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Chemical looping based ammonia production--A promising pathway for production of the noncarbon fuel

Science Bulletin 2022年第20期67卷 2124-2138,M0004页

作者： Qinghua Lai Tianyi Cai Shik Chi Edman Tsang Xia Chen Runping Ye Zhenghe Xu Morris D.Argyle Dong Ding Yongmei Chen Jianji Wang Armistead G.Russell Ye Wu Jian Liu Maohong Fan College of Engineering and Applied Science University of WyomingLaramie WY 82071USA School of Energy and Power Engineering Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China Wolfson Catalysis Department of ChemistryUniversity of OxfordOxford Ox13QRUK College of Chemistry and Chemical Engineering Ocean University of ChinaQingdao 266100China State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Chemical and Materials Engineering University of AlbertaEdmonton Alberta T6G1H9Canada Department of Chemical Engineering Brigham Young UniversityProvo UT 84602USA Idaho National Laboratory Idaho Falls ID83415USA College of Chemistry Beijing University of Chemical TechnologyBejing 100029China School of Chemistry and Environmental Science Henan Normal UniversityXinxiang 453007China School of Civil and Environmental Engineering Georgia Institute of TechnologyAtlanta GA 30332USA MIIT Key Laboratory of Thermal Control of Electronic Equipment School of Power EngineeringNanjing University of Science&TechnologyNanjing 210094China DICP-Surrey Joint Centre for Future Materials Department of Chemical and Process Engineeringand Advanced Technology InstituteUniversity of SurreyGuilford Surrey GU27XH UK

Ammonia, primarily made with Haber-Bosch process developed in 1909 and winning two Nobel prizes, is a promising noncarbon fuel for preventing global warming of 1.5 °C above pre-industrial levels. However,the undesired characteristics of the process, including high carbon footprint, necessitate alternative ammonia synthesis methods, and among them is chemical looping ammonia production(CLAP) that uses nitrogen carrier materials and operates at atmospheric pressure with high product selectivity and energy efficiency. To date, neither a systematic review nor a perspective in nitrogen carriers and CLAP has been reported in the critical area. Thus, this work not only assesses the previous results of CLAP but also provides perspectives towards the future of CLAP. It classifies, characterizes, and holistically analyzes the fundamentally different CLAP pathways and discusses the ways of further improving the CLAP performance with the assistance of plasma technology and artificial intelligence(AI).

关键词： Ammonia synthesis Chemical looping Nitrogen carrier Renewable fuels Energy carrier

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Modeling of water and temperature distribution in PEM fuel cell

引用

Kung Cheng Je Wu Li Hsueh Pao/Journal of engineering Thermophysics 2010年第12期31卷 2051-2056页

作者： Ma, Li-Zhong Shen, Shuang-Lin Jia, Fei Liu, Hong-Tan Guo, Lie-Jin State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China Dept. of Mechanical and Aerospace Engineering University of Miami Coral Gables FL 33124 United States

A two-phase flow, non-isothermal, three dimensional model was developed to study the transport phenomena in proton exchange membrane (PEM) fuel cell. Modeling results of water distribution and temperature distribution are presented in this paper. The modeling results show that water and temperature distributions are non-uniform. Along the flow direction, water concentration in anode is decreasing while that in cathode is increasing which liquid water present in cathode;in the cross section perpendicular to the flow direction, both water concentration and liquid water saturation under the shoulder are higher than that under the channel;liquid water distribution across cathode GDL is different at different discharging voltages. Local temperature is decreasing along the flow direction, with even higher gradient when the reactant gas is insufficient;temperatures under the shoulder are lower than those under the channel;in the direction across MEA, the highest temperature is in cathode catalyst layer, and temperature gradient increases as the discharging voltage decreases;at the same discharging voltage, the thicker the PEM is, the lower the local temperatures and the temperature gradient across MEA are.

关键词： Temperature distribution

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Pore-scale simulation of shale oil flow based on pore network model

引用

Fuel 2019年 251卷 683-692页

作者： Yongfei Yang Ke Wang Lei Zhang Hai Sun Kai Zhang Jingsheng Ma Key Laboratory of Unconventional Oil & Gas Development (China University of Petroleum (East China)) Ministry of Education Qingdao 266580 China Research Center of Multiphase Flow in Porous Media School of Petroleum Engineering China University of Petroleum (East China) Qingdao 266580 China Institute of Petroleum Engineering Heriot-Watt University Riccarton Edinburgh UK

The pore-grain characteristics of shale oil reservoir rocks are complex: nano-size pore throats, multi-scale of pore size and topology, and rich in organic matter. Generally, shale oil flow in nanoporous media is significantly affected by microscopic fluid slippage and adsorption on the pore surfaces, which give rise to variable slip length, viscosity ratio of adsorbed phase to bulk phase, and thickness of adsorption layer in organic & inorganic pore throats. In this study, a new pore network model is developed based on a modified shale oil flow equation to consider those combinational effects on shale oil permeability under different organic matter contents, and then is applied to provide an order analysis of those effects on the permeability of a representative shale model. Different flow patterns characterizing fluid-solid interaction are also discussed. Analysis results show that shale oil permeability is strongly influenced by the slip length. The effect of adsorption on permeability is negligible for cases considered. Shale oil flow is mainly controlled by inorganic pores when volumetric TOC is low. The influence of TOC on permeability depends on slippage and adsorption conditions in organic and inorganic matters, referred in this paper to as flow patterns. As the organic matter content increases, the connectivity of organic pores and throats improves, which further affects network permeability.

关键词： Shale oil Pore network model Slippage Adsorption effect Connectivity

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Effects of Flue Gas Recirculation on Combustion and Heat Flux Distribution in 660 Mw Double-Reheat Tower-Type Boiler

SSRN

引用

SSRN 2022年

作者： Deng, Lei Dong, Lingxiao Bai, Yang Wu, Yuhao Liu, Hu Belošević, Srdjan Tomanović, Ivan Che, Defu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an710049 China Guoshen Institute of Technology CHN ENERGY Xi'An710065 China Department of Thermal Engineering and Energy "VINČA" Institute of Nuclear Sciences National Institute of thе Republic of Serbia University of Belgrade Mike Petrovića Alasa 12-14 11351 Vinča PO Box 522 Belgrade11001 Serbia

The ultra-supercritical double-reheat boiler has attracted more attention because of high parameters, low pollution and large capacity. However, there are some difficulties in the development of this technology, such as adjusting the reheat steam temperature. In this study, computational fluid dynamics simulation is used to analyze a 660 MW double-reheat tower-type pulverized coal-fired boiler. The influence of flue gas recirculation (FGR) on heat transfer characteristics and combustion process in the furnace (including heating surfaces in the upper parts of the furnace) are evaluated. The user-defined function approach predicates CO reduction effect on NO x . The results show that the flow at the horizontal section through the centerline of recirculating flus gas nozzles is rotating. The velocity distribution changes into an elliptical rotating flow when FGR ratio is 20%. At higher FGR ratios, the high-temperature area (1565-1700 K) shrinks and both the NO x concentration at the low-temperature superheater outlet and oxygen concentration in the furnace descend. Oxygen concentration at low-temperature superheater outlet first increases and then decreases. In the main combustion zone, the heat flux peak of water-cooled wall is about 330 kW m -2 . As FGR ratio increases from 0% to 20%, the rate of water-cooled wall heat absorption to total boiler decreases by 3.50%. This rate for reheater and superheater increases by 2.53% and 2.13%, respectively. © 2022, The Authors. All rights reserved.

关键词： Temperature

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Numerical Investigations for the Pcm and Liquid Immersion Cooling Effects on Lithium Ion Battery Thermal Runaway Mitigation

SSRN

引用

SSRN 2023年

作者： Liu, Xinyu Zhou, Zhifu Wu, Wei-Tao Wei, Lei Wu, Weixiong Li, Yang Gao, Linsong Li, Yubai Song, Yongchen Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology Dalian116024 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China School of Mechanical Engineering Nanjing University of Science and Technology Nanjing210094 China Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen518055 China Energy and Electricity Research Center Jinan University Zhuhai519070 China

In this study, a three-dimensional (3D) thermal runaway (TR) model with conjugate heat transfer submodel is adopted. TR behaviors for a battery pack with 12 prismatic LIBs are then simulated. Three thermal safety measures of TR protection from internal shorting in Cell 1 to pack level configuration are compared and evaluated. Paraffin phase change material (PPCM) is firstly proposed to delay the TR propagation between LIBs with solid-liquid phase change as heat transfer mechanism. Different thicknesses of PPCMs are compared to verify the TR mitigation performance of the PPCM under thermal abuse condition. The TR time for the Cell 2 is delayed to be 64 s, 266 s and 414 corresponding to PPCM thickness of 1.8 mm, 3.6 mm and 5.4 mm. As the simulation results shows, this TR time can be further delayed to 798 s by a strategy with combing PPCM with insulation. In addition, this work proposes a novel thermal safety protection based on immersion cooling with pool boiling of fluorinated liquid as heat transfer mechanism. We observe that the average temperature of Cell 2 - Cell 12 tends to be within 34oC under immersive cooling condition, which indicates the possibility to prevent the TR. © 2023, The Authors. All rights reserved.

关键词： Lithium-ion batteries

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Corrigendum to ‘Numerical simulation on sonic steam jet condensation in subcooled water through a double-hole nozzle’ [Int. J. Heat Mass Transfer 115 (2017) 143–147]

引用

International Journal of Heat and Mass Transfer 2017年 115卷 1360-1360页

作者： Lutao Wang Daotong Chong Lun Zhou Weixiong Chen Junjie Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an 710049 PR China

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Experimental study on the submerged steam jet through side hole nozzle

引用

IOP Conference Series: Materials Science and engineering 2015年第1期88卷

作者： W Wang F Yuan Q B Zhao D T Chong W X Chen J J Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 PR China

In this paper, the steam shape parameters and the condensation oscillation characteristics of the direct contact condensation of submerged steam jet into subcooled water were investigated through a side hole nozzle. Meanwhile, the dimensionless jet length and the expansion ratio versus pool water temperature and steam mass flux were obtained by measuring the photographs taken by a high speed camera. Both of them increased gradually with rise of pool water temperature and steam mass flux. A comparison of the shape parameters of three different style nozzles was also achieved. And a correlation of the dimensionless jet length was obtained, the predicted data agreed well with the experimental data, while the discrepancy was within ±5%. For the pressure oscillation versus steam mass flux, the peaks and the root mean square value of pressure oscillation were almost consistent in the range of 150-400 kgm-2s-1, while both of them increase in the range of 400-800 kgm-2s-1. The positive peak and negative peak were completely symmetrical.

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Experimental Study on Deliquification with Atomizing Nozzle in Gas Well

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IOP Conference Series: Earth and Environmental Science 2020年第1期555卷

作者： Yutang Gao Xiaobai Li Peng Chang Lei Liu State Key Laboratory of Multiphase Flow in Power Engineering Xi'an 710049 Shaanxi P.R. China

Gas is a clean energy resource in comparison with oil and coal. Liquid-loading problem is frequently encountered in the process of gas production. It would directly cause the production of gas wells decreasing, even off production. A number of deliquification techniques have been suggested for solving this kind of problem, but the available techniques are not yet widely applicable. Based on the analysis, the method of deliquification with atomizing nozzle in gas wells was put forward. The test bench was designed for studying the atomization of nozzles and the liquid entrainment of gas flow. The size distribution of atomized droplets was measured by Malvern laser grain size analyzer. The Sauter mean diameters of atomized droplets were analysed under different two-phase flow conditions. The results indicate that the designed nozzles have good atomization performances and show potential application for reducing liquid loading in gas wells.

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Experimental investigations on flow instabilities in a forced circulation loop at near-critical and supercritical pressures

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AIP Conference Proceedings 2013年第1期1547卷

作者： Lei Zhang Haijun Wang Hongfang Gu Shouxu Qiao Xiaobao Shi Yushan Luo State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiao tong University Xi'an 710049 China

Properties of supercritical water will undergo drastic changes near the "pseudo critical" point which gives rise to a serious concern about flow instabilities under supercritical conditions. To investigate the fluid flow behaviors, experiments with different system pressures (near-critical and supercritical pressure) were conducted on the Xi'an Jiao tong University's (XJTU) supercritical water test facility. Large amplitudes of mass flow flux as well as inlet pressure were found in various operation conditions. Mechanism of this unusual flow instability behavior is discussed. The oscillation behavior occurring in the present work has also been compared with that under the subcritical pressures and parameters effects are also studied.

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Research on condensation of n-octane/n-nonane in throttling flow

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Kung Cheng Je Wu Li Hsueh Pao/Journal of engineering Thermophysics 2011年第SUPPL. 1期32卷 150-153页

作者： Lü, Xiao-Fei Liu, Hai Li, Ming-Sheng Chang, Chun Bai, Bo-Feng State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China First Gas Production Factory Xinjiang Oil field Company Karamay 834000 China

A numerical model was developed to simulate the condensation flow of the n-octane/n-nonane in three dimension throttle. With this model the condensation properties of n-octane/n-nonane in throttle were investigated, it was found that the maximum supersaturation ratio of n-octane/n-nonane vapor in the homogeneous condensation process was very high, in comparison n-nonane was harder to condense. The influence of inlet supersaturation ratio, total pressure and total temperature on the condensation of n-nonanein in throttling flow process was analyzed. From the results, the direct influences of inlet parameters were found on the wilson point location, average droplet radius and liquid phase mass fraction.

关键词： Condensation

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