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Dense carbon nanofiber self-supporting electrode fabricated by orientation/compaction strategy for high volumetric lithium storage capacity

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Progress in Natural science:Materials International 2025年第1期35卷 229-237页

作者： Haihui Liu Chaoqun Chen Qiang Xu Yan Song Xiangwu Zhang Chang Ma Tianjin Municipal Key Lab of Advanced Fiber and Energy Storage Technology Tiangong University CAS Key Laboratory of Carbon Materials Institute of Coal Chemistry Chinese Academy of Sciences Fiber and Polymer Science Program Department of Textile Engineering Chemistry and Science Wilson College of Textiles North Carolina State University

Low bulk density greatly restricts the large-scale application of electrospun carbon-based fiber membrane as electrode in energy storage devices. To solve the above challenges, herein an orientation-compaction densification strategy is proposed to enhance the bulk density and volumetric capacity of PAN-based carbon nanofiber membranes as self-supporting electrode used in lithium-ion batteries（LIBs）. Specifically, highly-oriented fibers are achieved by high-speed roller collecting during electrospinning, and compaction densification is conducted by hot-pressing treatment. The effects of collecting speed and hot-pressing pressure on the morphology, conductivity,bulk density, tensile strength, and flexibility of the obtained carbon nanofiber membrane are *** to conventional fiber membranes, of which fibers are disorderly stacked, the oriented fiber membrane is much easier to achieve dense stacking by compaction. The obtained dense carbon nanofiber membrane demonstrates a bulk density of 0.566 g cm-3, and shows a significantly-enhanced volumetric capacity(318.3 mA h cm-3), high-rate performance(86.6 mA h cm-3at 5 A g-1), and satisfactory cycling stability when used as selfsupporting electrode of LIBs.

关键词： Bulk density Densification Electrospinning Orientation-compaction Volumetric capacity

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High‑Speed Sirospun Conductive Yarn for Stretchable Embedded Knitted Circuit and Self‑Powered Wearable Device

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Advanced Fiber Materials 2023年第1期5卷 154-167页

作者： Li Niu Jin Wang Kai Wang Heng Pan Gaoming Jiang Chaoyu Chen Pibo Ma Engineering Research Center of Knitting Technology Ministry of EducationCollege of Textile Science and EngineeringJiangnan UniversityWuxi 214122China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200China

In the intelligent era,the textile technique is a high efficiency,mature and simple manufacturing solution capable of fabricat-ing fully flexible wearable ***,the external circuit with its integration and comfort limitations cannot satisfy the requirements of intelligent wearable and portable *** study presents an industrialized production method to fabricate core–shell structure conductive yarn for direct textile use,prepared by the high-speed sirospun *** integration and flexibility are significantly improved over previous *** sirospun conductive yarn(SSCY)and the intarsia technique can provide the SSCY seamless and convenient embedded knitted circuit(SSCY-EKC)to form a full textile electrical element as the channel of power and signals transmission,allowing for a stable resistance change and wide strain range for meeting practical *** based on the triboelectric nanogenerator(SSCY-TENG)can be designed as a caution carpet with attractive design and good washability for a self-powered sensor that recognizes human ***,intrinsic textile properties such as washability,softness,and comfort *** benefits such as excellent extension,fitting,and stretchability,the SSCY-EKC used herein can realize a fully flexible electrical textile with a high potential for physical detection,body gesture recognition,apparel fashion,and decoration.

关键词： Sirospun technique Embedded knitted circuit Intarsia technique Stretchable Wearable devices

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Influence of Bromo-Aromatic Substrates on Direct Arylation of EDOTs toward Higher Molecular Conjugate Polymer

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Chinese Journal of Polymer science 2025年第5期43卷 718-729页

作者： Xi-Lin Pei Quan Yang Yan-Lu Sun Wei Wu Jian-Yong Yu Yong He State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai201620China Innovation Center for Textile Science and Technology Donghua UniversityShanghai201620China School of Materials Science and Engineering Shanghai UniversityShanghai200444China

The influence of the electronic and steric properties of bromoaromatic substrates on direct arylation polymerization for synthesizing high-molecular-weight conjugated polymers was investigated through a combination of experiments and ***-aromatic substrates with electron-withdrawing fluoro substituents exhibited higher yields and degrees of polymerization under PPh3-assisted conditions compared to those with electron-donating or bulky methyl ***,excessive steric hindrance at ortho-sites or overly electrondeficient dibromoaromatic substrates leads to reaction *** indicated that electron-withdrawing substituents enhanced the electrophilicity of arylpalladium-PPh3intermediates,facilitating the activation of electron-rich arylative substrates and promoting polymer ***,steric hindrance from the substituents can influence the preferred reaction pathway,thereby increasing the real reaction *** experimental and computational results suggest that bromoaromatic substrates with optimized electron-deficient characteristics significantly improve monomer conversion and polymerization efficiency with n-hexylmethylether-substituted *** findings clarify how the electronic and steric properties of bromo-aromatic substrates affect EDOT derivative activation and are expected to aid in optimizing the polymerization conditions for the preparation of high-molecular-weight conjugated polymers.

关键词： 3,4-Ethylenedioxythiophene Direct arylation polymerization Bromo-aromatic substrate Concerted metalation-deptonation

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Occurrence and Decay of SARS-CoV-2 in Community Sewage Drainage Systems

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Engineering 2023年第7期26卷 214-219,I0008,I0009页

作者： Qian Dong 蔡俊雄刘艳臣凌海波 Qi Wang Luo-Jing Xiang Shao-Lin Yang Zheng-Sheng Lu Yi Liu Xia Huang 曲久辉 State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Hubei Provincial Academy of Eco-Environmental Sciences Wuhan 430072China Key Laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

The rapid spread of the coronavirus disease(COVID-19)pandemic in over 200 countries poses a substantial threat to human *** acute respiratory syndrome coronavirus 2(SARS-CoV-2),which causes COVID-19,can be discharged with feces into the drainage ***,a comprehensive understanding of the occurrence,presence,and potential transmission of SARS-CoV-2 in sewers,especially in community sewers,is still *** study investigated the virus occurrence by viral nucleic acid testing in vent stacks,septic tanks,and the main sewer outlets of community where confirmed patients had lived during the early days of the epidemic in Wuhan,*** results indicated that the risk of long-term emission of SARS-CoV-2 to the environment via vent stacks of buildings was low after confirmed patients were ***-CoV-2 were mainly detected in the liquid phase,as opposed to being detected in aerosols,and its RNA in the sewage of septic tanks could be detected for only four days after confirmed patients were *** surveillance of SARS-CoV-2 in sewage could be a sensitive indicator for the possible presence of asymptomatic patients in the community,though the viral concentration could be diluted more than ten times,depending on the sampling site,as indicated by the Escherichia coli *** comprehensive investigation of the community sewage drainage system is helpful to understand the occurrence characteristics of SARS-CoV-2 in sewage after excretion with feces and the feasibility of sewage surveillance for COVID-19 pandemic monitoring.

关键词： SARS-CoV-2 Transmission risk Drainage system Sewage Community

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High biomass yields of Chlorella protinosa with efficient nitrogen removal from secondary effluent in a membrane photobioreactor

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Journal of Environmental sciences 2024年第12期146卷 272-282页

作者： Min Yang Zhen Liu Aijie Wang Ingmar Nopens Hairong Hu Hong Chen School of Civil and Environmental Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China Key Laboratory of Dongting Lake Aquatic Eco-Environmental Control and Restoration of Hunan Province Changsha 410114China BIOMATH Department of Data Analysis and Mathematical ModellingGhent UniversityGent B 9000Belgium Key Laboratory of Environmental Biotechnology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China School of Materials Science and Engineering Hunan University of Science and TechnologyXiangtan 411201China

Further treatment of secondary effluents before their discharge into the receiving water bodies could alleviate water *** this study,the Chlorella proteinosa was cultured in a membrane photobioreactor to further remove nitrogen from the secondary *** effect of hydraulic retention time(HRT)on microalgae biomass yields and nutrient removal was *** results showed that soluble algal products concentration reduced in the suspension at low HRT,thereby alleviating microalgal growth *** addition,the lower HRT reduced the nitrogen limitation for Chlorella proteinosa’s growth through the phase-out of nitrogen-related functional *** a result,the productivity for Chlorella proteinosa increased from 6.12 mg/L/day at an HRT of 24 hr to 20.18 mg/L/day at an HRT of 8 *** highest removal rates of 19.7 mg/L/day,23.8 mg/L/day,and 105.4 mg/L/day were achieved at an HRT of 8 hr for total nitrogen(TN),ammonia,and chemical oxygen demand(COD),***,in terms of removal rate,TN and COD were the largest when HRT is 24 hr,which were 74.5%and 82.6%*** maximum removal rate of ammonia nitrogen was 99.2%when HRT was 8 hr.

关键词： Chlorella MPBR Fouling HRT SAP Nutrient

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CA-VTON: Correlation-Aware Image-Based Virtual Try-On Network 16

CA-VTON: Correlation-Aware Image-Based Virtual Try-On Networ...

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16th International Conference on Intelligent Human-Machine Systems and Cybernetics, IHMSC 2024

作者： Luo, Weihao Zhong, Yueqi Donghua University Ministry of Education College of Textiles Key Laboratory of Textile Science & Technology Shanghai China

ISBN: (纸本)9798331540241

Image-based virtual try-on technology aims to transfer a given clothing item onto the corresponding region of a human body image. Existing methods tend to suffer from generating significant amounts of artifacts, particularly when dealing with complex human poses or pose intersections. This limitation severely constrains the poses of input person image and consequently impacts the practicality of virtual try-on networks. To address this predicament, we propose a novel Correlation-Aware image-based Virtual Try-on Network (CA-VTON). Our method mainly consists of two components: a softmax-correlation-guided Optical Flow Warping Module (OFWM) to warp the clothing according to the pose of reference person, and a Try-on Image Synthesis Module (TISM) guided by pose correlation, which supervises the generation process of try-on results. Extensive qualitative and quantitative experiments validate the effectiveness of our proposed method. © 2024 IEEE.

关键词： Optical flows

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Ultra-high specific surface area activated carbon from Taihu cyanobacteria via KOH activation for enhanced methylene blue adsorption

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Chinese Journal of Chemical Engineering 2024年第3期67卷 106-116页

作者： Yifang Mi Wenqiang Wang Sen Zhang Yalong Guo Yufeng Zhao Guojin Sun Zhihai Cao Key Laboratory of Advanced Textile Materials and Manufacturing Technology and Engineering Research Center for Eco-Dyeing&Finishing of Textiles Ministry of EducationZhejiang Provincial Engineering Research Center for Green and Low-carbon Dyeing&FinishingZhejiang Sci-Tech UniversityHangzhou 310018China Key Laboratory for Technology in Rural Water Management of Zhejiang Province Zhejiang University of Water Resources and Electric PowerHangzhou 310018China

Cyanobacteria-based activated carbon(CBAC)was successfully prepared by pyrolysis-activation of Taihu *** the impregnation ratio and activated temperature were 2 and 800-C,respectively,the optimal CBACs possessed an ultra-high specific surface(2178.90 m^(2)·g^(-1))and plenty of micro-and meso-pores,as well as a high pore volume(1.01 cm^(3)·g^(-1)).Ascribed to ultra-high surface area,π-π interaction,electrostatic interaction,as well as hydrogen-bonding interactions,the CBACs displayed huge superiority in efficient dye *** saturated methylene blue adsorption capacity by CBACs could be as high as 1143.4 mg·g^(-1),superior to that of other reported biomass-activated *** adsorption was endothermic and modeled well by the pseudo-second-order kinetic,intra-particle diffusion,and Langmuir *** work presented the effectiveness of Taihu cyanobacteria adsorbent ascribed to its super large specific surface area and high adsorption ability.

关键词： Activated carbon Biomass Dye adsorption Taihu cyanobacteria

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C=C bond enables difluorideboron b-diketonate derivatives with high contrast mechanoresponsive luminescence for reversible writing and information encryption

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Journal of Materials Chemistry C 2024年第6期13卷 2868-2874页

作者： Xia, Yan Li, Geng Yin, Xiangkai Li, Jie Zhao, Juemin Guo, Kunpeng Tang, Yaxing Wang, Hua Ministry of Education Key Laboratory of Interface Science and Engineering in Advanced Materials College of Materials Science and Engineering Taiyuan University of Technology Taiyuan030024 China College of Textile Engineering Taiyuan University of Technology JinZhong030600 China

Promoting the contrast of mechanoresponsive luminescent materials is of great significance in the application of information storage and encryption. In this work, two D-p-A difluorideboron b-diketonate derivatives were developed by varying the structure of the p-bridge. By incorporating a C=C bond into the phenyl p-bridge of BF2-PhCz, BF2-PVCz with a phenyl vinyl p-unit achieved bathochromic fluorescence with a higher quantum yield and a higher contrast of mechanoresponsive luminescence (MRL). Theoretical calculations and experimental characterization revealed the C=C bond contributed to the enhanced oscillator strength of the molecule and head-to-head molecular packing in the crystal. The applications of reversible writing and information deep-encryption were then realized based on the high-contrast and reversible MRL behavior of BF2-PVCz. © The Royal Society of Chemistry 2025.

关键词： Cryptography

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Review of recent advances in ferrite-based materials:From synthesis techniques to electromagnetic wave absorption performance

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International Journal of Minerals,Metallurgy and Materials 2025年第3期32卷 591-608页

作者： Xingliang Chen Di Lan Luoting Zhou Hailing Liu Xiyu Song Shouyu Wang Zhuanyong Zou Guanglei Wu Shaoxing Key Laboratory of High Performance Fibers&Products Key Laboratory of Clean Dyeing and Finishing Technology of Zhejiang ProvinceShaoxing UniversityShaoxing 312000China School of Materials Science and Engineering Hubei University of Automotive TechnologyShiyan 442002China Chinatesta(Zhejiang)Testing Services Co. Ltd.Shaoxing 312000China Institute of Materials for Energy and Environment State Key Laboratory of Bio-fibers and Eco-textilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China

With the booming development of electronic information science and 5G communication technology,electromagnetic radi-ation pollution poses a huge threat and damage to *** novel and high-performance electromagnetic wave(EMW)ab-sorbers is an effective method to solve the above issue and has attracted the attention of many *** a typical magnetic material,ferrite plays an important role in the design of high-performance EMW absorbers,and related research focuses on diversified synthesis methods,strong absorption performance,and refined microstructure ***,we focus on the synthesis of ferrites and their composites and introduce recent advances in the high-temperature solid-phase method,sol-gel method,chemical coprecipitation method,and solvent thermal method in the preparation of high-performance EMW *** review aims to help researchers understand the advantages and disadvantages of ferrite-based EMW absorbers fabricated through these *** also provides important guidance and reference for researchers to design high-performance EMW absorption materials based on ferrite.

关键词： ferrite electromagnetic wave absorber sol-gel method magnetic material solvent thermal method

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Polyetherketoneketone/carbon fiber composites with an amorphous interface prepared by solution impregnation

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新型炭材料（中英文） 2024年第4期39卷 692-702页

作者： ZHANG Feng LI Bo-lan JIAO Meng-xiao LI Yan-bo WANG Xin YANG Yu YANG Yu-qiu ZHANG Xiao-hua MOE Key Laboratory of Textile Science&Technology College of TextilesInnovation Center for Textile Science and TechnologyDonghua UniversityShanghai 201620China Key Laboratory of Carbon Materials National Engineering Laboratory for Carbon Fiber TechnologyInstitute of Coal ChemistryChinese Academy of SciencesTaiyuan 030001China

Interfacial adhesion between carbon fibers(CF)and polyetherketoneketone(PEKK)is a key factor that affects the mechanical performances of their *** is therefore of great importance to impregnate the CF bundles with PEKK as effi-ciently as *** report that PEKK with a good dispersion in a mixed solution of 4-chlorophenol and 1,2-dichloroethane can be introduced onto CF surfaces by solution impregnation and curing at 280,320,340 and 360℃.The excellent wettability or infiltra-tion of the PEKK solution guarantees a full covering and its tight binding to CFs,making it possible to evaluate the interfacial shear strength(IFSS)with the microdroplet *** interior of the CF bundles is completely and uniformly filled with PEKK by solu-tion impregnation,leading to a high interlaminar shear strength(ILSS).The maximum IFSS and ILSS reached 107.8 and 99.3 MPa,*** superior shear properties are ascribed to the formation of amorphous PEKK in the small spaces between CFs.

关键词： Polyetherketoneketone Carbon fiber Wettability Amorphous adhesion Interfacial strength

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