检索结果-内蒙古大学图书馆

Glycine betaine modulates extracellular polymeric substances to enhance microbial salinity tolerance

environmental Science and Ecotechnology 2024年第4期20卷 259-268页

作者： Yan Xia Xinbai Jiang Shuaishuai Guo Yuxuan Wang Yang Mu Jinyou Shen Key Laboratory of Environmental Remediation and Ecological Health Ministry of Industry and Information TechnologySchool of Environmental and Biological EngineeringNanjing University of Science and TechnologyNanjing210094China CAS Key Laboratory of Urban Pollutant Conversion Department of Environmental Science and EngineeringUniversity of Science&Technology of ChinaHefei230026China

High salinity inhibits microbial activity in the bioremediation of saline *** alleviate osmotic stress,glycine betaine(GB),an osmoprotectant,is added to enhance the secretion of extracellular polymeric substances(EPS).These EPS are pivotal in withstanding environmental stressors,yet the intricate interplay between GB supplementation and microbial responses through EPS modificationsdencompassing composition,molecular architecture,and electrochemical featuresdremains elusive in hypersaline *** we show microbial strategies for salinity endurance by investigating the impact of GB on the dynamic alterations of EPS *** findings reveal that GB supplementation at 3.5%salinity elevates the total EPS(T-EPS)content from 12.50±0.05 to 24.58±0.96 mg per g dry cell *** observed shift in zeta potential from-28.95 to-6.25 mV at 0%and 3.5%salinity,respectively,with GB treatment,indicates a reduction in electrostatic repulsion and ***,the EPS protein secondary structure transition from b-sheet to a-helix,with GB addition,signifies a more compact protein configuration,less susceptible to salinity *** analyses,including cyclic voltammetry(CV)and differential pulse voltammetry(DPV),reveal GB's role in promoting the release of exogenous electron shuttles,such as flavins and c-type cytochromes(c-Cyts).The enhancement in DPV peak areas(Q_(DPV))with GB addition implies an increase in available extracellular electron transfer *** investigation advances our comprehension of microbial adaptation mechanisms to salinity through EPS modifications facilitated by GB in saline habitats.

关键词： High salinity Extracellular polymeric substances Glycine betaine Protein secondary structure Extracellular electron transfer

来源：评论

学校读者我要写书评

暂无评论

Enhanced Cd^(2+)removal from aqueous solution using olivine and magnesite combination:New insights into the mechanochemical synergistic effect

引用

Journal of environmental Sciences 2025年第1期147卷 714-725页

作者： Xiaofang Chen Chao Wang Min Chen Huimin Hu Junwei Huang Ting Jiang Qiwu Zhang School of Resources&Environmental Engineering Wuhan University of TechnologyWuhan 430070China State Environmental Protection Key Laboratory of Water Environmental Simulation and Pollution Control South China Institute of Environmental SciencesMinistry of Ecology and EnvironmentGuangzhou 510655China

In this study,an efficient stabilizer material for cadmium(Cd^(2+))treatment was successfully prepared by simply co-milling olivine with *** analyticalmethods including XRD,TEM,SEM and FTIR,combined with theoretical calculations(DFT),were used to investigate mechanochemical interfacial reaction between twominerals,and the reaction mechanism of Cd removal,with ion exchange between Cd^(2+)and Mg^(2+)as the main pathway.A fixation capacity of Cd^(2+)as high as 270.61 mg/g,much higher than that of the pristine minerals and even the individual/physical mixture of milled olivine and magnesite,has been obtained at optimized conditions,with a neutral pH value of the solution after treatment to allow its direct *** as-proposed Mg-based stabilizer with various advantages such as cost benefits,green feature etc.,will boosts the utilization efficiency of naturalminerals over the elaborately prepared adsorbents.

关键词： Olivine Magnesite Interface reaction Mechanochemical activation Cadmium removal

来源：评论

学校读者我要写书评

暂无评论

New insight into scale inhibition during tea brewing: Ca^(2+)/Mg^(2+) complexing and alkalinity consumption

引用

Journal of environmental Sciences 2023年第2期124卷 901-914页

作者： Linjun Li Jinsuo Lu Heliang Pang Zhiqiang Zhang Jing Yang Pengpeng Li Xiaoyu Yan Miaomiao Fan School of Environmental and Municipal Engineering Xi’an University of Architecture and TechnologyXi’an 710055China Shaanxi Key Laboratory of Environmental Engineering Xi’an University of Architecture and TechnologyXi’an 710055China State Key Laboratory of Green Building in West China Xi’an University of Architecture and TechnologyXi’an 710055China

Scale not only affects the taste and color ofwater,but also increases the risks of osteoporosis and cardiovascular diseases associated with drinking *** a popular beverage,tea is rich many substances that have considerable potential for scale inhibition,including protein,tea polyphenols and organic *** this study,the effect of tea brewing on scale formationwas *** was found that the proteins,catechins and organic acids in tea leaves could be released when the green tea was brewed in water with sufficient hardness and *** tea-released protein was able to provide carboxyl groups to chelate with calcium ions(Ca^(2+)),preventing the Ca^(2+)from reacting with the carbonate ions(CO_(3)^(2-)).The B rings of catechins were another important structure in the complexation of Ca^(2+)and magnesium ions(Mg2+).The carboxyl and hydroxyl groups on the organic acids was able to form fivemembered chelating rings with Ca^(2+)and Mg^(2+),resulting in a significant decrease in Ca^(2+)from 100.0 to 60.0 mg/***,the hydrogen ions(H^(+))provided by the organic acids consumed and decreased the alkalinity of the water from 250.0 to 131.4 mg/L,leading to a remarkable reduction in pH from 8.93 to *** further prevented the bicarbonate(HCO_(3)^(-))from producing CO_(3)^(2−)when the water was *** reaction of the tea constituents with the hardness and alkalinity inhibited the formation of scale,leading to a significant decrease in turbidity from 10.6 to 1.4 ***,this study provides information to help build towards an understanding of the scale inhibition properties of tea and the prospects of tea for anti-scaling in industrial applications.

关键词： Scale inhibition Tea brewing Chelation Hardness Alkalinity

来源：评论

学校读者我要写书评

暂无评论

Confined seepage analysis of saturated soils using fuzzy fields

引用

Journal of Rock Mechanics and Geotechnical engineering 2025年第3期17卷 1302-1320页

作者： Nataly A.Manque Kok-Kwang Phoon Yong Liu Marcos A.Valdebenito Matthias G.R.Faes Reliability Engineering TU Dortmund UniversityDortmund44227Germany Singapore University of Technology and Design Singapore487372Singapore State Key Laboratory of Water Resources Engineering and Management Wuhan UniversityWuhan430072China

Seepage refers to the flow of water through porous *** phenomenon has a crucial role in dam,slope,excavation,tunnel,and well *** seepage analysis usually is a challenging task,as one must cope with the uncertainty associated with the parameters such as the hydraulic conductivity in the horizontal and vertical directions that drive this ***,at the same time,the data on horizontal and vertical hydraulic conductivities are typically scarce in spatial *** this context,so-called non-traditional approaches for uncertainty quantification(such as intervals and fuzzy variables)offer an interesting alternative to classical probabilistic methods,since they have been shown to be quite effective when limited information on the governing parameters of a phenomenon is ***,the main contribution of this study is the development of a framework for conducting seepage analysis in saturated soils,where uncertainty associated with hydraulic conductivity is characterized using fuzzy *** method to characterize uncertainty extends interval fields towards the domain of fuzzy *** fact,it is illustrated that fuzzy fields are an effective tool for capturing uncertainties with a spatial component,since they allow one to account for available physical measurements.A case study in confined saturated soil shows that with the proposed framework,it is possible to quantify the uncertainty associated with seepage flow,exit gradient,and uplift force effectively.

关键词： Fuzzy fields Interval fields Seepage analysis Hydraulic conductivity Spatial uncertainty

来源：评论

学校读者我要写书评

暂无评论

Donor-acceptor covalent organic frameworks-confined ultrafine bimetallic Pt-based nanoclusters for enhanced photocatalytic H_(2)generation

引用

Nano Research 2024年第7期17卷 5835-5844页

作者： Yu Liu Yawen Shi Hua Wang Shengbo Zhang Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) Key Laboratory for Green Chemical Technology of the Ministry of EducationSchool of Chemical Engineering and TechnologyTianjin UniversityTianjin 300350China School of Environmental Science and Engineering Tianjin Key Laboratory of Biomass/Wastes UtilizationTianjin UniversityTianjin 300350China

Photocatalytic hydrogen generation from hydrogen storage media is an effective and promising approach for the green hydrogen industry as well as for achieving carbon neutrality ***,the lower photocatalytic efficiency due to the limited light trapping capacity,low electron transfer rate,and severe aggregation of nanoparticles caused by high surface energy seriously restricts their practical ***,we constructed a series of donor–acceptor(D–A)type covalent organic frameworks to confine ultrafine bimetallic Pt-based nanoclusters for photocatalytic hydrogen generation from ammonia borane(AB)*** visible light irradiation at 20℃,PtCo_(2)@covalent organic framework(COF)showed the highest photocatalytic activity with a turnover frequency(TOF)of 486 min−*** and density functional theory(DFT)calculations reveal that the high catalytic activity is mainly attributed to the strong electronic interactions between D–A type COF and ultrafine PtCo_(2)***,the D–A type COF can significantly enhance the light-trapping ability by fine-tuning the electron-acceptor type in the framework,and accelerate the photogenerated electron transfer from D–A type COF to PtCo_(2)nanocluster,which promotes the adsorption and activation of H_(2)O and AB molecules and accelerates hydrogen ***,PtCo_(2)@COF also exhibited ultra-high durability due to the significantly enhanced resistance to nanocluster aggregation caused by the nanopore confinement effect of D–A type *** believe that this work will provide a theoretical guide for the rational design of efficient D–A COFbased catalysts for photocatalysis.

关键词： light trapping electron transfer donor-acceptor covalent organic frameworks(D-A COFs) bimetallic nanoclusters photocatalysis

来源：评论

学校读者我要写书评

暂无评论

Pt nanoclusters modified porous g-C_(3)N_(4)nanosheets to significantly enhance hydrogen production by photocatalytic water reforming of methanol

引用

Chinese Journal of Chemical engineering 2024年第2期66卷 40-50页

作者： Yi-Fei Liang Jin-Rong Lu Shang-Kun Tian Wen-Quan Cui Li Liu Hebei Provincial Key Laboratory of Environmental Photocatalytic and Electrocatalytic Materials College of Chemical EngineeringNorth China University of Science and TechnologyTangshan 063210China

For the use of green hydrogen energy,it is crucial to have efficient photocatalytic activity for hydrogen generation by water reforming of methanol under mild *** attention has been paid to gC_(3)N_(4)as a promising photocatalyst for the generation of *** improve the separation of photogenerated charge,porous nanosheet g-C_(3)N_(4)was modified with Pt nanoclusters(Pt/g-C_(3)N_(4))through impregnation and following photo-induced *** catalyst showed excellent photocatalytic activity of water reforming of methanol fo r hydrogen production with a 17.12 mmol·g^(-1)·h^(-1)rate at room temperature,which was 311 times higher than that of the unmodified g-C_(3)N_(4).The strong interactions of Pt-N in Pt/g-C_(3)N_(4)constructed effective electron transfer channels to promote the separation of photogenerated electrons and holes *** addition,in-situ infrared spectroscopy was used to investigate the intermediates of the hydrogen production reaction,which proved that methanol and water eventually turn into H_(2)and CO_(2)via formaldehyde and *** study provides insights for understanding the photocatalytic hydrogen production in the water reforming of methanol.

关键词： Water reforming of methanol Photocatalysis g-C_(3)N_(4) Pt nanoclusters Hydrogen production

来源：评论

学校读者我要写书评

暂无评论

Research on Knowledge Representation Methods for Fire Incidents Based on Knowledge Graphs 5

Research on Knowledge Representation Methods for Fire Incide...

引用

5th International Conference on System reliability and Safety engineering, SRSE 2023

作者： Chu, Qiaohui Chen, Ying Beihang University Science and Technology on Reliability and Environmental Engineering Laboratory Beijing China

ISBN: (纸本)9798350305944

Sudden fire incidents have become one of the most frequent and common major disasters that threaten public safety and social development. The data released by authorities is mostly represented in text form, which provides limited and unclear descriptions of emergency response procedures. The low level of data structuring results in some data being unable to be effectively transformed into valuable information for reuse, leading to the wastage of data resources and hindering further processing as well as subsequent applications of case event information. In order to structure and process fire incident information, and enhance the value of information utilization for assisting decision-making, we focus on the fire incident data recorded in a state in the United States as the case data. Considering the characteristics of fire incident data, knowledge representation learning methods based on knowledge graphs such the TransE model and the TransH model are applied. By adopting the idea of distributed representation, the data is embedded into low-dimensional dense vectors, which can significantly improve computational efficiency, alleviate data sparsity issues, and meet the requirements of downstream applications. Finally, the effectiveness of the proposed research method is validated by evaluating the embedding effects of the knowledge representation process using the evaluation metrics of link prediction tasks. Our experimental results demonstrate that TransH significantly outperforms TransE on link prediction tasks. © 2023 IEEE.

关键词： Fires

来源：评论

学校读者我要写书评

暂无评论

In situ reconstruction induced oxygen-deficient multiphase Cu based species hybridized with Ni single atoms as tandem platform for CO_(2) electroreduction

引用

Nano Research 2024年第5期17卷 3888-3894页

作者： Juzhe Liu Yuheng Wang Pengpeng Mo Feng Yang Kaiqi Jiang Zhixiang Cheng Yuxuan Liu Zhiyi Sun Zheng Liu Yimei Zhang Wenxing Chen The Key Laboratory of Resources and Environmental System Optimization Ministry of EducationCollege of Environmental Science and EngineeringNorth China Electric Power UniversityBeijing 102206China Energy&Catalysis Center School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China SEPA Key Laboratory of Eco-Industry Chinese Research Academy of Environmental SciencesBeijing 100012China

Tandem catalysis,capable of decoupling individual steps,provides a feasible way to build a high-efficiency CO_(2) electro-conversion system for multicarbons(C_(2+)).The construction of electrocatalytic materials is one of focusing ***,we fabricated a single atom involved multivalent oxide-derived Cu composite material and found it inclined to reconstruct into oxygen-deficient multiphase Cu based species hybridized with monatomic Ni on N doped C *** this prototype,rapid CO generation and C-C coupling are successively achieved on NiN4 sites and surface amorphized Cu species with defects,resembling a micro-production *** this way,the in situ formed tandem catalyst exhibited a high Faradaic efficiency(FE)of~78%for C_(2+)products along with satisfactory durability over 50 ***,the reconstruction-induced amorphous layer with abundant asymmetric sites should be favorable to improve the ethanol selectivity(FE:63%),which is about 10 times higher than that of the non-tandem Cu-based contrast *** work offers a new approach for manipulating tandem catalyst systems towards enhancing C_(2+)products.

关键词： tandem catalysis single atom reconstruction amorphous CO_(2)reduction reaction

来源：评论

学校读者我要写书评

暂无评论

Competing esterification and oligomerization reactions of typical long-chain alcohols to secondary organic aerosol formation

引用

Journal of environmental Sciences 2023年第4期126卷 103-112页

作者： Jiaxin Wang Xiaohui Ma Yuemeng Ji Yongpeng Ji Yanpeng Gao Yuqi Xiao Guiying Li Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthInstitute of Environmental Health and Pollution controlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Key Laboratory of City Cluster Environmental Safety and Green DevelopmentSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Organosulfate (OSA) nanoparticles,as secondary organic aerosol (SOA) compositions,are ubiquitous in urban and rural ***,we systemically investigated the mechanisms and kinetics of aqueous-phase reactions of 1-butanol/1-decanol (BOL/DOL) and their roles in the formation of OSA nanoparticles by using quantum chemical and kinetic *** mechanism results show that the aqueous-phase reactions of BOL/DOL start from initial protonation at alcoholic OH^(-)groups to form carbenium ions (CBs),which engage in the subsequent esterification or oligomerization reactions to form OSAs/organosulfites (OSIs) or *** kinetic results reveal that dehydration to form CBs for BOL and DOL reaction systems is the rate-limiting ***,about 18%of CBs occur via oligomerization to dimers,which are difficult to further oligomerize because all reactive sites are *** rate constant of BOL reaction system is one order of magnitude larger than that of DOL reaction system,implying that relative short-chain alcohols are more prone to contribute OSAs/OSIs than long-chain *** results reveal that typical long-chain alcohols contribute SOA formation via esterification rather than oligomerization because OSA/OSI produced by esterification engages in nanoparticle growth through enhancing hygroscopicity.

关键词： Long-chain alcohols Organosulfates Aqueous phase reaction Reaction mechanisms Secondary organic aerosol

来源：评论

学校读者我要写书评

暂无评论

Recovering rare earths,lithium and fluorine from rare earth molten salt electrolytic slag using sub-molten salt method

引用

Journal of Rare Earths 2024年第9期42卷 1774-1781,I0005页

作者： Delong Yang Mingming Yu Yusufujiang Mubula Weiquan Yuan Zheyu Huang Bo Lin Guangjun Mei Tingsheng Qiu School of Resources and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou341000China Jiangxi Key Laboratory of Mining Engineering Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Environmental Engineering Wuhan University of TechnologyWuhan430070China Gannan Institute of Science and Technology Ganzhou341000China

Viewing the problem of high ene rgy consumption in the process of recovering rare earths from rare earth molten salt electrolysis slag,an environmentally friendly and low carbon process by sub-molten salt decomposition was *** thermodynamic analysis of sub-molten salt reaction indicates that the recovery of rare earths from the slag using sub-molten salt medium is thermodynamically *** this process,the rare earth fluoride and lithium in the slag are almost transformed into rare earth hydroxide,sodium fluoride and lithium hydroxide,fluorine and lithium are transferred into the washing solution,and the rare earths in the residues can be leached into solution by acid *** the optimum reaction conditions of reaction temperature 200℃,reaction time 3 h,NaOH initial concentration 80%,NaOH-Slag mass ratio 3:1,the leaching efficiency of rare earths,fluorine and lithium can reach to 99.05%,98.23% and 99.22%.After evaporation,the fluorine and lithium in the washing solution can be obtained in the forms of sodium fluoride and lithium fluoride,the recovery efficiency reach 95.5%and 92.8%,*** RE oxides(99.53%) can be obtained from the leaching solution after precipitation and roasting.

关键词： Rare earth electrolysis slag Sub-molten salt Green extraction Fluorine Lithium Recovery

来源：评论

学校读者我要写书评

暂无评论

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案：

请选择收藏分类：

通借通还

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：