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A probability theory for filtered ghost imaging

Chinese Physics B 2023年第4期32卷 329-337页

作者：刘忠源孟少英陈希浩 Key Laboratory of Optoelectronic Devices and Detection Technology College of PhysicsLiaoning UniversityShenyang 110036China

Based on probability density functions,we present a theoretical model to explain filtered ghost imaging(FGI)we first proposed and experimentally demonstrated in 2017[***.425290(2017)].An analytic expression for the joint intensity probability density functions of filtered random speckle fields is derived according to their probability ***,the normalized second-order intensity correlation functions are calculated for the three cases of low-pass,bandpass and high-pass filterings to study the resolution and visibility in the FGI *** simulations show that the resolution and visibility predicted by our model agree well with the experimental results,which also explains why FGI can achieve a super-resolution image and better visibility than traditional ghost imaging.

关键词： ltered ghost imaging probability density function super-resolution

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Resolution-enhanced single-pixel imaging using the Hadamard transform matrix

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Chinese Physics B 2023年第12期32卷 652-656页

作者：别书航王晨晖吕瑞兵鲍倩倩付强孟少英陈希浩 Key Laboratory of Optoelectronic Devices and Detection Technology College of PhysicsLiaoning UniversityShenyang 110036China

We propose a single-pixel imaging(SPI)method to achieve a higher-resolution image via the Hadamard transform *** traditional SPI schemes,this new method recovers images by correlating single-pixel signals with synchronized transformed patterns of Hadamard bases that are actually projected onto the digital micromirror *** transform pattern is obtained through the inverse Fourier transform of the pattern acquired by Gaussian filtering of each Hadamard basis in the frequency *** proposed scheme is based on a typical SPI experimental setup and does not add any hardware complexity,enabling the transformation of Hadamard matrices and image reconstruction through data processing ***,this approach could be considered as an alternative option for achieving fast SPI in a diffraction-limited imaging system,without the need for additional hardware.

关键词： single-pixel imaging Gaussian filtering resolution enhancement

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Advanced porous thermoelectric materials:Design,construction,and application

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Nano Research 2025年第4期18卷 469-492页

作者： Ruoyan Li Bangzhi Ge Chongjian Zhou State Key Laboratory of Solidification Processing and Key Laboratory of Radiation Detection Materials and Devices Ministry of Industry and Information TechnologyNorthwestern Polytechnical UniversityXi’an 710072China

Thermoelectric(TE)technology,capable of converting heat directly into electricity,holds great promise for applications requiring efficient energy output,such as wearable devices and aerospace ***,the widespread use of traditional TE materials is limited by challenges such as high density,brittleness,and coupling of thermoelectric *** TE materials offer a potential solution by enabling lightweight,enhancing mechanical flexibility,and reducing thermal conductivity by rational design and precise control of the pore *** review examined recent advances in the construction of optimized pore structures,including the size,distribution,and *** summarized the state-of-the-art synthesis and classification for porous TE materials,highlighting methods for tuning pore configurations to enhance TE ***,we also collected the cutting-edge device ensemble strategies and demonstrated their application such as aerospace,temperature management,and medical ***,we took an outlook on the rational and intelligent design of pore structures and their integration into systems for energy *** review provides new understanding of mechanisms and designs for porous TEs,and also offers valuable guidance for the development of next-generation materials and their application in innovative self-powered systems.

关键词： thermoelectric pores synthesis methods mechanical properties applications

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A low-cost wide bandgap polymer based on carboxylate substituted thiazole enables efficient organic solar cells with remarkable batch-to-batch reproducibility

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Science China Chemistry 2025年第2期68卷 733-744页

作者： Xiaodong Zhu Yuchen Lei Jianhong Gao Yanjun He Jinsicheng Liu Qian Guo Xiang Gao Liwei Xiong Xunchang Wang Renqiang Yang Zhitian Liu Hubei Engineering Technology Research Center of Optoelectronic and New Energy Materials Hubei Key Laboratory of Plasma Chemistry and Advanced MaterialsSchool of Materials Science and EngineeringWuhan Institute of TechnologyWuhan 430205China Key Laboratory of Optoelectronic Chemical Materials and Devices(Ministry of Education) School of Optoelectronic Materials&TechnologyJianghan UniversityWuhan 430056China

Constructing the low-cost,high-efficiency,and good batch-to-batch reproducibility polymer donor is vitally important for the application of organic solar ***,we develop a structurally simple carboxylate-substituted thiazole as an electronwithdrawing building block to construct a low-cost polymer,PBTTzE,containing a facilely prepared chlorinated benzo[1,2-b:4,5-b′]dithiophene(BDTCl)donor *** from synergistic electron deficient effects of chlorination and ester group and C=N,as well as the noncovalent interaction of S…O and S…N,PBTTzE exhibits a deep HOMO energy level(−5.59 eV),and a planar skeleton *** combined with the IT-4F acceptor,the polymer(54 kDa)demonstrated a champion PCE of 15.87%,which is the highest value in the IT-4F-based binary devices to ***,PBTTzE exhibits excellent batch-tobatch reproducibility due to its very similar PCEs within a range of 43–76 *** addition,an alloyed state and complementary absorption can be formed between PM6 and ***,in a ternary device with PBTTzE added to the PM6:BTP-eC9 blend,a top PCE of 18.76%is achieved due to the suppressed energy loss,prolonged exciton diffusion distance,and improved charge *** work demonstrates that the carboxylate-substituted thiazole is a highly promising acceptor unit for constructing low-cost and high-performance polymers.

关键词： carboxylate substituted thiazole polymer donor low-cost batch-to-batch reproducibility organic solar cells

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Infrared image super-resolution reconstruction based on residual fast fourier transform

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Multimedia Tools and Applications 2025年第9期84卷 6805-6823页

作者： Li, Xianguo Liu, Rui Yang, Yanli School of Electronics and Information Engineering Tiangong University Tianjin China Tianjin Key Laboratory of Optoelectronic Detection Technology and System Tianjin China

Infrared images have been widely used in military, civilian, and industrial fields. Due to the inherent limitations of sensors, infrared images usually have some disadvantages such as low resolution and blurred texture details. How to improve the resolution of infrared images without changing hardware devices has become a current research hotspot. Aiming at the problem that the existing infrared image super-resolution reconstruction methods do not utilize the image details sufficiently, this paper proposes an infrared image super-resolution reconstruction algorithm based on residual fast fourier transform(ISRRFT). The image features are extracted in both spatial domain and frequency domain, so as to fully extract the high-frequency and low-frequency information components of infrared images and improve the quality of reconstructed infrared images In addition, the learnable fast fourier transform loss function has been introduced, which is used in conjunction with the L1 loss function to calculate the loss from both the spatial and frequency domains, thus better optimizing the model parameters. The test results on three test sets, SR1280, IRData and Infrared20, show that the proposed algorithm has an optimal performance in terms of both objective and subjective evaluation metrics compared to current representative algorithms. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2024.

关键词： Image reconstruction

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Heptagonal intramolecular-lock strategy enables high-performance thermally activated delayed fluorescence emitters

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Science China Chemistry 2024年第4期67卷 1181-1186页

作者： Zhenmei Huang Dezhi Yang Dongge Ma Zhengyang Bin Jingsong You Key Laboratory of Green Chemistry and Technology of Ministry of Education College of ChemistrySichuan UniversityChengdu 610064China Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and DevicesSouth China University of TechnologyGuangzhou 510640China

The development of highly efficient thermally activated delayed fluorescence(TADF)emitters is persistently pursued for the application of organic light-emitting diodes(OLED)in full-colour display and solid-state ***,we present a heptagonal intramolecular-lock strategy to design high-performance TADF *** a proof-of-concept,a new type of tribenzotropone(TBP)acceptor has been designed and synthesized by a cascade decarboxylative cyclization of aryl oxoacetic acid derivative with biphenyl boronic *** with the unlocked benzophenone(BP)acceptor,the TBP acceptor has a highly twisted heptagonal geometry with moderate rigidity and flexibility,which enables a high-performance TADF emitter with a small single-triplet energy gap(ΔE_(ST))of 0.04 e V,a high photoluminescence quantum yield(Φ_(PL))of 99% and a large horizontal orientation factor(Θ_(//))of 84.0%.Consequently,highly efficient OLEDs with an external quantum efficiency as high as 33.8% are assembled,which is significantly higher than those of DPAC-BP with a highly rotatable BP acceptor(23.8%)as well as DPACFO with a rigid fluorenone(FO)acceptor(6.9%).

关键词： organic light-emitting diodes medium-ring intramolecular-lock thermally activated delayed fluorescence molecular orientation

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Sm^(2+)ions boost ammonia electrooxidation reaction on samarium oxide anode for hydrogen generation in non-aqueous electrolyte

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Nano Research 2024年第7期17卷 5856-5862页

作者： Xingyu Liu Xue Yang Han Sun Zekai Yang Haijun Chen Tianjin Key Laboratory of Optoelectronic Thin Film Devices and Technology College of Electronic Information and Optical EngineeringNankai UniversityTianjin 300350China

Ammonia has garnered recognition as a zero-carbon fuel due to its high-density hydrogen storage capacity and its convenience for storage and *** address the challenges associated with the direct usage of ammonia,the development of NH_(3)-to-H_(2)conversion technologies has emerged as a promising and effective ***,we present for the first time that crystallized Sm_(2)O_(3−x)electrodes demonstrate high and stable electrocatalytic activities,including N_(2)evolution rate and Faradaic efficiency,for ammonia electrolysis in a non-aqueous *** was observed that Sm^(2+)ions in samarium oxide play an indispensable role in the ammonia electrooxidation reaction on the ***,the mechanism of ammonia electrooxidation has also been elucidated,laying the foundation for a better understanding of the relationship between local structure and electrochemical properties in order to facilitate research on Pt-free electrocatalysts for the electrolysis of ammonia into H_(2).

关键词： NH_(3)-to-N_(2)conversion ammonia electrooxidation reaction ammonia electrolysis non-aqueous electrolyte samarium oxide

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Infrared Photodetectors and Image Arrays Made with Organic Semiconductors

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Chinese Journal of Polymer Science 2023年第10期41卷 1629-1637页

作者： Zhi-Ming Zhong Feng Peng Lei Ying Zhen-Qiang Huang Wen-Kai Zhong Gang Yu Yong Cao Fei Huang Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and DevicesSouth China University of TechnologyGuangzhou510640China

Combining the strategies of introducing larger heteroatom,regio-regular backbone and extended branching position of side-chain,we developed polymer semiconductors(PPCPD)with narrow band-gap to construct the photosensing layer of thin-film photodiodes and image *** spectral response of the resulting organic photodiodes spans from the near ultra-violet to short-wavelength infrared *** performance of these short-wavelength infrared photodiodes in 900–1200 nm range achieved a level competitive with that of indium gallium arsenide-based inorganic crystalline detectors,exhibiting a specific detectivity of 5.55×1012 Jones at 1.15µ*** photodetectivity and quantum efficiency in photodiode with amorphous/nanocrystalline thin-films of 100–200 nm thickness enabled high pixel-density image arrays without pixel-level-patterning in the sensing layer.1×256 linear diode arrays with 25µm×25µm pixel pitch were achieved,enabling high pixel-density short-wavelength infrared imaging at room temperature.

关键词： Conjugated polymer Organic semiconductor Infrared Photodetector Image array

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A Brief Introduction to Organic Electrodeposition and a Review of the Fabrication of OLEDs based on Electrodeposition technology

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Chinese Journal of Polymer Science 2023年第5期41卷 621-639,I0005页

作者： Bo-Han Wang Yu-Guang Ma Yong Cao Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and DevicesSouth China University of TechnologyGuangzhou 510640China

Electrodeposition is an old and effective method for the fabrication of organic *** electrodeposited organic films have been widely used in various applications,highly luminescent films have been a great challenge because the electrochemically doped state may strongly quench the *** the first part of this review,the organic electrodeposition techniques,along with general electropolymerization and other special electrodepositions are *** the second part of the review,we describe how to electrochemically fabricate luminescent films for organic light-emitting diodes(OLEDs).With the rational molecular design and well-controlled electrodeposition process,we have not only demonstrated high-performance OLEDs,but also paved a promising way to practice active-matrix OLEDs(AMOLEDs)and super-resolution *** particular,RGB 3×3 array OLEDs based on active-matrix substrates,RGB passive-matrix OLEDs(PMOLEDs)with a resolution of 210 ppi,and monochromatic OLEDs with a super-resolution of 2822 ppi have been successfully *** is highly anticipated that the organic electrodeposition technology is of comparable or perhaps even higher contenders in manufacturing and downscaling OLEDs and AMOLEDs with low-cost and high-resolution for the human-computer interaction fields such as augmented reality(AR),virtual reality(VR),etc.

关键词： Electrochemistry Organic electrodeposition Electropolymerization Luminescent films OLEDs

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In-situ solid-phase anion-exchange full-color perovskite light-emitting devices

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Science China Chemistry 2023年第6期66卷 1707-1713页

作者： Danyang Li Junjie Wang Jian Wang Junbiao Peng Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and DevicesSouth China University of TechnologyGuangzhou 510640China

Perovskite materials can realize the transition from green light to full-visible light spectrum by halogen anion ***,we designed an in-situ solid-phase anion-exchange method combined with inkjet printing to achieve full-color perovskite quantum dot light-emitting diodes(PeQD-LEDs).It was revealed that,in addition to the concentration,the anion-exchange rate was affected by the dielectric constant of the anion-exchange medium *** destroying the PeQD film,the higher the dielectric constant of the solvent,the faster the reaction *** at the same time,the solvent with higher dielectric constant will cause more defects,so the morphology,structure and properties of the perovskite films varied with *** chain length of amine salts in anion-exchange medium solute also played a key role in the stability of electroluminescence *** obtained blue-light devices had a maximum EQE of 4.6%at 481 nm and 6.6%at 493 nm prepared by *** inkjet printing,instead of printing red-,green-and blue-luminescent materials,we printed halogen-containing materials to achieve the in-situ solid-phase anion-exchange with underlying Pe QDs,and the inkjet-printed full-color device showed the current efficiency of 0.78 cd A^(-1).The method to achieve full-color devices by inkjet-printing halogen-containing materials can not only simplify the process,but also broaden the range of material selection,making the ink preparation more selective.

关键词： perovskite light-emitting diode inkjet print anion exchange full color

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