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Assessment of internal exposure risk from metals pollution of occupational and non-occupational populations around a non-ferrous metal smelting plant

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Journal of Environmental Sciences 2025年第1期147卷 62-73页

作者： Yingjun Wu Mengdie Qi Hang Yu Guiying Li Taicheng An Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and Health Guangdong Key Laboratory of Environmental Catalysis and Health Risk ControlInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Key Laboratory for City Cluster Environmental Safety and Green DevelopmentSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Non-ferrous metal smelting poses significant risks to public ***,the copper smelting process releases arsenic,a semi-volatile metalloid,which poses an emerging exposure risk to both workers and nearby *** comprehensively understand the internal exposure risks of metal(loid)s from copper smelting,we explored eighteen metal(loid)s and arsenic metabolites in the urine of both occupational and non-occupational populations using inductively coupled plasma mass spectrometry with high-performance liquid chromatography and compared their health *** showed that zinc and copper(485.38 and 14.00μg/L),and arsenic,lead,cadmium,vanadium,tin and antimony(46.80,6.82,2.17,0.40,0.44 and 0.23μg/L,respectively)in workers(n=179)were significantly higher compared to controls(n=168),while Zinc,tin and antimony(412.10,0.51 and 0.15μg/L,respectively)of residents were significantly higher than ***,workers had a higher monomethyl arsenic percentage(MMA%),showing lower arsenic methylation *** appointment analysis identified arsenic,lead,cadmium,antimony,tin and thallium as co-exposure metal(loid)s from copper smelting,positively relating to the age of *** hazard index(HI)of workers exceeded 1.0,while residents and control were approximately at ***,all three populations had accumulated cancer risks exceeding 1.0×10^(-4),and arsenite(AsIII)was the main contributor to the variation of workers and ***,residents living closer to the smelting plant had higher health *** study reveals arsenic exposure metabolites and multiple metals as emerging contaminants for copper smelting exposure populations,providing valuable insights for pollution control in non-ferrous metal smelting.

关键词： Arsenic metabolites Metal(loid)s Non-ferrous metal smelting Human biomonitoring Exposure Urine

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Impact of coking plant to heavy metal characteristics in groundwater of surrounding areas:Spatial distribution,source apportionment and risk assessments

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Journal of Environmental Sciences 2025年第3期149卷 688-698页

作者： Congqing Wang Wanjun Wang ChaoWang Shixing Ren Yingjun Wu Meicheng Wen Guiying Li Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory Environmental Catalysis and Pollution Control Key Laboratory of City Cluster Environmental Safety and Green developmentSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Coking industry is a potential source of heavy metals(HMs)***,its impacts to the groundwater of surrounding residential areas have not been well *** study investigated the pollution characteristics and health risks of HMs in groundwater nearby a typical coking *** HMs including Fe,Zn,Mo,As,Cu,Ni,Cr,Pb and Cd were *** average concentration of total HMswas higher in the nearby area(244.27μg/L)than that of remote area away the coking plant(89.15μg/L).The spatial distribution of pollution indices including heavy metal pollution index(HPI),Nemerow index(NI)and contamination degree(CD),all demonstrated higher values at the nearby residential areas,suggesting coking activity could significantly impact the HMs distribution *** sources of HMs were identified by Positive Matrix Factorization(PMF)model,which indicated coal washing and coking emission were the dominant sources,accounted for 40.4%,and 31.0%,*** ingestionwas found to be the dominant exposure pathway with higher exposure dose to children than *** quotient(HQ)values were below 1.0,suggesting negligible non-carcinogenic health risks,while potential carcinogenic risks were from Pb and Ni with cancer risk(CR)values>10−*** Carlo simulation matched well with the calculated results with HMs concentrations to be the most sensitive *** study provides insights into understanding how the industrial coking activities can impact the HMs pollution characteristics in groundwater,thus facilitating the implement of HMs regulation in coking industries.

关键词： Coking industry Heavy metal Groundwater Spatial distribution Source apportionment Monte Carlo simulation

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Achieving ultrahigh strength and ductility via high-density nanoprecipitates triggering multiple deformation mechanisms in a dual-aging high-entropy alloy with precold deformation

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材料科学技术（英文版） 2025年第2期205卷 27-41页

作者： Liyuan Liu Yang Zhang Zhongwu Zhang Key Laboratory of Superlight Materials and Surface Technology Ministry of EducationCollege of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001China Key Laboratory of Superlight Materials and Surface Technology Ministry of EducationCollege of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001China State Key Laboratory of Metal Materials for Marine Equipment and Application Anshan 114009China

How to achieve high-entropy alloys(HEAs)with ultrahigh strength and ductility is a challenging *** strengthening is one of the methods to significantly enhance strength,but unfortunately,ductility will be *** overcome the strength-ductility trade-off,the strategy of this study is to induce the formation of high-density nanoprecipitates through dual aging(DA),triggering multiple deformation mechanisms,to obtain HEAs with ultrahigh strength and ***,the effect of precold deforma-tion on precipitation behavior was studied using Ni35(CoFe)55V5Nb5(at.％)HEAas the *** results reveal that the activation energy of recrystallization is 112.2 kJ/*** the precold-deformation amount increases from 15％to 65％,the activation energy of precipitation gradually decreases from 178.8 to 159.7 kJ/*** precipitation time shortens,the size of the nanoprecipitate decreases,and the den-sity ***,the thermal treatment parameters were optimized,and the DA process was customized based on the effect of precold deformation on precipitation ***-density L12 nano-precipitates(～3.21 × 1025 m-3)were induced in the 65％precold-deformed HEA,which led to the si-multaneous formation of twins and stacking fault(SF)networks during *** yield strength(YS),ultimate tensile strength,and ductility of the DA-HEA are～2.0 GPa,～2.2 GPa,and～12.3％,*** with the solid solution HEA,the YS of the DA-HEA increased by 1,657 MPa,possessing an astonishing increase of～440％.The high YS stems from the precipitation strengthening contributed by the L12 nanoprecipitates and the dislocation strengthening contributed by precold *** synergistically enhanced ductility stems from the high strain-hardening ability under the dual support of twinning-induced plasticity and SF-induced plasticity.

关键词： High-entropy alloy Precold deformation Precipitation behavior Ultrahigh strength Deformation mechanism

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Experimental Study on Diesel Spray and Flame Asymmetry Characteristics of Dual-Orifice Nozzles for a Medium-Speed Engine

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Journal of Thermal Science 2025年第1期34卷 303-322页

作者： JU Dehao LIURui ZHENG Liang DENG Jiahui ZHANG Wenzheng HUO Jinlu HUANG Li Shanghai Marine Diesel Engine Research Institute Shanghai 201108China National Key Laboratory of Marine Engine Science and Technology Shanghai 201108China Key Laboratory for Power Machinery and Engineering Ministry of EducationShanghai Jiao Tong UniversityShanghai 200240China

The asymmetry of the multi-orifice spray will cause uneven heat load of the marine diesel engine,thereby affecting its working performance and service ***,an in-depth understanding of the spray and flame characteristics of multi-orifice nozzles will guide the optimization of the nozzle structure,needle design and diesel atomization and combustion *** this reason,four groups of dual-orifice nozzles with different hole diameters(0.1-0.55 mm)and mass flow rates covering the typical marine medium-speed diesel injections are designed and customized,and the constant volume chamber(CVC)with high temperature and pressure is used to simulate the actual in-cylinder working conditions of the diesel engine for the spray visualization *** study the asymmetry of the fuel sprays discharged from a diesel injector,the multi-orifice nozzle is simplified as a dual-orifice nozzle in this *** with X-ray Computed Tomography(CT)imaging technology,the influences of the nozzle internal structure on the spray and flame asymmetry are studied in the constructed supercritical *** is found that the asymmetry of the inlet angle and the equivalent length-diameter ratio is positively correlated with the inconsistency of the dual *** an increase in the injection pressure and nozzle diameter,the asymmetry of the dual spray becomes more pronounced,resulting in greater disparities in the ignition delay times and ignition positions of the two ***,the increase in nozzle diameter also leads to combustion instability,resulting in a flame with a serrated *** the increase of ambient temperature,the proportion of liquid phase in the jet decreases and the relative density of spray front decreases.

关键词： dual-orifice nozzle nozzle structure atomization spray flame asymmetry

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A Multi-AUV Collaborative Mapping System With Bathymetric Cooperative Active SLAM Algorithm

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IEEE Internet of Things Journal 2025年第9期12卷 12441-12452页

作者： Qi, Chi Ma, Teng Li, Ye Ling, Yu Liao, Yulei Jiang, Yanqing Harbin Engineering University National Key Laboratory of Autonomous Marine Vehicle Technology Heilongjiang Harbin150001 China

Autonomous underwater vehicles (AUVs) play a pivotal role in the underwater Internet of Things (IoT). However, their capacity to fulfil large-scale bathymetric mapping is often constrained by limitations in navigational capabilities. This article proposes a homogeneous distributed collaborative mapping system, consisting of bathymetric mapping vehicles and its isomorphic server vehicle. The system achieves accurate positioning through bathymetric cooperative active simultaneous localization and mapping (BCA-SLAM) technology. This article mainly focuses on the server’s online path planning in BCA-SLAM using D-optimality metrics of the Fisher information matrix (FIM), to maximize the positioning accuracy of the collaborative system. A method for predicting the intervehicle loop-closure factor FIM was proposed for selecting the subsequent target point for the server, while a lemma for multiple augmented matrix determinants was devised to mitigate its computational burden. Experimental results have proved both the accuracy and efficiency of the proposed algorithm have been tested in semi-physical simulation. © 2014 IEEE.

关键词： Fisher information matrix

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Novel dual-enhanced stimulation for safe and efficient marine hydrate production

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Petroleum Science 2025年第2期22卷 805-820页

作者： Yun Qi You-Hong Sun Bing Li Heng-Feng Shan Yi-Zhuo Liu Guo-Biao Zhang School of Engineering and Technology China University of Geosciences Key Laboratory of Polar Geology and Marine Mineral Resources (China University of Geosciences Beijing) Ministry of Education

The commercial exploitation of natural gas hydrates is currently facing several challenges,including low production rates,limited recovery areas,and brief periods of continuous *** address these issues,we propose a novel dual-enhanced stimulation(DES) method for marine hydrate *** method involves injecting a special slurry that solidifies into porous,high-permeability,and highstrength slurry *** veins not only enhance permeability,allowing for faster gas and water flow,but also improve reservoir *** study experimentally investigated the split grouting of clayey-silty sediments with dual-enhanced slurry to assess the feasibility of DES and to explo re the slurry diffusion mechanism and micro-pore structure of the *** results showed that split grouting with dual-enhanced slurry exhibited frequent fracture initiation with quick pressure spikes and sharp declines,suggesting shorter fractures in clayey-silty *** vertical stress increased,the primary diffusion direction of the dual-enhanced slurry shifted from horizontal to vertical,aligning with fracture propagation patterns observed during *** hydraulic fracturing in hard rocks,split grouting in clayey-silty sediments encountered more difficult *** veins formed through a recurring cycle of splitting into fractures and filling with slurry,occurring more frequently in weaker sediments with slower injection rates and higher vertical *** vertical stress hindered slurry vein diffu sion,easily resulting in compaction grouting near the grouting ***,three-dimensional laser scanning of the veins showed that those formed through split grouting were continuous and stable,with their thickness decreasing as diffusion distance *** morphology of these veins was shaped by factors such as grouting rate,formation stress,and elastic modulus,with higher rates and elastic moduli facilitating the formation of complex vein n

关键词： Natural gas hydrate Dual-enhanced stimulation Splitting grouting Hydrate production Pore structure

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Thermo-responsive microneedles patch for transdermal drug delivery via squeezing in diabetic foot ulcers

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材料科学技术（英文版） 2025年第2期205卷 299-314页

作者： Xiaotong Wu Dan Xia Tingting Shi Baoe Li Donghui Wang Chunyong Liang Mingdong Dong Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology School of Materials Science and EngineeringHebei University of TechnologyTianjin 300130China Hebei Key Laboratory of Biomaterials and Smart Theranostics School of Health Sciences and Biomedical EngineeringHebei University of TechnologyTianjin 300130China Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology School of Materials Science and EngineeringHebei University of TechnologyTianjin 300130China Hebei Key Laboratory of Biomaterials and Smart Theranostics School of Health Sciences and Biomedical EngineeringHebei University of TechnologyTianjin 300130China Interdisciplinary Nanoscience Center Aarhus UniversityAarhus CDK-8000Denmark

Microneedle(MN)patches could be a promising treatment for diabetic foot ulcers that plague thousands of people *** reducing skin resistance or increasing driving force can accelerate the effi-ciency of transdermal drug delivery with conventional MN patches,it can create toxic chemical residues or require the help of additional ***,a thermo-responsive microneedles patch(TMN)with high biocompatibility without additional equipment is *** TMN consisted of a bilayer mi-croneedles composed of sodium alginate(SA)-g-poly(N-isopropylacrylamide)layer(SA-g-PNIPAM)loaded with sucrose octasulfate sodium salt(SOS)and hyaluronic acid layer and a polycaprolactone/chitosan nanofiber membrane loading with tetracycline hydrochloride(TH)and *** accelerates drug re-lease by extruding the drug through a volumetric phase transition in response to temperature changes,and TH and SOS promote wound healing by inhibiting bacterial growth and promoting vascular regener-ation and epithelial *** results showed that the drug release of TMN was significantly faster,with the drug release rate of more than 80％in the 10th h,and the antibacterial rate of TMN could reach 800％.In addition,TMN had good biocompatibility and good healing effects in vivo,which may be helpful for the design of multifunctional dressings in the future.

关键词： Microneedles patch Thermal response Transdermal drug delivery Diabetic foot ulcers

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High concentration of Ti^(3+)in C-TiO_(x)nanosheets boosting efficient photodegradation

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Science China(Technological Sciences) 2025年第3期68卷 156-166页

作者： Chongbei WU Xuan LI Haibin WANG Jiaxin TANG Shuai WEI Yuanyuan WU Aobing WANG Jizhou JIANG Hebei Key Laboratory of Man-machine Environmental Thermal Control Technology and Equipment Hebei Vocational University of Technology and EngineeringXingtai054000China School of Materials Science and Engineering Key Laboratory of Green Chemical Engineering Process of Ministry of EducationEngineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationWuhan Institute of TechnologyWuhan430205China

Semiconductor photocatalysis holds significant promise for addressing dye-pollution in ***,the efficiency of photocatalytic water purification is constrained by the weak light absorption capacity and low active site distribution of *** a bottom-up approach,carbon-doped TiO_(x)(C-TiO_(x))nanosheets with high concentrations of Ti^(3+)active sites were fabricated by etching the Al element in Ti_(3)Ai C_(2)with H_(2)O_(2).Experimental evidence demonstrates that the optimal C-TiO_(x)nanosheets exhibit high activity for the photocatalytic degradation of methylene blue,achieving a degradation rate of 100%within 50 *** introduction of carbon into the C-TiO_(x)nanosheets induces a red shift in the absorption edge,boosting the migration of photo-generated charge ***,there is a significant correlation between the concentration of Ti^(3+)active sites and the density of oxygen vacancies in the C-TiO_(x)nanosheets,which synergistically influence the photocatalytic degradation performance of MB dye wastewater.

关键词： bottom-up strategies C-TiO_(x)nanosheets high-concentrations Ti^(3+) photocatalytic degradation

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Broad-Learning-System-Based Model-Free Adaptive Predictive control for Nonlinear MASs Under DoS Attacks

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IEEE/CAA Journal of Automatica Sinica 2025年第2期12卷 381-393页

作者： Hongxing Xiong Guangdeng Chen Hongru Ren Hongyi Li the School of Automation Guangdong-Hong Kong Joint Laboratory for Intelligent Decision and Cooperative Control Guangdong University of Technology Guangdong Provincial Key Laboratory for Intelligent Decision and Cooperative Control Guangdong University of Technology the College of Electronic and Information Engineering Southwest University IEEE

In this paper, the containment control problem in nonlinear multi-agent systems(NMASs) under denial-of-service(DoS) attacks is addressed. Firstly, a prediction model is obtained using the broad learning technique to train historical data generated by the system offline without DoS attacks. Secondly, the dynamic linearization method is used to obtain the equivalent linearization model of NMASs. Then, a novel model-free adaptive predictive control(MFAPC) framework based on historical and online data generated by the system is proposed, which combines the trained prediction model with the model-free adaptive control method. The development of the MFAPC method motivates a much simpler robust predictive control solution that is convenient to use in the case of DoS attacks. Meanwhile, the MFAPC algorithm provides a unified predictive framework for solving consensus tracking and containment control problems. The boundedness of the containment error can be proven by using the contraction mapping principle and the mathematical induction method. Finally, the proposed MFAPC is assessed through comparative experiments.

关键词： Broad learning technique denial-of-service (DoS) model-free adaptive predictive control (MFAPC) nonlinear multi-agent systems (NMASs)

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Physically informed hierarchical learning based soft sensing for aero-engine health management unit

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Chinese Journal of Aeronautics 2025年第3期38卷 374-385页

作者： Aina WANG Pan QIN Yunbo YUAN Guang ZHAO Ximing SUN School of Control Science and Engineering Dalian University of TechnologyDalian 116024China Key Laboratory of Intelligent Control and Optimization for Industrial Equipment of Ministry of Education Dalian 116024China School of Energy and Power Engineering Dalian University of TechnologyDalian 116024China

Partial Differential Equations(PDEs)are model candidates of soft sensing for aero-engine health management *** existing Physics-Informed Neural Networks(PINNs)have made ***,unmeasurable aero-engine driving sources lead to unknown PDE driving terms,which weaken PINNs *** this end,Physically Informed Hierarchical Learning followed by Recurrent-Prediction Term(PIHL-RPT)is ***,PIHL is proposed for learning nonhomogeneous PDE solutions,in which two networks NetU and NetG are *** is for learning solutions satisfying PDEs;NetG is for learning driving terms to regularize NetU ***,we propose a hierarchical learning strategy to optimize and couple NetU and NetG,which are integrated into a data-physics-hybrid loss ***,we prove PIHL-RPT can iteratively generate a series of networks converging to a function,which can approximate a solution to well-posed ***,RPT is proposed for prediction improvement of PIHL,in which network NetU-RP is constructed to compensate for information loss caused by data sampling and driving sources’***,artificial datasets and practical vibration process datasets from our wear experiment platform are used to verify the feasibility and effectiveness of PIHL-RPT based soft ***,comparisons with relevant methods,discussions,and PIHL-RPT based health monitoring example are given.

关键词： Hierarchical learning strategy Monitoring:Partial differen tial equations with unmeasurable driving terms Physically informed hierarchical learning followed by recurrent-prediction term Soft sensing

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