The Einstein-de Haas(EdH)effect,which establishes that changes in magnetization induce mechanical rotation,was experimentally demonstrated in 1915[1],independently of Richardson’s[2]earlier conceptual prediction rela...
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The Einstein-de Haas(EdH)effect,which establishes that changes in magnetization induce mechanical rotation,was experimentally demonstrated in 1915[1],independently of Richardson’s[2]earlier conceptual prediction related to this aspect.
Artificial synapses with full synapse-like functionalities are of crucial importance for the implementation of neuromorphic computing and bioinspired intelligent systems. In particular, the development of artificial s...
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Artificial synapses with full synapse-like functionalities are of crucial importance for the implementation of neuromorphic computing and bioinspired intelligent systems. In particular, the development of artificial synapses with the capability to emulate multiplexed neural transmission is highly desirable, but remains challenging. In this work, we proposed a hybrid ambipolar synaptic transistor that combines two-dimensional(2D) molybdenum disulfide(Mo S_(2)) sheet and crystalline one-dimensional(1D) poly(3-hexylthiophene-2,5-diyl) polymer nanowires(P3HT NWs) as dual excitatory channels. Essential synaptic functions, including excitatory postsynaptic current, paired-pulse facilitation, synaptic potentiation and depression, and dynamic filtering were emulated using the synaptic transistor. Benefitting from the dual excitatory channels of the synaptic transistor, the device achieved a fast switch between short-term and long-term memory by altering the charge carriers in the dual channels, i.e., electrons and holes. This emulated the multiplexed neural transmission of different excitatory neurotransmitters, e.g., dopamine and noradrenaline. The plasticity-switchable artificial synapse(PSAS) simulates the task-learning process of individuals under different motivations and the impact of success or failure on task learning and memory, which promises the potential to enable complex functionalities in future neuromorphic intelligent electronics.
Color formulation prediction aims to get different target colors based on a specified color range. It was difficult for existing color matching methods to achieve accurate nonlinear mapping from target colors to formu...
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A novel synthesis method of a sparse rectangular planar receiving array (SRPRA) to maximize the power transmission efficiency (PTE) for microwave power transmission (MPT) is proposed in this paper. The array element p...
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—A novel subarray layout method is proposed for the problems of high power dispersion and high complexity of the existing layout methods of receiving rectifier antenna arrays. By the traditional RF synthesis and DC s...
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The complicated and diverse deep defects,voids,and grain boundary in the CZTSSe absorber are the main reasons for carrier recombination and efficiency *** further improvement of the open-circuit voltage and fill facto...
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The complicated and diverse deep defects,voids,and grain boundary in the CZTSSe absorber are the main reasons for carrier recombination and efficiency *** further improvement of the open-circuit voltage and fill factor so as to increase the efficiency of CZTSSe device is *** this work,we obtained K-doped CZTSSe absorber by a simple solution *** medium-sized K atoms,which combine the advantages of light and heavy alkali metals,are able to enter the grain interior as well as segregate at grain *** K-Se liquid phase can improve the absorber *** find that the accumulation of the wide bandgap compound K_(2)Sn_(2)S_(5)at grain boundary can increase the contact potential difference of grain boundary,form more effective hole barriers,and enhance the charge separation *** the same time,K doping passivates the interface as well as bulk defects and suppresses the non-radiative *** improved crystallinity,enhanced charge transport capability and reduced defect density due to K doping result in a significant enhancement of the carrier lifetime,leading to 13.04%device *** study provides a new idea for simultaneous realization of grain boundary passivation and defect suppression in inorganic kesterite solar cells.
In this article,morpholine,a non-conjugated heterocycle,is embedded intoπsystem to construct single-component organic room temperature phosphorescence(RTP)*** effect of morpholine on intermolecular interaction,crysta...
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In this article,morpholine,a non-conjugated heterocycle,is embedded intoπsystem to construct single-component organic room temperature phosphorescence(RTP)*** effect of morpholine on intermolecular interaction,crystal packing modes,and RTP performance is investigated *** experimental and theoretical calculation results illustrate the versatility of morpholine in promoting the n-π*transition and intensifying the intermolecular interactions,which not only enhances the generation of triplet excitons,but also suppresses the nonradiative decay of triplet ***,TMPh containing three morpholine units shows an ultralong lifetime of 1.03 s and a visible afterglow up to 10 *** unique dual delayed emission and long afterglow property allow potential application of morpholine derivatives in data encryption,and the time-dependent color change of afterglow emission is realized after removing the excitation source,providing a high-level data *** article provides a new perspective for the design of purely organic RTP system without utilization of metal,or even any heavy atoms.
Lithium metal anode is considered the alternative to graphite anode due to its ultra-high theoretical capacity of 3860 mAh·g^(-1).However,serious Li dendrite growth and drastic electrolyte side reactions restrain...
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Lithium metal anode is considered the alternative to graphite anode due to its ultra-high theoretical capacity of 3860 mAh·g^(-1).However,serious Li dendrite growth and drastic electrolyte side reactions restrain the commercial application of Li metal *** this work,a Li_(3)Bi/LiF interfacial layer is constructed on the surface of the Li metal anode by a spontaneous substitution *** composite interfacial layer possesses excellent ionic conductivity,high mechanical strength,and great electrolyte wettability,which ensures fast Li-ion transfer and uniform Li deposition of the Li_(3)Bi/LiF@Li ***,the Li_3Bi/LiF@Li symmetric cell provides a cycle life of more than 400 h with only 73 mV voltage polarization at 10 mA·cm^(-2).By pairing with commercial NCM622 cathode,the Li_(3)Bi/LiF@Li full cell exhibits a long cycle at a rate of 2 C.
In recent years, due to the increasing demand for green energy, organic/polymer heterojunction solar cells have aroused great interest in the academic and industrial ***/polymer solar cells (OSCs) have a series of adv...
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In recent years, due to the increasing demand for green energy, organic/polymer heterojunction solar cells have aroused great interest in the academic and industrial ***/polymer solar cells (OSCs) have a series of advantages over their counterparts. The morphology of the active layer and the energy band structure of the device can be adjusted easily by changing the molecular ***-area low-cost modules can be prepared by roll-to-roll solution printing at room temperature.
Despite the great leap forward perovskite solar cells(PSCs)have achieved in power conversion efficiency,the device instability remains one of the major problems plaguing its ***-free hole transport material(HTM)has be...
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Despite the great leap forward perovskite solar cells(PSCs)have achieved in power conversion efficiency,the device instability remains one of the major problems plaguing its ***-free hole transport material(HTM)has been widely studied as an important strategy to improve the stability of PSCs due to its avoidance of moisture-sensitive dopants and cumbersome doping *** this work,a series of dopant-free HTMs L1F,L2F and L3F based on D-A-π-A-D configuration were synthesized through two steps of reaction.L3F presents a high glass transition temperature of 1800C and thermal decomposition temperature of ***,electron paramagnetic resonance signals of L1F,L2F and L3F powders indicate the open-shell quinoidal diradical resonance structure in their aggregation state due to aggregation-induced radical *** these HTMs present higher hole mobility than dopant-free Spiro-OMeTAD,and the dopant-free L3F-based PSC device achieves the highest power conversion efficiency of 17.6%among *** addition,due to the high hydrophobic properties of L1F,L2F and L3F,the perovskite films spin-coated with these HTMs exhibit higher humidity stability than doped *** results demonstrate a promising design strategy for high glass transition temperature dopant-free hole transport *** open-shell quinoid-radical organic semiconductors are not rational candidates for dopant-free HTMs for PSC devices.
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