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Atomic-Scale Insights into Flexoelectricity and the Enhanced Photovoltaic Effect at the Grain Boundary in Halide Perovskites

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Nano letters 2025年 2025 May 25页

作者： Yaonan Xiong Zhiming Luo Wenjing Chen Zhou Li Sanxia Yin Chenchen Peng Jinhua Hong Junlei Qi Meng-Qiu Cai Zhengguo Xiao Chao Ma Shulin Chen National Key Laboratory of Power Semiconductor and Integration Technology Engineering Research Center of Advanced Semiconductor Technology and Application of Ministry of Education College of Semiconductors (College of Integrated Circuits) Hunan University Changsha 410082 China. State Key Laboratory of Precision Welding & Joining of Materials and Structures Harbin Institute of Technology Harbin 150001 China. Hunan Provincial Key Laboratory of High-Energy Scale Physics and Applications School of Physics and Electronics Hunan University Changsha 410082 China. Hefei National Laboratory for Physical Science at the Microscale Department of Physics CAS Key Laboratory of Strongly-coupled Quantum Matter Physics University of Science and Technology of China Hefei 230026 China. College of Materials Science and Engineering Hunan University Changsha 410082 China.

Grain boundaries (GBs) generally exist in halide perovskites and are often accompanied by structural distortions or composition segregation, significantly altering their optoelectronic properties. However, the atomic-scale mechanisms underpinning these effects remain elusive due to the inherent complexity of the GB structures. By employing aberration-corrected transmission electron microscopy, we directly visualize the atomic structures of GBs in halide perovskites, uncovering the emergence of flexoelectricity and associated polarization-induced shift-currents. We demonstrate that a large strain gradient at 52° GBs induces significant flexoelectric polarization. This flexoelectricity is observed across GBs with different compositions and misorientation angles. First-principles calculations confirm that such flexoelectric polarization can enhance the photovoltaic effect, resulting in a shift-current of ∼15 μA V. These findings uncover a previously unrecognized role of GBs in halide perovskites and provide new insights into leveraging GB engineering to achieve flexoelectricity and regulate optoelectrical properties in halide perovskites.

关键词： TEM atomic scale flexoelectricity grain boundary halide perovskites

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A multi-channel wearable sensing patch based on gate-all-around field-effect transistors

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Lab on a chip 2025年 2025 May 28页

作者： Zhe Xing Qiang Liu Bo Lin Shuang Li Yuxin Liu Guanyang Zhang Wenjie Yu Zhenhua Wu Hongju Mao State Key Laboratory of Transducer Technology Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences Shanghai 200050 China. wuzhx@***. Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences Beijing 100049 China. National Key Laboratory of Materials for Integrated Circuits Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences Shanghai 200050 China. Academy of Medical Engineering and Translational Medicine Tianjin University Tianjin 300072 China. Center for Medical Research and Innovation Shanghai Pudong Hospital Fudan University Pudong Medical Center Shanghai 200120 China.

Field-effect transistors (FETs), known for their rapid response and signal amplification capabilities, have attracted significant research interest for the detection of biomarkers. However, the development of multi-channel sensors using FETs and their wearable applications are impeded by the rigid substrates and large areas. Here, we reported a wearable EGFET sensor array patch that integrates gate-all-around field-effect transistors (GAA FETs) and flexible printed circuit board (FPCB) patches to overcome these challenges. The patch takes advantage of the excellent electrical properties and small size of GAA FETs, allowing for multi-biomarker detection. Additionally, it integrates large-scale, low-cost FPCB-based electrodes to enhance the flexibility of the patch. Comprehensive characterization experiments have demonstrated the performance of the patch to detect multiple biomarkers, including glucose, lactate, Na, K, and Ca. This innovative patch is promising to facilitate the development of FET-based multi-channel wearable sensors, and has the potential to help realize more comprehensive health monitoring.

关键词： MISFET devices

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A Method to Recognize Sleeping Position Using an CNN Model Based on Human Body Pressure Image

A Method to Recognize Sleeping Position Using an CNN Model B...

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2019 IEEE International Conference on Power, Intelligent Computing and Systems, ICPICS 2019

作者： Liu, Zhong Wang, Xin'an Su, Mingliang Lu, Ken School of Electronics Engineering and Computer Science Peking University China Key Laboratory of Integrated Micro-System Science and Engineering Applications Peking University Shenzhen Graduate School Shenzhen China IFutureLab Inc. United States

ISBN: (纸本)9781728137209

Sleep is an important part of human life. Recognition of sleeping position is an important part of judging the quality of sleep, warning disease and prevention of pressure sores. At present, the body pressure is being used as a commonly method to recognize sleep gesture, and most of it is based on methods of extracting features, mainly based on local signs and global features. This paper proposes a deep learning method based on CNN deep learning method to deal with recognition of body pressure image. Compared with the previous methods, the method based on CNN neural network achieves higher accuracy of recognition at a lower cost and is suitable for complex application environments, which has good practical value. © 2019 IEEE.

关键词： Sleep research

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A Study on Sleep Position Recognition of Body Pressure Image based on KPCA and SVM

A Study on Sleep Position Recognition of Body Pressure Image...

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2019 IEEE International Conference on Power, Intelligent Computing and Systems, ICPICS 2019

作者： Liu, Zhong Wang, Xin'an Le, Yang Sun, Jone School of Electronics Engineering and Computer Science Peking University China Key Laboratory of Integrated Micro-System Science and Engineering Applications Peking University Shenzhen Graduate School Shenzhen China IFutureLab Inc. United States

ISBN: (纸本)9781728137209

Sleep is an important part of life, and sleep position recognition is an important indicator which reflects sleep quality, warns diseases and prevents pressure sores. Actually, sleep quality is usually related to the body pressure, which affects muscle comfort and blood circulation during sleep. However, in order to regulate the body pressure, one vital step is to recognize the sleep position. Body pressure is a common indicator of the recognition of sleep position. This investigation put forward a body pressure recognition method combining with kernel principal component analysis (KPCA) and support vector machine. The feature extraction based on KPCA can well solve the nonlinear separable problems as well as dimension reduction processing of PCA, and reduce the system's complexity. Compared with the image recognition method and computer vision recognition method, it realized a higher recognition accuracy at a lower cost. Ultimately, the recognition accuracy of six common sleep positions reached 96.5%. © 2019 IEEE.

关键词： Support vector machines

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Fungal diversity notes 1611-1716: taxonomic and phylogenetic contributions on fungal genera and species emphasis in south China

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Fungal Diversity 2023年第5期122卷 161-403页

作者： Indunil C.Senanayake Walter Rossi Marco Leonardi Alex Weir Mark McHugh Kunhiraman C.Rajeshkumar Rajnish K.Verma Samantha C.Karunarathna Saowaluck Tibpromma Nikhil Ashtekar Sreejith K.Ashtamoorthy Sanjay Raveendran Gurmeet Kour Aishwarya Singh Saúl De la Peña-Lastra Antonio Mateos Miroslav Kolařík Vladimír Antonín HanaŠevčíková Fernando Esteve-Raventós Ellen Larsson Fermín Pancorbo Gabriel Moreno Alberto Altés Yolanda Turégano Tian-Ye Du Li Lu Qi-Rui Li Ji-Chuan Kang Sugantha Gunaseelan Kezhocuyi Kezo Malarvizhi Kaliyaperumal Jizhen Fu Milan C.Samarakoon Yusufjon Gafforov Shakhnoza Teshaboeva Pradeep C.Kunjan Arya Chamaparambath Adam Flakus Javier Etayo Pamela Rodriguez-Flakus Mikhail P.Zhurbenko Nimali Ide Silva Danushka S.Tennakoon KPDeepna Latha Patinjareveettil Manimohan KNAnil Raj Mark S.Calabon Abdollah Ahmadpour Zeinab Heidarian Zahra Alavi Fatemeh Alavi Youbert Ghosta Razmig Azizi Mei Luo Min-Ping Zhao Nuwan D.Kularathnage Li Hua Yun-Hui Yang Chun-Fang Liao Hai-Jun Zhao Anis S.Lestari Subashini C.Jayasiri Feng-Ming Yu Lei Lei Jian-Wei Liu Omid Karimi Song-Ming Tang Ya-Ru Sun Yong Wang Ming Zeng Zin H.Htet Benedetto T.Linaldeddu Artur Alves Alan J.L.Phillips Carlo Bregant Lucio Montecchio AndréDe Kesel Vincent P.Hustad Andrew N.Miller Anna G.Fedosova Viktor Kučera Mubashar Raza Muzammil Hussain Yan-Peng Chen Vinodhini Thiyagaraja Deecksha Gomdola Achala R.Rathnayaka Asha J.Dissanayake Nakarin Suwannarach Sinang Hongsanan Sajeewa S.N.Maharachchikumbura Lakmali S.Dissanayake Nalin N.Wijayawardene Rungtiwa Phookamsak Saisamorn Lumyong E.B.Gareth Jones Neelamanie Yapa Dhanushka N.Wanasinghe Ning Xie Mingkwan Doilom Ishara S.Manawasinghe Jian-Kui(Jack)Liu Qi Zhao Biao Xu Kevin D.Hyde Jiage Song Innovative Institute for Plant Health/Key Laboratory of Green Prevention and Control On Fruits and Vegetables in South China Ministry of Agriculture and Rural AffairsZhongkai University of Agriculture and EngineeringHaizhu DistrictGuangzhou 510225GuangdongChina Center of Excellence in Fungal Research Mae Fah Luang UniversityChiang Rai 57100Thailand Guangdong Provincial Key Laboratory for Plant Epigenetics College of Life Science and OceanographyShenzhen University3688Nanhai AvenueNanshanShenzhen 518055GuangdongChina Sect.Environmental Sciences Department MeSVAUniversity of L’AquilaVia Vetoio67100 CoppitoAQItaly Department of Environmental Biology SUNY-ESF241 Illick Hall1 Forestry DriveSyracuseNY 13210USA National Fungal Culture Collection of India MACS Agharkar Research InstitutePuneMaharashtra 411004India Department of Plant Pathology Punjab Agricultural UniversityLudhianaPunjab 141004India Center for Yunnan Plateau Biological Resources Protection and Utilization College of Biological Resource and Food EngineeringQujing Normal UniversityQujing 655011YunnanChina Department of Forest Ecology Kerala Forest Research InstitutePeechiThrissurKerala 680653India Department of Botany The American CollegeTallakkulamMaduraiTamil Nadu 625002India Department of Zoology Savitribai Phule Pune UniversityGaneshkhind RdGaneshkhindPuneMaharashtra 411007India University of Santiago de Compostela 15782 Santiago de CompostelaSpain Sociedad Micológica Extremeña C/Sagitario 1410001 CáceresSpain Institute of Microbiology of the Czech Academy of Sciences Vídeňská108314220 Prague 4Czech Republic Department of Botany Moravian MuseumZelnýtrh 665937 BrnoCzech Republic Department of Life Sciences(Botany Unit) University of Alcalá28805 Alcaláde HenaresMadridSpain Biological and Enviromental Sciences University of Gothemburgand Gothemburg Global Biodiversity CentreBox 46140530 GöteborgSweden Madrid Mycological Society Real Jardín BotánicoC/Claudio Moyano 128014 MadridSpain State Ke

This article is the 15th contribution in the Fungal Diversity Notes series,wherein 115 taxa from three phyla,nine classes,28 orders,48 families,and 64 genera are *** taxa described and illustrated in the present study include a new family,five new genera,61 new species,five new combinations,one synonym,one new variety and 31 records on new hosts or new geographical *** *** introduced and accommodated in *** new genera introduced in this study are Ageratinicola,Kevinia,Pseudomultiseptospora(Parabambusicolaceae),Marasmiellomycena,and Vizzinia(Porotheleaceae).Newly described species are Abrothallus altoandinus,Ageratinicola kunmingensis,Allocryptovalsa aceris,Allophoma yuccae,Apiospora cannae,***,***,Boeremia wisteriae,Calycina papaeana,Clypeo-coccum lichenostigmoides,Coniochaeta riskali-shoyakubovii,Cryphonectria kunmingensis,Diaporthe angustiapiculata,***,***,Diatrypella guangdongense,Dothiorella franceschinii,Endocalyx phoenicis,Epicoc-cum terminosporum,Fulvifomes karaiensis,***,Ganoderma ghatensis,Hysterobrevium baoshanense,Inocybe avellaneorosea,***,Jahnula oblonga,Kevinia lignicola,Kirschsteiniothelia guangdongensis,Laboulbenia caprina,***,***,***,***,***,***,***,***,Laccaria rubriporus,Lasiodiplodia morindae,Lyophyllum agnijum,Marasmiellomycena pseudoomphaliiformis,Melomastia beihaiensis,Nemania guangdongensis,Nigrograna thailandica,Nigrospora ficuum,Oxydothis chinensis,***,Petriella thailandica,Phaeoacremonium chinensis,Phialocephala chinensis,Phytophthora debattistii,Polyplosphaeria nigrospora,Pronectria loweniae,Seriascoma acutispora,Setoseptoria bambusae,Stictis anomianthi,Tarzetta tibetensis,Tarzetta urceolata,Tetraploa obpyriformis,Trichoglossum beninense,and Tricoderma *** provide an emendation for Urnula ailaoshanensis Agaricus duplocingulatoides *** i

关键词： Agaricomycetes Ascomycota Basidiomycota Dothideomycetes Eurotiomycetes Fungal diversity Geoglossomycetes Geographical distribution Host records Incertae sedis Laboulbeniomycetes Lecanoromycetes Leotiomycetes Novel taxa New combination Oomycota Peronosporea Pezizomycetes Phylogeny Sordariomycetes South Chinese fungi Taxonomy

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Excitation to defect-bound band edge states in twodimensional semiconductors and its effect on carrier transport

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npj Computational Materials 2019年第1期5卷 1070-1075页

作者： Dan Wang Dong Han Damien West Nian-Ke Chen Sheng-Yi Xie Wei Quan Tian Vincent Meunier Shengbai Zhang Xian-Bin Li State Key Laboratory on Integrated Optoelectronics College of Electronic Science and EngineeringJilin University130012 ChangchunChina State Key Laboratory of Luminescence and Applications Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of Sciences130033 ChangchunChina Department of Physics Applied Physics&AstronomyRensselaer Polytechnic InstituteTroyNY 12180USA College of Chemistry and Chemical Engineering Chongqing UniversityHuxi Campus401331 ChongqingChina

The ionization of dopants is a crucial process for electronics,yet it can be unexpectedly difficult in two-dimensional materials due to reduced screening and *** first-principles calculations,here we propose a dopant ionization process for twodimensional semiconductors where charge carriers are only excited to a set of defect-bound band edge states,rather than to the true band edge states,as is the case in *** defect-bound states have small enough ionization energies but large enough spatial *** a modest defect density,carriers can transport through band by such states.

关键词： defect semiconductors states

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Corrigendum to “Epitaxial growth of wafer scale antioxidant single-crystal graphene on twinnedPt(111)” [Carbon 181 (2021) 225-233]

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Carbon 2021年 182卷 863-864页

作者： He Kang Pengtao Tang Haibo Shu Yanhui Zhang Yijian Liang Jing Li Zhiying Chen Yanping Sui Shike Hu Shuang Wang Sunwen Zhao Xuefu Zhang Chengxin Jiang Yulong Chen Zhongying Xue Miao Zhang Da Jiang Guanghui Yu Songang Peng Zhi Jin Xinyu Liu State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences Shanghai 200050 China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences Beijing 100049 China College of Optical and Electronic Technology China Jiliang University 310018 Hangzhou China Microwave Devices and Integrated Circuits Department Institute of Microelectronics Chinese Academy of Sciences Beijing 100029 China

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Nanomechanical Resonators: Toward Atomic Scale

arXiv

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arXiv 2022年

作者： Xu, Bo Zhang, Pengcheng Zhu, Jiankai Liu, Zuheng Eichler, Alexander Zheng, Xu-Qian Lee, Jaesung Dash, Aneesh More, Swapnil Wu, Song Wang, Yanan Jia, Hao Naik, Akshay Bachtold, Adrian Yang, Rui Feng, Philip X.-L. Wang, Zenghui Centre for Nano Science and Engineering Indian Institute of Science Karnataka Bangalore560012 India University of Michigan Shanghai Jiao Tong University Joint Institute Shanghai Jiao Tong University Shanghai200240 China School of Electronic Information and Electrical Engineering Shanghai Jiao Tong University Shanghai200240 China Department of Electrical and Computer Engineering Herbert Wertheim College of Engineering University of Florida GainesvilleFL32611 United States Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China Chengdu610054 China State Key Laboratory of Electronic Thin Films and Integrated Devices University of Electronic Science and Technology of China Chengdu610054 China Department of Physics ETH Zurich Zurich8093 Switzerland College of Integrated Circuit Science and Engineering Nanjing University of Posts and Telecommunications Nanjing210023 China Department of Electrical and Computer Engineering University of Texas at El Paso El PasoTX79968 United States Department of Electrical and Computer Engineering University of Nebraska-Lincoln LincolnNE68588 United States Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences Shanghai200050 China ICFO-Institut de Ciencies Fotoniques The Barcelona Institute of Science and Technology Barcelona08860 Spain

The quest for realizing and manipulating ever smaller man-made movable structures and dynamical machines has spurred tremendous endeavors, led to important discoveries, and inspired researchers to venture to previously unexplored grounds. Scientific feats and technological milestones of miniaturization of mechanical structures have been widely accomplished by advances in machining and sculpturing ever shrinking features out of bulk materials such as silicon. With the flourishing multidisciplinary field of low-dimensional nanomaterials, including one-dimensional (1D) nanowires/nanotubes and two-dimensional (2D) atomic layers such as graphene/phosphorene, growing interests and sustained effort have been devoted to creating mechanical devices toward the ultimate limit of miniaturization genuinely down to the molecular or even atomic scale. These ultrasmall movable structures, particularly nanomechanical resonators that exploit the vibratory motion in these 1D and 2D nano-to-atomic-scale structures, offer exceptional device-level attributes, such as ultralow mass, ultrawide frequency tuning range, broad dynamic range, and ultralow power consumption, thus holding strong promises for both fundamental studies and engineering applications. In this Review, we offer a comprehensive overview and summary of this vibrant field, present the state-of-the-art devices and evaluate their specifications and performance, outline important achievements, and postulate future directions for studying these miniscule yet intriguing molecular-scale machines. © 2022, CC BY-NC-ND.

关键词： Signal processing

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Construction of through-space charge transfer donor-acceptor coordination polymers through the combination of planar electron-deficient/rich ligands

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Chinese Chemical Letters 2025年

作者： Zhen-Wei Zhang Da-Shuai Zhang Wei Wang Xiao-Ting Liu Hui Hu Yong-Zheng Zhang Longlong Geng Bin Li Yuchen Deng Rongmin Wei Xiuling Zhang Yuexing Zhang Ze Chang Shandong Provincial Key Laboratory of Monocrystalline Silicon Semiconductor Materials and Technology Shandong Universities Engineering Research Center of Integrated Circuits Functional Materials and Expanded Applications College of Chemistry and Chemical Engineering Dezhou University Dezhou 253023 China. School of Chemistry and Chemical Engineering Shandong University of Technology Zibo 255000 China. College of Chemistry Zhengzhou University Zhengzhou 450001 China. School of Materials Science and Engineering Nankai University Tianjin 300350 China.

In this paper, a new series of donor-acceptor coordination polymers (DACPs), [Cd(dppz)(R-ndc)(H 2 O)] n (R = none, DZU-400; R = F, DZU-400-F; R = Br, DZU-400-Br; DZU is short for Dezhou University), [Cd(dppz)(adc)(H 2 O)] n (DZU-401), and {[Cd(dppz)(adb) 0.5 (HCOO)(H 2 O)]} n (DZU-402), have been successfully constructed through the combination of electron-deficient dipyrido[3,2-a:2′,3′-c]phenazine (dppz) as an acceptor and various dicarboxylic ligands (H 2 ndc = 2,3-naphthalenedicarboxylic acid, F-H 2 ndc = 6,7-difluoronaphthalene-2,3-dicarboxylic acid, Br-H 2 ndc = 6,7-dibromonaphthalene-2,3-dicarboxylic acid, H 2 adc = 9,10-anthracenedicarboxylic acid, and H 2 adb = 4,4′-(anthracene-9,10-diyl)dibenzoic acid) with electron-rich planar aromatic rings as donors. Structural analyses reveal closely parallel arrangement of the planar acceptor and donor units in these DACPs, which could facilitate the through-space charge transfer (TSCT) interactions of the D-A systems and the corresponding luminescent properties. Interestingly, the DACPs show highly regulable donor dependent photoluminescence from blue to orange. Based on the TSCT based luminescence and the high thermal stability of the DACPs, their thermal-stimuli responsive emission properties were further studied. Photoluminescence intensity of the DACPs all present good linearity with temperature (298-473 K), as proved by variable temperature fluorescence spectra. Importantly, the temperature sensing process is reversible and recyclable, suggesting the promising applications of the DACPs as thermal-stimuli responsive materials.

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Out-of-Plane Single-Copper-Site Catalysts for Room-Temperature Benzene Oxidation

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Angewandte Chemie 2024年第20期136卷

作者： Dr. Wei Che Dr. Pai Li Gao-Feng Han Dr. Hyuk-Jun Noh Dr. Jeong-Min Seo Jong-Pil Jeon Changqing Li Dr. Wei Liu Prof. Feng Li Prof. Qinghua Liu Prof. Jong-Beom Baek School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks Ulsan National Institute of Science and Technology (UNIST) Ulsan 44919 Republic of Korea State Key Laboratory of Integrated Circuit Materials Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences Shanghai 200050 P. R. China State Key Laboratory of Fine Chemicals Frontier Science Center for Smart Materials Department of Chemistry School of Chemical Engineering Dalian University of Technology Dalian 116024 P. R. China Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials Fudan University Shanghai 200433 P. R. China National Synchrotron Radiation Laboratory University of Science and Technology of China Hefei 230029 Anhui P. R. China

Crafting single-atom catalysts (SACs) that possess “just right” modulated electronic and geometric structures, granting accessible active sites for direct room-temperature benzene oxidation is a coveted objective. However, achieving this goal remains a formidable challenge. Here, we introduce an innovative in situ phosphorus-immitting strategy using a new phosphorus source (phosphorus nitride, P 3 N 5 ) to construct the phosphorus-rich copper (Cu) SACs, designated as Cu/NPC. These catalysts feature locally protruding metal sites on a nitrogen (N)-phosphorus (P)-carbon (C) support (NPC). Rigorous analyses, including X-ray absorption spectroscopy (XAS) and X-ray photoelectron spectroscopy (XPS), validate the coordinated bonding of nitrogen and phosphorus with atomically dispersed Cu sites on NPC. Crucially, systematic first-principles calculations, coupled with the climbing image nudged-elastic-band (CI-NEB) method, provide a comprehensive understanding of the structure-property-activity relationship of the distorted Cu−N 2 P 2 centers in Cu/NPC for selective oxidation of benzene to phenol production. Interestingly, Cu/NPC has shown more energetically favorable C−H bond activation compared to the benchmark Cu/NC SACs in the direct oxidation of benzene, resulting in outstanding benzene conversion (50.3 %) and phenol selectivity (99.3 %) at room temperature. Furthermore, Cu/NPC achieves a remarkable turnover frequency of 263 h −1 and mass-specific activity of 35.2 mmol g −1 h −1 , surpassing the state-of-the-art benzene-to-phenol conversion catalysts to date.

关键词： benzene hydroxylation electron localization geometric feature green chemistry single-atom catalysts

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