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Immobilization of antimony in soil and groundwater using ferro-magnesium bimetallic organic frameworks

Journal of Environmental Sciences 2023年第3期125卷 194-204页

作者： Le Yuan JianleWang Zuqi Zhong Jiguang Li Hong Deng School of Environment and Energy Guangdong Provincial Key Laboratory of Solid Wastes Pollution Control and Resource RecyclingSouth China University of TechnologyGuangzhou 510006China Guangxi Key Laboratory of Beibu Gulf Marine Biodiversity Conservation Beibu Gulf UniversityQinzhou 535000China Guangdong Engineering and Technology Research Center for Environmental Nanomaterials South China University of TechnologyGuangzhou 510006China

Sb(Ⅲ) is often detected in contaminated soil and groundwater. Hence, high-efficiency technology is needed. In this study, bimetallic organic frameworks were used for the first time to immobilize Sb(Ⅲ) from contaminated soil and groundwater. The materials were synthesized by the hydrothermal method. Both ends of the prepared material were hexagonal tip rods,and the length became shorter as the ratio of Fe/Mg decreased. The bimetallic organic framework with a Fe/Mg feeding ratio of 0.5 was the optimum material for Sb(Ⅲ) removal, which could effectively immobilize Sb(Ⅲ). The adsorption isotherm was fitted well with the Freundlich model, and the optimal adsorption capacity can reach 106.97 mg/g. The adsorption capacity of 84% can be completed in 10 min, which conformed to the pseudo-second-order kinetics. The Fe^(3+)could enhance the stability of the material, and the Mg^(2+)was conducive to freeing up adsorption sites for binding Sb(Ⅲ) and forming stable chemical adsorption. Ion exchange is the predominant mechanism to remove Sb(Ⅲ). After 14 days of remediation of Sb(Ⅲ) contaminated soil, the Toxicity Characteristic Leaching Procedure(TCLP)-leached concentrations of Sb(Ⅲ) were reduced by 86%, 91% and 94% when the material dosages were1%, 2% and 3%, respectively. Immobilization of Sb(Ⅲ) in soil resulted in a conversion of antimony speciation from more easily bioavailable species to less bioavailable species, further contributing to reduce the environmental risk of antimony. The results indicate that ferromagnesium bimetallic organic frameworks may serve as a kind of promising materials for the immobilization of Sb(Ⅲ) in contaminated soil and groundwater.

关键词： Antimony Ferro-magnesium bimetallic organic frameworks(MOFs) Soil Groundwater

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Development of a Compact Optical Layout for a Miniature Fluorescence Spectrometer: In-Situ Detection of Organic Pollutants in Aquatic Environment

Development of a Compact Optical Layout for a Miniature Fluo...

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2024 China Automation Congress, CAC 2024

作者： Fan, Xingyu Yu, Jie Zhang, Qiuhao Cao, Shuai Zhang, Lingke Xue, Fangjia State Key Laboratory of Industrial Control Technology College of Control Science and Engineering Zhejiang University Hangzhou China

ISBN: (纸本)9798350368604

In recent years, the increasing presence of emerging organic pollutants in rivers, lakes, and other aquatic environments has posed significant threats to human health and ecological safety. Current monitoring technologies for these pollutants face several challenges, including the high cost of equipment and the scarcity of trained professionals. Furthermore, existing portable fluorescence sensors are limited by inadequate data, unsuitability for in-situ water environments, and the ability to detect only specific pollutants. This paper proposes a novel design for an in-situ miniature fluorescence spectrometer, utilizing a compact optical layout to monitor organic pollutants in water. The design features a high-power UV LED combined with a lens group to enhance the fluorescence excitation effect of low-concentration organic pollutants. The system components are integrated into a compact layout centered around a flow cell, significantly reducing the device's size. In experimental validation, vitamin B was used as a model organic pollutant to test the prototype's detection capabilities. Within the concentration range of 1 - 100 μg/L, the fluorescence intensity exhibited a strong linear correlation with the vitamin B concentration, achieving an R2 value of 0.9945, comparable to that of commercial spectrometers. This portable device demonstrates excellent performance in detecting organic matter and offers significant advantages for in-situ monitoring applications, making it well-suited for real-time pollutant detection in rivers, lakes, and other aquatic environments. © 2024 IEEE.

关键词： Lake pollution

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Relabeling Abnormal Videos via Intra-Video Label Propagation for Weakly Supervised Video Anomaly Detection 14

Relabeling Abnormal Videos via Intra-Video Label Propagation...

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14th Asian control Conference, ASCC 2024

作者： Zhou, Wenhao Li, Yingxuan Zhao, Jiancheng Zhao, Chunhui College of Control Science and Engineering Zhejiang University State Key Laboratory of Industrial Control Technology Hangzhou China

ISBN: (纸本)9789887581598

Weakly supervised video anomaly detection is chal-lenging due to the lack of frame-level labels in abnormal videos. Previous work generally formulates it as a multiple instance learning (MIL) problem, in which abundant snippets especially including hard snippets in abnormal videos are underutilized, causing the training process to be dominated by redundant easy snippets. In this work, we introduce a semi-supervised learning perspective and aim to provide reliable snippet-level labels for abnormal videos to fully leverage them. Specifically, we propose a relabeling strategy by utilizing the Label Propagation Network (LPN) to propagate labels from confident snippets to hard snippets. Considering label propagation tends to be fragile and inaccurate in this case due to incorrect pseudo labels, we develop a feature relation module to enhance the intra-class compactness and inter-class dispersion, as well as a label separation module to enlarge the discrepancy of propagated labels. The overall model is designed to be concise and universal, which can be applied to existing weakly supervised methods to improve performance. Extensive experiments demonstrate that our method achieves state-of-the-art results on three benchmark datasets. © 2024 Asian control Association.

关键词： Self-supervised learning

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Prussian Blue/Cellulose Acetate Thin Film Composite Nanofiltration Membrane for Molecular Sieving and Catalytic Fouling Resistance

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Chinese Journal of Polymer Science 2023年第4期41卷 593-604,I0009页

作者： Hai-Bo Lin Jian-Guo Zhao Na Lu Qiu Han Jian-Qiang Wang Jian-Min Guan Xiao Wang Fu Liu Key Laboratory of Marine Materials and Related Technologies Zhejiang Key Laboratory of Marine Materials and Protective TechnologiesNingbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo315201China Qinghai University Qinghai810016China University of Chinese Academy of Sciences Beijing100049China

Nanofiltration(NF)membranes as high selective separators are appealing for molecular sieving,which still remains a great challenge for the mixed dyes with same *** this study,cellulose acetate(CA)membranes were firstly aminated by ethylene imine polymer(PEI),and then the thin film of metal organic frameworks(MOFs)were constructed onto aminated CA membrane through forward-diffusion,slow crystallization and in situ growth of Fe Co-Prussian blue(FeCo-PB)crystallization *** designed PB@CA composite NF membrane shows an ideal rejection for Congo red(CR)/methyl orange(MO)mixture solution,with 99.7%±0.2%for CR and 33.5%±2%for *** addition,the composite NF membrane demonstrated good efficiency for photocatalytic degradation of organic fouling(permeability recovery ratio was up to 92%)due to the active FeCo-PB ***,this work provides a practical strategy to prepare MOFs mediated thin film composite nanofiltration membrane for precise molecular sieving and catalytic antifouling performances.

关键词： Nanofiltration membrane Molecular sieving Catalytic fouling resistance Prussian blue

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Achieving anti-corrosion and anti-biofouling dual-function self-healing coating by natural carrier attapulgite loading with 2-Undecylimidazoline

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Journal of Materials Science & technology 2023年第17期148卷 222-234页

作者： Yinghao Wu Jinming Wei Xiaolu Shi Wenjie Zhao Key Laboratory of Marine Materials and Related Technologies Zhejiang Key Laboratory of Marine Materials and Protective TechnologiesNingbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China Ningbo New Material Testing and Evaluation Center Co. LtdNingbo 315048China

In the marine environment,the protective coatings face serious corrosion and biofouling problem,lim-itations,and challenges that made self-healing coatings unable to perform both anti-corrosion and anti-biofouling dual-function at the same *** we constructed the corrosion resistance and anti-biofouling self-healing coating by integrating nano-containers into the coating matrix,the 2-Undecylimidazoline(ULM)acted as a corrosion inhibitor and anti-biofouling dual-functional agent which was loaded on the natural container attapulgite(ATP).To obtain high healing efficiency,a fluidity-driven self-healing silicone oil coating was thickened by fibrous ATP to enhance its stability,which played a key role in the self-healing and long-term corrosion *** self-healing time of ULM@ATP rein-forced oil coating was 4 s at least in the air and up to 30 s in the 1 M HCl ***,the ULM@ATP can significantly enhance the corrosion resistance of the self-healing coating,with the best effect achieved when the content of ULM@ATP was 5 wt.%.The impedance modulus of ULM@ATP-2 still reached 1.62×10^(8)Ωcm^(2) after 480 immersion in 3.5 wt.%NaCl solution,which is 3 orders of magnitude high than pure Oil coating(2.17×10^(5)Ωcm^(2)).The restructure of the ATP network and the release of ULM could largely inhibit the corrosion of *** continuous open circuit potential of the compos-ite coating performed the potentially infinite self-healing *** self-healing performances of the composite coating in strong acid and base solutions exhibited high environmental *** anti-corrosion and anti-biofouling(the surface coverage of adhered chlorella decreased 96.88%)dual-function strategy of self-healing coatings could be also realized by many other porous nano-materials or function *** self-healing performances of the composite coating in strong acid and base solutions exhibited high environmental *** anti-corrosion and anti-biof

关键词： Self-healing Active corrosion resistance Anti-biofouling Attapulgite

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Surrogate-assisted optimization for anti-ship missile body configuration considering high-velocity water touching

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Chinese Journal of Aeronautics 2023年第12期36卷 268-281页

作者： Nianhui YE Teng LONG Junhui MENG Renhe SHI Baoshou ZHANG School of Aerospace Engineering Beijing Institute of TechnologyBeijing 100081China Key Laboratory of Dynamics and Control of Flight Vehicle Ministry of EducationBeijing 100081China

As a crucial weapon in the sea battle,anti-ship missiles generally employ a sea-skimming penetration strategy to reduce the probability of being detected by the target radar,which greatly increases the risk of touching water caused by sensor errors or random sea *** alleviate the large impact load by high-velocity water touching,a novel anti-ship missile body configuration is proposed in this paper,which is inspired by the idea of hydroplaning.A parametric geometry model is first developed to modify the configuration of the anti-ship missile ***,a structured arbitrary Lagrange-Eulerian based Fluid-Structure Interaction(FSI)model is established to analyze the kinematics parameters of the missile body during the hydroplaning process.A missile body configuration optimization problem is then formulated to minimize the impact load considering several constraints,e.g.,horizontal velocity loss,pitch angle after touching water,and inside capacity for *** to the time-consuming FSI simulation,a Kriging-assisted constrained differential evolution method is utilized to optimize the missile body configuration for reducing the impact *** the optimization process,radial basis function and Kriging are combined with evolutionary operators to lead the search to the vicinity of the optimum *** result shows that the proposed missile body configuration can reduce the impact load by 18.8%compared with the ordinary ***,the optimized configuration can further yield a 17.4%impact load decrease subject to all the constraints and avoid structural damage by the high-velocity water touching,which demonstrates the effectiveness and practicability of the proposed anti-ship missile body configuration and corresponding optimization framework for reducing the impact load.

关键词： Surrogate-assisted optimiza-tion Fluid-structureinteraction Arbitrary Lagrange-Eulerian Missile Conceptual design

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Identification of Mixed Organic Pollutants in River Water Based on Graph Convolutional Networks

Identification of Mixed Organic Pollutants in River Water Ba...

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2024 China Automation Congress, CAC 2024

作者： Cao, Shuai Yu, Jie Fan, Xingyu Zhang, Qiuhao Xue, Fangjia Hou, Dibo State Key Laboratory of Industrial Control Technology College of Control Science and Engineering Zhejiang University Hangzhou China

ISBN: (纸本)9798350368604

In the application of three-dimensional (3-D) fluorescence spectroscopy for river water pollutant detection, traditional feature extraction models often neglect wavelength information and complex intermolecular interrelationships. Moreover, experiments are frequently limited to single-substance classifications. This research addresses these limitations by proposing a novel model for organic pollutant recognition based on graph neural networks (GNNs). The proposed method begins by using the excitation-emission matrix and the wavelength information corresponding to each fluorescence intensity value as inputs. A convolutional neural network (CNN) is initially employed to extract preliminary features from the three-dimensional fluorescence spectra. Subsequently, the initial spectral features obtained during the pre-training stage are used to construct a graph neural network model. This model represents each category of organic pollutants as nodes within the graph, capturing the intrinsic connections between different pollution samples through node interactions. Finally, the model outputs a score vector for each category to classify the pollutants. To validate the proposed model, datasets comprising twelve common organic pollutants, both as single substances and mixtures, were collected. Comparative analysis with other methods demonstrates that the proposed approach achieves a high accuracy rate. ©2024 IEEE.

关键词： Graph neural networks

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Tracked robot with underactuated tension-driven RRP transformable mechanism:ideas and design

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Frontiers of Mechanical engineering 2024年第1期19卷 85-104页

作者： Ran XU Chao LIU School of Mechanical Electronic and Control EngineeringBeijing Jiaotong UniversityBeijing 100044China Key Laboratory of Vehicle Advanced Manufacturing Measuring and Control Technology(Ministry of Education)Beijing Jiaotong UniversityBeijing 100044China

Robots with transformable tracked mechanisms are widely used in complex terrains because of their high adaptability,and many studies on novel locomotion mechanisms have been conducted to make them able to climb higher *** underactuated transformable mechanisms for tracked robots could decrease the number of actuators used while maintaining the flexibility and obstacle-crossing capability of these robots,and increasing their cost ***,the underactuated tracked robots have appreciable research *** this paper,a novel tracked robot with a newly proposed underactuated revolute‒revolute‒prismatic(RRP)transformable mechanism,which is inspired by the sit-up actions of humans,was *** newly proposed tracked robot has only two actuators installed on the track pulleys for moving and does not need extra actuators for ***,it could concentrate the track belt’s tension toward one side,and the unbalanced tension would drive the linkage mechanisms to change its *** this method,the proposed underactuated design could change its external shape to create support points with the terrain and move its center of mass actively at the same time while climbing obstacles or crossing other kinds of terrains,thus greatly improving the climbing capability of the *** geometry and kinematic relationships of the robot and the crossing strategies for three kinds of typical obstacles are *** the basis of such crossing motions,the parameters of links in the robot are designed to make sure the robot has sufficient stability while climbing ***-crossing dynamic simulations were run and analyzed to prove the feasibility of the robot.A prototype was built and *** show that the proposed robot could climb platforms with heights up to 33.3%of the robot’s length or cross gaps with widths up to 43.5%of the robot’s length.

关键词： mechanical design tracked robot underactuated mechanisms RRP mechanism obstacle crossing strategy

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Simultaneous Degradation, Dehalogenation, and Detoxification of Halogenated Antibiotics by Carbon Dioxide Radical Anions

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engineering 2024年第6期37卷 78-86页

作者： Yanzhou Ding Xia Yu Shuguang Lyu Huajun Zhen Wentao Zhao Cheng Peng Jiaxi Wang Yiwen Zhu Chengfei Zhu Lei Zhou Qian Sui State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process School of Resources and Environmental EngineeringEast China University of Science and TechnologyShanghai 200237China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Academy of Environmental Sciences Shanghai 200233China

Despite the extensive application of advanced oxidation processes(AOPs)in water treatment,the efficiency of AOPs in eliminating various emerging contaminants such as halogenated antibiotics is constrained by a number of *** moieties exhibit strong resistance to oxidative radicals,affecting the dehalogenation and detoxification *** address these limitations of AOPs,advanced reduction processes(ARPs)have been ***,a novel nucleophilic reductant—namely,the carbon dioxide radical anion(CO_(2)^(·-))—is introduced for the simultaneous degradation,dehalogenation,and detoxification of florfenicol(FF),a typical halogenated *** results demonstrate that FF is completely eliminated by CO_(2)^(·-),with approximately 100%of Cland 46%of Freleased after 120 min of *** detoxification is observed,which exhibits a linear response to the release of free inorganic halogen ions(R^(2)=0.97,p<0.01).The formation of halogen-free products is the primary reason for the superior detoxification performance of this method,in comparison with conventional hydroxyl-radical-based *** identification and density functional theory(DFT)calculations reveal the underlying dehalogenation mechanism,in which the chlorine moiety of FF is more susceptible than other moieties to nucleophilic attack by CO_(2)^(·-).Moreover,CO_(2)^(·-)-based ARPs exhibit superior dehalogenation efficiencies(>75%)in degrading a series of halogenated antibiotics,including chloramphenicol(CAP),thiamphenicol(THA),diclofenac(DLF),triclosan(TCS),and ciprofloxacin(CIP).The system shows high tolerance to the pH of the solution and the presence of natural water constituents,and demonstrates an excellent degradation performance in actual groundwater,indicating the strong application potential of CO_(2)^(·-)-based ARPs in real ***,this study elucidates the feasibility of CO_(2)^(·-)for the simultaneous degradation,dehalogenation,and detoxification of halog

关键词： Carbon dioxide radical anions Advanced reduction processes Halogenated antibiotics Dehalogenation Detoxification

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Application of phononic crystals in modern engineering vibration and noise control, a review

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Noise and Vibration Worldwide 2025年第4-5期56卷 224-241页

作者： Huang, Wei Xu, Jian Yao, Yi Zhang, Yongliang Wang, Xin Han, Pengbo SINOMACH Academy of Science and Technology Co. Ltd SINOMACH Research Center of Engineering Vibration Control Technology Beijing100080 China Beijing China CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern Mechanics University of Science and Technology of China Anhui China Key Laboratory of Vibration Control for Key Process Equipment of Major Scientific Infrastructure in the Machinery Industry Beijing China

Phononic crystals are composite materials consisting of periodically distributed inclusions, and this structure enables wave band gaps under specific conditions. This characteristic allows for the suppression of elastic waves within certain frequency ranges, offering a new approach to vibration reduction and noise control. In this study, phononic crystals, with their periodic structure, tunable bandgap properties, topology optimization, and additive manufacturing technology, are reviewed. Some key hot issues, such as low-frequency vibration and noise control, intelligent materials, and tunable bandgap design, are discussed. In the future, phononic crystals will play a significant role in barrier vibration isolation, rail transit vibration isolation, power equipment vibration isolation, precision equipment vibration isolation, noise control, and underground protection engineering. This study constitutes a systematic summary and outlook of phononic crystals in modern engineering vibration and noise control. © The Author(s) 2025.

关键词： Precision engineering

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