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Utilization of Low-Energy Photons of Sunlight by Multiphoton Strategy: From Nature to Artificial Techniques

CCS Chemistry 2025年第1期7卷 10-21页

作者： Yu Zhang Zengqi Xie Yuguang Ma State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and DevicesGuangdong Provincial Key Laboratory of Luminescence from Molecular AggregatesGuangdong Basic Research Center of Excellence for Energy&Information Polymer MaterialsSouth China University of TechnologyGuangzhou 510640

The pursuit of enhancing solar energy utilization efficiency has led to the continuous development of innovative materials and devices and especially exploring new mechanisms in artificial solar energy *** photosensitizing systems with a single-photon process usually suffer from the waste of low-energy photons of sunlight;in this context,a multiphoton strategy have been proposed by mimicking the photosynthesis process in nature in order to overcome this *** review provides insights into various novel multiphoton strategies especially the consecutive photoinduced electron transfer *** significance of the effective utilization of low-energy photons is emphasized,presenting a key pathway for improving energy conversion efficiency in various artificial techniques including photocatalysis,photoelectrodes,and solar ***,the long-time stable intermediate charge separation states are highlighted as an essential issue for the multiphotonstrategy. Finally, a perspective is given on the possibletransplantation of the multiphoton strategy fromsolution to solid-state devices in the future.

关键词： solar energy utilization artificial photosynthesis multiphoton strategy photoinduced charge transfer long-lived charge separation state

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Niobium telluride absorber for a mode-locked vector soliton fiber laser

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Science China(Physics,Mechanics & Astronomy) 2023年第5期66卷 130-138页

作者： XinXin Shang NanNan Xu Jia Guo Shuo Sun HuaNian Zhang SWageh Ahmed AAl-Ghamdi Han Zhang DengWang Li Shandong Province Key Laboratory of Medical Physics and Image Processing Technology Shandong Provincial Key Laboratory of Optics and Photonic DeviceSchool of Physics and ElectronicsShandong Normal UniversityJinan 250014China Institute of Microscale Optoelectronics Collaborative Innovation Center for Optoelectronic Science&TechnologyKey Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong ProvinceCollege of Physics and Optoelectronic EngineeringShenzhen Key Laboratory of Micro-Nano Photonic Information TechnologyGuangdong Laboratory of Artificial Intelligence and Digital Economy(SZ)Shenzhen UniversityShenzhen 518060China School of Physics and Optoelectronic Engineering Shandong University of TechnologyZibo 255049China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia

Niobium telluride(NbTe_(2)),an emerging transition metal dichalcogenide material,has been theoretically predicted to have nonlinear absorption properties and excellent optical ***,only a few studies of the utilization of NbTe_(2)in ultrafast photonics have been *** this work,a NbTe_(2)-based saturable absorber(SA)was applied in an erbium-doped fiber as a mode-locked device,and a vector soliton based on NbTe_(2)was obtained for the first ***_(2)-PVA film SA was successfully prepared by the liquid-phase exfoliation and spin coating methods,with a modulation depth of up to 10.87%.The nonlinear absorption coefficient of NbTe_(2)-based SA film tested through the open-aperture Z-scan laser measurement is 0.62×10^(−11) m/W.A conventional soliton with a pulse duration of 858 fs was generated using NbTe_(2)-based SA,which was demonstrated to be a kind of polarization-locked vector soliton in further *** experimental results reveal the nonlinear optical properties of NbTe_(2)and broaden its applications in ultrafast photonic devices.

关键词： niobium telluride saturable absorber mode-locked pulse fiber laser

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Optimizing theπ-Bridge of Non-fullerene Acceptors to Suppress Dark Current in NIR Organic Photodetectors

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Chemical Research in Chinese Universities 2024年第4期40卷 712-721页

作者： SHAO Lin HUANG Yijun HONG Ling XU Zishuo YANG Xiye LIU Chunchen HUANG Fei CAO Yong State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and DevicesSchool of Materials Science and EngineeringSouth China University of TechnologyGuangzhou510640P.R.China Lumidar Technology Co. Ltd.Guangzhou510530P.R.China

Recently,the rapid development of non-fullerene acceptors(NFAs)has laid the foundation for performance improvements in near-infrared(NIR)organic photodetectors(OPDs).However,reducing the bandgap of NFAs to achieve strong absorption in the shorter-wave region usually leads to increased dark current density(J_(d))and decreased responsivity(R),severely limiting the detectivity(D*)of *** date,it remains challenging to manipulate the J_(d) of NIR-OPDs through rational structure engineering of ***,three NIR-NFAs,namely bis(2-decyltetradecyl)4,4′-(2′,7′-di-tert-butylspiro[cyclopenta[2,1-b:3,4-b′]dithiophene-4,9′-fluorene]-2,6-diyl)bis(6-(((Z)-1-(dicyanomethylene)-5,6-difluoro-3-oxo-1,3-dihydro-2H-inden-2-ylidene)methyl)thieno[3,4-b]thiophene-2-carboxylate)(TSIC-4F),bis(2-decyltetradecyl)6,6′-(2′,7′-di-tert-butylspiro[cyclopenta[2,1-b:3,4-b′]dithiophene-4,9′-fluorene]-2,6-diyl)bis(4-(((Z)-1-(dicyanomethylene)-5,6-difluoro-3-oxo-1,3-dihydro-2H-inden-2-ylidene)methyl)thieno[3,4-b]thiophene-2-carboxylate)(STIC-4F),and 2,2′-((2Z,2′Z)-(((2′,7′-di-tert-butylspiro[cyclopenta[2,1-b:3,4-b′]dithiophene-4,9′-fluorene]-2,6-diyl)bis(2,3-bis(5-(2-butyloctyl)thiophen-2-yl)thieno[3,4-b]pyrazine-7,5-diyl))bis(metha-neylylidene))bis(5,6-difluoro-3-oxo-2,3-dihydro-1H-indene-2,1-diylidene))dimalononitrile(TPIC-4F),were designed using the thieno[3,4-b]thiophene(TT)and thieno[3,4-b]pyrazine(TPy)derivatives as theπ-*** to the intramolecular S-S and S-N interactions,STIC-4F and TPIC-4F exhibited smaller backbone distortions than TSIC-4F.A significantly red-shifted absorption with a peak at 1015 nm was observed in TPIC-4F film,larger than that(ca.960 nm)for TSIC-4F and STIC-4F ***,OPDs operating in a photovoltaic mode were successfully fabricated,and TPIC-4F-based OPDs achieved the lowest J_(d) of 3.18×10^(-8) A/cm^(2) at-0.1 ***,although TPIC-4F-based OPDs exhibited the lowest R,higher shot-noise-limited specific detectivity(D_(sh)*)in 1000-1200 nm co

关键词： π-Bridge Near-infrared Non-fullerene acceptor Dark current Organic photodetector

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Low Temperature Tetragonal Tungsten Bronze Oxides for Li-ion Storage

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Chemical Research in Chinese Universities 2024年第5期40卷 922-926页

作者： XU Chengxin ZHANG Wenda LOU Chenjie LI Chengyu XU Ligang SHI Yongchao LIU Jie LUO Huajie FU Jipeng KUANG Xiaojun TANG Mingxue Guangxi Key Laboratory of Electrochemical and Magnetochemical Function Materials College of Chemistry and BioengineeringGuilin University of TechnologyGuilin541006P.R.China Center for High Pressure Science and Technology Advanced Research Beijing100193P.R.China Guangxi Key Laboratory of Optic and Electronic Materials and Devices Key Laboratory of New Processing Technology for Nonferrous Metals and MaterialsMinistry of EducationCollege of Materials Science and EngineeringGuilin University of TechnologyGuilin541004P.R.China School of Materials Science and Engineering&Key Laboratory of Advanced Materials and Devices for Post-Moore Chips Ministry of EducationUniversity of Science and Technology BeijingBeijing100083P.R.China Key Laboratory of Rare Earth Optoelectronic Materials and Devices of Zhejiang Province Institute of Optoelectronic Materials and DevicesChina Jiliang UniversityHangzhou310018P.R.China

Nb-based tungsten bronze oxides have emerged as attractive materials in various fields,owing to the structural openings and simple synthesis *** this work,the tetragonal tungsten bronze(TTB)NaWNbO_(6) was prepared by solid state reaction at a relatively low temperature of 775°*** local structure was systematically studied by solid state nuclear magnetic resonance(SSNMR)with the aid of transition electronic microscopy(TEM).The analysis indicates that NaWNbO6 has pentagonal,square,and triangular ***,square tunnels were partly occupied(50%)by Na,which creates the ability for the Li-ion storage with a volumetric capacity of 210 A·h·L^(−1)at 0.2 *** 2D ^(23)Na-^(23)Na EXSY results further suggest the ability of ions to fast exchange between the tetragonal and pentagonal tunnels,resulting in a high-rate performance 20 C.

关键词： Tetragonal tungsten bronze Solid-state^(23)Na NMR ^(93)Nb NMR spectrum Fast ion exchange

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High-performance flexible Sb_(2)Se_(3) thin-film photodetector for tunable color imaging and wearable physiological monitoring applications

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Nano Research 2025年第2期18卷 687-698页

作者： Shuo Chen Hong-Bo Li Yi Fu Guo-Qiang Liu Muhammad Ishaq Jun Luo Jian-Min Li Bo Che Jing-Ting Luo Liming Ding Tao Chen Guang-Xing Liang Shenzhen Key Laboratory of Advanced Thin Films and Applications Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong ProvinceState Key Laboratory of Radio Frequency Heterogeneous IntegrationCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China The Hospital of Shenzhen General Station of Exit and Entry Frontier Inspection Shenzhen 518024China Key Laboratory of Artificial Micro-and Nano-structures of Ministry of Education School of Physics and TechnologyWuhan UniversityWuhan 430072China Hefei National Research Center for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy ConversionDepartment of Materials Science and EngineeringUniversity of Science and Technology of ChinaHefei 230026China Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190China

Antimony selenide(Sb_(2)Se_(3))has recently made considerable photovoltaic,advancements in photoelectrochemical,and photodetector research scenarios,owing to its advantageous material merits and superior optoelectronic *** contrast,the exploration of flexible Sb_(2)Se_(3) photoelectric devices are less attempted,though it possesses unique one-dimensional(1D)crystal structure to enable large deformation ***,we develop a flexible Sb2Ses thin-film photodetector on polyimide *** to the high-quality SbSes light absorber and benign interfaces at both back contact and heterojunction regions,the carrier dynamics are effectively *** leading flexible Sb_(2)Se_(3) photodetector showcases self-powered and broadband features,with exceptional responsivity of 0.51 A·W^(-1) and realistic detectivity up to 1.32×10^(13) Jones,ultra-fast response speed of 49 ns/351 ns of rise and decay times,and remarkable mechanical deformation stability,flourishing the high-level development for flexible Sb_(2)Se_(3) ***,a tunable single/dual-color flexible imaging system under band alignment modulation,along with a wearable and accurate heart rate/arterial blood oxygen saturation photoplethysmography detection system highlights the great application potential for flexible Sb,Ses photodetectors.

关键词： Sb_(2)Se_(3) flexible thin-film photodetector color imaging heart rate arterial blood oxygen saturation

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Dual-band terahertz antenna based on a novel photonic band gap structure

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optoelectronics Letters 2023年第11期19卷 666-672页

作者： BAI Yukun LI Jie Tianjin Key Laboratory of Film Electronic and Communication Devices Engineering Research Center of Optoelectronic Devices and Communication TechnologyMinistry of EducationSchool of Integrated Circuit Science and EngineeringTianjin University of TechnologyTianjin300384China

In this paper,a novel dual-band photonic band gap(PBG) structure was proposed and applied to a dual-band micro-strip *** antenna resonates at 1.267 THz and 1.502 THz,exhibiting reflection coefficients of-58.177 dB and-49.462 dB,and gains of 3.173 dBi and 5.232 dBi,*** with the microstrip antenna based on the homogeneous silicon substrate,the designed dual-band antenna based on the novel PBG structure shows improved impedance matching,radiation efficiency,and *** paper simulated and analyzed the impacts of different filling dielectric materials and the variations of dimensions,position,period,and corrugation depths of the dual-band PBG structure on the resonances of the *** is expected that the proposed novel dual-band PBG structure has great application potentials,and such cancer diagnosis is done by utilizing the radiation characteristics of the antenna.

关键词： antenna structure band

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17.13% Efficiency and Superior Thermal Stability of Organic Solar Cells Based on a Comb-Shape Active Blend

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Energy & Environmental Materials 2023年第6期6卷 266-272页

作者： Zhipeng Yin Qingjie Wang Huan Zhao Haiqiao Wang Ning Li Weijie Song School of Materials Science and Engineering NingboTech UniversityNingbo 315100China Zhejiang Provincial Engineering Research Center of Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and DevicesSchool of Materials Science and EngineeringSouth China University of TechnologyGuangzhou 510640China

With rapid progress,organic solar cells(OSCs)are getting closer to the target of real ***,the stability issue is still one of the biggest challenges that have to be ***,the thermal stability of OSCs is far from meeting the requirements of the ***,based on the layer-by-layer(LBL)process and by utilizing the dissolubility nature of solvent and materials,binary inverted OSCs(ITO/AZO/PM6/BTP-eC9/MoO3/Ag)with comb shape active morphology are *** efficiency of 17.13%and simultaneous superior thermal stability(with 93%of initial efficiency retained in~9:00 h under 85℃in N_(2))are demonstrated,showing superior stability to reference *** enhancements are attributed to the formed optimal comb shape of the active layer,which could provide a larger D/A interface,thus more charge carriers,render the active blend a more stable morphology,and protect the electrode by impeding ion's migration and *** the best of our knowledge,this is the best thermal stability of binary OSCs reported in the literature,especially when considering the high efficiency of over 17%.

关键词： comb-shape blend high efficiency organic solar cell thermal stability

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Highly Reliable Multilayer Encryption Scheme With Constellation Shaping Based on Joint Index Modulation

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Journal of Lightwave technology 2025年第12期43卷 5689-5698页

作者： Zhu, Dongxu Liu, Bo Ren, Jianxin Mao, Yaya Song, Xiumin Chen, Shuaidong Zhao, Lilong Yin, Mengtong Dai, Wei Chen, Guoqing Cai, Junjie Institute of Optics and Electronics Nanjing University of Information Science & Technology Nanjing210044 China State Key Laboratory Cultivation Base of Atmospheric Optoelectronic Detection and Information Fusion Nanjing University of Information Science & Technology Nanjing210044 China Jiangsu International Joint Laboratory for Meteorological Photonics and Optoelectronic Detection Nanjing University of Information Science & Technology Nanjing210044 China Jiangsu Engineering Research Center for Intelligent Optoelectronic Sensing Technology of Atmosphere Nanjing University of Information Science & Technology Nanjing210044 China Beijing University of Posts and Telecommunications Beijing100876 China Department of Electronic Engineering Tsinghua University Beijing100084 China

This paper proposes a highly reliable multilayer encryption scheme with constellation shaping based on joint index modulation. Multilayer encryption is used to ensure the security of the scheme. We utilize the 3D-Zhang chaotic system to realize the multidimensional perturbation of bits, subcarriers, and symbols of the original signal. The key information is masked with the signal using joint index modulation (JIM). The cooperative transmission of the initial value of the chaotic system is realized through the position information of the silent subcarriers and the constellation modes of the corresponding subcarriers. The scheme interleaves the initial values of the two chaotic systems to encode them as index bits, realizing the first layer of masked keys. Additional constellation shaping is achieved by optimizing the index mapping rules and changing the distribution of constellation points in the center and in the dual mode. The rotational encryption of the constellation is realized using a one-dimensional sinusoidal chaotic system after the completion of JIM, and the second layer of spherical shell masking of the key information is completed. The experimental implementation demonstrates the successful transmission of a 14 Gb/s 3D-JIM -8QAM signal over a 2 km weakly coupled seven-core fiber. Results confirm that the multi-layer encryption approach ensures secure signal transmission even under partial key leakage, without introducing degradation to the system's transmission performance. Compared to a random constellation distribution, the optimized index mapping scheme provides a coding gain of 0.75 dB at an FEC (Forward Error Correction) threshold of 3.8×10-3. The proposed scheme achieves error-free key transmission, with a bit error rate (BER) consistently maintained at 0. Notably, even minor key misalignments result in a BER of 0.5, facilitating timely key updates. The scheme boasts a vast key space of 10150, effectively resisting brute-force attacks. Due to its hi

关键词： Forward error correction

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MBenes:Two-dimensional transition-metal borides with ordered metal vacancies

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Chinese Chemical Letters 2023年第1期34卷 3-4页

作者： Hui Yang Liang Chu Tianjin Key Laboratory for Optoelectronic Materials and Devices Key Laboratory of Display Materials and Photoelectric Devices(Ministry of Education)School of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China New Energy Technology Engineering Laboratory of Jiangsu Province&School of Science Nanjing University of Posts and TelecommunicationsNanjing 210023China

2D MBenes have been theoretically predicted to possess unique electronic structures and physicochemical properties,and thus shown great promise in various ***,the synthesis of individual single-layer MBene remains a grand challenge due to its orthorhombic structure of MAB ***,scientists from Link?ping University have fabricated 2D monolayer Mo4/3B2-xTzwith ordered metal *** results demonstrated the feasibility of top-down approach by chemical exfoliation of laminated compounds and provided the principle for further preparation of a wealth of MBenes.

关键词： Transition-metal borides i-MAB phases MBenes Monolayer Ordered metal vacancies

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Thiazoloisoindigo-based Polymer Semiconductors: Synthesis,Structure-Property Relationship, Charge Carrier Polarity, and Field-Effect Transistor Performance

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Chinese Journal of Polymer Science 2024年第1期42卷 24-31,I0006页

作者： Bo-Wen Li Miao Xiong Mei-Hua Liu Zhi-Gao Li Long Sang Zi-Han Xiong Biao Xiao Jian Pei Xiao-Bo Wan Key Laboratory of Optoelectronic Chemical Materials and Devices Ministry of EducationSchoolofOptoelectronic Materials&TechnologyJianghan UniversityWuhan430056China Bejing National Laboratoryfor Molecular Sciences the Key Laboratory of Bioorganic Chemistry and Molecular Engineering of Ministry of EducationCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

Developing new polymeric semiconductors with excellent device performance is essential for organic electronics. Herein, we synthesized two new thiazoloisoindigo(Tz II)-based polymers, namely, P(Tz II-d Th-d Th) and P(Tz II-d Th-d Tz), by copolymerizing thiophene-flanked Tz II with bithiophene and bithiazole, respectively. Owing to the more electron-deficient nature of bithiazole than bithiophene, P(Tz II-d Th-d Tz)possesses deeper LUMO/HOMO levels of-3.45/-5.47 e V than P(Tz II-d Th-d Th)(-3.34/-5.32 e V). The organic field-effect transistor(OFET) devices based on P(Tz II-d Th-d Th) exhibited p-type behaviors with an average hole mobility value as high as 1.43 cm^(2)·V^(-1)·s^(-1), while P(Tz II-d Th-d Tz)showed typical ambipolar characteristics with average hole and electron mobilities of 0.38 and 0.56 cm^(2)·V^(-1)·s^(-1). In addition, we compared the performances of both polymers with other Tz II-based polymers reported in our previous work, and showed that the charge carrier polarity can be manipulated by adjusting the number of the thiophene units between the acceptor unit. As the increase of the number of thiophene rings,charge carrier polarity shifts from electron-dominated ambipolar transport to hole-dominated ambipolar transport and then to unipolar hole transport in OFETs, which provides an effective molecular design strategy for further optimization of polymer OFET performance.

关键词： Field-effect transistor Charge carrier polarity Thiazoloisoindigo

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