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Characterization of the interfacial structure and fracture behavior of in situ synthesized ceramics to reinforce Ni-based composite coatings

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材料科学技术（英文版） 2025年第5期208卷 11-25页

作者： Yuxin Wang Yanchun Dong Yun Tian Jianing Liu Dongyao Zhang Chunli Qiu Yanqi Zhao Yong Yang School of Materials Science and Engineering Hebei University of TechnologyTianjin 300132China Key Lab.for New Type of Functional Materials in Hebei Province School of Materials Science and EngineeringState Key Laboratory of Reliability and Intelligence of Electrical EquipmentHebei University of TechnologyTianjin 300132China

This work used the in-situ synthesis of molten-state nitride ceramic phase-reinforced Ni-based alloy coat-ings,aiming to improve the phase-interface bonding through the interdependent co-solidification be-tween molten *** XRD was used to analyze the physical phases of the composite *** microstructure and phase-interface structure were characterized in detail by combining SEM,TEM,HRTEM,FFT,and SAED *** tester and microforce microhardness tester were em-ployed to measure the surface hardness and elastic modulus of the composite *** fracture be-havior of the composite coatings was characterized by observing the fracture morphology of the coatings using SEM combined with the EDS *** was found that the formation mechanisms of inter-facial misfit dislocation assistance,lattice distortion,aggregation of stacking faults,and specific growth orientation between the y-Ni matrix phase and each ceramic phase in NiCrBSi-TiCrN composite coat-ings improved the lattice matching between the two-phase interface,which resulted in the formation of atomically corresponding coherent lattice relations and stepped interfacial semi-coherent lattice relations,and enhanced the degree of phase-interface *** this basis,the composite coatings with high Cr content further inhibited the expansion of interphase penetration cracks due to the existence of Cr-rich zones at the phase interface,thus exhibiting high fracture *** work provides new opinions on the improvement of phase-interface bonding and composition design of Ni-based composite coatings.

关键词： In situ synthesis NiCrBSi-TiCrN composite coating Phase interface Fracture behavior

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Bamboo-like MnO_(2)·Co_(3)O_(4):High-performance catalysts for the oxidative removal of toluene

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Journal of environmental Sciences 2025年第1期147卷 617-629页

作者： Ali Rastegarpanah Jiguang Deng Yuxi Liu Lin Jing Wenbo Pei Jia Wang Hongxing Dai Beijing Key Laboratory for Green Catalysis and Separation Key Laboratory of Beijing on Regional Air Pollution ControlKey Laboratory of Advanced Functional MaterialsEducation Ministry of ChinaLaboratory of Catalysis Chemistry and NanoscienceDepartment of Chemical EngineeringFaculty of Environment and LifeBeijing University of TechnologyBeijing 100124China

Themanganese-cobalt mixed oxide nanorodswere fabricated using a hydrothermalmethod with different metal precursors(KMnO_(4)and MnSO_(4)·H_(2)O for MnOx and Co(NO3)2>6H_(2)O and CoCl_(2)>6H_(2)O for Co_(3)O_(4)).Bamboo-like MnO_(2)>Co_(3)O_(4)(B-MnO_(2)>Co_(3)O_(4)(S))was derived from repeated hydrothermal treatments with Co_(3)O_(4)@MnO_(2)and MnSO_(4)>H_(2)O,whereas Co_(3)O_(4)@MnO_(2)nanorods were derived from hydrothermal treatment with Co_(3)O_(4)nanorods and KMnO_(4).The study shows that manganese oxide was tetragonal,while the cobalt oxide was found to be cubic in the crystalline *** surface ions were present in multiple oxidation states(e.g.,Mn^(4+)and Mn^(3+))and surface oxygen *** content of adsorbed oxygen species and reducibility at low temperature declined in the sequence of BMnO_(2)>Co_(3)O_(4)(S)>Co_(3)O_(4)@MnO_(2)>MnO_(2)>Co_(3)O_(4),matching the changing trend in *** all the samples,B-MnO_(2)>Co_(3)O_(4)(S)showed the preeminent catalytic performance for the oxidation of toluene(T10%=187℃,T50%=276℃,and T90%=339℃).In addition,the B-MnO_(2)>Co_(3)O_(4)(S)sample also exhibited good H_(2)O^(-),CO_(2)^(-),and SO_(2)^(-)resistant *** good catalytic performance of B-MnO_(2)>Co_(3)O_(4)(S)is due to the high concentration of adsorbed oxygen species and good reducibility at low *** oxidation over B-MnO_(2)>Co_(3)O_(4)(S)proceeds through the adsorption of O_(2)and toluene to form O∗,OH∗,and H_(2)C(C6H5)∗species,which then react to produce benzyl alcohol,benzoic acid,and benzaldehyde,ultimately converting to CO_(2)and H_(2)*** findings suggest that B-MnO_(2)>Co_(3)O_(4)(S)has promising potential for use as an effective catalyst in practical applications.

关键词： Manganese-cobalt mixed oxide Nanorod Bamboo-like morphology Hydrothermal method Toluene oxidation

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Structure-performance relationship between denitration performance and catalytic interface morphologies of MnCeO_(x)/P84 catalytic filters

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Journal of Rare Earths 2025年第3期43卷 516-525,I0004页

作者： Bo Yang Yujie Lei Maosen Ni Liuying Wang Qiong Huang Mindong Chen Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology(CICAEET) Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution ControlSchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing210044China

MnCeO_(x)/P84 catalytic filters with spherical,flower-like,cubic and rod-like catalytic interfaces were synthesized respectively,and their catalytic activities in the NH_(3)-SCR reaction were *** MnCeO_(x)/P84 catalytic filter with spherical catalytic interfaces(recorded as S-MnCeO_(x)/P84)exhibits the best catalytic denitration *** NO_(x)removal efficiency of S-MnCeO_(x)/P84 reaches the highest value of 98.6%at 160℃when the catalyst loading is 100 g/m^(2).At the same time,S-MnCeO_(x)/P84 exhibits good SO_(2)resistance and stability,achieving a NO_(x)removal rate of 83%at 190℃with 30 ppm SO_(2).The characterization results illustrate that the MnCeO_x active component in S-MnCeO_(x)/P84 is present in weak crystalline states,tightly wrapped around the surface of the filter fiber,and uniformly dispersed,and the mesopore is the main pore structure of the S-MnCeO_(x)/P84,which can provide a channel for the catalytic reaction to *** the same time,transmission electron microscopy(TEM)characterization shows that y-MnO_(2)is the main form of MnO_(2)in the S-MnCeO_(x)/*** analysis of H_(2)temperature programmed reduction(H_(2)-TPR).NH_(3)temperature programmed desorption(NH_(3)-TPD)and in-situ diffuse reflectance infrared spectra(DRIFTS)show that S-MnCeO_(x)/P84 has good redox ability at 100-200℃and has abundant Lewis acid sites and Bronsteds acid sites,which provides an important guarantee for its superior low-temperature NH_(3)-SCR denitration performance.

关键词： Catalytic filter Nitrogen oxides(NO_x) Denitration Catalytic interface Rare earths

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High-precision numerical modeling of the pro jectile launch and failure mechanism analysis of pro jectile-borne components

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Applied Mathematics and Mechanics(English Edition) 2025年第5期46卷 885-906页

作者： Xindan GUO Qiming LIU Xu HAN Tao LI Bin’an JIANG Canwei CAI State Key Laboratory of Advanced Design and Manufacturing Technology for Vehicle College of Mechanical and Vehicle EngineeringHunan UniversityChangsha 410082China State Key Laboratory of Reliability and Intelligence of Electrical Equipment School of Mechanical EngineeringHebei University of TechnologyTianjin 300401China Artillery Ammunition Technology Laboratory PLA Army Academy of Artillery and Air DefenseHefei 230031China

As core components of precision-guided projectiles,projectile-borne components are highly susceptible to failure or even damage in complex high-overload environments,thereby significantly compromising launch reliability and ***,accurately characterizing the mechanical behavior of propellants remains challenging due to the limitations in the current internal ballistic theory and the constraints of large-scale artillery firing *** complicates the high-precision numerical modeling of projectile launch,and obstructs investigations into the failure mechanisms of projectile-borne ***,this paper identifies propellant parameters using the computational inverse method under uncertainty,further establishes high-precision numerical models of projectile launch,and explores the failure mechanisms of projectile-borne components in complex high-overload ***,a projectile launching experiment is meticulously designed and executed to obtain the breech pressure and muzzle ***,a general simulation model is built,and the powder burn model is used to simulate the ignition and ***,the propellant parameters are effectively identified with the computational inverse method by the combination of the experiments and simulations.A high-precision numerical model of projectile launch is modified with the parameters validated by another experiment,and the high-overload characteristics during projectile launch are thoroughly analyzed based on this ***,the high-overload characteristics of projectile-borne components are analyzed to elucidate the stress variation laws and to reveal the failure mechanisms influenced by time and spatial *** research provides an effective method for perfectly identifying propellant parameters and building high-precision numerical models of projectile ***,it provides significant guidance for the anti-high overload design and analysis of projectile-bo

关键词： projectile-borne component high-overload environment propellant parameter identification computational inverse technique failure mechanism

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Confined seepage analysis of saturated soils using fuzzy fields

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Journal of Rock Mechanics and Geotechnical engineering 2025年第3期17卷 1302-1320页

作者： Nataly A.Manque Kok-Kwang Phoon Yong Liu Marcos A.Valdebenito Matthias G.R.Faes Reliability Engineering TU Dortmund UniversityDortmund44227Germany Singapore University of Technology and Design Singapore487372Singapore State Key Laboratory of Water Resources Engineering and Management Wuhan UniversityWuhan430072China

Seepage refers to the flow of water through porous *** phenomenon has a crucial role in dam,slope,excavation,tunnel,and well *** seepage analysis usually is a challenging task,as one must cope with the uncertainty associated with the parameters such as the hydraulic conductivity in the horizontal and vertical directions that drive this ***,at the same time,the data on horizontal and vertical hydraulic conductivities are typically scarce in spatial *** this context,so-called non-traditional approaches for uncertainty quantification(such as intervals and fuzzy variables)offer an interesting alternative to classical probabilistic methods,since they have been shown to be quite effective when limited information on the governing parameters of a phenomenon is ***,the main contribution of this study is the development of a framework for conducting seepage analysis in saturated soils,where uncertainty associated with hydraulic conductivity is characterized using fuzzy *** method to characterize uncertainty extends interval fields towards the domain of fuzzy *** fact,it is illustrated that fuzzy fields are an effective tool for capturing uncertainties with a spatial component,since they allow one to account for available physical measurements.A case study in confined saturated soil shows that with the proposed framework,it is possible to quantify the uncertainty associated with seepage flow,exit gradient,and uplift force effectively.

关键词： Fuzzy fields Interval fields Seepage analysis Hydraulic conductivity Spatial uncertainty

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Impact of annealing on structural and corrosion resistance properties of Ti_(20)Zr_(20)Hf_(20)Be_(20)Ni_(20)high-entropy metallic glass

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Rare Metals 2025年第1期44卷 565-580页

作者： Ke-Ran Li Pan Gong Dong-Liang Wang Cheng Zhang Hu Huang Muhammad Yasir Mao Zhang Xin-Yun Wang State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China Research Institute of Huazhong University of Science and Technology in Shenzhen Shenzhen 518057China Key Laboratory of CNC Equipment Reliability Ministry of EducationSchool of Mechanical and Aerospace EngineeringJilin UniversityChangchun 130022China Department of Materials Science&Engineering Institute of Space TechnologyIslamabad 44000Pakistan

This study comprehensively investigates the effects of annealing on the structural,electrochemical properties and passivation film characteristics of Ti_(20)Zr_(20)Hf_(20)Be_(20)Ni_(20)(at%)high-entropy metallic glass(HE-MG).Subjected to various annealing temperatures,the samples were analyzed in a 3.5 wt%NaCl solution to evaluate changes in their microstructure and assess their corrosion *** reveal that the HE-MG undergoes multistage crystallization,displaying an amorphous matrix integrated with face centered cubic(FCC)and Ni_(7)Zr_(2)phases between 420 and 500℃,indicating robust thermal *** assessments identify a critical temperature threshold:Below the glass transition temperature(Tg),the HE-MG maintains excellent corrosion resistance,promoting stable passivation *** Tg,enhanced long-range atomic rearrangement during relaxation increases passivation layer defects and significantly diminishes corrosion resistance.X-ray photoelectron spectroscopy(XPS)analyses show that the primary components of the passivation layer are TiO_(2),ZrO_(2),HfO_(2)and *** annealing temperatures lead to enhanced Be and Ni content and decreased Ti,Zr and ***,high mixing entropy and significant atomic size mismatch suppress long-range atomic rearrangement and *** crystallization begins above Tg by_(20)℃,with crystalline phases evenly distributed within the matrix without drastically affecting corrosion *** investigation highlights the impact of thermal treatment on the properties of HE-MG,contributing valuable insights into optimizing their performance and applications.

关键词： High-entropy metallic glass Annealing Corrosion resistance Glass transition temperature Cluster

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Emerging Technologies for the Control of Biological Contaminants in Water Treatment: A Critical Review

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engineering 2025年 48卷 185-204页

作者： Gao, Rui Gao, Shu-Hong Li, Jun Su, Yiyi Huang, Fang Liang, Bin Fan, Lu Guo, Jianhua Wang, Aijie State Key Laboratory of Urban Water Resource and Environment School of Civil and Environmental Engineering Harbin Institute of Technology Shenzhen518055 China State Key Laboratory of Urban Water Resource and Environment School of Environment Harbin Institute of Technology Harbin150090 China Shenzhen518055 China The University of Queensland BrisbaneQLD4072 Australia

Biological contaminants (BCs), including but not limited to various pathogens and their endogenous pollutants such as intracellular pathogens and antimicrobial resistance genes (ARGs), are ubiquitously detected in effluent of wastewater and drinking water treatment systems which were originally designed to remove common indicator bacteria, resulting in potential impacts on public health. Although there are many emerging technologies that showing promising antimicrobial effects, few have progressed to the actual water scenarios. It's crucial to understand the main knowledge gaps and thereby design the future developments to better meet engineering requirements. In this review, we first summarize the performance of conventional water treatment towards BCs removal. Then we showcase the advances of proof-of-concept strategies, including nanotechnology, advanced oxidation process, biological control process and integrated techniques, for BCs control in light of antimicrobial mechanisms, characteristics, proper niches in water treatment, challenges and latest improvements. Further, we proposed a semi-quantitative framework coupling life cycle assessment (LCA) and analytic hierarchy process (AHP) to assess and compare the application potential of representative pilot technologies, in which the antimicrobial effects, economic issues and sustainability are comprehensively considered. For wastewater treatment, non-thermal plasma weights highest among the emerging technologies and outperforms conventional disinfection in terms of efficacy indicators (overall inactivation rate, ARGs removal rate, and growth inhibition), but fall behind overall mainly due to more energy input. Bacteriophage-based treatment has the potential to synergistically inactive the persistent pathogens in combination with conventional disinfection, serving as a cost-effective and environmental-friendly supplement. For drinking water treatment, the integrated photocatalytic nanocomposite receives the highe

关键词： Effluent treatment

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Review of bumper materials for spacecraft shield against orbital debris hypervelocity impact

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Defence technology(防务技术) 2025年第3期45卷 137-177页

作者： Siyuan Ren Pinliang Zhang Qiang Wu Qingming Zhang Zizheng Gong Guangming Song Renrong Long Liangfei Gong Mingze Wu Beijing Institute of Spacecraft Environment Engineering China Academy of Space TechnologyBeijing100094China State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing100081China School of Civil Engineering Chongqing Jiaotong UniversityChongqing400074China

It is widely known that the hypervelocity impact of orbital debris can cause serious damage to spacecraft,and enhancing the impact resistance is the great concern of spacecraft shield *** paper provides a comprehensive overview of advances in the development of bumper materials for spacecraft shield *** particular,the protective mechanism and process of the bumper using different materials against hypervelocity impact are reviewed and *** advantages and disadvantages of each material used in shield were discussed,and the performance under hypervelocity impact was given according to the specific *** review provides the useful reference and basis for researchers and engineers to create bumper materials for spacecraft shield applications,and the contemporary challenges and future directions for bumper materials for spacecraft shield were presented.

关键词： Orbital debris Spacecraft shield Hypervelocity impact Bumper materials Protective mechanism

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Effectiveness of Precursor Emission Reductions for the Control of Summertime Ozone and PM2.5 in the Beijing–Tianjin–Hebei Region under Different Meteorological Conditions

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Advances in Atmospheric Sciences 2025年第4期42卷 653-669页

作者： Jing QIAN Hong LIAO Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing 210044JiangsuChina

We used observed concentrations of air pollutants,reanalyzed meteorological parameters,and results from the Goddard Earth Observing System Chemical Transport Model to examine the relationships between concentrations of maximum daily 8-h average ozone(MDA8 O_(3)),PM_(2.5)(particulate matter with diameter of 2.5μm or less),and PM_(2.5)components and 2-m temperature(T2)or relative humidity(RH),as well as the effectiveness of precursor emission reductions on the control of O_(3) and PM_(2.5) in Beijing–Tianjin–Hebei(BTH)under different summertime temperature and humidity *** observed(simulated)MDA8 O_(3) and PM_(2.5) concentrations increased as T2 went up,with linear trends of 4.8(3.2)ppb℃^(−1) and 1.9(1.5)μg m^(−3)℃^(−1),*** results showed that the decreases in MDA8 O_(3) from precursor emission reductions were more sensitive to T2 than to *** a larger proportion of volatile organic compound(VOC)emissions at higher T2 was more effective for the control of summertime O_(3) in *** the control of summertime PM_(2.5) in BTH,reducing nitrogen oxides(NOx)combined with a small proportion of VOCs was the best *** magnitude of reduction in PM_(2.5) from reducing precursor emissions was more sensitive to RH than to T2,with the best efficiency at high *** from this study are helpful for formulating effective policies to tackle O_(3) and PM_(2.5) pollution in BTH.

关键词： ozone PM_(2.5) emission reductions meteorological conditions

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Insight into catalytic performance and reaction mechanism for toluene total oxidation over Cu-Ce supported catalyst

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Journal of environmental Sciences 2025年第3期149卷 476-487页

作者： Xuan Liang Jin Zhang Juntai Tian Zenghua Xie Yue Liu Peng Liu Daiqi Ye School of Environment and Energy South China University of TechnologyGuangzhou 510006China National Engineering Laboratory for VOCs Pollution Control Technology and Equipment Guangzhou 510006China Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control South China University of TechnologyGuangzhou 510006China Guangdong Provincial Engineering and Technology Research Centre for Environmental Risk Prevention and Emergency Disposal South China University of TechnologyGuangzhou 510006China

Herein,three supported catalysts,CuO/Al_(2)O_(3),CeO_(2)/Al_(2)O_(3),and CuO-CeO_(2)/Al_(2)O_(3),were synthesized by the convenient impregnation method to reveal the effect of CeO_(2)addition on catalytic performance and reaction mechanism for toluene *** with CuO/Al_(2)O_(3),the T_(50)and T_(90)(the temperatures at 50%and 90%toluene conversion,respectively)of CuO-CeO_(2)/Al_(2)O_(3)were reduced by 33 and 39°C,respectively.N_(2)adsorptiondesorption experiment,XRD,SEM,EDS mapping,Raman,EPR,H_(2)-TPR,O_(2)-TPD,XPS,NH_(3)-TPD,Toluene-TPD,and in-situ DRIFTS were conducted to characterize these *** excellent catalytic performance of CuO-CeO_(2)/Al_(2)O_(3)could be attributed to its strong coppercerium interaction and high oxygen vacancies ***,in-situ DRIFTS proved that CuO-CeO_(2)/Al_(2)O_(3)promoted the conversion of toluene to benzoate and accelerated the deep degradation path of *** work provided valuable insights into the development of efficient and economical catalysts for volatile organic compounds.

关键词： Cu-Ce supported catalyst Copper-cerium interaction Oxygen vacancies Toluene oxidation Reaction mechanism

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