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arXiv 2024年

作者： Niu, Jiarui R. Wang, W.Y. Jiang, J.C. Qu, Y. Zhou, D.J. Zhu, W.W. Lee, K.J. Han, J.L. Zhang, B. Li, D. Cao, S. Fang, Z.Y. Feng, Y. Fu, Q.Y. Jiang, P. Jing, W.C. Li, J. Li, Y. Luo, R. Meng, L.Q. Miao, C.C. Miao, X.L. Niu, C.H. Pan, Y.C. Wang, B.J. Wang, F.Y. Wang, H.Z. Wang, P. Wu, Q. Wu, Z.W. Xu, H. Xu, J.W. Xu, L. Xue, M.Y. Yang, Y.P. Yuan, M. Yue, Y.L. Zhao, D. Zhang, C.F. Zhang, D.D. Zhang, J.S. Zhang, S.B. Zhang, Y.K. Zhu, Y.H. National Astronomical Observatories Chinese Academy of Sciences 20A Datun Road Chaoyang District Beijing100101 China School of Astronomy and Space Science University of Chinese Academy of Sciences Beijing100049 China The Nevada Center for Astrophysics University of Nevada Las VegasNV89154 United States Department of Physics and Astronomy University of Nevada Las VegasNV89154 United States Kavli Institute for Astronomy and Astrophysics Peking University Beijing100871 China Department of Astronomy Peking University Beijing100871 China Yunnan Observatories Chinese Academy of Sciences P.O.Box110 Yunnan Kunming650011 China Zhejiang Lab Kechuang Avenue Zhongtai Sub-District Yuhang District Zhejiang Province Hangzhou China School of Computer Science and Engineering Beihang University Beijing100191 China Purple Mountain Observatory Chinese Academy of Sciences Nanjing210023 China Department of Astronomy School of Physics and Materials Science Guangzhou University Guangzhou510006 China Institute of Astrophysics Central China Normal University Wuhan430079 China School of Astronomy and Space Science Nanjing University Nanjing210093 China Key Laboratory of Modern Astronomy and Astrophysics Nanjing University Ministry of Education China Lanzhou University Lanzhou730000 China Faculty of Electrical engineering and Computer Science Ningbo University Ningbo315211 China Pengcheng Laboratory Shenzhen518055 China South-Western Institute for Astronomy Research Yunnan University Yunnan Kunming650504 China National Space Science Center Chinese Academy of Sciences Beijing100190 China School of Physics and Electronic Science Guizhou Normal University Guiyang550025 China Guizhou Provincial Key Laboratory of Radio Astronomy and Data Processing Guizhou Normal University Guiyang550025 China

We report the first detection of polarization angle (PA) orthogonal jumps, a phenomenon previously only observed from radio pulsars, from a fast radio burst (FRB) source FRB 20201124A. We find three cases of orthogonal jumps in over two thousand bursts, all resembling those observed in pulsar single pulses. We propose that the jumps are due to the superposition of two orthogonal emission modes that could only be produced in a highly magnetized plasma, and they are caused by the line of sight sweeping across a rotating magnetosphere. The shortest jump timescale is of the order of one-millisecond, which hints that the emission modes come from regions smaller than the light cylinder of most pulsars or magnetars. This discovery provides convincing evidence that FRB emission originates from the complex magnetosphere of a magnetar, suggesting an FRB emission mechanism that is analogous to radio pulsars despite a huge luminosity difference between two types of objects. Copyright © 2024, The Authors. All rights reserved.

关键词： Polarization

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Fungal diversity notes 1036-1150:taxonomic and phylogenetic contributions on genera and species of fungal taxa

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Fungal Diversity 2019年第3期96卷 1-242页

作者： Kevin D.Hyde Danushka S.Tennakoon Rajesh Jeewon DJayarama Bhat Sajeewa S.N.Maharachchikumbura Walter Rossi Marco Leonardi Hyang Burm Lee Hye Yeon Mun Jos Houbraken Thuong T.T.Nguyen Sun Jeong Jeon Jens Christian Frisvad Dhanushka N.Wanasinghe Robert Lucking Andre Aptroot Marcela E.S.Caceres Samantha C.Karunarathna Sinang Hongsanan Rungtiwa Phookamsak Nimali Ide Silva Kasun M.Thambugala Ruvishika S.Jayawardena Indunil C.Senanayake Saranyaphat Boonmee Jie Chen Zong-Long Luo Chayanard Phukhamsakda Olinto L.Pereira Vanessa P.Abreu Andre Wilson Campos Rosado Buyck Bart Emile Randrianjohany Vale rie Hofstetter Tatiana B.Gibertoni Adriene Mayrada Silva Soares Helio Longoni Plautz Jr Helen Maria Pontes Sotao William Kalhy Silva Xavier Jadson Diogo Pereira Bezerra Thays Gabrielle Linsde Oliveira Cristina Mariade Souza-Motta Oliane Maria Correia Magalhaes Digvijayini Bundhun Dulanjalee Harishchandra Ishara S.Manawasinghe Wei Dong Sheng-Nan Zhang Dan-Feng Bao Milan C.Samarakoon Dhandevi Pem Anuruddha Karunarathna Chuan-Gen Lin Jing Yang Rekhani H.Perera Vinit Kumar Shi-Ke Huang Monika C.Dayarathne Anusha H.Ekanayaka Subashini C.Jayasiri Yuanpin Xiao Sirinapa Konta Tuula Niskanen Kare Liimatainen Yu-Cheng Dai Xiao-Hong Ji Xue-Mei Tian Armin Mesic Sanjay K.Singh Kunthida Phutthacharoen Lei Cai Touny Sorvongxay Vinodhini Thiyagaraja Chada Norphanphoun Napalai Chaiwan Yong-Zhong Lu Hong-Bo Jiang Jin-Feng Zhang Pranami D.Abeywickrama Janith V.S.Aluthmuhandiram Rashika S.Brahmanage Ming Zeng Thilini Chethana Deping Wei Martina Reblova Jacques Fournier Jana Nekvindova Renan do Nascimento Barbosa Jose Ewerton Felintodos Santos Neiva Tintide Oliveira Guo-Jie Li Damien Ertz Qiu-Ju Shang Alan J.L.Phillips Chang-Hsin Kuo Erio Camporesi Timur S.Bulgakov Saisamorn Lumyong E.B.Gareth Jones Putarak Chomnunti Eleni Gentekaki Frank Bungartz Xiang-Yu Zeng Sally Fryar Zdenko Tkalcec Junmin Liang Guangshuo Li Ting-Chi Wen Paras Nath Singh Yusufjon Gafforov Itthayakorn Promputtha Erandi Yasanthika Ishani D.Goonasekara Rui-Lin Zhao Qi Zhao Paul M Key Laboratory for Plant Diversity and Biogeography of East Asia Kunming Institute of BotanyChinese Academy of ScienceKunming 650201YunnanPeople’s Republic of China School of Science Mae Fah Luang UniversityChiang Rai 57100Thailand Center of Excellence in Fungal Research Mae Fah Luang UniversityChiang Rai 57100Thailand East and Central Asia Regional Office World Agroforestry Centre(ICRAF)Kunming 650201YunnanPeople’s Republic of China Department of Biology Faculty of ScienceChiang Mai UniversityChiang Mai 50200Thailand Mushroom Research Foundation 128 M.3 Ban Pa Deng T.Pa PaeA.Mae TaengChiang Mai 50150Thailand Department of Plant Medicine National Chiayi University300 Syuefu RoadChiayi City 60004TaiwanPeople’s Republic of China Department of Health Sciences Faculty of ScienceUniversity of MauritiusReduitMauritius Formerly Department of Botany Goa UniversityGoaIndia No.128/1-J Azad Housing SocietyCurcaGoa Velha 403108India Department of Crop Sciences College of Agricultural and Marine SciencesSultan Qaboos UniversityPO Box 8123 Al KhoudOman Sect.Environmental Sciences Dept.MeSVAUniversity of L’Aquila67100 CoppitoAQItaly Division of Food Technology Biotechnology&AgrochemistryCollege of Agriculture&Life SciencesChonnam National UniversityGwangju 61186Korea Fungal Resources Research Division NNIBRSangju-si 37242Korea Westerdijk Fungal Biodiversity Institute Uppsalalaan 83584 CT UtrechtThe Netherlands Department of Biotechnology and Biomedicine DTUBioengineeringTechnical University of Denmark2800 Kongens LyngbyDenmark Botanischer Garten und Botanisches Museum Berlin Freie Universitat BerlinKonigin-Luise-StraßBe 6-814195 BerlinGermany Laboratorio de Botanica/Liquenologia Instituto de BiocienciasUniversidade Federal de Mato Grosso do SulAvenida Costa e Silva s/nBairro UniversitarioCampo GrandeMatto Grosso do Sul CEP 79070-900Brazil Departamento de Biociencias Universidade Federal de SergipeItabaianaSergipe CEP:49500-000Brazil Shenzhen Key Laboratory of Microbial

This article is the tenth series of the Fungal Diversity Notes,where 114 taxa distributed in three phyla,ten classes,30 orders and 53 families are described and *** described in the present study include one new family(*** in Dothideomycetes),five new genera(Caatingomyces,Cryptoschizotrema,Neoacladium,Paramassaria and Trochilispora)and 71 new species,(*** thailandica,Amniculicola aquatica,***,Angustimassarina sylvatica,Blackwellomyces lateris,Boubovia gelatinosa,Buellia viridula,Caatingomyces brasiliensis,Calophoma humuli,Camarosporidiella mori,Canalisporium dehongense,Cantharellus brunneopallidus,***,Castanediella meliponae,Coprinopsis psammophila,Cordyceps succavus,Cortinarius minusculus,***,Diaporthe italiana,***,Diatrypella delonicis,Dictyocheirospora aquadulcis,***,Digitodesmium chiangmaiense,Distoseptispora dehongensis,***,Dothiorella styphnolobii,Ellisembia aurea,Falciformispora aquatic,Fomitiporia carpinea,***,Grammothele aurantiaca,***,Hermatomyces bauhiniae,Jahnula queenslandica,Kamalomyces mangrovei,Lecidella yunnanensis,Micarea squamulosa,Muriphaeosphaeria angustifoliae,Neoacladium indicum,Neodidymelliopsis sambuci,Neosetophoma miscanthi,***,Nodulosphaeria aquilegiae,***,Paramassaria samaneae,Penicillium circulare,***,***-pumilae,***,***,Phaeoisaria siamensis,Phaeopoacea asparagicola,Phaeosphaeria penniseti,Plectocarpon galapagoense,Porina sorediata,Pseudoberkleasmium chiangmaiense,Pyrenochaetopsis sinensis,Rhizophydium koreanum,Russula prasina,Sporoschisma chiangraiense,Stigmatomyces chamaemyiae,***,***,***,***,Thysanorea uniseptata,Torula breviconidiophora,***,Trochilispora schefflerae and Vaginatispora palmae).Further,twelve new combinations(*** cryptotrema,Prolixandromyces australi,***,***,***,P.

关键词： 71 new taxa Ascomycota Basidiomycota Dothideomycetes Eurotiomycetes Lecanoromycetes Leotiomycetes Pezizomycetes Phylogeny Taxonomy

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Chromatin 3D structure, phase separation and disease

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Life Medicine 2023年第2期2卷 3页

作者： Lili Fan Xinyi Liu Diana Guallar Junjun Ding Guangzhou Key Laboratory of Formula-Pattern of Traditional Chinese Medicine School of Traditional Chinese Medicine Jinan University Guangzhou 510632 China RNA Biomedical Institute Sun Yat-sen Memorial Hospital Zhongshan School of Medicine Sun Yat-sen University Guangzhou 510080 China Advanced Medical Technology Center The First Affiliated Hospital Zhongshan School of Medicine Sun Yat-sen University Guangzhou 510006 China Center for Stem Cell Biology and Tissue Engineering Key Laboratory for Stem Cells and Tissue Engineering Ministry of Education Zhongshan School of Medicine Sun Yat-sen University Guangzhou 510006 China Center for Research in Molecular Medicine and Chronic Diseases Universidade de Santiago de Compostela Santiago de Compostela 15782 Spain RNA Biomedical Institute Sun Yat-sen Memorial Hospital Zhongshan School of Medicine Sun Yat-sen University Guangzhou 510080 China Advanced Medical Technology Center The First Affiliated Hospital Zhongshan School of Medicine Sun Yat-sen University Guangzhou 510006 China Center for Stem Cell Biology and Tissue Engineering Key Laboratory for Stem Cells and Tissue Engineering Ministry of Education Zhongshan School of Medicine Sun Yat-sen University Guangzhou 510006 China Department of Histology and Embryology School of Basic Medical Sciences Guangzhou Medical University Guangzhou 511436 China West China Biomedical Big Data Center West China Hospital Sichuan University Chengdu 610041 China

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Changing life expectancy in European countries 1990–2021: a subanalysis of causes and risk factors from the Global Burden of Disease Study 2021

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The Lancet Public Health 2025年第3期10卷 e172-e188页

作者： Steel, Nicholas Bauer-Staeb, Clarissa Maria Mercedes Ford, John A. Abbafati, Cristiana Abdalla, Mohammed Altigani Abdelkader, Atef Abdi, Parsa Zuñiga, Roberto Ariel Abeldaño Abiodun, Olugbenga Olusola Abolhassani, Hassan Abu-Gharbieh, Eman Abukhadijah, Hana J. Abu-Zaid, Ahmed Addo, Isaac Yeboah Addolorato, Giovanni Adekanmbi, Victor Adetunji, Juliana Bunmi Adeyeoluwa, Temitayo Esther Agardh, Emilie E. Agyemang-Duah, Williams Ahmad, Danish Ahmed, Ayman Ahmed, Syed Anees Akinosoglou, Karolina Akkaif, Mohammed Ahmed Al Awaidy, Salah Al Hasan, Syed Mahfuz Al Zaabi, Omar Ali Mohammed Aldridge, Robert W. Algammal, Abdelazeem M. Al-Gheethi, Adel Ali Saeed Ali, Abid Ali, Mohammed Usman Ali, Syed Shujait Ali, Waad Alicandro, Gianfranco Alif, Sheikh Mohammad Al-Jumaily, Adel Allebeck, Peter Alrawashdeh, Ahmad Al-Rifai, Rami H. Alsabri, Mohammed A. Alshahrani, Najim Z. Aluh, Deborah Oyine Al-Wardat, Mohammad Al-Zyoud, Walid A. Amiri, Sohrab Anderlini, Deanna Andrei, Catalina Liliana Anil, Abhishek Anvari, Saeid Anyasodor, Anayochukwu Edward Appiah, Seth Christopher Yaw Aquilano, Michele Arabloo, Jalal Arafat, Mosab Areda, Demelash Aremu, Abdulfatai Armani, Keivan Armocida, Benedetta Ärnlöv, Johan Asaduzzaman, Muhammad Astell-Burt, Thomas Aujayeb, Avinash Ausloos, Marcel Azadnajafabad, Sina Aziz, Shahkaar Azzam, Ahmed Y. Babu, Giridhara Rathnaiah Badache, Andreea Corina Badiye, Ashish D. Bahramian, Saeed Baig, Atif Amin Baker, Jennifer L. Bansal, Hansi Bärnighausen, Till Winfried Barone, Mark Thomaz Ugliara Barrow, Amadou Barteit, Sandra Bashir, Shahid Bashiru, Hameed Akande Basso, João Diogo Bastan, Mohammad-Mahdi Basu, Sanjay Batra, Kavita Bauckneht, Matteo Baune, Bernhard T. Beghi, Massimiliano Beiranvand, Maryam Béjot, Yannick Bell, Michelle L. Bello, Olorunjuwon Omolaja Belo, Luis Beloukas, Apostolos Beneke, Alice A. Bettencourt, Paulo J.G. Bhagavathula, Akshaya Srikanth Bhala, Neeraj Bhaskar, Sonu Bisulli, Francesca Bjørge, Tone Bodunrin, Aadam Olalekan Carvajal, Alejandro Botero Bouaoud, Souad Brayne, Carol Brenner, H Department of Primary Care and Public Health University of East Anglia Norwich United Kingdom Office for Health Improvement and Disparities Department of Health and Social Care London United Kingdom Department of Legal and Economic Studies La Sapienza University Rome Italy Rome Italy Hull York Medical School University of Hull Hull United Kingdom Department of Mathematics and Sciences Ajman University Ajman United Arab Emirates Department of Medicine Memorial University St. John's NL Canada Postgraduate Department University of Sierra Sur Miahuatlan de Porfirio Diaz Mexico Yhteiskuntadatatieteen keskus (Centre for Social Data Science) Helsinki Finland Department of Internal Medicine Federal Medical Centre Abuja Nigeria Research Center for Immunodeficiencies Tehran University of Medical Sciences Tehran Iran Department of Medical Biochemistry and Biophysics Karolinska Institutet (Karolinska Institute) Stockholm Sweden Department of Clinical Sciences University of Sharjah Sharjah United Arab Emirates Department of Biopharmaceutics and Clinical Pharmacy University of Jordan Amman Jordan Medical Research Center Hamad Medical Corporation Doha Qatar Department of Biochemistry and Molecular Medicine Alfaisal University Riyadh Saudi Arabia College of Graduate Health Sciences University of Tennessee Memphis TN United States School of Medicine Sydney NSW Australia Centre for Social Research in Health University of New South Wales Sydney NSW Australia Internal Medicine and Alcohol Related Disease Unit Fondazione Policlinico Universitario A. Gemelli IRCCS Rome Italy Department of Medical and Surgical Sciences Università Cattolica di Roma (Catholic University of Rome) Rome Italy Department of Obstetrics and Gynecology University of Texas Medical Branch Galveston TX United States Department of Biochemistry Osun State University Osogbo Nigeria Department of Pharmacology and Therapeutics University of Medical Sciences Ondo Ondo Nigeria Department of Veteri

Background: Decades of steady improvements in life expectancy in Europe slowed down from around 2011, well before the COVID-19 pandemic, for reasons which remain disputed. We aimed to assess how changes in risk factors and cause-specific death rates in different European countries related to changes in life expectancy in those countries before and during the COVID-19 pandemic. Methods: We used data and methods from the Global Burden of Diseases, Injuries, and Risk Factors Study 2021 to compare changes in life expectancy at birth, causes of death, and population exposure to risk factors in 16 European Economic Area countries (Austria, Belgium, Denmark, Finland, France, Germany, Greece, Iceland, Ireland, Italy, Luxembourg, the Netherlands, Norway, Portugal, Spain, and Sweden) and the four UK nations (England, Northern Ireland, Scotland, and Wales) for three time periods: 1990–2011, 2011–19, and 2019–21. Changes in life expectancy and causes of death were estimated with an established life expectancy cause-specific decomposition method, and compared with summary exposure values of risk factors for the major causes of death influencing life expectancy. Findings: All countries showed mean annual improvements in life expectancy in both 1990–2011 (overall mean 0·23 years [95% uncertainty interval [UI] 0·23 to 0·24]) and 2011–19 (overall mean 0·15 years [0·13 to 0·16]). The rate of improvement was lower in 2011–19 than in 1990–2011 in all countries except for Norway, where the mean annual increase in life expectancy rose from 0·21 years (95% UI 0·20 to 0·22) in 1990–2011 to 0·23 years (0·21 to 0·26) in 2011–19 (difference of 0·03 years). In other countries, the difference in mean annual improvement between these periods ranged from –0·01 years in Iceland (0·19 years [95% UI 0·16 to 0·21] vs 0·18 years [0·09 to 0·26]), to –0·18 years in England (0·25 years [0·24 to 0·25] vs 0·07 years [0·06 to 0·08]). In 2019–21, there was an overall decrease in mean annual life expectancy a

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Single Atom Bi Decorated Copper Alloy Enables C−C Coupling for Electrocatalytic Reduction of CO2into C2+Products**

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Angewandte Chemie 2023年第30期135卷

作者： Yucheng Cao Suya Chen Shuowen Bo Dr. Wenjun Fan Jiangnan Li Dr. Chunmei Jia Prof. Dr. Zhen Zhou Prof. Dr. Qinghua Liu Dr. Lirong Zheng Prof. Dr. Fuxiang Zhang State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian National Laboratory for Clean Energy Dalian 116023 Liaoning China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences Beijing 100049 China Contribution: Formal analysis (lead) Investigation (lead) Methodology (lead) Writing - original draft (lead) School of Materials Science and Engineering Institute of New Energy Material Chemistry Renewable Energy Conversion and Storage Center (ReCast) Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Nankai University Tianjin 300350 China Contribution: Data curation (equal) Formal analysis (equal) Investigation (equal) Methodology (equal) National Synchrotron Radiation Laboratory University of Science and Technology of China Hefei 230029 Anhui China Contribution: Investigation (supporting) Methodology (supporting) Beijing Synchrotron Radiation Facility Institute of High Energy Physics Chinese Academy of Sciences Beijing 100049 China

Single atom alloy (SAA) catalysts have been recently explored for promotion of various heterogeneous catalysis, but it remains unexplored for selective electrocatalytic reduction of carbon dioxide (CO 2 ) into multi-carbon (C 2+ ) products involving C−C coupling. Herein we report a single-atomic Bi decorated Cu alloy (denoted as BiCu-SAA) electrocatalyst that could effectively modulate selectivity of CO 2 reduction into C 2+ products instead of previous C 1 ones. The BiCu-SAA catalyst exhibits remarkably superior selectivity of C 2+ products with optimal Faradaic efficiency (FE) of 73.4 % compared to the pure copper nanoparticle or Bi nanoparticles-decorated Cu nanocomposites, and its structure and performance can be well maintained at current density of 400 mA cm −2 under the flow cell system. Based on our in situ characterizations and density functional theory calculations, the BiCu-SAA is found to favor the activation of CO 2 and subsequent C−C coupling during the electrocatalytic reaction, as should be responsible for its extraordinary C 2+ selectivity.

关键词： C−C Coupling CO2 Reduction Electrocatalyst Selectivity Single Atom Catalyst

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In Situ Polymerized 1,3-Dioxolane Electrolyte for Integrated Solid-State Lithium Batteries

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Angewandte Chemie 2023年第12期135卷

作者： Ye Qian Mi Wei Deng Chaohui He Prof. Dr. Osman Eksik Yi Ping Zheng De Kun Yao Dr. Xian Bin Liu Yan Hong Yin Ye Sheng Li Prof. Dr. Bao Yu Xia Prof. Dr. Zi Ping Wu Ganzhou Key Laboratory of Advanced Metals and Functional Materials Faculty of Materials Metallurgy and Chemistry Jiangxi University of Science and Technology Ganzhou 341000 China Contribution: Data curation (lead) Contribution: Formal analysis (lead) Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education) Hubei Key Laboratory of Material Chemistry and Service Failure Wuhan National Laboratory for Optoelectronics School of Chemistry and Chemical Engineering Huazhong University of Science and Technology Wuhan 430074 China Institute of Nanotechnology Gebze Technical University Gebze 41400 Turkey Contribution: Investigation (equal) Contribution: Methodology (lead) Contribution: Supervision (equal) Writing - original draft (lead) Contribution: Resources (lead) Contribution: Conceptualization (lead) Supervision (lead) Visualization (lead) Writing - review & editing (equal) Contribution: Project administration (lead) Supervision (lead) Validation (lead) Writing - original draft (lead)

Solid-state lithium batteries are promising and safe energy storage devices for mobile electronics and electric vehicles. In this work, we report a facile in situ polymerization of 1,3-dioxolane electrolytes to fabricate integrated solid-state lithium batteries. The in situ polymerization and formation of solid-state dioxolane electrolytes on interconnected carbon nanotubes (CNTs) and active materials is the key to realizing a high-performance battery with excellent interfacial contact among CNTs, active materials and electrolytes. Therefore, the electrodes could be tightly integrated into batteries through the CNTs and electrolyte. Electrons/ions enable full access to active materials in the whole electrode. Electrodes with a low resistance of 4.5 Ω □ −1 and high lithium-ion diffusion efficiency of 2.5×10 −11 cm 2 s −1 can significantly improve the electrochemical kinetics. Subsequently, the batteries demonstrated high energy density, amazing charge/discharge rate and long cycle life.

关键词： Interface Lithium Battery Polymerization Solid-State Electrolyte

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Corrigendum to: Multi-Swarm Cuckoo Search Algorithm withQ-Learning Model

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The Computer Journal 2022年第7期65卷 1938-1938页

作者： Li, Juan Xiao, Dan-dan Zhang, Ting Liu, Chun Li, Yuan-xiang Wang, Gai-ge School of Artificial Intelligence Wuhan Technology and Business University Wuhan 430065 China School of Artificial Intelligence Wuchang University of Technology Wuhan 430223 China Key Laboratory of Symbolic Computation and Knowledge Engineering of Ministry of Education Jilin University No. 2699 Qianjin Street Gaoxin District Changchun Jilin China 130012 School of Computer Wuhan University No. 299 Bayi Street Wuchang District Wuhan Hubei China 430072 Department of Computer Science and Technology Ocean University of China No. 238 Songling Street Laoshan District Qingdao Shandong China 266100 Institute of Algorithm and Big Data Analysis Northeast Normal University No. 5268 Renmin Street Nanguan District Changchun Jilin China 130117

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engineering residues on C interface to improve thermostability of nitrilase for biosynthesis of Pregabalin precursor

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AIChE Journal 2023年第11期69卷

作者： Xia-Feng Lu Xiao-Ling Tang Chen-Hui Xu Hong-Juan Diao Zhe-Ming Wu Ren-Chao Zheng Yu-Guo Zheng Key Laboratory of Bioorganic Synthesis of Zhejiang Province College of Biotechnology and Bioengineering Zhejiang University of Technology Hangzhou People's Republic of China Engineering Research Center of Bioconversion and Biopurification of Ministry of Education Zhejiang University of Technology Hangzhou People's Republic of China Contribution: Investigation (lead) Methodology (supporting) Writing - original draft (lead) Contribution: Formal analysis (supporting) Investigation (supporting) Writing - original draft (supporting) Contribution: Data curation (supporting) Formal analysis (supporting) Contribution: Formal analysis (lead) Contribution: Data curation (supporting) Contribution: Conceptualization (lead) Funding acquisition (lead) Project administration (lead) Supervision (lead) Contribution: Project administration (supporting) Supervision (supporting)

Nitrilase-mediated bioprocesses exhibited great potential in the production of value-added carboxylic acids. However, poor thermostability of nitrilases usually restricts their industrial applications. Herein, the thermostability of nitrilase Ba NIT M0 was significantly improved by engineering the amino acid residues on the intersection of two dimers (C interface). Except for simultaneous enhancement of enantioselectivity and activity, the best variant V82L/M127I/L159M/F166Q/C237S/Q260H ( Ba NIT M4 ) showed a 10.8-fold increase in half-life at 30°C compared with Ba NIT M0 . Structural analysis demonstrated that additional hydrogen bonds were formed between the residues on the C interface, which strengthened the interactions of two symmetrical regions and spirals. Subsequently, the engineered nitrilase was immobilized onto epoxy resins LXTE-603 and the immobilized nitrilase exhibited excellent stability over 12 repeated cycles, which indicated a great industrial potential for biosynthesis of Pregabalin precursor.

关键词： C interface immobilized nitrilase Pregabalin precursor protein engineering thermostability

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Favoring CO Intermediate Stabilization and Protonation by Crown Ether for CO2Electromethanation in Acidic Media

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Angewandte Chemie 2023年第50期135卷

作者： Keqiang Xu Jinhan Li Fangming Liu Xijie Chen Tete Zhao Fangyi Cheng Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Engineering Research Center on High-Efficiency Energy Storage (Ministry of Education) Renewable Energy Conversion and Storage Center College of Chemistry Nankai University Tianjin 300071 China Contribution: Data curation (lead) Formal analysis (lead) Investigation (lead) Methodology (lead) Visualization (lead) Writing - original draft (equal) Contribution: Data curation (supporting) Formal analysis (equal) Investigation (supporting) Methodology (equal) Software (equal) Validation (equal) Frontiers Science Center for New Organic Matter Nankai University Tianjin 300071 China Contribution: Formal analysis (equal) Funding acquisition (supporting) Methodology (equal) Project administration (lead) Validation (supporting) Writing - review & editing (lead) Contribution: Data curation (supporting) Formal analysis (supporting) Investigation (supporting) Methodology (supporting) Validation (supporting) Contribution: Data curation (supporting) Formal analysis (supporting) Investigation (supporting) Visualization (supporting) Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192 China Contribution: Conceptualization (lead) Formal analysis (equal) Methodology (equal) Resources (lead) Supervision (lead) Writing - review & editing (equal)

The large-scale deployment of CO 2 electroreduction is hampered by deficient carbon utilization in neutral and alkaline electrolytes due to CO 2 loss into (bi)carbonates. Switching to acidic media mitigates carbonation, but suffers from low product selectivity because of hydrogen evolution. Here we report a crown ether decoration strategy on a Cu catalyst to enhance carbon utilization and selectivity of CO 2 methanation under acidic conditions. Macrocyclic 18-Crown-6 is found to enrich potassium cations near the Cu electrode surface, simultaneously enhancing the interfacial electric field to stabilize the *CO intermediate and accelerate water dissociation to boost *CO protonation. Remarkably, the mixture of 18-Crown-6 and Cu nanoparticles affords a CH 4 Faradaic efficiency of 51.2 % and a single pass carbon efficiency of 43.0 % toward CO 2 electroreduction in electrolyte with pH=2. This study provides a facile strategy to promote CH 4 selectivity and carbon utilization by modifying Cu catalysts with supramolecules.

关键词： CO2 Electroreduction Copper Catalyst Crown Ether Methanation Protonation

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Cooperative Catalysis of Polysulfides in Lithium-Sulfur Batteries through Adsorption Competition by Tuning Cationic Geometric Configuration of Dual-active Sites in Spinel Oxides

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Angewandte Chemie 2022年第8期135卷

作者： Dr. Hongtai Li Pei Shi Lei Wang Tianran Yan Tong Guo Xiao Xia Prof. Chi Chen Prof. Jing Mao Prof. Dan Sun Prof. Liang Zhang Institute of Functional Nano & Soft Materials (FUNSOM) Soochow University Suzhou 215123 China Contribution: Conceptualization (lead) Formal analysis (lead) Writing - original draft (lead) CAS Key Laboratory of Design and Assembly of Functional Nanostructures Fujian Key Laboratory of Nanomaterials Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences Fuzhou 350002 China Xiamen Institute of Rare Earth Materials Haixi Institute Chinese Academy of Sciences Xiamen 361021 China Contribution: Data curation (lead) Investigation (equal) Contribution: Investigation (equal) Validation (equal) Contribution: Investigation (equal) Key Laboratory for Soft Chemistry and Functional Materials of Ministry of Education Nanjing University of Science and Technology Nanjing 210094 China Contribution: Data curation (equal) Investigation (equal) School of Materials Science and Engineering Zhengzhou University Zhengzhou 450001 China Contribution: Investigation (equal) Supervision (equal) Jiangsu Key Laboratory of Advanced Negative Carbon Technologies Soochow University Suzhou 215123 China Contribution: Conceptualization (lead) Funding acquisition (lead) Supervision (lead) Writing - review & editing (lead)

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