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2011 MRS Spring Meeting

作者： Shen, Shaohua Kronawitter, Coleman X. Jiang, Jiangang Guo, Liejin Mao, Samuel S. State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 China Environmental Energy Technologies Division Lawrence Berkeley National Laboratory Berkeley CA 94720 United States

ISBN: (纸本)9781618395238

α-Fe2O3 nanorod arrays were fabricated by a low-temperature aqueous chemical growth (ACG) technique and followed by an annealing process. For the surface doping of α-Fe2O3 nanorods, β-FeOOH nanorods obtained via ACG were coated with a thin layer of Cr3+ precursor solution by spin coating, and then underwent the annealing treatment in air. Conducting polymer polypyrrole (PPy) decorated α-Fe2O3 nanorods were prepared by electrodeposition method using malic acid contained pyrrole aqueous solution. Primary results showed that the photocurrents of α-Fe2O3 nanorod array photoanodes were greatly enhanced by surface doping of Cr3+, as well as PPy decoration. This might be due to the retarded charge recombination and promoted surface reaction rate of photogenerated holes with water. Further investigation on surface modification of α-Fe2O3 nanorod array photoanodes is currently conducted in our group. © 2011 Materials Research Society.

关键词： Nanorods

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Study on the Radiation Distribution in A Fluidized Tubular Reactor for Heterogeneous Photocatalytic Hydrogen Production

Study on the Radiation Distribution in A Fluidized Tubular R...

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2011 International Conference on Energy and Environment(ICEE 2011)

作者： Zhao Liang Fan Liangliang Jing Dengwei Liu Wenxu Cao Fei Zhu Xule Yang Junyin Zhang Hailong State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

Radiation distribution study is of importance for the design and the optimization of fluidized photocatalytic tubular reactor which has been developed for photocatalytic hydrogen production under direct solar light. In the present study, the radiation distribution in such reactor was successfully simulated by adopting Monte Carlo method and the six-flux radiation absorption-scattering models. Both the incident angles of light around the reactor and the concentration distribution of photocatalyst were taken into account. Our analysis indicates that the angles and the intensity of the incident rays significantly affect the radiation distribution. Moreover, it was also found that the equilibrium radiation distribution has a close relationship with the density distribution of the photocatalysts. The simulated results are expected to be helpful for obtaining the optimal operating parameters for solar photocatalytic hydrogen production.

关键词： radiation distribution,fluidized tubular reactor,nanometer catalyst,compound parabolic concentrators

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A Model for Wave Properties in Churn flow

A Model for Wave Properties in Churn Flow

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The Fifth China-Korea Workshop on Nuclear Reactor Thermal Hydraulics

作者： Ke Wang Bofeng Bai Jiahuan Cui State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

A model for wave properties, such as wave velocity and amplitude in churn flow has been developed in this paper. The results demonstrate that the wave behavior differs from that in annular flow. In addition, the critical amplitude A c decreases with the increase in gas flow rate. Moreover, the maximum amplitude A max decreases with the increasing of gas mass flux but increase with the increasing of liquid mass flux. The average absolute deviations (AAD) for A c and A max are 16.29% and 7.10%, respectively.

关键词： A Model for Wave Properties in Churn flow Model

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An Adaptive VOF Method on Unstructured Grid

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AIP Conference Proceedings 2011年第1期1376卷 642-644页

作者： L. L. Wu M. Huang B. Chen State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an 710049 China

In order to improve the accuracy of interface capturing and keeping the computational efficiency, an adaptive VOF method on unstructured grid is proposed in this paper. The volume fraction in each cell is regarded as the criterion to locally refine the interface cell. With the movement of interface, new interface cells (0 ≤ f ≤ 1) are subdivided into child cells, while those child cells that no longer contain interface will be merged back into the original parent cell. In order to avoid the complicated redistribution of volume fraction during the subdivision and amalgamation procedure, a predictor‐corrector algorithm is proposed to implement the subdivision and amalgamation procedures only in empty or full cell ( f = 0 or 1). Thus volume fraction in the new cell can take the value from the original cell directly, and the interpolation of the interface is avoided. The advantage of this method is that the re‐generation of the whole grid system is not necessary, so its implementation is very efficient. Moreover, an advection flow test of a hollow square was performed, and the relative shape error of the result obtained by adaptive mesh is smaller than those by non‐refined grid, which verifies the validation of our method.

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Study on the Radiation Distribution in A Fluidized Tubular Reactor for Heterogeneous Photocatalytic Hydrogen Production

Study on the Radiation Distribution in A Fluidized Tubular R...

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2011 International Conference of Environmental Science and engineering（ICESE 2011）

作者： Zhao Liang Fan Liangliang Jing Dengwei Liu Wenxu Cao Fei Zhu Xule Yang Junyin Zhang Hailong State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

关键词： Radiation distribution,Fluidized tubular reactor,Nanometer catalyst Compound parabolic concentrators

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Eosin Y-sensitized ZnO/TiO 2 for efficient visible light photocatalytic hydrogen evolution

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MRS Online Proceedings Library 2011年第1期1326卷 1-6页

作者： Haipei Liu Dengwei Jing Liejin Guo State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an P. R. China

In this work a series of Eosin Y-ZnO(x%)/TiO2 were prepared. ZnO well dispersed on the surface of TiO2, which improves the adsorption of Eosin Y and the excited electron to transfer to the conduction band of TiO2. Therefore the visible light activity of 0.2%Pt-Eosin Y-ZnO(x%)/TiO2 is much higher than that of the 0.2%Pt-Eosin Y-TiO2 and 0.2%Pt-Eosin Y-ZnO. The 0.2%Pt-Eosin Y- ZnO(1.5%)/TiO2 has the highest visible light activity among the catalysts coupled with various ZnO amount, whose activity is increased by a factor of 3.5 compared to that of 0.2%Pt-Eosin Y-TiO2. It is proposed that, 0.2%Pt-Eosin Y-ZnO(1.5%)/TiO2 has the optimal trapping sites of carriers and thickness of the space-charge layer on the TiO2 particle surface, so these factors result a more efficient charge separation, an increased lifetime of the charge carriers, and the enhanced of hydrogen production.

关键词： catalytic hydrogenation energy generation

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Photocatalytic reforming of formic acid with simultaneous hydrogen production under visible light over CdS sensitized Na 2 Ti 2 O 4 (OH) 2

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MRS Online Proceedings Library 2011年第1期1326卷 1-6页

作者： Wendong Tang Dengwei Jing Liejin Guo State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an P. R. China

The present work reports the renewable hydrogen production by an anaerobic photocatalytic reforming of formic acid over CdS sensitized Na2Ti2O4(OH)2 nanotubes. the Na2Ti2O4(OH)2 nanotube was prepared and charactered by X-ray diffraction, UV-visible absorption, transmission electron microscopy, etc. The activity of the catalyst in formic acid was investigated. The greatest photocatalytic reforming activity of formic acid occurs as the formic acid initial concentration is 20 v.%. A probable mechanism for the photocatalytic reforming process was proposed and discussed.

关键词： nanostructure photochemical hydrothermal

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Experimental investigation of heat transfer for supercritical pressure water flowing in vertical annular channels

Experimental investigation of heat transfer for supercritica...

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作者： Gang, Wu Bi, Qincheng Yang, Zhendong Wang, Han Zhu, Xiaojing Hao, Hou Leung, L.K.H. State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an 710049 China Atomic Energy of Canada Limited Chalk River ON K0J 1J0 Canada

An experiment has recently been completed at Xi'an Jiaotong University (XJTU) to obtain wall-temperature measurements at supercritical pressures with upward flow of water inside vertical annuli. Two annular test sections were constructed with annular gaps of 4 and 6 mm, respectively, and an internal heater of 8 mm outer diameter. Experimental-parameter ranges covered pressures of 23-28 MPa, mass fluxes of 350-1000 kg/m2/s, heat fluxes of 200-1000 kW/m2, and bulk inlet temperatures up to 400 °C. Depending on the flow conditions and heat fluxes, two distinctive heat transfer regimes, referring to as the normal heat transfer and deteriorated heat transfer, have been observed. At similar flow conditions, the heat transfer coefficients for the 6 mm gap annular channel are larger than those for the 4 mm gap annular channel. A strong effect of spiral spacer on heat transfer has been observed with a drastic reduction in wall temperature at locations downstream of the device in the annuli. Two tube-data-based correlations have been assessed against the experimental heat transfer results. The Jackson correlation agrees with the experimental trends and overpredicts slightly the heat transfer coefficients. The Dittus-Boelter correlation is applicable only for the normal heat transfer region but not for the deteriorated heat transfer region. © 2011 Published by Elsevier B.V.

关键词： Heat transfer coefficients

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Improved Photocatalytic H 2 Evolution from Inorganic/Organic Sacrificial Solution over Ni-Doped (CuIn) 0.2 Zn 1.6 S 2 Photocatalysts

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MRS Online Proceedings Library 2011年第1期1326卷 1-6页

作者： Xianghui Zhang Dengwei Jing Liejin Guo State Key Lab of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an PR China

The Ni-doped (CuIn)0.2Zn1.6S2 photocatalysts were prepared via a two-step ultrasonic-hydrothermal method under an environmental-friendly condition. XRD pattern profiles suggested that Ni2+ successfully doped into (CuIn)0.2Zn1.6S2 lattice. UV-Vis spectra indicated that the optical properties of the photocatalysts greatly depended on the amount of Ni doped. SEM images show that the samples were microspheres. The microsphere structures were gradually damaged with the increment of Ni doping amount. The photoactivity of (CuIn)0.2Zn1.6S2 was enhanced when Ni2+ was doped into the crystal structure. The H2 evolution performance over the prepared samples from inorganic/organic sacrificial solution was systematic investigated.

关键词： catalytic energy generation hydrogenation

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Deposition of Cement Kiln Ash on the Tubes of Waste Heat Recovery Boiler

Deposition of Cement Kiln Ash on the Tubes of Waste Heat Rec...

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IEEE PES Asia-Pacific power and Energy engineering Conference (APPEEC)

作者： Yufeng Wang Chunyun Hu Shi'en Hui Qinxin Zhao Qulan Zhou State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi China

Deposition of cement kiln ash on the tubes of heat recovery boiler affects the heat exchange efficiency. The basic characteristic of cement kiln ash and the deposition on the tubes with different arrangements are presented. Numerical simulation and experiment measurement show that flow field feature, especially the low-velocity zone and vortex street, causes different shape of ash deposit around the tube. The effect of ash concentration, tube arrangement and gas velocity on the deposition is analyzed. The effect of the tube diameter and the gas composition is also discussed.

关键词： Ash Electron tubes Surface treatment Heat recovery Waste heat Shape Boilers

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