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A novel N-stable Co 2 P nano-catalyst for the synthesis of quinoxalines by annulation of alkynes and 1,2-diaminobenzenes

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Chinese Chemical Letters 2025年第8期36卷

作者： Xiaochun Liu Gaoyan Chen Xiaodong Yue Chaoyue Wang Xue-Xin Zhang Xuecheng Ran Yingxiao Zong Junke Wang Xicun Wang Gansu Key Laboratory of Polymer Materials College of Chemistry and Chemical Engineering Northwest Normal University Lanzhou 730070 China Key Laboratory of Hexi Corridor Resources Utilization of Gansu College of Chemistry and Chemical Engineering Hexi University Zhangye 734000 China Key Laboratory of Opto-Electronic Technology and Intelligent Control (Ministry of Education) Lanzhou Jiaotong University Lanzhou 730070 China Hubei Key Laboratory of Processing and Application of Catalytic materials Huanggang Normal University Huanggang 438000 China

Designing efficient, recyclable, and low-cost catalysts is crucial for the synthesis of quinoxaline derivatives. In this context, a novel N -stable Co 2 P nano-catalyst (CoP@N C-1.5) was developed using a template-sacrificial approach. The catalyst demonstrated a broad substrate scope and good functional group tolerance, achieving yields of up to 84 %. Additionally, the catalyst exhibited reusability and can be recycled up to three times. The CoP@N C-1.5 was characterized using X-ray powder diffraction (XRD), scanning electron microscopy (SEM), and transmission electron microscopy (TEM). The results indicated that the catalyst contained Co 2 P nanoparticles. The X-ray photoelectron spectroscopy (XPS) further confirms the presence of Co-P. Analysis of the characterization data and experimental results revealed that the active site of the catalyst comprises N -stable Co 2 P nanoparticles.

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3D model retrieval using density-based silhouette descriptor

3D model retrieval using density-based silhouette descriptor

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2nd International Conference on Pattern Recognition Applications and Methods, ICPRAM 2013

作者： Tang, Qi Yang, Xin Institute of Image Processing and Pattern Recognition Shanghai Jiao Tong University Shanghai China Key Laboratory of System Control and Information Processing Ministry of Education of China Shanghai 200240 China

ISBN: (纸本)9789898565419

In this paper we present a new content-based retrieval descriptor, density-based silhouette descriptor (DBS). It characterizes a 3D object with multivariate probability functions of its 2D silhouette features. The new descriptor is computationally efficient and induces a permutation property that guarantees invariance at the matching stage. Also, it is insensitive to small shape perturbations and mesh resolution. The retrieval performance on several 3D databases shows that the DBS provides state-of-art discrimination over a broad and heterogeneous set of shape categories.

关键词： Probability density function

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Changes in spectrum mapping in rhythmic movement involved in walking after spinal cord injury

Changes in spectrum mapping in rhythmic movement involved in...

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2013 IEEE International Conference on Medical Imaging Physics and Engineering, ICMIPE 2013

作者： Wei, Li Zhiqiao, Yan Yue, Huang Jiang, Xu Image Processing and Intelligent Control Key Laboratory Education Ministry of China China School of Automation Huazhong University of Science and Technology Wuhan 430074 China Rehabilitation Department Tongji Hospital Wuhan 430074 China

ISBN: (纸本)9781467360128

Spectrum mapping reflects the strength of brain electrical activity in different frequency band. The current study analyzes changes in electroencephalography (EEG) after spinal cord injury (SCI) on the basis of spectrum mapping. Comparing spectrum mappings of SCI patients and normal subjects, the fact that beta rhythm dominated in brain electrical activity during walking period was concluded. In addition, the proportion of delta wave increased and slightly exceeded that of beta wave after spinal cord injury and power values in delta band of SCI patients performed greater than that of normal subjects. © 2013 IEEE.

关键词： Electroencephalography

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Integrating segmentation and classification accuracy for accuracy assessment in object-based image analysis

Integrating segmentation and classification accuracy for acc...

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2012 3rd IEEE/IET International Conference on Audio, Language and image processing, ICALIP 2012

作者： Li, Nan Huo, Hong Fang, Tao Institute of Image Processing and Pattern Recognition Department of Automation Shanghai Jiao Tong University Shanghai China Key Laboratory of System Control and Information Processing Ministry of Education Shanghai China

ISBN: (纸本)9781467301718

An accuracy assessment method that integrates segmentation and classification accuracy is proposed to meet the requirements of object-based image analysis. Segmentation errors are measured by establishing the relationship between pixels and their corresponding segments according to the overlaps of segments and reference polygons. Then, two improved confusion matrices that take the segmentation errors into consideration are used: one for pixel-level classification results, and the other for object-level classification results. A final accuracy assessment combines the statistics of these two confusion matrices. The proposed method can be applied to segmentation scale selection in the hierarchical interpretation system. An experiment on a SPOT5 image demonstrates the effectiveness of this method for segmentation scale selection, which can guide the fusion of objects of different scales to obtain a higher accuracy. © 2012 IEEE.

关键词： image analysis

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Runway detection of an unmanned landing aerial vehicle based on vision

Runway detection of an unmanned landing aerial vehicle based...

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MIPPR 2005: SAR and Multispectral image processing

作者： Wang, Hongqun Peng, Jiaxiong Li, Lingling Institute for Pattern Recognition and Artificial Intelligence State Education Commission Key Laboratory for Image Processing and Intelligent Control Huazhong University of Science and Technology Wuhan 430074

When an monocular vision-based unmanned aerial vehicle (UAV) based on vision is flown to the final approach fix to intercept the glide slope without the navigation of Global Positioning System (GPS), the position and orientation of the airport runway in image must be detected accurately so as to a host of suitable procedures have to be followed. The optimum length of the final approach is about five miles from the runway threshold. The front view of the runway, which is achieved at the moment, is very illegible. The approaching marking (cross bar) of the runway are showed as some white spots of high intensity and the complicated backgrounds of the airport are included in the images. In this case, spots with high intensity should be extracted and classified, some of these spots are just the images of the background noises and the pseudo-targets, which can't be separated with the spots of the runway as in the view there is no significant characteristic difference among them ostensibly. Fortunately, in the terrestrial coordinate space, most of the runway marks are located at the apexes of a rectangle, having some geometric relationships. The relationship among the projection coordinates of the runway spots in the images can be determined according to the perspective principle, the constraint condition of the rectangle as well as the front shot constraint condition of the target, by using this relationship, the runway approaching marks can be separated, the position and the direction of the runway in the images can be identified. In this paper, the clustering management is adopted so as to greatly reduce the computing time. The consequence of the experiments shows that by this algorithm, even from a place far away from the runway whose marks are unclear, we also can effectively detect the runway.

关键词： Unmanned vehicles

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Lithium-ion battery state-of-charge estimation using a real-time moving horizon estimation algorithm

Lithium-ion battery state-of-charge estimation using a real-...

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2021 CAA Symposium on Fault Detection, Supervision, and Safety for Technical Processes, SAFEPROCESS 2021

作者： Yan, Jiayu Li, Song Wan, Yiming Huazhong University of Science and Technology Key Laboratory of Image Processing and Intelligent Control Ministry of Education Wuhan China 29th Research Institute of China Electronics Technology Group Corporation Chengdu China

ISBN: (纸本)9781665401159

For battery management systems, it is significant to reliably estimate state-of-charge (SOC) from limited measurements in real time. Based on a nonlinear SOC-dependent equivalent circuit model, we propose a real-time moving horizon estimation (MHE) algorithm for SOC estimation. For efficient computation, the sequential quadratic programming strategy is applied, and each quadratic programming (QP) iteration is solved via the structure-exploiting forward and backward recursions. To account for the limited computation time allowed within each sampling interval, the proposed algorithm does not fully solve the receding horizon optimization problem over each sliding window, but performs fixed number of QP iterations. The simulation results show that compared to the existing fully solved MHE applied to SOC estimation, the proposed real-time MHE algorithm significantly saves computation time at the cost of a slight loss of estimation performance. © 2021 IEEE.

关键词： Quadratic programming

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Optimal Power and Gas Flow of Energy Internet with Non-Isothermal Process and Energy Storage 43

Optimal Power and Gas Flow of Energy Internet with Non-Isoth...

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43rd Chinese control Conference, CCC 2024

作者： Liu, Chen He, Shiyuan Wang, Xinyi Liu, Xiao-Kang Huazhong University of Science and Technology School of Artificial Intelligence and Automation Wuhan430074 China Huazhong University of Science and Technology Ministry of Education Key Laboratory of Image Processing and Intelligent Control Wuhan430074 China

ISBN: (纸本)9789887581581

The electrical-gas coupled power flow problem is one of the most basic problems under Energy Internet. In order to achieve a more complete analysis of the electric-gas coupled power flow, this paper establishes a novel integrated energy system model that considers electricity and natural gas. This model integrates the power system AC power flow model and the non-isothermal process of natural gas pipeline transmission, achieving a more accurate description of the power grid and gas network power flow. At the same time, the beneficial effects of energy storage units on the network of each part of the system are analyzed. Through simulation design, the benefits of energy storage access on system cost and security are analyzed and quantified. © 2024 Technical Committee on control Theory, Chinese Association of Automation.

关键词： Energy storage

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An improved mapping method of buffer for line-based architecture of 2-D DWT

An improved mapping method of buffer for line-based architec...

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2005 International Conference on Communications, Circuits and Systems

作者： Xiong, Cheng-Yi Wang, Cheng-Jun Tian, Jin-Wen Liu, Jian College of Electronic Information Engineering South-Center University for Nationalities Wuhan 430074 China Key Laboratory of Education Huazhong University of Science and Technology Ministry for Image Processing and Intelligent Control Wuhan 430074 China

ISBN: (纸本)0780390156

The number of arithmetic units used in one-dimensional (1-D) discrete wavelet transform (DWT) is the main consideration for reducing the area of VLSI implementation of 1-D DWT, while the size of intermediate memory used for data buffering is another dominate factor of effecting hardware complexity of VLSI implementation for two-dimensional (2-D) DWT. In this paper, we exploit the essential relationship between the size of temporal buffer (TB) required in the line-based architecture for 2-D DWT (LBA2DDWT) and the number of register used in 1-D DWT module, and present an improved method of mapping the registers used in 1-D DWT to the TB required in LBA2DDWT. Comparison results with the other design reported in previous literature demonstrate that, the proposed mapping method can reduce efficiently the size of memory required in LBA2DDWT. © 2005 IEEE.

关键词： Wavelet transforms

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Learning from Noisy Labels with Coarse-to-Fine Sample Credibility Modeling 17th

Learning from Noisy Labels with Coarse-to-Fine Sample Cred...

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17th European Conference on Computer Vision, ECCV 2022

作者： Zhang, Boshen Li, Yuxi Tu, Yuanpeng Peng, Jinlong Wang, Yabiao Wu, Cunlin Xiao, Yang Zhao, Cairong YouTu Lab Shenzhen China Tongji University Shanghai China Key Laboratory of Image Processing and Intelligent Control Ministry of Education School of Artificial Intelligence and Automation Huazhong University of Science and Technology Wuhan China

ISBN: (纸本)9783031250620

Training deep neural network (DNN) with noisy labels is practically challenging since inaccurate labels severely degrade the generalization ability of DNN. Previous efforts tend to handle part or full data in a unified denoising flow via identifying noisy data with a coarse small-loss criterion to mitigate the interference from noisy labels, ignoring the fact that the difficulties of noisy samples are different, thus a rigid and unified data selection pipeline cannot tackle this problem well. In this paper, we first propose a coarse-to-fine robust learning method called CREMA, to handle noisy data in a divide-and-conquer manner. In coarse-level, clean and noisy sets are firstly separated in terms of credibility in a statistical sense. Since it is practically impossible to categorize all noisy samples correctly, we further process them in a fine-grained manner via modeling the credibility of each sample. Specifically, for the clean set, we deliberately design a memory-based modulation scheme to dynamically adjust the contribution of each sample in terms of its historical credibility sequence during training, thus alleviating the effect from noisy samples incorrectly grouped into the clean set. Meanwhile, for samples categorized into the noisy set, a selective label update strategy is proposed to correct noisy labels while mitigating the problem of correction error. Extensive experiments are conducted on benchmarks of different modality, including image classification (CIFAR, Clothing1M etc.) and text recognition (IMDB), with either synthetic or natural semantic noises, demonstrating the superiority and generality of CREMA. © 2023, The Author(s), under exclusive license to Springer Nature Switzerland AG.

关键词： Deep neural networks

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An advanced actor-critic algorithm for training video game ai 1st

An advanced actor-critic algorithm for training video game a...

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1st International Conference on Neural Computing for Advanced Applications, NCAA 2020

作者： Zha, Zhong Yi Tang, Xue Song Wang, Bo Key Laboratory of Ministry of Education for Image Processing and Intelligent Control Artificial Intelligence and Automation School Huazhong University of Science and Technology Wuhan430074 China College of Information and Science Donghua University Shanghai China

ISBN: (纸本)9789811576690

This paper presents an improved deep reinforcement learning (DRL) algorithm, namely Advanced Actor Critic (AAC), which is based on Actor Critic (AC) algorithm, to the video game Artificial intelligence (AI) training. The advantage distribution estimator, Normal Constraint (NC) function and exploration based on confidence are introduced to improve the AC algorithm, in order to achieve accurate value estimate, select continuous spatial action correctly, and explorate effectively. The aim is to improve the performance of conventional AC algorithm in a complex environment. A case study of video game StarCraft II mini-game AI training is employed. The results verify that the improved algorithm effectively improves the performance in terms of the convergence rate, maximum reward, average reward in every 100 episode, and time to reach a specific reward, etc. The analysis on how these modifications improve the performance is also given through interpretation of the feature layers in the mini-games. © Springer Nature Singapore Pte Ltd. 2020.

关键词： Reinforcement learning

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