A stable and highly active core‐shell heterostructure electrocatalyst is essential for catalyzing oxygen evolution reaction(OER).Here,a dual‐trimetallic core‐shell heterostructure OER electrocatalyst that consists ...
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A stable and highly active core‐shell heterostructure electrocatalyst is essential for catalyzing oxygen evolution reaction(OER).Here,a dual‐trimetallic core‐shell heterostructure OER electrocatalyst that consists of a NiFeWS_(2) inner core and an amorphous NiFeW(OH)_(z)outer shell is designed and synthesized using in situ electrochemical *** electrochemical measurements of different as‐synthesized catalysts with a similar mass loading suggest that the core‐shell Ni_(0.66)Fe_(0.17)W_(0.17)S_(2)@amorphous NiFeW(OH)_(z) nanosheets exhibit the highest overall performance compared with that of other bimetallic reference catalysts for the ***,the nanosheet arrays were in situ grown on hydrophilic‐treated carbon paper to fabricate an integrated three‐dimensional electrode that affords a current density of 10 mA cm^(−2) at a small overpotential of 182 mV and a low Tafel slope of 35 mV decade^(−1) in basic *** Faradaic efficiency of core‐shell Ni_(0.66)Fe_(0.17)W_(0.17)S_(2)@amorphous NiFeW(OH)_(z) is as high as 99.5% for *** scanning electron microscope,transmission electron microscope,and X‐ray photoelectron spectroscopy analyses confirm that this electrode has excellent stability in morphology and elementary composition after long‐term electrochemical ***,density functional theory calculations further indicate that the core‐shell heterojunction increased the conductivity of the catalyst,optimized the adsorption energy of the OER intermediates,and improved the OER *** study provides a universal strategy for designing more active core‐shell structure electrocatalysts based on the rule of coordinated regulation between electronic transport and active sites.
1 *** visual speech representations from talking face videos is an important problem for several speech-related tasks,such as lip reading,talking face generation,and audiovisual speech separation[1,2].The key difficul...
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1 *** visual speech representations from talking face videos is an important problem for several speech-related tasks,such as lip reading,talking face generation,and audiovisual speech separation[1,2].The key difficulty lies in tackling speech-irrelevant factors presented in the videos,such as lighting,resolution,viewpoints,and head motion.
Although Convolutional Neural Networks(CNNs)have significantly improved the development of image Super-Resolution(SR)technology in recent years,the existing SR methods for SAR image with large scale factors have rarel...
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Although Convolutional Neural Networks(CNNs)have significantly improved the development of image Super-Resolution(SR)technology in recent years,the existing SR methods for SAR image with large scale factors have rarely been studied due to technical difficulty.A more efficient method is to obtain comprehensive information to guide the SAR image ***,the co-registered High-Resolution(HR)optical image has been successfully applied to enhance the quality of SAR image due to its discriminative *** by this,we propose a novel Optical-Guided Super-Resolution Network(OGSRN)for SAR image with large scale ***,our proposed OGSRN consists of two sub-nets:a SAR image SuperResolution U-Net(SRUN)and a SAR-to-Optical Residual Translation Network(SORTN).The whole process during training includes two *** stage-1,the SR SAR images are reconstructed by the *** an Enhanced Residual Attention Module(ERAM),which is comprised of the Channel Attention(CA)and Spatial Attention(SA)mechanisms,is constructed to boost the representation ability of the *** stage-2,the output of the stage-1 and its corresponding HR SAR images are translated to optical images by the SORTN,*** then the differences between SR images and HR images are computed in the optical space to obtain feedback information that can reduce the space of possible SR *** that,we can use the optimized SRUN to directly produce HR SAR image from Low-Resolution(LR)SAR image in the testing *** experimental results show that under the guidance of optical image,our OGSRN can achieve excellent performance in both quantitative assessment metrics and visual quality.
Visual relation detection aims to describe the relationships between objects in a scene by using the form of a triplet . Existing methods not only suffer from the huge number of combinations of triples, but also make ...
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In high-precision occasions, three-phase voltage PWM rectifier based on conventional voltage-current dual closed-loop control suffer from current harmonics and poor interference immunity. In order to effectively allev...
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This work focuses on the evolution behaviors of ring dark solitons(RDSs) and the following vortices after the collapses of RDSs in spin-1 Bose–Einstein condensates. We find that the weighted average of the initial de...
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This work focuses on the evolution behaviors of ring dark solitons(RDSs) and the following vortices after the collapses of RDSs in spin-1 Bose–Einstein condensates. We find that the weighted average of the initial depths of three components determines the number and motion trajectories of vortex dipoles. For the weighted average of the initial depths below the critical depth, two vortex dipoles form and start moving along the horizontal *** the weighted average depth above the critical depth, two or four vortex dipoles form, and all start moving along the vertical axis. For the RDS with weighted average depth at exactly the critical point, four vortex dipoles form, half of the vortex dipoles initiate movement vertically, and the other half initiate movement *** conclusion is applicable to the two-component system studied in earlier research, indicating its universality.
Open world object detection aims to simulate the human process of recognizing objects in real life scenarios. It can identify categories not introduced during the training phase as unknown during the testing phase and...
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IoT devices have been widely used with the advent of *** devices contain a large amount of private data during *** is primely important for ensuring their ***,we proposed a lightweight block cipher based on dynamic S-...
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IoT devices have been widely used with the advent of *** devices contain a large amount of private data during *** is primely important for ensuring their ***,we proposed a lightweight block cipher based on dynamic S-box named *** is introduced for devices with limited hardware resources and high throughput *** is a 128-bit block cipher supporting 64-bit key,which is based on a new generalized Feistel variant *** retains the consistency and significantly boosts the diffusion of the traditional Feistel *** SubColumns of round function is implemented by combining bit-slice technology with *** S-box is dynamically associated with the *** has been demonstrated that DBST has a good avalanche effect,low hardware area,and high *** S-box has been proven to have fewer differential features than RECTANGLE *** security analysis of DBST reveals that it can against impossible differential attack,differential attack,linear attack,and other types of attacks.
Controlling networks aims to study the models, structures,and related dynamics of complex networks. The primary problem of controlling networks is to determine whether they are controllable. Nowadays, controllability ...
Controlling networks aims to study the models, structures,and related dynamics of complex networks. The primary problem of controlling networks is to determine whether they are controllable. Nowadays, controllability has been widely studied and applied to system engineering and control theory, power systems, aerospace, and quantum systems. Various classical criteria include the Gram matrix criterion, Kalman rank criterion, and PBH test.
The accurate and automatic segmentation of retinal vessels fromfundus images is critical for the early diagnosis and prevention ofmany eye diseases,such as diabetic retinopathy(DR).Existing retinal vessel segmentation...
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The accurate and automatic segmentation of retinal vessels fromfundus images is critical for the early diagnosis and prevention ofmany eye diseases,such as diabetic retinopathy(DR).Existing retinal vessel segmentation approaches based on convolutional neural networks(CNNs)have achieved remarkable ***,we extend a retinal vessel segmentation model with low complexity and high performance based on U-Net,which is one of the most popular *** view of the excellent work of depth-wise separable convolution,we introduce it to replace the standard convolutional *** complexity of the proposed model is reduced by decreasing the number of parameters and calculations required for *** ensure performance while lowering redundant parameters,we integrate the pre-trained MobileNet V2 into the ***,a feature fusion residual module(FFRM)is designed to facilitate complementary strengths by enhancing the effective fusion between adjacent levels,which alleviates extraneous clutter introduced by direct ***,we provide detailed comparisons between the proposed SepFE and U-Net in three retinal image mainstream datasets(DRIVE,STARE,and CHASEDB1).The results show that the number of SepFE parameters is only 3%of U-Net,the Flops are only 8%of U-Net,and better segmentation performance is *** superiority of SepFE is further demonstrated through comparisons with other advanced methods.
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