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Diversity and dynamic response of anaerobic ammonia oxidation granular sludge

Journal of environmental Sciences 2025年第6期152卷 262-275页

作者： Jiahong Ye Xiang Li Yan Yuan Yayi Wang Yong Huang JunMa Han Wang Pengze Dang Pei-ling Xu School of Environmental Science and Engineering Suzhou University of Science and TechnologySuzhou 215009China State Key Laboratory of Pollution Control and Resources Reuse Shanghai Institute of Pollution Control and Ecological SecurityCollege of Environmental Science and EngineeringTongji UniversityShanghai 200092China State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090China

Red anaerobic ammonia oxidation (Anammox) granular sludge (AnGS) has been reported insuccessfully operating Anammox systems, and its color is associated with sludge ***, in long-term operating systems, AnGS exhibits different sensory colors, physicalstructures, community structures, and denitrification performance, but the relationship betweenthem has not yet been *** AnGS of the Anammox system, which has beenin operation for more than a decade, can be divided into twomain categories: red and *** specific Anammox activity (SAA) in conventional red AnGS increased continuously asthe particle size increased from <0.51 mm to 6.02 ± 0.84 mm. The SAA of white AnGS wereslightly lower than those of red AnGS with similarly-size granules but significantly higherthan AnGS with smaller red granules. Compared with red AnGS, the extracellular polymericsubstances of white AnGS were significantly reduced,mainly due to the higher intracellulariron content, resulting in lower heme c concentration. Thus, heme c may prove not to bean evaluative tool for measuring Anammox activity. Red and white AnGS, whether throughself-aggregation or adsorption by hydroxyl apatite and other carriers, will face the fate ofinternal voids during particle size growth. White AnGS exhibited amore complex microbialcommunity than red AnGS. Candidatus Brocadia was abundant in red AnGS and the abundanceincreased with increasing granule size. Candidatus Kuenenia and Candidatus Jetteniamade significant contributions to denitrification in white AnGS. This study provides a newperspective on particle selection for anammox engineering applications.

关键词： Anaerobic ammonium oxidation granular sludge Sensory diversity Intracellular iron Heme Enzyme activity Microbial diversity

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Fault Diagnosis Model for UAV with Small Sample Size and Imbalanced Data 15

Fault Diagnosis Model for UAV with Small Sample Size and Imb...

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15th IEEE Global reliability and Prognostics and Health Management Conference, PHM-Beijing 2024

作者： Song, Guoqing Ma, Ke Yang, Yang Dong, Yanchen Han, Danyang Suo, Mingliang School of Reliability and Systems Engineering Beihang University Beijing100191 China No.31850 People's Liberation Army of China Beijing102200 China Institute of Reliability Engineering National Key Laboratory of Science and Technology on Reliability and Environmental Engineering School of Reliability and Systems Engineering Beihang University Beijing100191 China

ISBN: (纸本)9798350354010

With the development of Unmanned Aerial Vehicles (UAV), their application scenarios and task requirements have become more complex, demanding higher standards for subsequent fault diagnosis and equipment maintenance. The actual flight data of UAV usually exhibits small sample sizes and imbalanced characteristics. To achieve more efficient fault prediction for UAV, this paper establishes a SMOTE-IWOA-RF fault diagnosis model. This model optimizes the Whale Optimization Algorithm (WOA) using chaotic initialization, nonlinear convergence factors, and Lévy flight strategies, resulting in better convergence accuracy and global search capability, as well as faster convergence speed. The model is compared with other classification models on data with different imbalance ratios, demonstrating that it is more efficient and accurate in UAV fault diagnosis, with the F1 score improving by about 10% compared to the pre-optimization state. Furthermore, the IWOA-RF model is combined with other data preprocessing methods, showing that SMOTE-IWOA-RF performs better on UAV operational data, indicating its practical value. © 2024 IEEE.

关键词： Fault detection

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The exposure risks associated with pathogens and antibiotic resistance genes in bioaerosol from municipal landfill and surrounding area

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Journal of environmental Sciences 2023年第7期129卷 90-103页

作者： Zhishu Liang Yun Yu Xiaolong Wang Wen Liao Guiying Li Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Guangdong Key Laboratory of Environmental Catalysis and Health Risk ControlSchool of Environmental Science and EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China

Pathogenic microbes with antibiotic resistance can thrive on municipal solid waste as nutrients and be aerosolized and transported to vicinities during waste disposal ***,the characterization of pathogenic bioaerosols and assessment of their exposure risks are ***,particle size,concentration,activity,antibiotic resistance,and pathogenicity of airborne microorganisms were assessed in different sectors of a typical *** showed that active sector in downwind direction has the highest bioaerosol level(1234 CFU/m3),while residential area has the highest activity(14.82 mg/L).Botanical deodorizer from mist cannon can effectively remove *** bioaerosols can be inhaled into respiratory system till bronchi with sizes ranging from 2.1−3.3 and 3.3−4.7μ*** bacteria(Bacilli,Bacillus,and Burkholderia-Paraburkholderia)and allergenic fungi(Aspergillus,Cladosporium,and Curvularia)prevailed in *** high abundance of microbial volatile organic compounds(mVOCs)producing bioaerosols were detected,these mVOCs contributed little to odor issues in ***,surrounding areas have higher levels of antibiotic-resistance genes(ARGs)than inner landfill with tetC,acrB,acrF,mdtF,and bacA as dominant *** ARGs were significantly correlated with bacterial community,while environmental parameters mainly influenced fungal *** findings can assist in reducing and preventing respiratory allergy or infection risks in occupational environments relating to waste management.

关键词： Bioaerosol Pathogenic community mVOCs Antibiotic-resistance genes Health risk Botanical deodorizer

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Peracetic acid catalytic activation using Co_(3)O_(4) nanocluster decorated graphitic carbon nitride for cefapirin degradation in water

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Science China(Technological Sciences) 2024年第10期67卷 3103-3115页

作者： YIN ShiMei GAO YiXuan CHEN Long LI Fan LIU XiaoNa QI Fei LIU Wen Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China Key Laboratory of Water and Sediment Sciences(Ministry of Education) College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China School of Environmental Science and Engineering Taiyuan University of TechnologyTaiyuan 030024China State Environmental Protection Key Laboratory of All Material Fluxes in River Ecosystems Peking UniversityBeijing 100871China Beijing National Laboratory for Molecular Sciences Peking UniversityBeijing 100871China

This study innovated cobalt-based catalytic nanocomposites(CCNs)for the heterogeneous activation of peracetic acid(PAA),a green and efficient advanced oxidation process for removing antibiotics from *** Co_(3)O_(4) catalysts exhibit limited activity due to stable electronic *** overcome this,CCNs were synthesized using a one-step condensation method,incorporating a size control strategy that anchors Co_(3)O_(4) nanoclusters within 4‒5 nm onto six-fold cavity of g-C3N4,simultaneously modifying the coordination environment of *** alteration significantly enhances the adsorption energy of PAA and catalytic activity compared to commercial Co_(3)O_(4).The improved performance of CCN2,in particular,is attributed to a shift in the cobalt d band center towards the Fermi level,facilitating electron delocalization and transfer,enhancing Co‒O bonding,and accelerating PAA ***2’s superior activity,with a cefapirin(CFP)degradation kinetic rate constant(k1=0.760 min^(−1))~11 times that of PAA direct oxidation(k1=0.070 min^(−1))and~5 times that of commercial Co_(3)O_(4)/PAA system(k1=0.164 min^(−1)),is due to its ability to generate dominant reactive species for antibiotic degradation,including alkoxy radicals(CH3C(=O)OO•),high valence metal(Co^(Ⅳ)(=O)^(2+)),and singlet oxygen(^(1)O_(2)),with the latter two being crucial for the degradation *** degradation of CFP involved three mechanisms,including direct oxidation by PAA,decarboxylation,and open-ring reactions at nitrogen *** research provides insights into developing high-activity catalysts for efficient PAA activation and antibiotic removal,leveraging the strategy of shifting the transition metal d band center.

关键词： peracetic acid Co_(3)O_(4)nanocluster high valence metal singlet oxygen cefapirin

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Underestimated contribution of fugitive emission to VOCs in pharmaceutical industry based on pollution characteristics, odorous activity and health risk assessment

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Journal of environmental Sciences 2023年第4期126卷 722-733页

作者： Qinhao Lin Zhong Gao Weikun Zhu Jiangyao Chen Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Technology Research Center for Photocatalytic Technology Integration and Equipment EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and Health Guangzhou Key Laboratory of Environmental Catalysis and Pollution ControlSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Fugitive emission has been becoming an important source of volatile organic compounds(VOCs) in pharmaceutical industry,but the exact contribution of fugitive emission remains incompletely *** present study,pollution characteristics,odorous activity and health risk of stack and fugitive emissions of VOCs from four functional units (e.g.,workshop,sewage treatment station,raw material storage and hazardous waste storage) of three representative pharmaceutical factories were *** was the dominant contributor to VOCs of fugitive emission in comparison with other functional *** high concentration of VOCs from fugitive emission in unsealed workshop (94.87 mg/m^(3))was observed relative to sealed one (1.18 mg/m^(3)),accounting for 31%and 5%of total VOCs,*** emission of VOCs in the unsealed workshop mainly consisted of nhexane,1-hexene and *** activity indexes and non-cancer hazard ratios of these VOCs from fugitive emission in the unsealed workshop were as high as that from stack ***,cancer risk of dichloromethane from fugitive emission and stack exhaust was up to (1.6-1.8)×10^(-5).Odorous activity or health risk index of the VOCs from fugitive emission was up to 13 or 11 times of the corresponding threshold value,posing remarkable health threat on pharmaceutical ***?ndings highlighted the possibly underestimated contribution of fugitive emission on VOCs in the pharmaceutical industry.

关键词： Pharmaceutical industry VOC pollution Fugitive emission Odorous activity index Health risk

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Progress on mechanical and tribological characterization of 2D materials by AFM force spectroscopy

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Friction 2024年第12期12卷 2627-2656页

作者： Shuai WU Jie GU Ruiteng LI Yuening TANG Lingxiao GAO Cuihua AN Qibo DENG Libin ZHAO Ning HU Key Laboratory of Hebei Province on Scale-span Intelligent Equipment Technology School of Mechanical EngineeringHebei University of TechnologyTianjin 300401China Advanced Equipment Research Institute Co. Ltd.of Hebei University of TechnologyTianjin 300401China Key Laboratory of Advanced Intelligent Protective Equipment Technology Ministry of EducationTianjin 300401China State Key Laboratory of Reliability and Intelligence Electrical Equipment Hebei University of TechnologyTianjin 300130China

Two-dimensional(2D)materials are potential candidates for electronic devices due to their unique structures and exceptional physical properties,making them a focal point in nanotechnology *** assessment of the mechanical and tribological properties of 2D materials is imperative to fully exploit their potential across diverse ***,their nanoscale thickness and planar nature pose significant challenges in testing and characterizing their mechanical *** the in situ characterization techniques,atomic force microscopy(AFM)has gained widespread applications in exploring the mechanical behaviour of nanomaterials,because of the easy measurement capability of nano force and displacement from the AFM ***,AFM-based force spectroscopy is a common approach for studying the mechanical and tribological properties of 2D *** review comprehensively details the methods based on normal force spectroscopy,which are utilized to test and characterize the elastic and fracture properties,adhesion,and fatigue of 2D ***,the methods using lateral force spectroscopy can characterize the interfacial properties of 2D materials,including surface friction of 2D materials,shear behaviour of interlayers as well as nanoflake-substrate *** influence of various factors,such as testing methods,external environments,and the properties of test samples,on the measured mechanical properties is also *** the end,the current challenges and issues in AFM-based measurements of mechanical and tribological properties of 2D materials are discussed,which identifies the trend in the combination of multiple methods concerning the future development of the in situ testing techniques.

关键词： two-dimensional(2D)materials atomic force microscopy(AFM) mechanical properties nanomechanical testing nanotribology

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Particulate matter capturing over manganese dioxides with different crystal structures

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Journal of environmental Sciences 2023年第5期127卷 667-677页

作者： Rui Liu Huan-Huan Yang Hao Zhou Xianliang Yi Yang Liu Key Laboratory of Industrial Ecology and Environmental Engineering(Ministry of Education) School of Ocean Science and TechnologyDalian University of TechnologyPanjin 124221China

Particulate matter(PM)is the main contributor to air pollution,and filtration has been reported to be promising for PM *** the complexity of polluted air(volatile organic compounds(VOCs)and ozone are likely concomitant with PM particles)and in view of the versatility of MnO_(2) for the degradation of VOCs and ozone,the feasibility of MnO_(2) materials as PM filteringmediawas investigated in this study,and the effect of crystal structure on PM filtration was *** with the layeredδ-MnO_(2),the MnO_(2) with tunnel structure(including 1×2-,2×2-and 3×3-MnO_(2))exhibited greatly enhanced PM removal efficiencies,and particularly,the 3×3-MnO_(2) possessed not only significant activity for adsorbing PM particles but also high utilization efficiency of the active *** properties of the adsorbents were studied by XRD,ATR,isothermal N_(2) adsorption,SEM and(HR)*** correlation between pore characteristics and particle elimination activity demonstrates that the most developed mesoporous structure of the 3×3-MnO_(2) sample played an important role in strengthening the PM adsorption *** comparison of the surface properties of the fresh and spent samples reveals that with respective to the occasion ofδ-MnO_(2),the structure of 3×3-MnO_(2) was robust enough to resist collapse after PM capturing and the great accommodation of the inorganic and organic PM substances in the voluminous pores induced strong affinity between PM particles and 3×3-MnO_(2).Thereby,a higher particle filtration ability was retained.

关键词： Particulate matter filtration Manganese oxides Crystal structure Pore structure

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Enhanced CO_(2) adsorption properties with bimetallic ZnCe-MOF prepared using a microchannel reactor

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Frontiers of Chemical Science and engineering 2025年第2期19卷 93-102页

作者： Pin Cui Ying Tang Aixia Guo Chenxu Wang Minmin Liu Wencai Peng Feng Yu Key Laboratory for Green Processing of Chemical Engineering of Xinjiang Bingtuan School of Chemistry and Chemical EngineeringShihezi UniversityShihezi 832003China Carbon Neutralization and Environmental Catalytic Technology Laboratory Bingtuan Industrial Technology Research InstituteShihezi UniversityShihezi 832003China

The use of metal-organic frameworks (MOFs) as CO_(2)-gas-capture materials has attracted extensive research attention. In this study, two types of MOFs—Zn-MOF and ZnCe-MOF—were synthesized utilizing the microchannel reaction method, with water being employed as the solvent. The specific surface area, pore size, and pore volume of Zn-MOF and ZnCe-MOF were 1566.4 and 15.6 m^(2)·g^(-1), 0.65 and 7.32 nm, as well as 1.65 and 0.03 cm^(3)·g^(-1), respectively. Furthermore, Ce doping not only increased the pore size of ZnCe-MOF but also its adsorption energy from −0.19 eV (Zn-MOF) to −0.53 eV (ZnCe-MOF). At 298 K, the adsorption capacities of Zn-MOF and ZnCe-MOF were 0.66 and 0.74 mmol·g^(-1), respectively. In addition, the CO_(2) adsorption behaviors of Zn-MOF and ZnCe-MOF were linear and logarithmic, respectively. Theoretical calculations show that the results of adsorption thermodynamic simulations were consistent with the experiments. Thus, the preparation of ZnCe-MOF materials using a microchannel reactor provides a new approach for the continuous preparation of MOFs.

关键词： Metal-organic framework microchannel reactor reaction mechanism CO_(2)capture adsorption

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Multimodal Machine Learning Guides Low Carbon Aeration Strategies in Urban Wastewater Treatment

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engineering 2024年第5期36卷 51-62页

作者： Hong-Cheng Wang Yu-Qi Wang Xu Wang Wan-Xin Yin Ting-Chao Yu Chen-Hao Xue Ai-Jie Wang State Key Laboratory of Urban Water Resource and Environment School of Civil and Environmental EngineeringHarbin Institute of Technology(Shenzhen)Shenzhen 518055China Key Laboratory of Drinking Water Safety and Distribution Technology of Zhejiang Province College of Civil Engineering and ArchitectureZhejiang UniversityHangzhou 310058China

The potential for reducing greenhouse gas(GHG)emissions and energy consumption in wastewater treatment can be realized through intelligent control,with machine learning(ML)and multimodality emerging as a promising ***,we introduce an ML technique based on multimodal strategies,focusing specifically on intelligent aeration control in wastewater treatment plants(WWTPs).The generalization of the multimodal strategy is demonstrated on eight ML *** results demonstrate that this multimodal strategy significantly enhances model indicators for ML in environmental science and the efficiency of aeration control,exhibiting exceptional performance and *** random forest with visual models achieves the highest accuracy in forecasting aeration quantity in multimodal models,with a mean absolute percentage error of 4.4%and a coefficient of determination of *** testing in a full-scale plant reveals that the multimodal model can reduce operation costs by 19.8%compared to traditional fuzzy control *** potential application of these strategies in critical water science domains is *** foster accessibility and promote widespread adoption,the multimodal ML models are freely available on GitHub,thereby eliminating technical barriers and encouraging the application of artificial intelligence in urban wastewater treatment.

关键词： Wastewater treatment Multimodal machine learning Deep learning Aeration control Interpretable machine learning

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Next generation desalination membrane with exceptional chlorine resistance

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Science China Chemistry 2024年第11期67卷 3500-3502页

作者： Shihong Lin Xinglin Lu Department of Civil and Environmental Engineering Vanderbilt UniversityNashville TN 37235USA CAS Key Laboratory of Urban Pollutant Conversion Department of Environmental Science and EngineeringNational Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230026China

This highlight draws inspiration from a recent publication in Science where Zhang and co-workers [1] from Nanjing University of Science and technology reported a novel multifunctional polyester reverse osmosis(RO) membrane and its application in seawater desalination. This research represents a notable advancement in the field, as polyester membranes may potentially compete with state-of-the-art polyamide RO membranes in the mainstream market.

关键词： polyester exceptional chlorine

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