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Flexible, self-cleaning, and high-performance ceramic nanofiber-based moist-electric generator enabled by interfacial engineering

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science China(Technological sciences) 2022年第2期65卷 450-457页

作者： WANG LiMing FENG LanLan SUN Zhao Yang HE XinYang WANG RongWu QIN XiaoHong YU JianYong Key Laboratory of Textile Science&Technology Ministry of EducationCollege of TextilesDonghua UniversityShanghai 201620China Innovation Center for Textile Science and Technology Donghua UniversityShanghai 201620China

Due to their long-term stability, even under extreme conditions, oxide ceramics have attracted significant attention in emerging fields like moist-electric generation. However, the inherent brittleness and low voltage output of oxide ceramic-based moistelectric generators(MEGs) limit their applications in wearable electronics. Herein, a facile strategy involving the combination of sol-gel electrospinning and calcination is used to fabricate flexible and freestanding Ti O_(2)/Zr O_(2)(TZ) composite nanofiber-based MEGs. The excellent flexibility of the TZ nanofiber membranes can be attributed to the suppression of their crystal structure transformation, dispersion of stress concentration, and reduction of crack propagation via interfacial engineering. The porous structure of the electrospun nanofiber membrane features an abundance of charged narrow channels for the diffusion of water molecules and generates a streaming potential. The optimal voltage output reached ~0.8 V, which is the highest value reported for an oxide ceramic-based MEG. Furthermore, the as-fabricated nanofiber-based MEG exhibits good self-cleaning capability to degrade organic pollutants under ultraviolet irradiation. By integrating mechanical flexibility, high performance, and a selfcleaning effect, this work presents a new idea for exploring diverse, efficient, and wearable oxide ceramic-based MEGs.

关键词： moist-electric generation ceramic nanofiber electrospinning flexible self-cleaning

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Reconfiguration and self-healing integrated Janus electrospinning nanofiber membranes for durable seawater desalination

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Nano Research 2023年第1期16卷 489-495页

作者： Huijie Liu Jiatai Gu Ye Liu Lei Yang Liming Wang Jianyong Yu Xiaohong Qin Key Laboratory of Textile Science&Technology of Ministry of Education College of TextilesDonghua UniversityShanghai 201620China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials International Joint Laboratory for Advanced Fiber and Lowdimension MaterialsCollege of Materials Science and EngineeringDonghua UniversityShanghai 201620China Innovation Center for Textile Science and Technology Donghua UniversityShanghai 201620China

Janus electrospinning nanofiber membranes have attracted extensive attention in the fields such as solar-driven interfacial desalination,liquid filtration,and waterproof and breathable ***,the Janus structures suffer from weak interfacial bonding and vulnerability to damage,making the durability and sustainability are highly sought after in real-word ***,we fabricate the simply reconfigurable and entirely self-healing Janus evaporator by electrospinning polypropylene glycol based polyurethane(PPG@PU)and polydimethylsiloxane based polyurethane-CNTs(PDMS@PU-CNTs)with different wettability,which are both designed based on dynamic Diels–Alder(DA)*** interface of the Janus membrane is stitched by the covalent bonds to directly improve the interface adhesion to 22 N·m−1,constructing an integrated evaporator,and thereby achieving a stable desalination rate of 1.34 kg·m−2·h−1 under one *** dissociation of DA networks allows the evaporators for self-healing and reconfiguration abilities,after which the photothermal performance is *** is the first work for the crosslinked self-healing polymer to be directly electrospun,achieving the improved interfacial bond and reconfiguration of entire evaporators,which presented promising new design principles and materials for interfacial solar seawater desalination.

关键词： Janus nanofiber membrane electrospinning interfacial bonding solar steam generation seawater desalination

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Antioxidative MXene@GA‑Decorated textile Assisted by Metal Ion for Efficient Electromagnetic Interference Shielding,Dual‑Driven Heating,and Infrared Thermal Camouflage

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Advanced Fiber Materials 2023年第6期5卷 2080-2098页

作者： Biaobiao Yan Xueming Bao Yilei Gao Man Zhou Yuanyuan Yu Bo Xu Li Cui Qiang Wang Ping Wang Key Laboratory of Science and Technology of Eco‑Textile Ministry of EducationJiangnan University1800 Lihu AvenueWuxi 214122People’s Republic of China

Two-dimensional transition metal carbide/nitride(MXene)-based textiles have been developed in many fields;however,the high sensitivity to oxidation and weak interfacial bonding hinder their ***,we present a strategy for the preparation of a highly antioxidative MXene@gallic acid(MXene@GA,MG)hybrid dispersion,and further covalently grafted it onto carboxylated cotton fabric through interaction with metal ions(Fe^(3+))for fabricating wearable multifunctional *** to the cross-linking effect of Fe^(3+)and the remarkable antioxidant activity of natural polyphenol GA,the MG coatings firmly adhere to the textile surfaces and can withstand conventional washing,exhibiting favorable service stability and potential application ***,the obtained MG-decorated textile has the inherent characteristics of good breathability,moisture permeability,flexibility,and biocompatibility of the original fabric,which are conducive to the wearability of smart ***,by utilizing the outstanding conductivity(~330 S/m)and photothermal convertibility of the MG coating,the functional textile achieves high electromagnetic interference(EMI)shielding efficiency(~35 dB),excellent dual-driven(Joule and solar)heating warmth retention,and infrared thermal *** to the green and scalable preparation process,favorable durability,excellent comfort,and multifunctionality,the MG-decorated textiles are anticipated to be promising candidates for the next generation of smart wearable personal protective clothing.

关键词： Antioxidative MXene@GA Metal ion-assisted deposition Durable stability Multifunctional protective textile

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Waste Cotton-Derived Fiber-Based Thermoelectric Aerogel for Wearable and Self-Powered Temperature-Compression Strain Dual-Parameter Sensing

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Engineering 2024年第8期39卷 235-243页

作者： Xinyang He Mingyuan Liu Jiaxin Cai Zhen Li Zhilin Teng Yunna Hao Yifan Cui Jianyong Yu Liming Wang Xiaohong Qin Key Laboratory of Textile Science&Technology Ministry of EducationCollege of TextilesDonghua UniversityShanghai 201620China Key Laboratory of Science and Technology of Eco-Textiles Ministry of EducationJiangnan UniversityWuxi 214122China Innovation Center for Textile Science and Technology Donghua UniversityShanghai 201620China

The rapid development of the global economy and population growth are accompanied by the production of numerous waste *** leads to a waste of limited resources and serious environmental pollution problems caused by improper *** rational recycling of wasted textiles and their transformation into high-value-added emerging products,such as smart wearable devices,is ***,we propose a novel roadmap for turning waste cotton fabrics into three-dimensional elastic fiber-based thermoelectric aerogels by a one-step lyophilization process with decoupled self-powered temperature-compression strain dual-parameter sensing *** thermoelectric aerogel exhibits a fast compression response time of 0.2 s,a relatively high Seebeck coefficient of 43μV·K^(-1),and an ultralow thermal conductivity of less than 0.04 W·m^(-1)·K^(-1).The cross-linking of trimethoxy(methyl)silane(MTMS)and cellulose endowed the aerogel with excellent elasticity,allowing it to be used as a compressive strain sensor for guessing games and facial expression *** addition,based on the thermoelectric effect,the aerogel can perform temperature detection and differentiation in self-powered mode with the output thermal voltage as the stimulus ***,the wearable system,prepared by connecting the aerogel-prepared array device with a wireless transmission module,allows for temperature alerts in a mobile phone application without signal interference due to the compressive strains generated during ***,our strategy is significant for reducing global environmental pollution and provides a revelatory path for transforming waste textiles into high-value-added smart wearable devices.

关键词： Waste textiles High value-added recycling Thermoelectrics Elasticity Decoupled sensing

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3D printing of glycerol-mediated alginate hydrogels with high strength and stiffness

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材料科学技术（英文版） 2025年第10期213卷 268-275页

作者： Deshuai Kong Biao Yang Hua Yuan Cong Du Yeqiang Tan State Key Laboratory of Bio-Fibers and Eco-Textiles Collaborative Innovation Center of Marine Biobased Fiber and Ecological Textile TechnologyInstitute of Marine Biobased MaterialsCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China

As a biomass material with biodegradability and biocompatibility,sodium alginate(SA)is a good candidate for constructing hydrogels for tissue-mimicking and biomedical scaffold fabricating through extrusion-based 3D printing ***,the mechanical strength and stiffness of alginate hy-drogels are still not comparable with biological tissues such as tendons and the printability of SA so-lutions is often ***,a novel strategy for 3D printing of alginate hydrogels with high mechanical performance is developed by using glycerol as a co-solvent for SA *** addition of glycerol(GL)enables the formation of a homogenous SA/GL solution with a high solid content of 12-20 wt.％and en-dows crosslinked SA hydrogels with high *** applying uniaxial stretches,hydrogel filaments prepared with concentrated SA/GL solutions reveal a high tensile strength of 36.6-161.3 MPa,Young's modulus of 59.2-1964.2 MPa,and elongation at break of 8.5％-106.2％due to the high orientated and closely packed SA ***/GL solutions become more solid-like with increasing SA concentration,and the solution with a solid content of 16 wt.％exhibits optimal 3D printability because of the appropri-ate rheological properties and thixotropic *** designing the deforming-and-fixing process,3D printed high-strength alginate hydrogels with complex structures are prepared,broadening the applica-tion of alginate hydrogels in load-bearing and biomedical fields.

关键词： Sodium alginate 3D printing High strength Anisotropic structure

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Conductive fibers for biomedical applications

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Bioactive Materials 2023年第4期22卷 343-364页

作者： Leqian Wei Shasha Wang Mengqi Shan Yimeng Li Yongliang Wang Fujun Wang Lu Wang Jifu Mao Key Laboratory of Textile Science&Technology Ministry of EducationCollege of TextilesDonghua UniversityShanghai201620China Key Laboratory of Textile Industry for Biomedical Textile Materials and Technology Donghua UniversityShanghai201620China School of Health and Life Sciences University of Health and Rehabilitation SciencesQingdao CityShandong Province266071China

Bioelectricity has been stated as a key factor in regulating cell activity and tissue function in electroactive ***,various biomedical electronic constructs have been developed to interfere with cell behaviors to promote tissue regeneration,or to interface with cells or tissue/organ surfaces to acquire physiological status via electrical *** from the outstanding advantages of flexibility,structural diversity,customizable mechanical properties,and tunable distribution of conductive components,conductive fibers are able to avoid the damage-inducing mechanical mismatch between the construct and the biological environment,in return to ensure stable functioning of such constructs during physiological ***,this review starts by presenting current fabrication technologies of conductive fibers including wet spinning,microfluidic spinning,electrospinning and 3D printing as well as surface modification on fibers and fiber *** provide an update on the biomedical applications of conductive fibers and fiber assemblies,we further elaborate conductive fibrous constructs utilized in tissue engineering and regeneration,implantable healthcare bioelectronics,and wearable healthcare *** conclude,current challenges and future perspectives of biomedical electronic constructs built by conductive fibers are discussed.

关键词： Conductive fibers Conductive biomaterials Tissue repair Implantable bioelectronics Wearable bioelectronics

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Interfacial Ru nanoclusters in tandem with single atoms on oxygen-vacancy regulated CeO_(2)for anion exchange membrane seawater-splitting

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Journal of Energy Chemistry 2025年第3期102卷 618-627页

作者： Yue Wang Jing Li Pengfei Yang Hongdong Li Guangrui Xu Yunmei Du Caixia Li Wei Jin Tianyi Ma Zexing Wu Lei Wang Key Laboratory of Eco-chemical Engineering Ministry of EducationInternational Science and Technology Cooperation Base of Eco-chemical Engineering and Green ManufacturingCollege of Chemistry and Molecular EngineeringCollege of Chemical EngineeringQingdao University of Science&TechnologyQingdao 266042ShandongChina College of Chemical Engineering Qingdao University of Science and TechnologyQingdao 266042ShandongChina College of Materials Science and Engineering Qingdao University of Science&TechnologyQingdao 266042ShandongChina College of Environment and Safety Engineering Qingdao University of Science and TechnologyQingdao 266042ShandongChina School of Environmental Science and Engineering Suzhou University of Science and TechnologySuzhou 215009JiangsuChina School of Science STEM CollegeRMIT University 3083VictoriaAustralia

A hydrogen spillover-bridged water dissociation/hydrogen formation could concurrently promote Volmer/Tafel process and improve the efficiency of hydrogen evolution reaction(HER)under alkaline ***,it is still challenging to promote occurrence of hydrogen spillover for the large interfacial transport barriers of H_(2)O and hydrogen on active ***,the strategy of energy barrier gradient to induce hydrogen spillover was proposed by constructing Ru nanoclusters coupled with single atom onto oxygen vacancy cerium dioxide(Ru/CeO_(2)-Ov-2).Density functional theory(DFT)calculations uncover that the adsorption/desorption of H2O occurs at the Ru clusters sites and then the dissociated H*spontaneously overflows from Ru clusters with high binding energy into the adjacent Ru single atom sites with low binding energy,which facilitate the hydrogen ***,the synthesized Ru/CeO_(2)-Ov-2 exhibits a small overpotential of 41 mV at 10 mA cm^(-2)and good stability at 500 mA cm^(-2)for 100 h in alkaline seawater,which could be ascribed to the rapid hydrogen spillover and strong coupling interaction between Ru and CeO_(2)-O_(v).This work provides a novel insight that synthesizing cooperative sites with energy barrier gradient helps to promote hydrogen spillover and accelerate the Volmer/Tafel process of HER.

关键词： Electrocatalyst CeO_(2) Ru Oxygen vacancy Hydrogen evolution reaction

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Molten metal-organic complex to synthesize versatile ultrathin nonlayered oxides

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Nano Research 2024年第4期17卷 3147-3155页

作者： Kaisi Liu Jiabin Wu Qun Li Hongrun Jin Yongxin Luo Bei Qi Simin Dai Jianquan Zhao Liang Huang Jun Zhou Hubei Key Laboratory of Biomass Fibers and Eco-Dyeing&Finishing Wuhan Textile UniversityWuhan 430200China Wuhan National Laboratory for Optoelectronics School of Optical and Electronic InformationHuazhong University of Science and TechnologyWuhan 430074China Analytical and Testing Center Huazhong University of Science and TechnologyWuhan 430074China

Two-dimensional(2D)materials have attracted a great deal of research interest because of their unique electrical,magnetic,optical,mechanical,and catalytic properties for various *** date,however,it is still difficult to fabricate most functional oxides as 2D materials unless they have a layered ***,we report a one-step universal strategy for preparing versatile non-layered oxide nanosheets by directly annealing the mixture of metal nitrate and dimethyl imidazole(2-MI).The 2-MI plays the key role for 2D oxides since 2-MI owns a very low molten point and sublimation temperature,in which its molten liquid can coordinate with metal ions,forming a metal-organic framework,and easily puffing by its gas molecules.A total of 17 materials were prepared by this strategy,including non-layered metal oxide nanosheets as well as metal/metal oxide loaded nitrogen-doped carbon *** as-prepared cobalt particle-loaded nitrogen-doped carbon nanosheets(Co@N/C)exhibit remarkable bifunctional oxygen reduction reaction(ORR)and oxygen evolution reaction(OER)electrocatalytic activity and ***,the Zn-air battery utilizing a Co@N/C catalyst exhibits high power density of 174.3 mW·cm^(-2).This facile strategy opens up a new way for large-scale synthesis of 2D oxides that holds great potential to push 2D oxides for practical applications.

关键词： non-layered oxide nanosheet metal/metal oxide@N/C oxygen evolution reaction(OER) oxygen reduction reaction(ORR) Zn-air battery

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Enzymatic synthesis of sodium alginate-g-poly (acrylic acid) grafting copolymers as a novel printing thickener

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Coloration technology 2022年第3期138卷 278-290页

作者： Zhang, Nan Tian, Zhensheng Yu, Yuanyuan Wang, Ping Zhou, Man Wang, Qiang Key Laboratory of Science and Technology of Eco-Textile Ministry of Education Jiangnan University Jiangsu Wuxi China

Grafting modification is a common method for improving the specific properties of polysaccharides. Herein, we synthesised sodium alginate-g-poly (acrylic acid) (NaAlg-g-PAA) as a novel printing thickener via catalysis of horseradish peroxidase and hydrogen peroxide in the presence of acetylacetone. The synthesised products were characterised by Fourier Transform–infrared spectroscopy and polar nuclear magnetic resonance spectroscopy, which confirmed that the PAA was successfully grafted onto the hydroxyl groups at carbon atoms (C2) of sodium alginate. The optimal grafting percentage and grafting efficiency reached 51% and 96%, respectively. Compared with native sodium alginate, the grafted copolymer NaAlg-g-PAA exhibited better thermal stability, rheological and printing properties. This work provides an efficient and promising approach for modifying polysaccharides like alginates and could be used as an alternative to conventional chemical modification. © 2021 Society of Dyers and Colourists.

关键词： Sodium alginate

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Predictably synthesizing a library of white-light-emitting perovskites

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science China Chemistry 2023年第3期66卷 760-767页

作者： Ludan Niu Lili Zhao Deyu Li Qian Chen Mingming Zhang Jing Luan Lei Wang Weigao Xu Jun Xing Key Laboratory of Eco-chemical Engineering Ministry of EducationCollege of Chemistry and Molecular EngineeringQingdao University of Science&TechnologyQingdao 266042China Key Laboratory of Mesoscopic Chemistry Ministry of EducationSchool of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China School of Materials Science and Technology Qingdao University of Science&TechnologyQingdao 266042China Shandong Engineering Research Center for Marine Environment Corrosion and Safety Protection College of Environment and Safety EngineeringQingdao University of Science and TechnologyQingdao 266042China

The low-dimensional organic-inorganic halide perovskites with self-trapped exciton emission have promising prospects for single-phase white-light emitters. However, so far, these broadband white-light-emitting(BWLE) perovskites were synthesized by trial-and-error testing spacing molecules. Here, we developed a steric hindrance regulation strategy to predictably synthesize BWLE perovskites. The molecules containing C–C(–NH_(2))–C groups were introduced into low-dimensional perovskites, which brings a large steric hindrance in-plane orientation. The bigger C–C(–NH_(2))–C bond angle would induce larger structural distortion in perovskites, which leads to the higher rate of self-trapping of excitons and the deeper self-trapping depth. The photoluminescence spectra of the synthesized perovskites can cover the cool-to-warm white light region. Overall, we fabricated a material library consisting of 40 kinds of BWLE compounds according to this strategy. Our findings develop a general strategy to synthesize BWLE perovskites and offer a material platform for optoelectronic applications.

关键词： white-light emission halide perovskite steric hindrance two-dimensional

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