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Overall Mass Transfer Coefficient of CO 2 Absorption in a Diameter-varying Spray Tower

Energy Procedia 2017年 114卷 1665-1670页

作者： Xiaomei Wu Min He Yunsong Yu Zhen Qin Zaoxiao Zhang School of Chemical Engineering and Technology Xi’an Jiaotong University No.28 Xianning West Road Xi’an 710049 P.R. China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University No.28 Xianning West Road Xi’an 710049 P.R. China

The application of spray towers for CO 2 capture is a development trend in recent years. However, most of the previous jobs were conducted in a cylindrical tower by using a single spray nozzle, whose configuration and performance is not good enough for industrial application. To solve this problem, the present work proposed a diameter-varying spray tower and a new spray mode of dual-nozzle opposed impinging spray to enhance the absorption performance of CO 2 spray absorption process. Experiments were conducted to investigate the effects of varies operating parameters on the overall mass transfer coefficient in various operating conditions. Experimental results showed that liquid to gas ratio and mole ratio of MEA to CO 2 are key factors which affect the performance of CO 2 absorption process and the maximum overall mass transfer coefficient for the diameter-varying dual-nozzle opposed impinging spray tower is 0.4773 kmol·m -3 ·h -1 ·kPa -1 .

关键词： CO 2 capture diameter-varying spray tower overall mass transfer coefficient absorption performance

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Model for seawater fouling and effects of temperature,flow velocity and surface free energy on seawater fouling

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Chinese Journal of Chemical engineering 2016年第5期24卷 658-664页

作者： Dazhang Yang Jianhua Liu Xiaoxue E Linlin Jiang School of Energy and Power Engineering University of Shanghai for Science and TechnologyShanghai 200093China Shanghai Key Laboratory of Multi-phase Flow and Heat Transfer Shanghai 200093China

A kinetic model was proposed to predict the seawater fouling process in the seawater heat *** new model adopted an expression combining depositional and removal behaviors for seawater fouling based on the Kern–Seaton *** present model parameters include the integrated kinetic rate of deposition(k d)and the integrated kinetic rate of removal(k r),which have clear physical signi ficance.A seawater-fouling monitoring device was established to validate the *** experimental data were well fitted to the model,and the parameters were obtained in different *** and EDX analyses were performed after the experiments,and the results show that the main components of seawater fouling are magnesium hydroxide and aluminum *** effects of surface temperature,flow velocity and surface free energy were assessed by the model and the experimental *** results indicate that the seawater fouling becomes aggravated as the surface temperature increased in a certain range,and the seawater fouling resistance reduced as the flow velocity of seawater ***,the effect of the surface free energy of metals was analyzed,showing that the lower surface free energy mitigates the seawater fouling accumulation.

关键词： Fouling Seawater Model Surface temperature flow velocity Surface free energy

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Connectivity control of effective sorption capacity and kinetics in heterogeneous porous media

Connectivity control of effective sorption capacity and kine...

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第一届全国水处理与回用学术会议

作者： Li Wang Hang Wen Li Li Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power Department of Energy and Mineral Engineering Penn State UniversityUniversity ParkPA 16802USA Department of Civil and Environmental Engineering Penn State UniversityUniversity ParkPA 16802USA

This work examines the effects of spatial heterogeneity in regulating Cr(Ⅵ)sorption under different geostatistical characteristics and spatial scale *** flow-through experiments in heterogeneous columns of 0.1 meters have shown that sorption in heterogeneous media can be characterized by three effective quantities: sorption capacity(Csc,m),early-stage fast sorption rate(kc1),and late-stage slow sorption rate(kc2).Two-dimensional reactive transport models are developed by calibrating these data from these columns of different illite distribution patterns and permeability contrasts between illite and quartz *** models were further run in geostatistical fields of different permeability variance(σ2lnκ,0.2 and 4.5)and length scale(0.1 to 1.0 m)conditions to quantify their role in determining effective sorption capacity and *** results indicate that in highly-connected columns with high permeability variance and long s,Cr(Ⅵ)-containing flow travels mostly through the high permeability,non-sorbing quartz *** therefore occurs mostly at the illite-quartz *** capacity and early fast rates(kc1)therefore depend strongly on the connectivity and properties that control advective transport of the *** longer time scales,diffusive transport determines the late-stage slow rates(kc2)and the breakthrough tailing,which depend less on connectivity and more on the size of the low-permeability illite zones and transverse dispersivity α*** to homogeneous columns of the same illite content,highly-connected patterns can reduce effective sorption capacity by up to a factor of 6.7,fast sorption rates by a factor of 25.0,and slow sorption rate by a factor of more than 2.0 orders of *** the domain length increases,the effects of spatial heterogeneities on sorption capacity and early stage fast sorption rates diminish due to longer length scales for mixing;these effects however persist for the late-stage slow sorp

关键词： connectivity sorption capacity spatial heterogeneity length scales reactive transport modeling

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Numerical simulation of complex membrane characteristics of elastic capsules

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Kung Cheng Je Wu Li Hsueh Pao/Journal of engineering Thermophysics 2016年第2期37卷 337-341页

作者： Luo, Zheng-Yuan Bai, Bo-Feng State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

Dynamics of elastic capsules (elastic membrane enclosing viscous fluid) under flow, which is determined by membrane mechanical characteristics, significantly influence mass transfer across the capsule membrane. Based on front tracking method, a three-dimensional model with considering membrane elasticity and bending resistance was developed to study the effect of bending resistance on the capsule deformation and membrane tensions. It is found that as the bending resistance increases, both the capsule deformation and membrane tensions decrease. Besides, the inclusion of bending resistance inhibits the formation of membrane buckles, thus enhances the membrane stability of capsules. © 2016, Science Press. All right reserved.

关键词： Membranes

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Research progress concerning turbulent drag reduction of surfactant solution

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Huagong Jinzhan/Chemical Industry and engineering Progress 2016年第6期35卷 1660-1675页

作者： Wei, Jinjia Huang, Chonghai Xu, Na State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'anShaanxi710049 China

In turbulent flow drag reduction applications, surfactant additive is more applicable than polymer for the flow with high shear or in the closed circulation system due to its reversible mechanical degradation advantage. However, there is not enough understanding of the complicated rheology and drag-reduction mechanism of surfactant solution, limiting its practical application in the drag reduction field. This review introduces the research progress of surfactant drag reduction conducted by the authors in recent years on microstructure, complicated rheology characteristics, turbulent structure, as well as their relations with drag reduction and heat transfer, and analyzes the combined drag reduction effect of surfactant additives in the flow and microgroove fabricated on the wall. The stretch devices can significantly improve the heat transfer performance of surfactant drag-reducing flow with a lower pressure loss penalty. To the shortages of present surfactant drag reduction research, several suggestions are given for the future study. The first is to develop environmentally friendly and effective surfactant, the second is optimal design and layout of heat transfer enhancement device for drag-reducing flow, the third is the study on synergetic effect of drag reduction by combing surfactant drag reduction and other drag-reducing ways, and the final one is practical industrial application research on the scale-up, anticorrosion and persistence effect of surfactant drag reduction. © 2016, Chemical Industry Press. All right reserved.

关键词： Heat transfer

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Effects of surface wettability on boiling nucleation

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Kung Cheng Je Wu Li Hsueh Pao/Journal of engineering Thermophysics 2016年第1期37卷 111-115页

作者： Zheng, Wen-Xiu Li, Si-Jie Bai, Bo-Feng State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

We established a gas-liquid-solid three phase pool boiling system from molecular dynamics insight, introducing the interactions between the wall and the fluid as an additional force. The effects of wall wettability on the boiling nucleation were studied from three aspects of the nucleation position, the average kinetic energy and the interface contact thermal resistance. The results show that strong surface wettability means strong constraint to the near surface molecules and gas nuclear position is farther from the surface. For stronger surface wettability, the molecular average kinetic energy for the molecules adjacent to the surface is significantly larger than that for the molecules far from the surface, for weaker surface wettability, molecular kinetic energy has a uniform distribution in the vertical direction of the wall. As increasing the surface wettability the interface contact thermal resistance increases and accordingly the boiling nucleation is weakened. © 2016, Science Press. All right reserved.

关键词： Nucleation

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Overexpressing F0/F1 operon of ATPase in Rhodobacter sphaeroides enhanced its photo-fermentative hydrogen production

Overexpressing F0/F1 operon of ATPase in Rhodobacter sphaero...

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作者： Zhang, Yang Yang, Honghui Feng, Jiali Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an710049 China Department of Environmental Science and Engineering Xi'An Jiaotong University Xi'an710049 China

The effect of atp genes overexpression in Rhodobacter sphaeroides HY01 on the amount of ATP, nitrogenase activity and hydrogen production were studied. The ATP content of ZTHF0 (F0 operon+), ZTHF1 (F1 operon+) and ZTHFF (F0 operon+, F1 operon+) was 6.5 ± 0.2 nmol/mL, 7.6 ± 0.2 nmol/mL and 8.3 ± 0.3 nmol/mL, respectively, which enhanced by 20.3%, 40.7%, and 53.7% compared with that of the control strain ZTH (pRK415+), respectively. However, the nitrogenase activities of ZTHF0, ZTHF1 and ZTHFF were 35.8 ± 0.5 nmol acetylene/(min·mg-dcw), 40.1 ± 0.7 nmol acetylene/(min·mg-dcw) and 29.3 ± 0.7 nmol acetylene/(min·mg-dcw), respectively, which increased by 18.2%, 32.3% and 0% compared with that of ZTH, respectively. The expression level of atp genes by real-time PCR showed that ZTHF0 or ZTHF1 only enhanced the expression of F0 operon or F1 operon, respectively, and ZTHFF enhanced the expression of both F0 and F1 operons. At the 5000 ± 200 lux with 10 mL culture, the hydrogen yields of ZTHF0 and ZTHF1 were 7636 ± 59 mL/L-culture and 8458 ± 76 mL/L, which increased by 10.5% and 27.8% compared with that of the control strain, respectively. Moreover, the maximum hydrogen evolution rate of ZTHF0 and ZTHF1 were 94.5 ± 4.1 mL/(Lh) and 103.1 ± 5.0 mL/(Lh), which enhanced by 15.4% and 20.6% compared with that of the control strain, respectively. The results suggested that overexpressing F0 operon or F1 operon could improve ATP content and hydrogen production performance in R. sphaeroides. © 2016, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.

关键词： Hydrogen production

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Experimental Investigation on Heat Transfer Characteristics of Water in Inclined Downward Tube of a Supercritical Pressure CFB Boiler

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Journal of Thermal Science 2015年第5期24卷 478-487页

作者： WANG Siyang YANG Dong XIE Beibei WANG Long WANG Yongjie State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University

In this study, experiments have been performed for an investigation on heat transfer of water in an inclined downward tube with an inner diameter of 20 mm and an inclined angle of 45° from the horizon, with the range of pressure from 11.5 to 28 MPa, mass flux from 450 to 1550 kg/(m2 s), and heat flux from 50 to 585 k W/m2. Based on the experimental data, the temperature distribution in the tube wall was derived. The heat transfer characteristics of inclined downward flow were compared with that of vertical downward flow. The effects of heat flux on wall temperature were analyzed and the corresponding empirical correlations were presented. The results show that heat transfer characteristics of water in the inclined downward tube are not uniform along the circumference from the top surface to the bottom surface. An increase in heat flux exacerbates the non-uniformity. At subcritical pressures, both dry-out and departure from nucleate boiling(DNB) occur at the top surface of the inclined downward tube; inversely, only dry-out takes place on the bottom surface of the inclined downward tube and in the vertical downward tube. At near-critical pressures, DNB and dry-out occur in the comparing tubes with greater possibility. At supercritical pressures, heat transfer gets enhanced in the pseudo-critical enthalpy region; in the high enthalpy region, the top surface temperature of the inclined downward tube decreases obviously.

关键词： inclined downward tube wall temperature circumferential non-uniformity heat transfer deterioration

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Industrialization prospects for hydrogen production by coal gasification in supercritical water and novel thermodynamic cycle power generation system with no pollution emission

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Science China(Technological Sciences) 2015年第12期58卷 1989-2002页

作者： GUO LieJin JIN Hui GE ZhiWei LU YouJun CAO ChangQing State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

Energy conversion and utilization, particularly carbon-based fuel burning in air phase, have caused great environmental pollution and serious problems to society. The reactions in water phase may have the potential to realize clean and efficient energy conversion and utilization. Coal gasification in supercritical water is a typical carbon-based fuel conversion process in water phase, and it takes the advantages of the unique chemical and physical properties of supercritical water to convert organic matter in coal to H2 and CO2. N, S, P, Hg and other elements are deposited as inorganic salts to avoid pollution emission. The State key laboratory of multiphase flow in power engineering has obtained extensive experimental and theoretical results based on coal gasification in supercritical water. Supercritical water fluidized bed reactor was developed for coal gasification and seven kinds of typical feedstock were selected. The hydrogen yield covers from 0.67 to 1.74 Nm3/kg and the carbon gasification efficiency is no less than 97%. This technology has a bright future in industrialization not only in electricity generation but also in hydrogen production and high value-added chemicals. Given the gas yield obtained in laboratory-scale unit, the hydrogen production cost is U.S.$ 0.111 Nm3 when the throughput capacity is 2000 t/d. A novel thermodynamic cycle power generation system based on coal gasification in supercritical water was proposed with the obvious advantages of high coal-electricity conversion efficiency and zero pollutant emission. The cost of U.S.$ 3.69 billion for desulfuration, denitration and dust removal in China in 2013 would have been saved with this technology. Five kinds of heat supply methods are analyzed and the rates of return of investment are roughly estimated. An integrated cooperative innovation center called a new type of high-efficient coal gasification technology and its large-scale utilization was founded to enhance the industrialization o

关键词： industrialization prospects hydrogen production supercritical water gasification power generation zero emission

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Laser-induced breakdown spectroscopy in Asia

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Frontiers of physics 2016年第6期11卷 231-255页

作者： Zhen-ZhenWang Yoshihiro Deguchi Zhen-Zhen Zhang Zhe Wang Xiao-Yan Zeng Jun-Jie Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China Graduate School of Advanced Technology and Science Tokushima University Tokushima 770-8501 Japan State Key Lab of Power Systems Department of Thermal Engineering Tsinghua-BP Clean Energy Center Tsinghua University Beijing 100084 China Wuhan National Laboratory for Optoelectronics (WNLO) Huazhong University of Science and Technology Wuhan ~3007~ China

Laser-induced breakdown spectroscopy (LIBS) is an analytical detection technique based on atomic emission spectroscopy to measure the elemental composition. LIBS has been extensively studied and developed due to the non-contact, fast response, high sensitivity, real-time and multi-elemental detection features. The development and applications of LIBS technique in Asia are summarized and discussed in this review paper. The researchers in Asia work on different aspects of the LIBS study in fundamentals, data processing and modeling, applications and instrumentations. According to the current research status, the challenges, opportunities and further development of LIBS technique in Asia are also evaluated to promote LIBS research and its applications.

关键词： laser-induced breakdown spectroscopy (LIBS) quantitative analysis signal enhancement applications challenges

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