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Realization of Multilocal Gradient-Doping Pcn by Alkali Metal Ion Sustained Release Capsules for Enhanced Photocatalytic Water Splitting

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SSRN 2023年

作者： Yan, Jiawei Fang, Fenjian Wei, Zhidong Chi, Jiasheng Chen, Mingxia Jiang, Zhi Jiang, Kun Shen, Shaohua Shangguan, Wenfeng Research Center for Combustion and Environment Technology Shanghai Jiao Tong University Shanghai200240 China College of Smart Energy Shanghai Jiao Tong University Shanghai200240 China College of Electrical Energy and Power Engineering Institute of Fuel Cells Shanghai Jiao Tong University Shanghai200240 China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China

The gradient-doping technique has been widely applied to induce an oriented built-in electric-field. However, it is still not efficient enough for charge mobility especially for particulate semiconductors, as the field is primarily in one direction from inner to surface. Here, we propose a multilocal gradient-doping technique that a nano-capsule is designed to store dopants and then release them into semiconductors nonuniformly. As an illustration, scattered pyrochlore-type K2Ta2O6 nanoparticles have been validated the capability of storing and releasing K+, which subsequently diffuse into the substrate PCN. Multi point-radiative gradient in K+ concentration, confined within the K2Ta2O6’s vicinity, will construct several 3D potential wells which can not only accelerate the carrier separation but also offer more migration channels for both photo-induced electrons and holes to the surface. Consequently, the multilocal K+ gradient-doping PCN shows the longest carriers’ lifetime and highest AQY (~21.8% at 400 nm) compared with the other uniformly doping techniques. © 2023, The Authors. All rights reserved.

关键词： Charge transfer

Effect of Channel Structure on the Thermal-Hydrodynamic Characteristics of Micro-Oscillating Heat Pipes

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SSRN 2022年

作者： Sun, Qin Qu, Jian School of Energy and Power Engineering Jiangsu University Zhenjiang212013 China Jiangsu Key Laboratory of Micro and Nano Heat Fluid Flow Technology and Energy Application Suzhou University of Science and Technology Suzhou215011 China

Simultaneous visualization and temperature measurement experiments were conducted to investigate the effect of cross-section structure on the thermo-hydrodynamic characteristics of two silicon-based micro-oscillating heat pipes, one having expanding channels (micro-OHPEC) and another having straight channels (micro-OHPSC). The hydraulic diameter of each parallel straight channel was 332.4 μm, while the diameters at the two ends of each expanding channel were about 364.4 and 287.0 μm, respectively. R141b was used as the working fluid at a volumetric filling-ratio of 50%. Fluid oscillatory motions, including small oscillation/stop-over (S-O), large oscillation (L-O) and bulk oscillation (B-O), were observed in these two micro-devices accompanied by bubbly flow, slug flow and annular/semi-annular flow. Compared with the micro-OHPSC, which exhibited a longer period of S-O motions, the micro-OHPEC was endowed with better thermal performance owing to the longer durations of L-O/B-O motions. The thermal resistance of the micro-OHPEC was reduced by about 26.8% in comparison with that of the micro-OHPSC at a heating power of about 6.3 W. As a simple and effective design strategy, expanding channel design can significantly increase the capillary driving force and intensify bubble nucleation within the micro-OHP, contributing to device performance enhancement. © 2022, The Authors. All rights reserved.

关键词： flow patterns

Liquid mean velocity and turbulence in a horizontal air-water bubbly flow

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Nuclear Science and Techniques 2003年第2期000卷

作者： YANG Jian ZHANG Ming-Yuan ZHANG Chao-Jie SU Yu-Liang The State Key Lab of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049

The liquid phase turbulent structure of an air-water bubbly horizontal flow in a circular pipe has been investigated experimentally. Three-dimensional measurements were implemented with two "X" type probes oriented in different planes, and local liquid-phase velocities and turbulent stresses were simultaneously obtained. Systematic measurements were conducted covering a range of local void fraction from 0 to 11.7%. The important experiment results and parametric trends are summarized and discussed.

关键词： Air-water bubbly flow Hot-film anemometry Liquid velocity Turbulence

Measurement of falling film thickness around a horizontal tube using laser-induced fluorescence technique

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Journal of Physics: Conference Series 2009年第1期147卷

作者： Xiaofei Wang Maogang He Hualiang Fan Ying Zhang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 People's Republic of China

An optical method for the non-intrusive measurement of falling film thickness on the perimeter of the horizontal tube is described. This non-intrusive measurement method is based on the visualization of the falling film flowing around the horizontal tube and uses the laser induced fluorescence and image processing techniques. The falling film thickness around a Turbo-CII horizontal tube and a plain horizontal tube was measured when water flushed the tube vertically with a stable velocity. The results for the Turbo-CII tube are compared with those for the plain tube, and show that the film thickness around the Turbo-CII tube varies with the same trend as that around the plain tube, and the minimal values of the film thickness tend to locate at different angular position of 95°-120° under different conditions. The film thickness around the enhanced tube changes within a smaller range with time than that around the plain tube. The corresponding effects on flow uniformity have also been discussed.

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Numerical study on the influence of plugging rate on the performance of adjustable steam ejector

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International Journal of Fluid Engineering

International Journal of Fluid engineering 2024年第2期1卷 50-60页

作者： Jianxiang Gao Zepeng Yuan Yuyan Hou Weixiong Chen State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049People’s Republic of China

During the operation of thermal power plant systems, severe challenges to the quality and safety of the heat supply arise owing to the effects of peak regulation. Steam ejectors, widely employed in the district heating sector, often exhibit poorer performance under off-design conditions as a result of their fixed structure. This study analyzes the effects of varying plugging rate, primary pressure, and induced pressure on the performance of adjustable steam ejectors. As the plugging rate increases, the mass flow rate of the primary fluid decrease, potentially falling below 32%, and that of the induced fluid initially experiences a minor increase, followed by a rapid decrease. Concurrently, the critical back pressure also decreases with an increase in the plugging rate, potentially falling by up to 65%. By contrast, the entrainment ratio surges with increasing plugging rate, with the maximum increase reaching up to 4.75 times. Under the same primary steam pressure and induced steam pressure, there exists an optimal entrainment ratio. Furthermore, both the critical back pressure and the optimal entrainment ratio increase as the primary steam pressure and induced steam pressure increase.

关键词： performance steam optimal

Strengthening Chlorobenzene Catalytic Degradation Rate and Selectivity Over Laxsr1-Xmno3±Δ by Anchoring Interfacial Oxygen Vacancy

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SSRN 2022年

作者： Li, Lu Tao, Dan Zhao, Qi Fu, Shuangshuang Min, Xin Chen, Changwei Tian, Mingjiao Shi, Jianwen He, Chi State Key Laboratory of Electrical Insulation and Power Equipment Center of Nanomaterials for Renewable Energy School of Electrical Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China College of Geology and Environment Xi’an University of Science and Technology Shaanxi Xi’an710054 China Faculty of Electronic and Information Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China School of Environmental and Municipal Engineering Xi’an University of Architecture and Technology Shaanxi Xi’an710055 China School of Environmental Science and Engineering Shanghai Jiao Tong University 800 Dongchuan Road Shanghai200240 China

Surficial lattice oxygen in perovskite compounds is a common participant during chloroaromatic catalytic destruction. Herein, we proposed a facile oxygen vacancy construction strategy for preparing high active LaxSr1-xMnO3±δ (LSMO) via NaBH4 treatment. Results reveal that LSMO composites are not only reduced by NaBH4 under mild condition, but trigger a significant Sr segregation effect, which plays a key role in oxygen vacancy formation accounting to the electron donation from Sr to Mn acceptor and subsequent lattice oxygen activation. Moreover, the concentration of interfacial active oxygen species can be regulated by taming the La-Sr interaction with different Sr substitution proportions. The anchored oxygen vacancies (OVs) take advantage of electron capture or transfer and induce molecule oxygen into active oxygen species to react with chlorobenzene molecules, resulting in a preferential catalytic oxidation capacity. Amongst, reduced La0.5Sr0.5MnO3±δ catalyst displays superior chlorobenzene destruction efficiency with 90% of which converted as low as 236 °C, which also exhibited a stable performance in long-time operation. However, the OVs would be refilled by water H2O molecules resulting in a weaker water resistance for OVs anchored catalyst. In summary, the annihilation of OVs is the most important factor for catalyst deactivation. The research offers a new avenue to construct interfacial oxygen species in perovskite oxides during the chlorobenzene deep oxidation process. © 2022, The Authors. All rights reserved.

关键词： Catalytic oxidation

Corrosion Behavior of Low Carbon 9cr-Ods Steel in High Temperature Oxygen-Saturated Lead-Bismuth Eutectic

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SSRN 2024年

作者： Yang, Chongdou Xu, Yuwen Yun, Di Zhao, Bingyao Liu, Wenguan Gao, Rui Xie, Shijing Qiu, Jie School of Nuclear Science and Technology Xi’an Jiaotong University Xi’an710049 China State Key Laboratory of Multiphase Flow Xi’an Jiaotong University Xi’an710049 China Sino-French Institute of Nuclear Engineering and Technology Sun Yat-Sen University Zhuhai519082 China

The corrosion behavior of low-carbon 9Cr-ODS steel were carried out in oxygen saturated LBE. It was found that the thickness of the oxide film increased with increasing corrosion time, but the growth rate gradually slows down with increasing time. TEM and XRD results show that the main structure of the oxide layer formed on 9Cr-ODS steel is multilayered structure, consist of an (Fe,Cr)3O4 spinel inner layer, mixed with some nano precipites FeCr2O4, Cr3O4, Mn3O4 and morphous at the grain boundaries, nanocrystal transition layer and a Fe3O4 outer layer. The corrosion mechanism of 9Cr-ODS steel in liquid LBE is discussed. © 2024, The Authors. All rights reserved.

关键词： Manganese oxide

Corrigendum to “Multi-scale coupling analysis of the flow blockage accident in the typical LFR” [Int. J. Therm. Sci., 195, January 2024, 108615]

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International Journal of Thermal Sciences 2024年 204卷

作者： Hanrui Qiu Mingjun Wang Jing Zhang Wenxi Tian G.H. Su State Key Laboratory of Multiphase Flow in Power Engineering School of Nuclear Science and Technology Xi'an Jiaotong University Xi'an 710049 China

Research on droplets growth of Marangoni condensation during the time-series process

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Journal of Physics: Conference Series 2017年第1期925卷

作者： Y Li J Wang K Xia N Chen J Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'lan 710049 P.R. China

In this paper, the condensate droplets growth of Marangoni condensation during the time-series process was experimentally studied. The photographs taken in the experiments were handled by image processing method. The droplets coverage ratio was introduced to analyse the growth process. As the time-series process went on, the condensate droplets coverage ratio increased fast at first, and then increased slowly until reaching a stable state. The droplets coverage ratio increased with the increase in the vapor-to-surface temperature difference and decreased with the increase in the ethanol vapor concentration.

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