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222Long-term mortality after early famine exposure: findings from the china Kadoorie Biobank

International Journal of Epidemiology 2021年第SUPPLEMENT_1期50卷

作者： Meng, Ruogu Yu, Canqing Guo, Yu Bian, Zheng Yang, Ling Chen, Yiping Du, Huaidong Chen, Junshi Chen, Zhengming Lv, Jun Li, Liming National Institute of Health Data Science Peking University Beijing China Center for Data Science in Health and Medicine Peking University Beijing China Department of Epidemiology and Biostatistics School of Public Health Peking University Health Science Center Beijing China Chinese Academy of Medical Sciences Beijing China Medical Research Council Population Health Research Unit at the University of Oxford Oxford United Kingdom Clinical Trial Service Unit & Epidemiological Studies Unit (CTSU) Nuffield Department of Population Health University of Oxford Oxford United Kingdom China National Center for Food Safety Risk Assessment Beijing China Key Laboratory of Molecular Cardiovascular Sciences (Peking University) Ministry of Education Beijing China Peking University Institute of Environmental Medicine Beijing China

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engineering residues on C interface to improve thermostability of nitrilase for biosynthesis of Pregabalin precursor

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AIChE Journal 2023年第11期69卷

作者： Xia-Feng Lu Xiao-Ling Tang Chen-Hui Xu Hong-Juan Diao Zhe-Ming Wu Ren-Chao Zheng Yu-Guo Zheng Key Laboratory of Bioorganic Synthesis of Zhejiang Province College of Biotechnology and Bioengineering Zhejiang University of Technology Hangzhou People's Republic of China Engineering Research Center of Bioconversion and Biopurification of Ministry of Education Zhejiang University of Technology Hangzhou People's Republic of China Contribution: Investigation (lead) Methodology (supporting) Writing - original draft (lead) Contribution: Formal analysis (supporting) Investigation (supporting) Writing - original draft (supporting) Contribution: Data curation (supporting) Formal analysis (supporting) Contribution: Formal analysis (lead) Contribution: Data curation (supporting) Contribution: Conceptualization (lead) Funding acquisition (lead) Project administration (lead) Supervision (lead) Contribution: Project administration (supporting) Supervision (supporting)

Nitrilase-mediated bioprocesses exhibited great potential in the production of value-added carboxylic acids. However, poor thermostability of nitrilases usually restricts their industrial applications. Herein, the thermostability of nitrilase Ba NIT M0 was significantly improved by engineering the amino acid residues on the intersection of two dimers (C interface). Except for simultaneous enhancement of enantioselectivity and activity, the best variant V82L/M127I/L159M/F166Q/C237S/Q260H ( Ba NIT M4 ) showed a 10.8-fold increase in half-life at 30°C compared with Ba NIT M0 . Structural analysis demonstrated that additional hydrogen bonds were formed between the residues on the C interface, which strengthened the interactions of two symmetrical regions and spirals. Subsequently, the engineered nitrilase was immobilized onto epoxy resins LXTE-603 and the immobilized nitrilase exhibited excellent stability over 12 repeated cycles, which indicated a great industrial potential for biosynthesis of Pregabalin precursor.

关键词： C interface immobilized nitrilase Pregabalin precursor protein engineering thermostability

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Impact of Electrostatic Interaction on Non-radiative Recombination Energy Losses in Organic Solar Cells Based on Asymmetric Acceptors

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Angewandte Chemie 2023年第35期135卷

作者： Yongjie Cui Dr. Peipei Zhu Prof. Huawei Hu Xinxin Xia Prof. Xinhui Lu Dr. Shicheng Yu Dr. Hermann Tempeld Prof. Rüdiger-A. Eichel Prof. Xunfan Liao Prof. Yiwang Chen National Engineering Research Center for Carbohydrate Synthesis/Key Laboratory of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education Jiangxi Normal University 99 Ziyang Avenue Nanchang 330022 China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials & College of Materials Science and Engineering Donghua University 2999 North Renmin Road Shanghai 201620 China Contribution: Conceptualization (equal) Data curation (lead) Formal analysis (equal) Writing - original draft (lead) Contribution: Formal analysis (supporting) Department of Physics Chinese University of Hong Kong Hong Kong 999077 China Contribution: Data curation (supporting) Institut für Energie- und Klimaforschung (IEK-9: Grundlagen der Elektrochemie) Forschungszentrum Jülich 52425 Jülich Germany Contribution: Formal analysis (equal) Supervision (equal) Writing - original draft (supporting) Contribution: Conceptualization (equal) Supervision (equal)

Reducing non-radiative recombination energy loss (Δ E 3 ) is one key to boosting the efficiency of organic solar cells. Although the recent studies have indicated that the Y-series asymmetric acceptors-based devices featured relatively low Δ E 3 , the understanding of the energy loss mechanism derived from molecular structure change is still lagging behind. Herein, two asymmetric acceptors named BTP-Cl and BTP-2Cl with different terminals were synthesized to make a clear comparative study with the symmetric acceptor BTP-0Cl. Our results suggest that asymmetric acceptors exhibit a larger difference of electrostatic potential (ESP) in terminals and semi-molecular dipole moment, which contributes to form a stronger π–π interaction. Besides, the experimental and theoretical studies reveal that a lower ESP-induced intermolecular interaction can reduce the distribution of PM6 near the interface to enhance the built-in potential and decrease the charge transfer state ratio for asymmetric acceptors. Therefore, the devices achieve a higher exciton dissociation efficiency and lower Δ E 3 . This work establishes a structure-performance relationship and provides a new perspective to understand the state-of-the-art asymmetric acceptors.

关键词： Asymmetric Acceptor Electrostatic Potential Hybridization Intermolecular Interaction Non-Radiative Recombination Energy Loss

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The DIRECT consortium and the REST-meta-MDD project:towards neuroimaging biomarkers of major depressive disorder

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Psychoradiology 2022年第1期2卷 32-42页

作者： Xiao Chen Bin Lu Hui-Xian Li Xue-Ying Li Yu-Wei Wang Francisco Xavier Castellanos Li-Ping Cao Ning-Xuan Chen Wei Chen Yu-Qi Cheng Shi-Xian Cui Zhao-Yu Deng Yi-Ru Fang Qi-Yong Gong Wen-Bin Guo Zheng-Jia-Yi Hu Li Kuang Bao-Juan Li Le Li Tao Li Tao Lian Yi-Fan Liao Yan-Song Liu Zhe-Ning Liu Jian-Ping Lu Qing-Hua Luo Hua-Qing Meng Dai-Hui Peng Jiang Qiu Yue-Di Shen Tian-Mei Si Yan-Qing Tang Chuan-Yue Wang Fei Wang Hua-Ning Wang Kai Wang Xiang Wang Ying Wang Zi-Han Wang Xiao-Ping Wu Chun-Ming Xie Guang-Rong Xie Peng Xie Xiu-Feng Xu Hong Yang Jian Yang Shu-Qiao Yao Yong-Qiang Yu Yong-Gui Yuan Ke-Rang Zhang Wei Zhang Zhi-Jun Zhang Jun-Juan Zhu Xi-Nian Zuo Jing-Ping Zhao Yu-Feng Zang the DIRECT consortium Chao-Gan Yan CAS Key Laboratory of Behavioral Science Institute of PsychologyChinese Academy of SciencesBeijing 100101China International Big-Data Center for Depression Research Chinese Academy of SciencesBeijing 100101China Magnetic Resonance Imaging Research Center Institute of PsychologyChinese Academy of SciencesBeijing 100101China Department of Psychology University of Chinese Academy of SciencesBeijing 100049China Sino-Danish College University of Chinese Academy of SciencesBeijing 101408China Sino-Danish Center for Education and Research Graduate University of Chinese Academy of SciencesBeijing 101408China Department of Child and Adolescent Psychiatry NYU Grossman School of MedicineNew YorkNY 10016USA Nathan Kline Institute for Psychiatric Research OrangeburgNew YorkNY 10962USA 9Affiliated Brain Hospital of Guangzhou Medical UniversityGuangzhou 510370China Capital Normal University Beijing 100089China Department of Psychiatry Sir Run Run Shaw HospitalZhejiang University School of MedicineHangzhou 310020ZhejiangChina Department of Psychiatry First Affiliated Hospital of Kunming Medical UniversityKunmingYunnan 650032China Shanghai Mental Health Center Shanghai Jiao Tong University School of MedicineShanghai 200030China Huaxi MR Research Center(HMRRC) Department of RadiologyWest China Hospital of Sichuan UniversityChengduSichuan 610044China Research Unit of Psychoradiology Chinese Academy of Medical SciencesChengduSichuan 610052China Department of Psychiatry and National Clinical Research Center for Mental DisordersThe Second Xiangya Hospital of Central South UniversityChangsha 410011HunanChina Department of Psychiatry The First Affiliated Hospital of Chongqing Medical UniversityChongqing 400042China Xijing Hospital of Air Force Military Medical University Xi’anShaanxi 710032China Center for Cognitive Science of Language Beijing Language and Culture UniversityBeijing 100083China Affiliated Mental Health Center&Hangzhou Seventh People’s Hospital Zhejiang University School of

Despite a growing neuroimaging literature on the pathophysiology of major depressive disorder(MDD),repro-ducible findings are lacking,probably reflecting mostly small sample sizes and heterogeneity in analytic *** address these issues,the Depression Imaging REsearch ConsorTium(DIRECT)was *** REST-meta-MDD project,pooling 2428 functional brain images processed with a standardized pipeline across all participating sites,has been the first effort from *** this review,we present an overview of the moti-vations,rationale,and principal findings of the studies so far from the REST-meta-MDD *** from the first round of analyses of the pooled repository have included alterations in functional connectivity within the default mode network,in whole-brain topological properties,in dynamic features,and in functional *** well-powered exploratory observations have also provided the basis for future longitudinal hypothesis-driven *** these fruitful explorations,DIRECT has proceeded to its second stage of data sharing that seeks to examine ethnicity in brain alterations in MDD by extending the exclusive Chinese original sample to other ethnic groups through international collaborations.A state-of-the-art,surface-based preprocessing pipeline has also been introduced to improve *** images from patients with bipolar disorder and schizophrenia will be included to identify shared and unique abnormalities across diag-nosis *** addition,large-scale longitudinal studies targeting brain network alterations following antidepressant treatment,aggregation of diffusion tensor images,and the development of functional magnetic resonance imaging-guided neuromodulation approaches are *** these endeavours,we hope to accelerate the translation of functional neuroimaging findings to clinical use,such as evaluating longitudinal effects of antidepressant medications and developing individualized

关键词： major depressive disorder DIRECT R-fMRI database neuroimaging

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Amorphous Mo-doped NiS0.5Se0.5Nanosheets@Crystalline NiS0.5Se0.5Nanorods for High Current-density Electrocatalytic Water Splitting in Neutral Media

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Angewandte Chemie 2022年第6期135卷

作者： Dr. Yang Wang Dr. Xiaopeng Li Dr. Zhong Huang Dr. Haozhi Wang Dr. Zelin Chen Dr. Jinfeng Zhang Prof. Xuerong Zheng Prof. Yida Deng Prof. Wenbin Hu State Key Laboratory of Marine Resource Utilization in South China Sea School of Materials Science and Engineering Hainan University Haikou 570228 P. R. China Contribution: Data curation (lead) Investigation (lead) Methodology (lead) Validation (lead) Writing - original draft (lead) School of Materials Science and Engineering Tianjin Key Laboratory of Building Green Functional Materials Tianjin Chengjian University Tianjin 300384 China Contribution: Formal analysis (equal) State Key Laboratory of Marine Resource Utilization in South China Sea College of Information and Communication Engineering Hainan University Haikou 570228 P. R. China Contribution: Methodology (equal) Software (equal) Validation (equal) Contribution: Methodology (equal) Software (equal) School of Materials Science and Engineering Tianjin Key Laboratory of Composite and Functional Materials Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of Education Tianjin University Tianjin 300072 P. R. China Contribution: Methodology (equal) Contribution: Conceptualization (equal) Investigation (equal) Supervision (equal) Contribution: Funding acquisition (lead) Supervision (equal) Contribution: Funding acquisition (supporting)

It is vitally important to develop highly active, robust and low-cost transition metal-based electrocatalysts for overall water splitting in neutral solution especially at large current density. In this work, amorphous Mo-doped NiS 0.5 Se 0.5 nanosheets@crystalline NiS 0.5 Se 0.5 nanorods (Am−Mo−NiS 0.5 Se 0.5 ) was synthesized using a facil one-step strategy. In phosphate buffer saline solution, the Am−Mo−NiS 0.5 Se 0.5 shows tiny overpotentials of 48 and 209 mV for hydrogen evolution reaction (HER), 238 and 514 mV for oxygen evolution reaction (OER) at 10 and 1000 mA cm −2 , respectively. Moreover, Am−Mo−NiS 0.5 Se 0.5 delivers excellent stability for at least 300 h without obvious degradation. Theoretical calculations revealed that the Ni sites in the defect-rich amorphous structure of Am−Mo−NiS 0.5 Se 0.5 owns higher electron state density and strengthened the binding energy of H 2 O, which will optimize H adsorption/desorption energy barriers and reduce the adsorption energy of OER determining step.

关键词： Amorphous Crystalline High-Current-Density Neutral Environment Water Splitting

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A Molybdenum Disulfide Nanozyme with Charge-Enhanced Activity for Ultrasound-Mediated Cascade-Catalytic Tumor Ferroptosis

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Angewandte Chemie 2022年第11期135卷

作者： Longwei Wang Xiaodi Zhang Zhen You Zhongwei Yang Dr. Mengyu Guo Jiawei Guo He Liu Xiaoyu Zhang Zhuo Wang Prof. Aizhu Wang Prof. Yawei Lv Dr. Jian Zhang Prof. Xin Yu Prof. Jing Liu Prof. Chunying Chen CAS Key Laboratory for Biomedical Effects of Nanomaterials and Nanosafety & CAS Center for Excellence in Nanoscience National Center for Nanoscience and Technology of China University of Chinese Academy of Science Beijing 100190 China Key Laboratory of Resource Biology and Biotechnology in Western China Ministry of Education School of Medicine Northwest University Xi'an 710069 China Contribution: Data curation (lead) Formal analysis (lead) Investigation (lead) Methodology (lead) Institute for Advanced Interdisciplinary Research School of Chemistry and Chemical Engineering University of Jinan Jinan 250022 China Contribution: Data curation (equal) Contribution: Investigation (equal) Methodology (equal) Contribution: Formal analysis (supporting) Contribution: Methodology (supporting) Contribution: Investigation (supporting) Contribution: Formal analysis (supporting) Software (lead) School of Physics and Electronics Hunan University Changsha 410082 China Contribution: Software (lead) Department of Biology and Biological Engineering Chalmers University of Technology Kemivägen 10 41296 Göteborg Sweden Contribution: Data curation (lead) Formal analysis (lead) Writing - original draft (lead) Contribution: Data curation (lead) Formal analysis (lead) Funding acquisition (equal) Writing - original draft (equal) Writing - review & editing (lead) Contribution: Conceptualization (lead) Funding acquisition (lead) Writing - review & editing (lead)

The deficient catalytic activity of nanozymes and insufficient endogenous H 2 O 2 in the tumor microenvironment (TME) are major obstacles for nanozyme-mediated catalytic tumor therapy. Since electron transfer is the basic essence of catalysis-mediated redox reactions, we explored the contributing factors of enzymatic activity based on positive and negative charges, which are experimentally and theoretically demonstrated to enhance the peroxidase (POD)-like activity of a MoS 2 nanozyme. Hence, an acidic tumor microenvironment-responsive and ultrasound-mediated cascade nanocatalyst (BTO/MoS 2 @CA) is presented that is made from few-layer MoS 2 nanosheets grown on the surface of piezoelectric tetragonal barium titanate (T-BTO) and modified with pH-responsive cinnamaldehyde (CA). The integration of pH-responsive CA-mediated H 2 O 2 self-supply, ultrasound-mediated charge-enhanced enzymatic activity, and glutathione (GSH) depletion enables out-of-balance redox homeostasis, leading to effective tumor ferroptosis with minimal side effects.

关键词： Ferroptosis Nanozymes Reactive Oxygen Species Tumor Therapy

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Electron Acceptor Molecule Doping Induced π–π Interaction to Promote Charge Transport Kinetics for Efficient and Stable 2D/3D Perovskite Solar Cells

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Angewandte Chemie 2023年第26期135卷

作者： Lian Wang Bohong Chang Hui Li Yutong Wu Luyuan Zhang Longwei Yin Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials Ministry of Education School of Materials Science and Engineering Shandong University 250061 Jinan P. R.China Contribution: Conceptualization (lead) Data curation (lead) Formal analysis (lead) Investigation (lead) Methodology (lead) Writing - original draft (lead) Contribution: Data curation (supporting) Investigation (supporting) Methodology (supporting) Writing - original draft (supporting) Contribution: Formal analysis (supporting) Investigation (supporting) Methodology (supporting) Writing - original draft (supporting) Contribution: Conceptualization (supporting) Methodology (supporting) Writing - original draft (supporting) Contribution: Formal analysis (supporting) Investigation (supporting) Writing - original draft (supporting) Contribution: Conceptualization (lead) Data curation (lead) Funding acquisition (lead) Investigation (lead) Methodology (lead) Writing - original draft (lead)

Although the incorporation of 2D perovskite into 3D perovskite can greatly enhance intrinsic stability, power conversion efficiency (PCE) of 2D/3D perovskite is still inferior to its 3D counterpart due to poor carrier transport kinetics resulted from the quantum and dielectric confinement of 2D component. To overcome this issue, the electron acceptor molecule 1,2,4,5-tetracyanobenzene (TCNB) was introduced to trigger intermolecular π–π interaction in 2D perovskite along with the electronic doping of 2D/3D perovskite to improve charge transfer efficiency. By virtue of high electron affinity, TCNB can undergo electron transfer reaction and subsequently establish π–π interaction with 1-naphthalenemethylammonium (NMA) cations, greatly strengthening lattice rigidity and reducing exciton binding energy. Transmission electron microscopy results demonstrate that 2D phases are mainly distributed at grain boundaries, reducing defect density and weakening nonradiative recombination. Meanwhile, the p-type doping of perovskite by TCNB optimizes energy level alignment at perovskite/hole transport layer interface. Consequently, PCE of champion device is significantly boosted to 24.01 %. The unencapsulated device retains an initial efficiency close to 94 % after exposure to ambient environment for over 1000 h. This work paves a novel path for designing new mixed-dimensional perovskite solar cells with high PCE and superior stability.

关键词： 2D/3D Perovskite Charge Transport Electron Acceptor Molecule Solar Cells π–π Interaction

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Author Correction: The Genome Sequences of 90 Mushrooms

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Scientific reports 2020年第1期10卷 8460页

作者： Huiying Li Surui Wu Xiao Ma Wei Chen Jing Zhang Shengchang Duan Yun Gao Ling Kui Wenli Huang Peng Wu Ruoyu Shi Yifan Li Yuanzhong Wang Jieqing Li Xiang Guo Xiaoli Luo Qiang Li Chuan Xiong Honggao Liu Mingying Gui Jun Sheng Yang Dong Kunming University of Science and Technology Kunming 650500 Yunnan China. Kunming Edible Fungi Institute of All China Federation of Supply and Marketing Cooperatives Kunming 650032 Yunnan China. Yunnan Plateau Characteristic Agricultural Industry Research Institute Kunming 650201 Yunnan China. Key Laboratory of Puer Tea Science Ministry of Education Yunnan Agricultural University Kunming 650201 Yunnan China. College of Biological Big Data Yunnan Agriculture University Kunming 650201 Yunnan China. Nowbio Biotechnology Company Kunming 650201 Yunnan China. State Key Laboratory of Genetic Resources and Evolution Kunming Institute of Zoology Chinese Academy of Sciences Kunming 650223 Yunnan China. Kunming College of Life Science University of Chinese Academy of Sciences Kunming 650204 Yunnan China. Biotechnology and Nuclear Technology Research Institute Sichuan Academy of Agricultural Sciences Chengdu 610061 Sichuan China. College of Agronomy and Biotechnology Yunnan Agricultural University Kunming 650201 Yunnan China. Kunming Edible Fungi Institute of All China Federation of Supply and Marketing Cooperatives Kunming 650032 Yunnan China. guimingying@***. Yunnan Plateau Characteristic Agricultural Industry Research Institute Kunming 650201 Yunnan China. shengj@***. Key Laboratory of Puer Tea Science Ministry of Education Yunnan Agricultural University Kunming 650201 Yunnan China. shengj@***. College of Biological Big Data Yunnan Agriculture University Kunming 650201 Yunnan China. loyalyang@***. State Key Laboratory for Conservation and Utilization of Bio-Resources in Yunnan Yunnan Agricultural University Kunming 650201 Yunnan China. loyalyang@***. Key Laboratory for Agro-biodiversity and Pest Control of Ministry of Education Yunnan Agricultural University Kunming 650201 Yunnan China. loyalyang@***.

An amendment to this paper has been published and can be accessed via a link at the top of the paper.

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Virus Detection: Nanopore Targeted Sequencing for the Accurate and Comprehensive Detection of SARS-CoV-2 and Other Respiratory Viruses (Small 32/2020)

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Small 2020年第32期16卷

作者： Ming Wang Aisi Fu Ben Hu Yongqing Tong Ran Liu Zhen Liu Jiashuang Gu Bin Xiang Jianghao Liu Wen Jiang Gaigai Shen Wanxu Zhao Dong Men Zixin Deng Lilei Yu Wu Wei Yan Li Tiangang Liu Department of Clinical Laboratory Renmin Hospital of Wuhan University Wuhan 430060 China Key Laboratory of Combinatorial Biosynthesis and Drug Discovery Ministry of Education and Wuhan University School of Pharmaceutical Sciences Wuhan 430071 China CAS Key Laboratory of Computational Biology CAS-MPG Partner Institute for Computational Biology Shanghai Institute of Nutrition and Health University of Chinese Academy of Sciences Chinese Academy of Sciences Shanghai 200031 China Wuhan Dgensee Clinical Laboratory Co. Ltd. Wuhan 430075 China Wuhan Institute of Virology Chinese Academy of Sciences Wuhan 430071 China Department of Internal Medicine Renmin Hospital of Wuhan University Wuhan 430060 China Center for Biomedical Informatics Shanghai Engineering Research Center for Big Data in Pediatric Precision Medicine Shanghai Children's Hospital Shanghai Jiao Tong University Shanghai 200040 China

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Solid–Liquid Interfacial Coordination Chemistry Enables High-Capacity Ammonium Storage in Amorphous Manganese Phosphate

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Angewandte Chemie 2022年第37期134卷

作者： Duo Yang Prof. Yu Song Ming-Yue Zhang Zengming Qin Jie Liu Prof. Xiao-Xia Liu Department of Chemistry Northeastern University 3-11 Wenhua Road Heping district Shenyang 110819 China School of Resources and Civil Engineering Northeastern University 3-11 Wenhua Road Heping district Shenyang 110819 China National-local Joint Engineering Research Center of High-efficient Exploitation Technology for Refractory Iron Ore Resources Shenyang 110819 Liaoning China National Frontiers Science Center for Industrial Intelligence and Systems Optimization Northeastern University 3-11 Wenhua Road Heping district Shenyang 110819 China Key Laboratory of Data Analytics and Optimization for Smart Industry Northeastern University) Ministry of Education China 3-11 Wenhua Road Heping district Shenyang 110819 China

Ammonium (NH 4 + ) ion as charge carrier is attracting attention in aqueous batteries. Yet, most NH 4 + host materials are still limited by the relatively low capacities. Here, we fabricated a manganese phosphate (MP-20) for NH 4 + ion storage. MP-20 displays a high capacity of 299.6 mAh g −1 at 1 A g −1 in ammonium acetate (NH 4 Ac) electrolyte, outperforming other reported NH 4 + host materials. Spectroscopy studies suggest a new NH 4 + /H + co-insertion mechanism. We surprisingly discover that the NH 4 Ac electrolyte plays an important role in improving the charge storage capability of the materials. Experimental and computational results indicate acetate ions can form coordination bonds with the Mn atoms, tailoring the electronic structure of the Mn atoms and the surrounding O atoms, and therefore facilitating the NH 4 + storage process. Our findings provide a new NH 4 + host material and propose the important role of the electrolyte-electrode coordination effect in aqueous ammonium batteries.

关键词： Aqueous Ammonium-Ion Batteries Charge Storage Mechanism Coordination Electrochemical Deposition Manganese Phosphate

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