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Pore-scale modelling on hydrogen transport in porous media: Implications for hydrogen storage in saline aquifers

International Journal of Hydrogen Energy 2023年第37期48卷 13922-13933页

作者： Jinlei Wang Yongfei Yang Shaobin Cai Jun Yao Quan Xie Key Laboratory of Unconventional Oil & Gas Development (China University of Petroleum (East China)) Ministry of Education Qingdao 266580 PR China Research Center of Multiphase Flow in Porous Media School of Petroleum Engineering China University of Petroleum (East China) Qingdao 266580 PR China WA School of Mines: Minerals Energy and Chemical Engineering Curtin University 26 Dick Perry Avenue 6151 Kensington Western Australia Australia

Hydrogen energy has tremendous potential as a clean fuel in this energy transition. To build up the full-scale hydrogen energy supply chain, large-scale hydrogen storage is of vital importance. Underground hydrogen storage in saline aquifers has been perceived as an important means to achieve large-scale hydrogen storage. Therefore, we investigated hydrogen transport in pore network in a sandstone porous media at strongly water-wet and weakly water-wet (hydrogen-wet). We performed direct numerical simulation through volume of fluid method to investigate the transport of hydrogen at pore-scale under different wetting conditions with input hydrogen-rock physics data from literature. Our results showed that during primary drainage process (hydrogen injection for storage purpose), increasing hydrogen wetting decreased snap-off effect, enabling a greater pore space for hydrogen storage. During primary imbibition process (hydrogen extraction), increasing hydrogen wetting promoted the size and stability of hydrogen clusters, which is unfavorable to hydrogen extraction process. Given the significant high interfacial tension between brine and hydrogen and low viscous force of hydrogen, snap-off effect dominates the flow in both hydrogen injection and extraction process regardless of wetting conditions. This physical process causes the recovery factor even below 20%. We therefore suggest that storing hydrogen in depleted gas reservoirs under irreducible water saturation would have much less risks in hydrogen trapping during extraction process.

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Theoretical investigation on heat-electricity decoupling technology of low-pressure steam turbine renovation for CHPs

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IOP Conference Series: Earth and Environmental Science 2019年第4期227卷

作者： Qingbo Hu Kun Wang Li Zhang Liansheng Zhou Rong Chen Shan Wang Yu Zhang Guohao Li Tianjin Electric Power Science & Research Institute Tianjin 300384 State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiao Tong University Xi'an 710049.

The power grid peaking capacity is insufficient due to the increasing installed capacity of renewable power. Moreover, it is also restricted by the operation mode of combined heat and power units (CHPs), the minimum electricity loads of which are determined by the heat load. It is significant to study the heat-electricity decoupling technologies for CHPs. Therefore, the low-pressure steam turbine renovation technology is studied in this paper with a 300MW unit as reference case. Results show that the minimum electric load rate and the coal consumption are decreased, and the heat-electricity ratio is increased significantly for CHP with low-pressure steam turbine renovation. When the heat load is 1200 GJ/h, the minimum electric load rate and coal consumption with low-pressure steam turbine renovation can be reduced by 32.4 and 30.9 % respectively. The heat-electricity ratio can be increased by 68.8 % after renovation of low-pressure steam turbine.

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Current Density Regulating Lithium Metal Directional Deposition for Long Cycle Life Lithium Metal Batteries

SSRN

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SSRN 2020年

作者： Mao, Heng Yu, Wei Cai, Zhuanyun Liu, Guixian Liu, Limin Wen, Rui Su, Yaqiong Xi, Kai Li, Benqiang Da, Xinyu Kou, Huari Yan, Wei Ding, Shujiang Xi'an Key Laboratory of Sustainable Energy Materials Chemistry School of Chemistry Xi’an Jiaotong University & Shaanxi Quantong Joint Research Institute of New Energy Vehicles Power Xi’an Jiaotong University Xi’an710049 China State Key Laboratory of Physical Chemistry of Solid Surfaces Department of Chemistry College of Chemistry and Chemical Engineering Xiamen University Xiamen361005 China Key Laboratory of Molecular Nanostructure and Nanotechnology Beijing National Laboratory for Molecular Sciences CAS Research/Education Center for Excellence in Molecular Sciences Institute of Chemistry Chinese Academy of Sciences Beijing100190 China Cambridge Graphene Centre Department of Engineering University of Cambridge CambridgeCB3 0FA United Kingdom Department of Mechanical Engineering University of Michigan-Dearborn DearbornMI48128 United States Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

Uncontrolled dendrite formation in the high energy density of lithium metal batteries (LMBs) may pose serious safety risks. Numerous works have been reported to protect separator. However, these methods still couldn’t inhibit the dendrite upward growth to protect the separator, effectively. Here, we introduce a novel “orientated-growth” strategy that makes the depositional interface transfer to the anode/current collector interface from the anode/separator interface. We placed a layer of cellulose/graphene carbon composite aerogel (CCA) between the current collector and the anode (CCA-Li). This layer works as the charge organizer;it induces a higher current density distribution and makes Li prefer to deposit in the bottom CCA layer of CCA-Li electrode. Both in-situ and ex-situ images of the electrode demonstrate the anode part of the cell has been flipped;with the new deposited particles facing the current collector and smooth surface facing the separator. Electrochemical characterization of the electrode in half and full cells showed outstanding cyclic stability and rate capability, with the CCA-Li/LPF full cell able to maintain 94% of its initial capacity after 1000 cycles. We believe that the innovative strategy would promote the leapfrog development for LMBs. © 2020, The Authors. All rights reserved.

关键词： Electric current collectors

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Boosted Photocatalytic Co2 Reduction by Induced Electromotive Force in Rotating Magnetic Field

SSRN

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SSRN 2023年

作者： Lu, Danchen Ren, Yuqi Yang, Ya Cheng, Miao Wang, Ke Wang, Nan Liu, Maochang Zhou, Jiancheng Chen, Wenshuai Li, Naixu School of Chemistry and Chemical Engineering Southeast University No.2 Dongnandaxue Road Jiangsu Nanjing211189 China CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and Sensor Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of Sciences Beijing101400 China Key Laboratory of Bio-Based Material Science and Technology Ministry of Education Northeast Forestry University No. 26 Hexing Road Harbin150040 China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University No.28 Xianning West Road Shaanxi Xi'An710049 China

Charge separation plays a crucial role in semiconductor-based photocatalytic CO2 conversion. Herein, we report a unique induced electric field, which can actively manipulate carrier behavior at the minuscule, leading to significantly boosted photocatalytic CO2 reduction in H2O vapor. The success relies on the development a monolithic photocatalyst made of a copper foam substrate and nanosized ZnO/NiO/Au heterostructures that can effectively couple a special rotating magnetic field (RMF). Specifically, the copper foam cuts the magnetic induction line, leading to the periodic generation of induced electric field. This induced electric field could significantly increase the carriers' density by preventing their recombination. Moreover, NiO and Au as the active sites for oxidation and reduction, respective, synergistically magnify this effect. As a result, compared with the photocatalytic reaction without adding RMF, the utilization rate of photogenerated electrons increases by 5.24 times after coupling RMF, with the yield of CO and CH4 improved by 5.50 times and 5.18 times. This strategy by integrating unique RMF into the reaction system provides new insights for improving photocatalytic CO2 conversion. © 2023, The Authors. All rights reserved.

关键词： Carbon dioxide

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Quantitative Statistical Evaluation of Micro Residual Oil after Polymer Flooding Based on X-ray Micro Computed-Tomography Scanning

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Energy & Fuels 2020年第9期34卷 10762-10772页

作者： Yongfei Yang Liu Tao Stefan Iglauer S. Hossein Hejazi Jun Yao Wenjie Zhang Kai Zhang Key Laboratory of Unconventional Oil & Gas Development China University of Petroleum (East China) Ministry of Education Qingdao 266580 People’s Republic of China Research Center of Multiphase Flow in Porous Media School of Petroleum Engineering China University of Petroleum (East China) Qingdao 266580 People’s Republic of China Petroleum Engineering School of Engineering Edith Cowan University Joondalup 6027 Western Australia Australia Porous Media Laboratory Department of Chemical and Petroleum Engineering University of Calgary Calgary Alberta Canada T2N 1N4

Polymer flooding is an important tertiary recovery method. However, even after its application, more than 50% of the oil remains in the formation layers. It is thus important for efficient resource use that both residual oil distribution and the mechanisms associated with polymer flooding are better understood. In the work described in this paper, a series of in situ X-ray tomography experiments were carried out, and different displacement stages were imaged. Then, rock, water, oil, and polymer were identified in the imagery and quantified, while interchanges among the different types of residual oil, and their associated microscopic polymer displacement mechanisms, were discussed. We also studied the impact of permeability on polymer flooding efficiency, and our results showed that polymer flooding could mobilize residual oil that was not accessible via water flooding. Mechanistically, the polymer flood caused the big continuous residual oil clusters to split, dispersing them into smaller clusters. The polymer also changed fluid flow pathways, thus increasing sweep efficiency, while its viscoelasticity was helpful for recovering singlet and film residual types of oil. We found that the polymer could only drive oil locally, and that a large amount of residual oil remained in the middle of the core. We also noted that polymer flooding was more effective for higher permeability samples, which showed that, after polymer flooding, the recovery rate for the samples with permeabilities of 3989, 1543, and 814 millidarcys (mD) were enhanced by 10.13, 6.30, and 4.34%, respectively. Higher permeability samples remained as network-type and multiple-type residual oils after polymer flooding, while samples with lower permeability showed multiple-type and singlet-type residual oils. Thus, our results and conclusions showed that different enhanced oil recovery methods could be applied for further development.

关键词： Saturation Lipids Cluster chemistry Permeability Polymers

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Corrigendum to “Huge wave and drop entrainment mechanism in gas–liquid churn flow” [Chem. Eng. Sci. 108 (2013) 638–646]

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Chemical engineering Science 2017年 158卷 624-624页

作者： Ke Wang Bofeng Bai Weimin Ma State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi 710049 China Royal Institute of Technology (KTH) Stockholm 10691 Sweden

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Erosion of water-based fracturing fluid containing particles in a sudden contraction of horizontal pipe

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Journal of Physics: Conference Series 2017年第1期916卷

作者： Jiarui Cheng Yinping Cao Yihua Dou Zhen Li State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China. Department of Mechanical Engineering Xi'an Shiyou University Xi'an China.

A lab experiment was carried out to study the effects of pipe flow rate, particle concentration and pipe inner diameter ratio on proppant erosion of the reducing wall in hydraulic fracturing. The results show that the erosion rate and erosion distribution are different not only in radial direction but also in circumferential direction of the sample. The upper part of sample always has a minimum erosion rate and erosion area. Besides, the erosion rate of reducing wall is most affected by fluid flow velocity, and the erosion area is most sensitive to the change in the diameter ratio. Meanwhile, the erosion rate of reducing wall in crosslinked fracturing fluid is mainly determined by the fluid flowing state due to the high viscosity of the liquid. In general, the increase in flow velocity and diameter ratio not only cause the expansion of erosion-affected flow region in sudden contraction section, but also lead to more particles impact the wall.

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Numerical Study of Percolation and Seepage Behaviors in Ion-Adsorption-Type Rare Earth Ore Leaching Process

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Mathematical Problems in engineering 2023年第1期2023卷

作者： Dianyu, E. Su, Zhongfang Zeng, Jia Yang, Liuyimei Li, Jing Xu, Qiang Wang, Lin Cui, Jiaxin Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science and Technology Nanchang330013 China International Institute for Innovation Jiangxi University of Science and Technology Nanchang330013 China Ganjiang Innovation Academy Chinese Academy of Sciences Ganzhou341000 China ARC Research Hub for Computational Particle Technology Department of Chemical and Biological Engineering Monash University ClaytonVIC3800 Australia State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an710049 China Delft University of Technology Delft Netherlands

Ionic rare earth ore is a type of featured rare earth ore in China. Its mining process suffers from a long leaching cycle and considerable consumption of leaching agents. Improving mining efficiency requires a sound physical understanding of the leaching process. In this study, the CFD-based numerical model is used to analyze the physical process of leaching through porous media formed by particles. The simulation results indicate that a lower packing porosity and smaller particles packed granular porous medium result in much larger energy dissipation during seepage, and the energy dissipation increases with seepage velocity. It is found that when the seepage velocity increases to a certain high value, the energy dissipation exceeds the value predicted by Darcy's law, which is mainly caused by liquid turbulence. Additionally, the effect of particle shape is examined. The results show that the granular medium composed of prolate particles causes larger energy dissipation than oblate particles, and spherical particles play the least role. This phenomenon may result from the particle shape affecting the area of the frontal contact surface between particles and liquid. The results provide new insights into the fundamental understanding of percolation and seepage behaviors in the ion-adsorption-type rare earth ore leaching process. © 2023 E. Dianyu et al.

关键词： Energy dissipation

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聚丙烯酸酯修饰铜电极用于电化学二氧化碳还原选择性生成多碳产物（英文）

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Science Bulletin 2024年第15期 2395-2404页

作者：石玉川张凯妮董崇礼 Ta Thi Thuy Nga 汪淼魏代星王佳琳王亦清沈少华 International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Department of Physics Tamkang University

Highly selective production of value-added multicarbon(C2+) products via electrochemical CO2reduction reaction（eCO2RR） on polycrystalline copper（Cu） remains ***,the facile surface modification using poly（α-ethyl cyanoacrylate）(PECA) is presented to greatly enhance the C2+selectivity for eCO2RR over polycrystalline Cu,with Faradaic efficiency（FE） towards C2+products increased from30.1% for the Cu electrode to 72.6% for the obtained Cu-PECA electrode at -1.1 V *** hydrogen electrode（RHE）.Given the well-determined FEs towards C2+products,the partial current densities for C2+production could be estimated to be-145.4 mA cm-2for the Cu-PECA electrode at -0.9 V *** in a homemade flow ***-situ spectral characterizations and theoretical calculations reveal that PECA featured with electron-accepting-C≡N and-COOR groups decorated onto the Cu electrode could inhibit the adsorption of *H intermediates and stabilize the *CO intermediates,given the redistributed interfacial electron density and the raised energy level of d-band center（Ed） of Cu active sites,thus facilitating the C-C coupling and then the C2+selective *** study is believed to be guidable to the modification of electrocatalysts and electrodes with polymers to steer the surface adsorption behaviors of reaction intermediates to realize practical eCO2RR towards value-added C2+products with high activity and selectivity.

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Activated Overall Water Splitting Over a Ni-Fe Layered Double Hydroxide Electrocatalyst by V Doping and Sulfuration

SSRN

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SSRN 2023年

作者： Wu, Wentong Peng, Lei Min, Boya Huang, Jie Liu, Saiya Lu, Kejian Lu, Shijian Jing, Dengwei Zheng, Mingsheng Liu, Maochang International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China No. 8 Oil Production Plant of PetroChina Changqing Oilfield Company Shaanxi Xi’an710016 China Carbon Neutrality Institute Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization China University of Mining and Technology Jiangsu Xuzhou221008 China Gree Altairnano New Energy Inc Zhuhai519040 China School of Chemistry and Biological Engineering University of Science and Technology Beijing Beijing100083 China

Ni-Fe layered double hydroxide (NiFe-LDH) is regarded as one of the promising non-noble electrocatalyst. However, the limited number of active sites and poor electrical conductivity impede its further development. Herein, we report the synthesis of a Ni foam supported NiFe-LDH electrocatalyst modified by V doping and vulcanization (NiFeV-S/NF). This modification endows the catalyst excellent property toward hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and overall water splitting. Only 211 mV and 127 mV of the overpotentials are required to achieve the current density of 10 mA cm-2 for OER and HER in 1 M KOH electrolyte, respectively. Particularly, the prepared NiFeV-S/NF could serve as a bifunctional electrocatalyst for overall water splitting, with a cell voltage of 1.573 V to reach a current density of 10 mA cm-2. In principle, the success relies on the intrinsically improved conductivity, increased specific surface area and the number of active sites, as well as the heterojunction structure of the catalyst. Therefore, this work provides a new idea for the design and preparation of more efficient noble-metal-free bifunctional electrocatalysts. © 2023, The Authors. All rights reserved.

关键词： Electrocatalysts

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