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Assessment on the Long Term Performance of a LaNi 5 based Hydrogen Storage System

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Energy Procedia 2012年 29卷 720-730页

作者： Fusheng Yang Xinxin Cao Zaoxiao Zhang Zewei Bao Zhen Wu Nyallang Nyamsi Serge State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an 710049 P. R.China Suzhou Research Institute Xi’an Jiaotong University Suzhou 215123 P. R. China

Metal hydride represents a promising candidate for hydrogen storage, because the technique is essentially safe, compact and flexible. However, the properties of the metal hydride tend to change in repeated hydriding/dehydriding cycles, which will inevitably affect the performance of corresponding hydrogen storage system. The effect is investigated in this paper by numerical simulation using a commercial package COMSOL MULTIPHYSICS 3.5a, and a typical material- LaNi5 is chosen for discussion. Through sensitivity analysis, the influences of variation in key properties over repeated cycles on the charging time of a tank-type storage system, are evaluated and some useful conclusions are drawn.

关键词： Metal hydride Hydrogen storage system Hydriding/dehydriding cycles Charging time Reaction kinetics

Improvement on Quantitative Measurement of Fly Ash Contents Using Laser-Induced Breakdown Spectroscopy

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Journal of flow Control, Measurement & Visualization 2015年第1期3卷 10-21页

作者： Zhenzhen Wang Yoshihiro Deguchi Hiroaki Watanabe Ryoichi Kurose Junjie Yan Jiping Liu State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an China Graduate School of Advanced Technology and Science The University of Tokushima Tokushima Japan Energy Engineering Research Laboratory The Central Research Institute of Electric Power Industry Kanagawa Japan Department of Mechanical Engineering and Science Advanced Research Institute of Fluid Science and Engineering Kyoto University Kyoto Japan

Contents of fly ash are important factors for the operation of coal-fired plants. Real-time monitoring of coal and fly ash such as unburned carbon in fly ash can be an indicator of the combustion conditions. Because of the strong signal intensity and the relative simplicity of the LIBS (Laser- Induced Breakdown Spectroscopy) technique, LIBS can be applicable for real-time composition measurement of coal and fly ash. This research presented here focused on the clarification of the effects of plasma temperature and coexisting materials on quantitative measurement of fly ash contents. Quantitative capability of LIBS was improved using the proposed plasma temperature correction method. The CO2 effect was also discussed to accurately evaluate unburned carbon in fly ash in exhausts. Using the results shown in this study, quantitative measurement of fly ash contents has been improved for wider applications of LIBS to practical fields.

关键词： Laser-Induced Breakdown Spectroscopy Fly Ash Temperature Correction CO2 Effect

Bionic microchannels for step lifting transpiration

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International Journal of Extreme Manufacturing 2023年第2期5卷 244-252页

作者： Zhaolong Wang Qiu Yin Ziheng Zhan Wenhao Li Mingzhu Xie Huigao Duan Ping Cheng Ce Zhang Yongping Chen Zhichao Dong Interdisciplinary Research Center of Low-carbon Technology and Equipment College of Mechanical and Vehicle EngineeringHunan UniversityChangsha 410082People’s Republic of China MOE Key Laboratory for Power Machinery and Engineering School of Mechanical EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China Qian Xuesen Laboratory of Space Technology China Academy of Space Technology(CAST)Beijing 100094People’s Republic of China Jiangsu Key Laboratory of Micro and Nano Heat Fluid Flow Technology and Energy Application School of Environmental Science and EngineeringSuzhou University of Science and TechnologySuzhouJiangsu 215009People’s Republic of China Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096People’s Republic of China Chinese Academy of Sciences Key Laboratory of Bio-inspired Materials and Interface Sciences Technical Institute of Physics and ChemistryChinese Academy of Sciences100190 BeijingPeople’s Republic of China

Those various cross-sectional vessels in trees transfer water to as high as 100 meters,but the traditional fabrication methods limit the manufacturing of those vessels,resulting in the non-availability of those bionic ***,we fabricate those bionic microchannels with various cross-sections by employing projection micro-stereolithography(PμSL)based 3D printing *** circumradius of bionic microchannels(pentagonal,square,triangle,and five-pointed star)can be as small as 100μm with precisely fabricated sharp ***'s more,those bionic microchannels demonstrate marvelous microfluidic performance with strong precursor effects enabled by their sharp *** significantly,those special properties of our bionic microchannels enable them outstanding step lifting performance to transport water to tens of millimeters,though the water can only be transported to at most 20 mm for a single bionic *** mimicked transpiration based on the step lifting of water from bionic microchannels is also *** precisely fabricated,low-cost,various cross-sectional bionic microchannels promise applications as microfluidic chips,long-distance unpowered water transportation,step lifting,mimicked transpiration,and so on.

关键词： bionic microchannel microfluidics water transportation step lifting 3D printing

Enhanced Low-Temperature Behavior of Selective Catalytic Reduction of Nox by Co on Fe-Based Catalyst with Looping Oxygen Vacancy

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SSRN 2022年

作者： Pan, Yuqing Li, Na Li, Ke Ran, Shiyuan Wu, Chenyang Zhou, Qulan Liu, Jiyuan Li, Shuzhou State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China School of Materials Science and Engineering Nanyang Technological University Singapore639798 Singapore Singapore138634 Singapore

The industrial applications of de-NOx require the high activity window of the catalysts to be shifted from high to low temperatures for energy saving. Selective catalytic reduction (SCR) of NOx by CO, as an alternative to NH3-SCR, is a promising de-NOx technology that facilitates the synergistic removal of pollutants. Herein, we report a new Fe2O3/amorphous SiO2 catalyst with high low-temperature activity for CO-SCR. A combination of experiments and density functional theory (DFT) calculations obtains direct evidence that an optimal content of oxygen vacancy enhances the low-temperature NO conversion ratio and N2 selectivity of Fe2O3-based catalyst to over 80% and maintain 100% CO conversion by promoting NN coupling via ONNO/N2O and NCO/NNCO2 intermediates. Compared with conventional defect engineering, such as doping other metals or artificially generating oxygen defects, the α-Fe2O3 (110) facet automatically enables an oxygen vacancy generation-filling cycle in the CO-SCR reaction, following Mars-van Krevelen (MvK) mechanism. This work advances a fundamental understanding of CO-SCR reaction mechanism over Fe2O3-based catalysts and provides insights for future studies to improve heterogeneous metal oxide catalysts. © 2022, The Authors. All rights reserved.

关键词： Oxygen vacancies

Boosting photocatalytic hydrogen production by creating isotype heterojunctions and single-atom active sites in highly-crystallized carbon nitride

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Science Bulletin 2022年第5期67卷 520-528,M0004页

作者： Shaohua Shen Jie Chen Yiqing Wang Chung-Li Dong Fanqi Meng Qinghua Zhang Yiliang Huangfu Zhi Lin Yu-Cheng Huang Yanrui Li Mingtao Li Lin Gu International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China School of Chemical Engineering and Technology Xi’an Jiaotong UniversityXi’an 710049China Department of Physics Tamkang UniversityNew Taipei City 25137TaiwanChina Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China

Carbon nitride-based photocatalysts hold an enormous potential in producing hydrogen.A strategy to simultaneously create isotype heterojunctions and active sites in highly-crystallized carbon nitride is anticipated to significantly boost the photocatalytic activity,but is yet to be ***,we find that cobalt salt added in the ionothermal synthesis can promote the phase transition of heptazine-based crystalline carbon nitride(CCN)to triazine-based poly(triazine imide)(PTI),rendering the creation of singleatom cobalt coordinated isotype CCN/PTI ***-CCN/PTI exhibits an appreciable apparent quantum yield of 20.88%at 425 nm for photocatalytic hydrogen production with a rate achieving3538μmol h^(-1)g^(-1)(λ>420 nm),which is 4.8 times that of CCN and 27.6 times that of *** high photocatalytic activity is attributed to the Type II isotype highly-crystallized CCN/PTI heterojunction for promoting charge carrier migration,and the single-atom Co sites for accelerating surface oxidation reaction.

关键词： Photocatalytic hydrogen production Single-atom cobalt Crystalline carbon nitride Poly(triazine imide) Isotype heterojunctions

Sensitively Detection of Ascorbic Acid in Orange Samples with Ionic Liquid Functionalized Carbon Dots and Lanthanide Complexes

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SSRN 2024年

作者： Li, Ying Xia, Ji-Ji Lu, Jia-Zhen Wang, Zi-Long Wang, Mi-Tang School of Materials and Chemistry University of Shanghai for Science and Technology Shanghai200093 China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai200093 China

In the food industry, ascorbic acid (AA) is widely used as an antioxidant. However, the concentration of AA is influenced by various factors, including temperature, time, and pH value during food preparation and storage, leading to its instability in content. This makes the accurate detection of AA content particularly important. Precise determination of AA content in food and pharmaceuticals is crucial for ensuring the adequate intake of essential vitamins and maintaining good health. Herein, we have developed a successful preparation method of an imidazole-based ionic liquid functionalized CDs hybrids APM-CDs. A novel photo functional hybrid probe Eu3+@APM-CDs was obtained via an ion-exchange reaction between APM-CDs and lanthanide complex Eu(DPA)3. The obtained hybrid probe was extensively characterized in detail. What’s more, the results show that the FL intensity of Eu3+@APM-CDs has a good linear response to AA concentrations in the range of 0-500 μM (R2 = 0.99), with a detection limit of 80 nM. The fluorescence probe demonstrates good selectivity and sensitivity toward AA and has the potential for significant application in AA detection by simplifying procedures and reducing interference from impurities. © 2024, The Authors. All rights reserved.

关键词： Probes

Analysis of fracture propagation and shale gas production by intensive volume fracturing

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Applied Mathematics and Mechanics(English Edition) 2023年第8期44卷 1385-1408页

作者： Qingdong ZENG Long BO Lijun LIU Xuelong LI Jianmeng SUN Zhaoqin HUANG Jun YAO College of Energy and Mining Engineering Shandong University of Science and TechnologyQingdao 266590Shandong ProvinceChina Research Center of Multiphase Flow in Porous Media China University of Petroleum(East China)Qingdao 266580Shandong ProvinceChina State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum UniversityChengdu 610500China College of Energy Chengdu University of TechnologyChengdu 610059China College of Geoscience China University of Petroleum(East China)Qingdao 266580Shandong ProvinceChina

This paper presents an integrated study from fracture propagation modeling to gas flow modeling and a correlation analysis to explore the key controlling factors of intensive volume *** fracture propagation model takes into account the interaction between hydraulic fracture and natural fracture by means of the displacement discontinuity method(DDM)and the Picard iterative *** shale gas flow considers multiple transport mechanisms,and the flow in the fracture network is handled by the embedded discrete fracture model(EDFM).A series of numerical simulations are conducted to analyze the effects of the cluster number,stage spacing,stress difference coefficient,and natural fracture distribution on the stimulated fracture area,fractal dimension,and cumulative gas production,and their correlation coefficients are *** results show that the most influential factors to the stimulated fracture area are the stress difference ratio,stage spacing,and natural fracture density,while those to the cumulative gas production are the stress difference ratio,natural fracture density,and cluster *** indicates that the stress condition dominates the gas production,and employing intensive volume fracturing(by properly increasing the cluster number)is beneficial for improving the final cumulative gas production.

关键词： fracture network propagation shale gas fow intensive volume fracturing displacement discontinuity method(DDM) embedded discrete fracture model(EDFM)

Visualization Experiments and Piston Effect of Heat Transfer on Supercritical Carbon Dioxide in a Mini Vertical Upward flow

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SSRN 2022年

作者： Lyu, Haicai Wang, Han Bi, Qincheng Niu, Fenglei School of Nuclear Science and Engineering North China Electric Power University Beijing102206 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University No.28 Xianning West Road Xi’an710049 China

The characteristics of supercritical heat transfer and flow patterns visualization were investigated experimentally. System parameters are pressure of 7.4 ~ 8.44 MPa, the mass flux of 600 ~ 1600 kg·m -2 ·s -1 and heat flux up to 319 kW·m -2 . The basic experimental data of heat transfer coefficient and frictional pressure drop were obtained. Local heat transfer coefficient was calculated with respect to the mass flux, heat flux and pressure. The scenario of in-tube supercritical carbon dioxide was presented by a high-resolution camera. Experimental results show that the heat transfer peak happens when the wall temperature is above the pseudo-critical temperature, and in-tube fluid is lower than the pseudo-critical temperature. Exciting phenomenon of critical opalescence is observed under the pressure of 7.4 MPa and a temperature of 31.68 ˚C. Rapid alternation of sky blue and milky white was captured in an extremely short period time, which may be related to Rayleigh scattering due to drastic density fluctuation. Piston effect of strongly uneven aggregation was formed due to the variation of thermal physical property, which can be used to exposit the mechanism of supercritical heat transfer peak near the pseudo-critical temperature. Ration of density and volumetric coefficient of expansion can be represented for the piston effect to produce the modified Jackson’s correlation, which owns the average error of -0.69% and root-mean-square error of 10.35%. © 2022, The Authors. All rights reserved.

关键词： Visualization

Depth from Defocus Technique for High Number Densities and Non-Spherical Particles

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SSRN 2024年

作者： Xu, Rixin Huang, Zuojie Gong, Wenchao Zhou, Wu Tropea, Cameron School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer for Power Engineering Shanghai China Institute for Fluid Mechanics and Aerodynamics Technical University of Darmstadt Darmstadt Germany

The Depth from Defocus (DFD) imaging technique for measuring the size and number concentration of particles in a dispersed two-phase flow has up to now been restricted to relatively sparse particle densities and to identifying only spherical particles. The present study examines two advancements to the technique, widening its range of application significantly. The first advancement introduces an image processing procedure which can identify and size particle images which are overlapping. This increases the tolerable number concentration of particles which can be identified and processed within the measurement volume. The second advancement explores the possibility of determining the size and position of non-spherical particles within an observation volume. These enhancements are experimentally validated using a dedicated apparatus in which particles of known size, shape and degree of overlapping images can be systematically varied. This experimental setup provides benchmark data to quantify the accuracy and limitations of the processing algorithms. © 2024, The Authors. All rights reserved.

关键词： Two phase flow