issues in current air pollution prevention and control in *** attention has been paid to industrial activities due to their large and relatively complex VOCs *** present research aims to provide a comprehensive review on whole-process control of industrial VOCs,which mainly includes source reduction,collection enhancement and end-pipe *** VOCs materials including water-borne ones are the keys to source substitution in industries related to coating and solvent usage,leak detection and repair(LDAR)should be regarded as an efficient means of source reduction in refining,petrochemical and other chemical *** types of VOCs collection methods such as gas-collecting hoods,airtight partitions and others are discussed,and airtight collection at negative pressure yields the best collection *** end-pipe treatments like UV oxidation,low-temperature plasma,activated carbon adsorption,combustion,biodegradation,and adsorption-combustion are discussed in ***,several recommendations are made for future advanced treatment and policy development in industrial VOCs emission control.

关键词： Volatile organic compounds Materials substitution Collection enhancement End-pipe treatments

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Significant changes in the physicochemical properties of BC-containing particles during the cold season in Beijing

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Journal of environmental Sciences 2025年第5期151卷 667-676页

作者： Shuya Hu Linghan Zeng Gang Zhao Shiyi Chen Chunsheng Zhao Weilun Zhao Min Hu State Key Joint Laboratory of Environmental Simulation and Pollution Control International Joint Research Center for Atmospheric Research(IJRC)College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China Department of Atmospheric and Oceanic Sciences School of PhysicsPeking UniversityBeijing 100871China Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Nanjing University of Information Science and TechnologyNanjing 210044China

The ambient air quality has improved significantly under strict emission controls in Beijing,China over the last *** carbon(BC),as a short-lived climate forcer in ambient aerosols,profoundly impacts the air quality and *** studies have demonstrated a decline in the mass concentration of *** this study,we characterized the chemical compositions and size distributions of BC-containing particles during the cold season of 2022 in Beijing using state-of-the-art instruments capable of exclusively measuring BCcontaining *** optical properties of BC-containing particles were further calculated based on the Mie ***,we compared the properties of BC-containing particles in 2022 with the results of previous *** results showed that the diameters of BC cores became larger while the coating thickness of BC-containing particles became thinner in *** the coating materials,the mass fraction of nitrate increased obviously,and even replaced organic matter as the dominant component during the peak of the pollution *** in chemical compositions and size distributions resulted in lower mass absorption cross-sections(MAC)of BC-containing particles from 10.5±1.1 m^(2)/g in 2016 to 7.3±0.8 m^(2)/g in 2022,reduced by 30.5%.Our results demonstrate the synergistic benefits of air pollution control in improving air quality and mitigating climate ***,the MAC of BC adopted in climate models should vary with the changing air pollution *** study emphasizes that it is imperative to conduct long-term observations of BC-containing particles to better estimate BC’s climate effects.

关键词： Black carbon Chemical composition Size distribution Light absorption ability

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Improved atmospheric mercury simulation using updated gas-particle partition and organic aerosol concentrations

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Journal of environmental Sciences 2022年第9期34卷 106-118页

作者： Kaiyun Liu Qingru Wu Shuxiao Wang Xing Chang Yi Tang Long Wang Tonghao Liu Lei Zhang Yu Zhao Qin’geng Wang Jinsheng Chen State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Institute of Atmospheric Environment Guangdong provincial academy of environmental scienceGuangzhou 510045China China National Environmental Monitoring Centre Beijing 100012China State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing210023China Center for Excellence in Regional Atmos.Environ. Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China

The gaseous or particulate forms of divalent mercury(HgⅡ) significantly impact the spatial distribution of atmospheric mercury concentration and deposition flux(FLX). In the new nested-grid GEOS-Chem model, we try to modify the HgⅡ gas-particle partitioning relationship with synchronous and hourly observations at four sites in China. Observations of gaseous oxidized Hg(GOM), particulate-bound Hg(PBM), and PM 2.5 were used to derive an empirical gas-particle partitioning coefficient as a function of temperature( T) and organic aerosol(OA) concentrations under different relative humidity(RH). Results showed that with increasing RH, the dominant process of HgⅡ gas-particle partitioning changed from physical adsorption to chemical desorption. And the dominant factor of HgⅡ gas-particle partitioning changed from T to OA concentrations. We thus improved the simulated OA concentration field by introducing intermediate-volatility and semi-volatile organic compounds(I/SVOCs) emission inventory into the model framework and refining the volatile distributions of I/SVOCs according to new filed tests in the recent literatures. Finally, normalized mean biases(NMBs) of monthly gaseous element mercury(GEM), GOM, PBM, WFLX were reduced from-33%–29%, 95%–300%, 64%–261%, 117%–122% to-13%–0%,-20%–80%,-31%–50%,-17%–23%. The improved model explains 69%–98% of the observed atmospheric Hg decrease during 2013–2020 and can serve as a useful tool to evaluate the effectiveness of the Minamata Convention on Mercury.

关键词： Nested GEOS-Chem model HgⅡgas-particle partitioning Organic aerosol atmospheric mercury Mercury deposition flux

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Effects of organic fertilizers produced using different techniques on rice grain yield and ammonia volatilization in double-cropping rice fields

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Pedosphere 2024年第1期34卷 110-120页

作者： Mingcheng HU Andrew JWADE Weishou SHEN Zhenfang ZHONG Chongwen QIU Xiangui LIN Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Collaborative Innovation Center of Atmospheric Environment and Equipment Technologyand School of Environmental Science and EngineeringNanjing University of Information Science and TechnologyNanjing 210044China Department of Geography and Environmental Science University of ReadingReading RG65DWUK Haina Research Institute of Guangdong Haina Agricultural Co. Ltd.Huizhou 516000China State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil ScienceChinese Academy of SciencesNanjing 210008China

Ammonia(NH_(3)) volatilization from rice fields contributes to poor air quality and indicates low nitrogen use efficiency. Although organic fertilizers can meet the nitrogen requirement for rice growth, the simultaneous effects of organic fertilizers on NH_(3) volatilization and rice yield in paddy fields are poorly understood and quantified. To address this gap in our knowledge, experimental field plots were established in a conventional double-cropping paddy field in the Pearl River Delta region, southern China. Five fertilizer treatments were used besides the control with no fertilizer: fresh organic fertilizer, successively composted organic fertilizer, chemically composted organic fertilizer, mixture of chemically composted organic fertilizer with inorganic fertilizer, and chemical fertilizer. Ammonia volatilization was measured using a batch-type airflow enclosure method. No significant differences in grain yield were observed among organic and chemical fertilizer treatments. However, compared with chemical fertilizer, chemically composted organic fertilizer and successively composted organic fertilizer significantly decreased total NH_(3) volatilization by 70% and 68%, respectively. The ammonium-nitrogen concentration in field surface water correlated strongly(P < 0.01) and positively with NH_(3) volatilization across fertilization treatments. Our findings demonstrate that chemically composted organic fertilizer can sustain rice yield while reducing NH_(3) volatilization. An important future step is to promote these field measurements to similar rice cultivation areas to quantify the regional-and national-scale impact on air quality and nitrogen deposition in sensitive areas, and to design and implement better fertilizer management practices.

关键词： air quality crop production manure NH_(3)emission nitrogen use efficiency

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