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nanoscale phase management of the 2D/3D heterostructure toward efficient perovskite solar cells

science Bulletin 2024年第18期69卷 2853-2861页

作者： Hao Gu Annan Zhu Junmin Xia Wang Li Jiahao Zheng Tao Yang Shengwen Li Nan Zhang Shiliang Mei Yongqing Cai Shi Chen Chao Liang Guichuan Xing Joint Key Laboratory of the Ministry of Education Institute of Applied Physics and Materials EngineeringUniversity of MacaoMacao 999078China State Key Laboratory of Organic Electronics and Information Displays&Institute of Advanced Materials(IAM) Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)Nanjing University of Posts&Telecommunications(NUPT)Nanjing 210023China MOE Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed Matter School of PhysicsNational Innovation Platform(Center)for Industry-Education Integration of Energy Storage TechnologyXi’an Jiaotong UniversityXi’an 710049China Ministry of Industry and Information Technology Key Lab of Micro-Nano Optoelectronic Information System Guangdong Provincial Key Laboratory of Semiconductor Optoelectronic Materials and Intelligent Photonic SystemsHarbin Institute of TechnologyShenzhen 518055China Institute for Electric Light Sources School of Information Science and TechnologyFudan UniversityShanghai 200433China

The stabilization of the formamidinium lead iodide(FAPbI_(3))structure is pivotal for the development of efficient photovoltaic *** two-dimensional(2D)layers to passivate the threedimensional(3D)perovskite is essential for maintaining the a-phase of FAPbI_(3) and enhancing the power conversion efficiency(PCE)of perovskite solar cells(PSCs).However,the role of bulky ligands in the phase management of 2D perovskites,crucial for the stabilization of FAPbI_(3),has not yet been *** this study,we synthesized nanoscale 2D perovskite capping crusts with=1 and 2 Ruddlesden-Popper(RP)perovskite layers,respectively,which form a type-Ⅱ 2D/3D *** heterostructure stabilizes the a-phase of FAPbI_(3),and facilitates ultrafast carrier extraction from the 3D perovskite network to transport contact *** introduced tri-fluorinated ligands to mitigate defects caused by the halide vacancies and uncoordinated Pb^(2+)ions,thereby reducing nonradiative carrier recombination and extending carrier *** films produced were incorporated into PSCs that not only achieved a PCE of 25.39%but also maintained 95%of their initial efficiency after 2000 h of continuous light exposure without *** findings underscore the effectiveness of a phase-pure 2D/3D heterostructure-terminated film in inhibiting phase transitions passivating the iodide anion vacancy defects,facilitating the charge carrier extraction,and boosting the performance of optoelectronic devices.

关键词： Phase-pure 2D perovskite 2D/3D heterostructure Type-II energy alignment Carrier dynamic FAPbI_(3)

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Dynamic mesophase transition induces anomalous suppressed and anisotropic phonon thermal transport

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npj Computational Materials 2024年第1期10卷 239-248页

作者： Linfeng Yu Kexin Dong Qi Yang Yi Zhang Zheyong Fan Xiong Zheng Huimin Wang Zhenzhen Qin Guangzhao Qin State Key Laboratory of Advanced Design and Manufacturing Technology for Vehicle College of Mechanical and Vehicle EngineeringHunan UniversityChangsha410082People’s Republic of China College of Physical Science and Technology Bohai UniversityJinzhou121013People’s Republic of China Hunan Key Laboratory for Micro-Nano Energy Materials&Device and School of Physics and Optoelectronics Xiangtan UniversityXiangtan411105 HunanChina School of Physics and Microelectronics Zhengzhou UniversityZhengzhou450001China Research Institute of Hunan University in Chongqing Chongqing401133China Greater Bay Area Institute for Innovation Hunan UniversityGuangzhou511300 Guangdong ProvinceChina

The physical/chemical properties undergo significant transformations in the different states arising from phase ***,due to the lack of a dynamic perspective,transitional mesophases are largely underexamined,constrained by the high resource burden of first ***,usingmolecular dynamics(MD)simulations empowered by the machine-learning potential,we proffer an innovative paradigm for phase transition:regulating the thermal transport properties via the transitional mesophase triggered by a uniaxial force *** investigate the mechanical,electrical,and thermal transport properties of the two-dimensional carbon allotrope of Janus-graphene with strain-engineered phase ***,we found that the transitional mesophase significantly suppresses the thermal conductivity and induces strong anisotropy near the phase transition *** machine-learning-driven MD simulations,we achieved highprecision atomic-level simulations of *** results show that thermal vibrationinduced intermediate amorphous or interfacial phases induce strong and anisotropic interfacial thermal *** investigation not only endows uswith a novel perspective onmesophases during phase transitions but also enhances our holistic comprehension of the evolution of material properties.

关键词： thermal transition transport

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Reliable and broad-range layer identification of Au-assisted exfoliated large area MoS_(2)and WS_(2)using reflection spectroscopic fingerprints

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nano Research 2022年第9期15卷 8470-8478页

作者： Bo Zou Yu Zhou Yan Zhou Yanyan Wu Yang He Xiaonan Wang Jinfeng Yang Lianghui Zhang Yuxiang Chen Shi Zhou Huaixin Guo Huarui Sun School of Science and Ministry of Industry and Information Technology Key Laboratory of Micro-Nano Optoelectronic Information System Harbin Institute of Technology ShenzhenShenzhen 518055China Collaborative Innovation Center of Extreme OpticsShanxi UniversityTaiyuan 030006China State Key Laboratory of Superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China University of Science and Technology of China Hefei 230026China Science and Technology on Monolithic Integrated Circuits and Modules Laboratory Nanjing Electronic Devices InstituteNanjing 210016China

The emerging Au-assisted exfoliation technique enables the production of a wealth of large-area and high-quality ultrathin two dimensional(2D)***,damage-free,and reliable determination of the layer number of such 2D films can greatly promote layer-dependent physical studies and device ***,an optical method has been developed for simple,high throughput,and accurate determination of the layer number for Au-assisted exfoliated MoS_(2)and WS_(2)films in a broad thickness *** method is based on quantitative analysis of layer-dependent white light reflection spectra(WLRS),revealing that the intensity of exciton-induced reflection peaks can be used as a clear indicator for identifying the layer *** simple yet robust method will facilitate fundamental studies on layer-dependent optical,electrical,and thermal properties and device applications of 2D *** technique can also be readily combined with photoluminescence(PL)and Raman spectroscopies to study other layer-dependent physical properties of 2D materials.

关键词： Au-assisted exfoliation MoS_(2)and WS_(2) layer identification white light reflection spectra excitonic peaks

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Multitarget gas alarm system for high-performance and anti-interference chemical warfare agents simulants detection

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science China(Technological sciences) 2025年第3期68卷 349-358页

作者： Yubin YUAN Qiang WU Menglong JIAO Haiyang WU Weihua LIU Xuming WANG Xiangrui BU Gong LI Chuanyu HAN Long HU Xin LI Xiaoli WANG Shool of Microelectronics School of Electronics and Information EngineeringXi’an Jiaotong UniversityXi’an710049China The Key Lab of Micro-nano Electronics and System Integration of Xi’an City Xi’an710049China Hangzhou Institute for Advanced Study University of Chinese Academy of SciencesHangzhou310024China School of Automation and Information Engineering Xi’an University of TechnologyXi’an710048China Key Laboratory for Physical Electronics and Devices of the Ministry of Education Xi’an Jiaotong UniversityXi’an710049China School of Science Xi’an Jiaotong UniversityXi’an710049China

Chemical warfare agents(CWAs)can cause significant harm to health and even death in a very short time even when inhaled in small amounts(~100 mg min/m^(3)).Detection equipment based on conventional techniques,including gas chromatography-mass spectrometry,Raman spectroscopy,fluorescence spectroscopy,and ion mobility spectrometry,have the disadvantages of high cost,long detection time,and high power ***,portable,and convenient equipment for target CWAs detection under interference is a *** this study,we propose an alarm system comprising a multitype micro sensor array and a field-programmable gate array-based readout circuit for CWAs simulants *** common volatile organic compound,temperature,and water vapor interference,the proposed multitype sensor-based detection system realizes an alarm function in less than 20 s with thresholds of 1 ppm dimethyl methylphosphonate(DMMP),4.6 ppm 2,2'-dichlorodiethyl ether(DCE),and 20 ppm SO_(2).Furthermore,the proposed detection system was evaluated outside the laboratory and passed the wilderness test,demonstrating its reliability in the *** believe that the proposed alarm system will contribute to the development of intelligent,portable,low-cost,and anti-interference CWAs detection technology.

关键词： alarm system CWAs simulants surface acoustic wave sensor mixed gas anti-interference

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trans-2-Enoyl-CoA Reductase Tecr-Driven Lipid Metabolism in Endothelial Cells Protects against Transcytosis to Maintain Blood-Brain Barrier Homeostasis

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Research 2022年第3期2022卷 75-89页

作者： Jinxuan Wang Jianxiong Xu Guangchao Zang Tao Zhang Qi Wu Hongping Zhang Yidan Chen Yi Wang Weixi Qin Shuang Zhao Erdai Qin Juhui Qiu Xiaojuan Zhang Lin Wen Yeqi Wang Guixue Wang Key Laboratory for Biorheological Science and Technology of Ministry of Education State and Local Joint Engineering Laboratory for Vascular ImplantsBioengineering College of Chongqing UniversityChongqing 400030China Institute of Life Science Laboratory of Tissue and Cell BiologyLab Teaching&Management CenterChongqing Medical UniversityChongqing 400016China Chongqing Key Laboratory of Nano/Micro Composite Material and Device School of Metallurgy and Materials EngineeringChongqing University of Science and TechnologyChongqing 401331China College of Basic Medical Sciences Chongqing Medical UniversityChongqing 400016China

The transport and metabolism of lipids in cerebrovascular endothelial cells(ECs)have been hypothesized to regulate blood-brain barrier(BBB)maturation and ***-chain polyunsaturated fatty acids(LCPUFAs)as the important lipids components of cell membranes are essential for the development and function of BBB,but the direct links of lipid metabolism and ECs barrier function remain to be ***,we comprehensively characterize the transcriptomic phenotype of developmental cerebrovascular ECs in single-cell resolution and firstly find that trans-2-enoyl-CoA reductase(Tecr),a verylong-chain fatty acid synthesis,is highly expressed during barriergenesis and decreased after BBB ***-specific knockout of Tecr compromises angiogenesis due to delayed vascular ***,EC-specific deletion of Tecr loss restrictive quality of vascular permeability from neonatal stages to adulthood,with high levels of transcytosis,but maintains the vascular tight ***,lipidomic analysis shows that the expression of Tecr in ECs is associated with the containing of omega-3 fatty acids,which directly suppresses caveolae vesicles *** results reveal a protective role for Tecr in BBB integrity and suggest that Tecr as a novel therapeutic target in the central nervous system(CNS)diseases associated with BBB dysfunction.

关键词： metabolism barrier Blood

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Nonvolatile Reconfigurable Phase-change-materials Integrated Silicon Photonics

Nonvolatile Reconfigurable Phase-change-materials Integrated...

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2024 Photonics and Electromagnetics Research Symposium, PIERS 2024

作者： Xu, Kai Wei, Maoliang Tang, Bo Li, Junying Yun, Yiting Lei, Kunhao Wu, Yingchun Li, Lan Lin, Hongtao Zhejiang University State Key Laboratory of Modern Optical Instrumentation Key Laboratory of Micro-Nano Electronics and Smart System of Zhejiang Province College of Information Science and Electronic Engineering Hangzhou China Institute of Microelectronics of the Chinese Academy of Sciences Beijing China University of Chinese Academy of Sciences Hangzhou Institute for Advanced Study Hangzhou China Westlake University Key Laboratory of 3D Micro/Nano Fabrication and Characterization of Zhejiang Province School of Engineering Hangzhou China Westlake Institute for Advanced Study Institute of Advanced Technology Hangzhou China

ISBN: (纸本)9798350375909

The emergence of integrated photonic technology provides an attractive solution of high speed, broad bandwidth and strong parallelism for large-scale information transmission and processing in interconnection, communication and computing. Reconfigurability is necessary for photonic processors to adapt varieties of application scenarios in the fields of data exchange, microwave photonics and neural networks. As yet, thermo-optical effect and carrier plasma dispersion effect are the most common phenomena for optical modulation. However, the volatility not only requires continuous power supply to maintain the devices' state, but also accompanies with serious thermal crosstalk induced by active regions. Hence, the nonvolatile methods that can reconfigure and fix on the current state for a long time after a single external excitation are considered as one of the significant technologies in the next generation of integrated photonics. Nonvolatile reconfiguration has been achieved through trapped-charge effect, bistable micro-electromechanical system (MEMS) with nano-latch mechanism and ferroelectric materials, which suffer from high loss, lower stability and complex process flow. Chalcogenide phase change materials (PCM) have become a promising method to realize compact and nonvolatile reconfigurable integrated photonic devices due to the high optical constant contrast between amorphous state and crystalline state, superiorly stable property and low temperature deposition possibility. Here, we developed a monolithic back-end-of-line integration technology of PCM in silicon photonics, supporting "Zero-change"heterogeneous integration platform at wafer scale. On this basis, nonvolatile integrated photonic devices with excellent performance have been fabricated. It lays a foundation for improving the energy efficiency and integration density of integrated photonic processors and suppressing thermal crosstalk between integrated photonic devices. © 2024 IEEE.

关键词： Silicon wafers

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3D bioprinting of in vitro porous hepatoma models:establishment,evaluation,and anticancer drug testing

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Bio-Design and Manufacturing 2024年第2期7卷 137-152页

作者： Xiaoyuan Wang Zixian Liu Qianqian Duan Boye Zhang Yanyan Cao Zhizhong Shen Meng Li Yanfeng Xi Jianming Wang Shengbo Sang Shanxi Key Laboratory of Micro Nano Sensors and Artificial Intelligence Perception College of Electronic Information and Optical EngineeringTaiyuan University of TechnologyTaiyuan 030024China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of TechnologyTaiyuan 030024China Shanxi Institute of 6D Artificial Intelligence Biomedical Science Taiyuan 030031China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030024China Department of Pathology Shanxi Provincial Cancer HospitalTaiyuan 030024China General Hospital of Taiyuan Iron and Steel Company Taiyuan 030809China

Traditional tumor models do not tend to accurately simulate tumor growth in vitro or enable personalized treatment and are particularly unable to discover more beneficial targeted *** address this,this study describes the use of threedimensional(3D)bioprinting technology to construct a 3D model with human hepatocarcinoma SMMC-7721 cells(3DP-7721)by combining gelatin methacrylate(GelMA)and poly(ethylene oxide)(PEO)as two immiscible aqueous phases to form a bioink and innovatively applying fluorescent carbon quantum dots for long-term tracking of *** GelMA(10%,mass fraction)and PEO(1.6%,mass fraction)hydrogel with 3:1 volume ratio offered distinct pore-forming characteristics,satisfactorymechanical properties,and biocompatibility for the creation of the 3DP-7721 *** analysis and quantitative real-time fluorescence polymerase chain reaction(PCR)were used to evaluate the biological properties of the *** with the two-dimensional culture cell model(2D-7721)and the 3D mixed culture cell model(3DM-7721),3DP-7721 significantly improved the proliferation of cells and expression of tumor-related proteins and ***,we evaluated the differences between the three culture models and the effectiveness of antitumor drugs in the three models and discovered that the efficacy of antitumor drugs varied because of significant differences in resistance proteins and genes between the three *** addition,the comparison of tumor formation in the three models found that the cells cultured by the 3DP-7721 model had strong tumorigenicity in nude *** evaluation of the levels of biochemical indicators related to the formation of solid tumors showed that the 3DP-7721 model group exhibited pathological characteristics of malignant tumors,the generated solid tumors were similar to actual tumors,and the deterioration was *** research therefore acts as a foundation for the application of 3DP-7721 models in drug devel

关键词： 3D bioprinting Hepatoma tumor models Drug screening Antitumor drug development

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Array of single crystalline anatase TiO2 nanotubes with significant enhancement of photoresponse

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Progress in Natural science:Materials International 2021年第4期31卷 536-540页

作者： Lvchao Qiu Ke Fang Yubo Li Shutao Huang Guanxing Li Songda Li Hu He Wentao Yuan Hangsheng Yang Wei Tian Yong Wang State Key Laboratory of Silicon Materials School of Materials Science and Engineering Zhejiang University Center of Electron Microscopy School of Materials Science and Engineering Zhejiang University Key Laboratory of Micro-Nano Electronic Device and Smart System of Zhejiang Province College of Information Science & Electronic Engineering Zhejiang University School of Physical Science and Technology Soochow University

Anatase TiO2nanotubes array（ATONA） has attracted tremendous attention owing to its promising applications in solar cells, water splitting and organic pollutants photocatalytic degradation. However, the activity of ATONAs was greatly suppressed by the grain boundaries existed in the tube walls, which acted as carrier scattering and recombination centers. Herein, we report a novel strategy to prepare array of single crystalline anatase TiO2nanotubes（SC-ATONAs） with significant enhancement of the photocatalytic activity and UV photo response performance compared to the polycrystalline counterparts. The growth of SC-ATONAs was achieved by establishing a crystallization temperature gradient along the tube wall, which ensured the crystallization started from the nucleation of a single nucleus at the bottom of amorphous TiO2nanotubes prepared by Ti anodization. These findings pave the way to prepare single-crystalline nanotubes with superior performance for other materials.

关键词： Single crystallineTiO2 nanotube Crystallization temperature gradient Photo response Photocatalysis

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Molten salt as ultrastrong polar solvent enables the most straightforward pyrolysis towards highly efficient and stable single-atom electrocatalyst

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Journal of Energy Chemistry 2021年第3期30卷 519-527页

作者： Nannan Li Wei Liu Chao Zhu Ce Hao Jingya Guo Hongyu Jing Jinwen Hu Cuncun Xin Danyang Wu Yantao Shi State Key Laboratory of Fine Chemicals Department of ChemistrySchool of Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina SEU-FEI Nano-Pico Center Key Laboratory of MEMS of Ministry of EducationCollaborative Innovation Center for Micro/Nano FabricationDevice and SystemSoutheast University2 No.4 PailouNanjing 210096JiangsuChina

Currently,pyrolysis as the most widely used method still has some key issues not well resolved for synthesis of carbon-supported single-atom catalysts(C-SACs),e.g.,the sintering of metal atoms at high temperature as well as the high cost and complicated preparations of *** this report,molten salts are demonstrated to be marvellous medium for preparation of C-SACs by pyrolysis of small molecular precursors(ionic liquid).The ultrastrong polarity on one hand establishes robust interaction with precursor and enables better carbonization,resulting in largely enhanced *** the other hand,the aggregation of metal atoms is effectively refrained while no nanoparticle or cluster is *** this strategy,a C-SAC with atomically dispersed Fe-N_(4) sites and a high specific area over 2000 m^(2) g^(-1) is obtained,which illustrates high ORR activity in both acid and alkaline ***,this SAC exhibits superior methanol tolerance and stability after acid soaking at 85℃ for 48 *** is believed that the molten-salts-assisted pyrolysis can be developed into a routine strategy as it not only can largely simply the synthesis of C-SACs,but also can be extended to prepare other types of SACs.

关键词： Ultrastrong polar solvent Molten salts one-pot pyrolysis Carbon-supported single atom catalysts Oxygen reduction reaction

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Graphene-based dual-function acoustic transducers for machine learning-assisted human-robot interfaces

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InfoMat 2023年第2期5卷 66-79页

作者： Hao Sun Xin Gao Liang-Yan Guo Lu-Qi Tao Zi Hao Guo Yangshi Shao Tianrui Cui Yi Yang Xiong Pu Tian-Ling Ren Institute of Microelectronics and Beijing National Research Center for Information Science and Technology(BNRist) Tsinghua UniversityBeijingPeople's Republic of China CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and SensorBeijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijingPeople's Republic of China State Key Laboratory of Power Transmission Equipment and System Security and New Technology School of Electrical EngineeringChongqing UniversityChongqingPeople's Republic of China School of Computer Science&Technology Beijing Institute of TechnologyBeijingPeople's Republic of China School of Automation and Electrical Engineering University of Science and Technology BeijingBeijingPeople's Republic of China

Human–robot interface(HRI)electronics are critical for realizing robotic ***,we report graphene-based dual-function acoustic transducers for machine learning-assisted human–robot interfaces(GHRI).The GHRI functions both an artificial ear through the triboelectric acoustic sensing mechanism and an artificial mouth through the thermoacoustic sound emission *** success of the integrated device is also attributed to the multifunctional laser-induced graphene,as either triboelectric materials,electrodes,or thermoacoustic *** systematically optimizing the structure parameters,the GHRI achieves high sensitivity(4500 mV Pa^(–1))and operating durability(1000000 cycles and 60 days),capable of recognizing speech identities,emotions,content,and other information in the human *** the assistance of machine learning,30 speech categories are trained by a convolutional neural network,and the accuracy reaches 99.66%and 96.63%in training datasets and test ***,GHRI is used for artificial intelligence communication based on recognized speech *** work shows broad prospects for the development of robotic intelligence.

关键词： human-robot interface laser-induced graphene machine learning thermoacoustic triboelectric nanogenerator

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