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2011 MRS Spring Meeting

作者： Liu, Haipei Jing, Dengwei Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an 710049 China

ISBN: (纸本)9781618395238

In this work a series of Eosin Y-ZnO(x%)/TiO2 were prepared. ZnO well dispersed on the surface of TiO2, which improves the adsorption of Eosin Y and the excited electron to transfer to the conduction band of TiO2. Therefore the visible light activity of 0.2%Pt-Eosin Y-ZnO(x%)/TiO2 is much higher than that of the 0.2%Pt-Eosin Y-TiO2 and 0.2%Pt-Eosin Y-ZnO. The 0.2%Pt-Eosin Y-ZnO(1.5%)/TiO 2 has the highest visible light activity among the catalysts coupled with various ZnO amount, whose activity is increased by a factor of 3.5 compared to that of 0.2%Pt-Eosin Y-TiO2. It is proposed that, 0.2%Pt-Eosin Y-ZnO(1.5%)/TiO2 has the optimal trapping sites of carriers and thickness of the space-charge layer on the TiO2 particle surface, so these factors result a more efficient charge separation, an increased lifetime of the charge carriers, and the enhanced of hydrogen production. © 2011 Materials Research Society.

关键词： Titanium dioxide

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Exhaust recovery of vehicle gasoline engine based on organic rankine cycle

Exhaust recovery of vehicle gasoline engine based on organic...

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SAE 2011 World Congress and Exhibition

作者： Zhang, Xinxin Zeng, Ke Bai, Sujuan Zhang, Ying He, Maogang State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an Shaanxi 710049 China

When the global energy consumption continues to increase, the research hotspot in the field of internal combustion engine (ICE) is how to improve the fuel utilization efficiency to achieve the energy saving. But as far as the engine efficiency is concerned, it has been very difficult to improve the fuel utilization efficiency after the Gasoline Direct-Injection (GDI) and Homogeneous Charge Compression Ignition (HCCI) technology were adopted. In this study, the exothermic distribution of fuel was studied detailedly when a TOYOTA 8A-FE gasoline engine operated at different working conditions through conducting steady-state experiment. Only one third of fuel's chemical energy is converted into effective work by engine, the rest is released to the environment in the form of waste heat generated from cooling and exhaust gas. But except the waste heat that has to be released to the environment according to the second law of thermodynamics, the rest can be theoretically utilized. If the waste heat of the vehicle engine can be recovered, the engine efficiency will be evidently improved. Results on the exergy analysis show that the exergy in the exhaust gas is about 45-70% and it will evidently increase with the increase of engine load and revolution. So it will have a good effect on exhaust recovery when the engine has a heavy load. Considering the character of exhaust gas, the Organic Rankine Cycle(ORC) is adopted to recover the waste heat of engine's exhaust gas. The thermodynamic performances of the cycle were analyzed and R113 was determined to be the working fluid. The experimental exhaust gas recovery system used to testify the aforementioned theoretical calculation was designed and established. The system consists of exhaust gas simulation device, expander, condenser, dynamometer, pump and data acquisition and processing system. In experiment, the performance parameter and power output of the Organic Rankine Cycle were measured. The expander show a high isentropic ef

关键词： Recovery

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Photocatalytic reforming of formic acid with simultaneous hydrogen production under visible light over CdS sensitized Na2Ti 2O4(OH)2

Photocatalytic reforming of formic acid with simultaneous hy...

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2011 MRS Spring Meeting

作者： Tang, Wendong Jing, Dengwei Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 China

ISBN: (纸本)9781618395238

The present work reports the renewable hydrogen production by an anaerobic photocatalytic reforming of formic acid over CdS sensitized Na 2Ti2O4(OH)2 nanotubes, the Na 2Ti2O4(OH)2 nanotube was prepared and charactered by X-ray diffraction, UV-visible absorption, transmission electron microscopy, etc. The activity of the catalyst in formic acid was investigated. The greatest photocatalytic reforming activity of formic acid occurs as the formic acid initial concentration is 20 v.%. A probable mechanism for the photocatalytic reforming process was proposed and discussed. © 2011 Materials Research Society.

关键词： Cadmium sulfide

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Rapid calculation for density of water and steam on p-T thermodynamic surface

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Yingyong Jichu yu Gongcheng Kexue Xuebao/Journal of Basic Science and engineering 2012年第SUPPL.期20卷 190-198页

作者： An, Bin Wang, Xiaodong Duan, Yuanyuan Wang, Zhixue State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources North China Electric Power University Beijing 102206 China Beijing Key Laboratory of Multiphase Flow and Heat Transfer for Low Grade Energy North China Electric Power University Beijing 102206 China Key Laboratory for Thermal Science and Power Engineering of MOE Department of Thermal Engineering Tsinghua University Beijing 100084 China

This paper develops a rapid calculation method for thermodynamic properties of water and steam on p-T thermodynamic surface with 273.16K

关键词： Steam

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Performance of a domestic refrigerator using TiO2-R600a nano-refrigerant as working fluid

Performance of a domestic refrigerator using TiO2-R600a nano...

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作者： Bi, Shengshan Guo, Kai Liu, Zhigang Wu, Jiangtao State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 China

In this work, an experimental work was investigated on the nano-refrigerant. TiO2-R600a nano-refrigerants were used in a domestic refrigerator without any system reconstruction. The refrigerator performance was then investigated using energy consumption test and freeze capacity test. The results indicate that TiO2-R600a nano-refrigerants work normally and safely in the refrigerator. The refrigerator performance was better than the pure R600a system, with 9.6% less energy used with 0.5 g/L TiO2-R600a nano-refrigerant. Thus, using TiO2-R600a nano-refrigerant in domestic refrigerators is feasible. © 2010 Elsevier Ltd. All rights reserved.

关键词： Refrigerators

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Shock tube study on auto-ignition characteristics of kerosene/air mixtures

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Chinese Science Bulletin 2011年第13期56卷 1399-1406页

作者： ZHANG YingJia HUANG ZuoHua WANG JinHua XU ShengLi State Key Laboratory of Multiphase Flow in Power Engineering Xi' an Jiaotong University Xi' an 710049 China Department of Modern Mechanics University of Science and Technology of China Hefei 230026 China

Ignition delay times are obtained for kerosene/air mixtures behind the reflected shock waves at temperatures between 1445 and 1650 K,at a pressure of 0.11 MPa and an equivalence ratio of 1.0.A nebulization device with Laval nozzle is used to nebulize kerosene and form an aerosol phase,which evaporates and diffuses rapidly behind the incident shock *** auto-ignite behind the reflected shock *** ICCD is used to visualize the kerosene/air mixture's ignition *** mixture's ignition intensity increases with increase in initial *** and irregular flames exist below 1515 K while plane and discontinuous flames exist over 1560 *** delay times decrease with increase in initial *** data shows good agreement with results reported previously in the literature.A new surrogate (consisting of 10% toluene,10% ethylbenzene and 80% n-decane) is proposed for *** et al.'s mechanism is used to simulate the ignition of kerosene with calculations agreeing well with the experimental *** sensitivity of reaction H+O2 <=>OH+O,which shows the highest sensitivity to the ignition delay time,increases with an increase in *** chain breaching reaction of CH3 with O2 accelerates the total reaction rate and the H-atom abstraction of n-decane controls the total reaction *** rate of production and instantaneous heat production indicate that two reactions,H+O2 <=>OH+O and O+H2 <=>OH+H,are the key reactions to the formation of OH radicals,as well as the main endothermic ***,the reaction of R3 is the main heat release reaction during *** structure analysis shows that initial pressure is increased slightly as CO and H2O will appear before main ignition.

关键词：空气混合物煤油自燃特性点火延迟时间冲击管反应速率初始温度数据显示

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TiO2-SnO2:F interfacial electronic structure investigated by soft x-ray absorption spectroscopy

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Physical Review B 2012年第12期85卷 125109-125109页

作者： Coleman X. Kronawitter Mukes Kapilashrami Jonathan R. Bakke Stacey F. Bent Cheng-Hao Chuang Way-Faung Pong Jinghua Guo Lionel Vayssieres Samuel S. Mao Department of Mechanical Engineering University of California at Berkeley Berkeley California 94720 USA Environmental Energy Technologies Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA Advanced Light Source Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Chemical Engineering Stanford University Stanford California 94305 USA Department of Physics Tamkang University Tamsui Taiwan Republic of China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi 710049 People's Republic of China

The electronic structure of the titanium dioxide (TiO2)-fluorine-doped tin dioxide (SnO2:F) interface is investigated by soft x-ray absorption spectroscopy using synchrotron radiation. The measurements probe the site- and symmetry-selected unoccupied density of states and reflect the interaction between an early transition-metal-oxide (d0) semiconductor and a post-transition-metal-oxide (d10) degenerate semiconductor. The distinct interfacial electronic structure of TiO2-SnO2:F is established by contrasting spectra with those for anatase and rutile TiO2, SnO2:F, and ZnO-SnO2:F and CdO-SnO2:F interfaces. Oxygen 1s absorption spectra, which relate to the O 2p partial density of states of the conduction band, indicate that the interface is associated with a reduction in Ti d-O p orbital hybridization and an alteration of the TiO2 crystal field. These observations are consistent with measured titanium 2p absorption spectra, which in addition provide evidence for distortion of long-range order around the cation site in the interfacial TiO2. The TiO2-SnO2:F interface is a functional component of a number of optoelectronic devices, perhaps most notably within the anode structure of solar cell architectures. In nonequilibrium conditions, such as those found in operating solar cells, interfacial electronic structure directly influences performance by modifying, for instance, the quasi-Fermi level electrons and the potential distribution at the transparent electrode.

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Radiant performance of opacifiers in opcifier-loaded silica aerogel-based composites

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Yingyong Jichu yu Gongcheng Kexue Xuebao/Journal of Basic Science and engineering 2012年第SUPPL.期20卷 181-189页

作者： Sun, Duo Wang, Xiaodong Duan, Yuanyuan Zhao, Junjie State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources North China Electric Power University Beijing 102206 China Department of Thermal Engineering University of Science and Technology Beijing Beijing 100083 China Beijing Key Laboratory of Multiphase Flow and Heat Transfer for Low Grade Energy North China Electric Power University Beijing 102206 China Key Laboratory for Thermal Science and Power Engineering of MOE Department of Thermal Engineering Tsinghua University Beijing 100084 China

Since the opacifier-loaded silica aerogel composites have strong ability to inhibit radiant heat transfer compared to the pure silica aerogel, they can improve effectively the insulation performance at high temperature conditions and have been used extensively as thermal insulation materials in a variety of industrial applications. This paper developed a theoretical model to predict the radiant performance of opacifiers by using the Mie scattering theory, Beer law and a radiant heat transfer equations. The model was used to calculate the radiant performance of carbon black opacifier with various particle diameters and the radiant performance of three opacifiers, carbon black, SiC and ZrO2. The results showed that the opacifier-loaded silica aerogel composites had much higher extinction coefficient than the pure silica aerogel in a range of 3-7.5 μm wave band or in medium and high temperature ranges, which significantly improved the insulation performance of composites. With a fixed opacifier mass fraction, the optimal particle diameter was 2-3 μm for carbon black opacifier. Among the three opacifiers, carbon black opacifier had better opaque property than that of SiC and ZrO2 opacifiers. Due to poor thermostability for carbon black opacifier at high temperature conditions, the optimal material design for opacifier-loaded silica aerogel composites should be as follows: SiC or ZrO2 are added on high temperature side of aerogel and carbon black is added on low temperature side.

关键词： Thermal conductivity

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Analysis of CHF in saturated forced convective boiling on a heated surface with impinging jets using artificial neural network and genetic algorithm

Analysis of CHF in saturated forced convective boiling on a ...

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作者： Cong, Tenglong Chen, Ronghua Su, Guanghui Qiu, Suizheng Tian, Wenxi School of Nuclear Science and Technology State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an 710049 China

In this paper, a three-layer Back Propagation (BP) algorithm artificial neural network (ANN) for predicting critical heat flux (CHF) in saturated forced convective boiling on a heated surface with impinging jets was trained successfully with a root mean square (RMS) error of 17.39%. The input parameters of the ANN are liquid-to-vapor density ratio, ρl/ ρv, the ratio of characteristic dimension of the heated surface to the diameter of the impinging jet, L/d, reciprocal of the Weber number, 2σ/ρlu2(L - d), and the number of impinging jets, Nj. The output is dimensionless heat flux, qco/ ρvHfgu. Based on the trained ANN, the influence of principal parameters on CHF has been analyzed as follows. CHF increases with an increase in jet velocity and decreases with an increase in L/d and N j. CHF increases with an increase in pressure at first and then decreases. Besides, a new correlation was generalized using genetic algorithm (GA) as a comparison with ANN to confirm the advantage of ANN. © 2011 Published by Elsevier B.V.

关键词： Heat flux

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Improved photocatalytic H2 evolution from inorganic/organic sacrificial solution over Ni-doped (CuIn)0.2Zn1.6S 2 photocatalysts

Improved photocatalytic H2 evolution from inorganic/organic ...

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2011 MRS Spring Meeting

作者： Zhang, Xianghui Jing, Dengwei Guo, Liejin State Key Lab of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

ISBN: (纸本)9781618395238

The Ni-doped (CuIn)0.2Zn1.6S2 photocatalysts were prepared via a two-step ultrasonic-hydrothermal method under an environmental-friendly condition. XRD pattern profiles suggested that Ni2+ successfully doped into (CuIn)0.2Zn 1.6S2 lattice. UV-Vis spectra indicated that the optical properties of the photocatalysts greatly depended on the amount of Ni doped. SEM images show that the samples were microspheres. The microsphere structures were gradually damaged with the increment of Ni doping amount. The photoactivity of (CuIn)0.2Zn1.6S2 was enhanced when Ni 2+ was doped into the crystal structure. The H2 evolution performance over the prepared samples from inorganic/organic sacrificial solution was systematic investigated. © 2011 Materials Research Society.

关键词： Microspheres

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