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SpectrumChain: a disruptive dynamic spectrum-sharing framework for 6G

science China(information sciences) 2023年第3期66卷 26-39页

作者： Qihui WU Wei WANG Zuguang LI Bo ZHOU Yang HUANG Xianbin WANG College of Electronic and Information Engineering Nanjing University of Aeronautics and Astronautics Key Laboratory of Dynamic Cognitive System of Electromagnetic Spectrum Space Ministry of Industry and Information Technology No.8511 Research Institute of CASIC Department of Electrical and Computer Engineering Western University

The sixth-generation(6G) wireless network will support ubiquitous connectivity and diversified scenarios to satisfy the requirements of various emerging applications. Full spectrum is a key enabler for6G to achieve the ambitious goal of a Tbps-scale data rate. In this paper, we first review the scenario and potential spectrum plan for 6G and then focus on SpectrumChain, a blockchain-based dynamic spectrumsharing(DSS) framework for 6G. The unique characteristics of blockchain for DSS are presented along with key technologies. Finally, the conclusion and future development trends are discussed.

关键词： dynamic spectrum sharing blockchain 6G

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Sequence structure controllable polymerization-induced self-assembly

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science China Chemistry 2024年第1期67卷 390-397页

作者： Zi-Xuan Chang Ren-Man Zhu Chun-Yan Hong Wen-Jian Zhang Department of Polymer Science and Engineering University of Science and Technology of ChinaHefei 230026China Institute of Physical Science and Information Technology Anhui UniversityHefei 230601China Key Laboratory of Environment-Friendly Polymeric Materials of Anhui Province Anhui UniversityHefei 230601China

Polymerization-induced self-assembly(PISA)combines synthesis and self-assembly of artificial polymers in one-pot,which brings us one step closer to emulating ***,the reported PISA formulations primarily focus on developing nano-objects with new chemical compositions and rarely on structural regulation of polymers with specific ***,sequence structure controllable polymerization-induced self-assembly(SCPISA)is reported by using 7-(2-methacryloyloxyethoxy)-4-methylcoumarin(CMA)as a *** the copolymerization of 2-hydroxyethyl methacrylate(HEMA)and CMA,controlled incorporation of CMA units into the polymer chains can be realized by programmable light/heat ***-based P(HEMA-co-CMA)copolymers with the same composition but different sequence structures generate a range of ***,the morphologies of the resultant nano-objects can also be controlled by regulating the feed molar ratio of CMA and HEMA,which is similar to the conventional PISA,but the synthesis procedure is obviously simplified in *** versatility of the methodology is further demonstrated by the fabrication of different functional nano-objects with sequence structure-dependent morphologies in SCPISA systems with different functional monomers.

关键词： polymerization-induced self-assembly sequence-controlled polymers PET-RAFT polymerization

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Transfer learning enables the rapid design of single crystal superalloys with superior creep resistances at ultrahigh temperature

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npj Computational Materials 2024年第1期10卷 1718-1732页

作者： Fan Yang Wenyue Zhao Yi Ru Siyuan Lin Jiapeng Huang Boxuan Du Yanling Pei Shusuo Li Shengkai Gong Huibin Xu School of Materials Science and Engineering Beihang UniversityBeijing 100191China Key Laboratory of Aerospace Materials and Performance(Ministry of Education) Key Laboratory of High-temperature Structural Materials&Coating Technology(Ministry of Industry and Information Technology)BeijingChina Tianmushan Laboratory Yuhang District311115 HangzhouZhejiang ProvinceChina

Accelerating the design of Ni-based single crystal(SX)superalloys with superior creep resistance at ultrahigh temperatures is a desirable goal but extremely challenging *** the present work,a deep transfer learning neural network with physical constraints for creep rupture life prediction at ultrahigh temperatures is *** learning enables deep learning model breaks through the generalization performance barrier in the extrapolation space of ultrahigh temperature creep properties in the case of a very small dataset,which is the key to achieving the above design goal.

关键词： creep resistance ultrahigh

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Photothermal catalytic C-C coupling to ethylene from CO_(2) with high efficiency by synergistic cooperation of oxygen vacancy and half-metallic WTe_(2)

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Journal of Energy Chemistry 2024年第6期93卷 547-556,I0014页

作者： Xiaoyue Zhang Yong Yang Yingjie Hu Lijun Xiong Tianyu Wang Panjie Li Jinyou Shen Key Laboratory of Environmental Remediation and Ecological Health Ministry of Industry and Information TechnologySchool of Environmental and Biological EngineeringNanjing University of Science and TechnologyNanjing 210094JiangsuChina School of Chemistry and Chemical Engineering Nanjing University of Science and TechnologyNanjing 210094JiangsuChina Nanjing Key Laboratory of Advanced Functional Materials Nanjing Xiaozhuang UniversityNanjing 210094JiangsuChina Jiangsu Environmental Engineering Technology Co.Ltd Nanjing 210019JiangsuChina

Photothermal catalytic CO_(2) conversion provides an effective solution targeting carbon neutrality by synergistic utilization of photon and ***,the C-C coupling initiated by photothermal catalysis is still a big ***,a three-dimensional(3D)hierarchical W_(18)O_(49)/WTe_(2) hollow nanosphere is constructed through in-situ embodying of oxygen vacancy and tellurium on the scaffold of WO_(3).The light absorption towards near-infrared spectral region and CO_(2) adsorption are enhanced by the formation of half-metal WTe_(2) and the unique hierarchical hollow *** with the generation of oxygen vacancy with strengthened CO_(2) capture,the photothermal effect on the samples can be sufficiently exploited for activating the CO_(2) *** particular,the close contact between W_(18)O_(49)and WTe_(2) largely promotes the photoinduced charge separation and mass transfer,and thus the~*CHO intermediate formation and fixedness are *** a result,the C-C coupling can be evoked between tungsten and tellurium atoms on WTe_(2).The ethylene production by optimized W_(18)O_(49)/WTe_(2) reaches 147.6μmol g^(-1)with the selectivity of 80%.The in-situ diffuse reflectance infrared Fourier transform spectroscopy(DRIFTS)and density functional theory(DFT)calculations are performed to unveil the presence and significance of aldehyde intermediate groups in C-C *** half-metallic WTe_(2) cocatalyst proposes a new approach for efficient CO_(2) conversion with solar energy,and may especially create a new platform for the generation of multi-carbon products.

关键词： Photothermal catalysis Half-metal WTe_(2) C–C coupling Carbon neutrality

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Two-dimensional Cu-porphyrin nanosheet membranes for nanofiltration

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Nano Research 2023年第5期16卷 6290-6297页

作者： Jiahao Cai Shizheng Song Lijie Zhu Qipeng Lu Zong Lu Yanying Wei Haihui Wang School of Chemistry&Chemical Engineering Guangdong Provincial Key Lab of Green Chemical Product TechnologyState Key Laboratory of Pulp and Paper EngineeringSouth China University of TechnologyGuangzhou 510640China School of Instrument Science and Opto-Electronics Engineering Beijing Information Science and Technology UniversityBeijing 100192China School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083China Beijing Key Laboratory for Membrane Materials and Engineering Department of Chemical EngineeringTsinghua UniversityBeijing 100084China

A kind of two-dimensional(2D)metal-organic framework(MOF)material,Cu-meso-tetrakis(4-carboxyphenyl)porphine(Cu-TCPP)nanosheets with wrinkled and flat morphologies are used as building blocks to assemble membranes by vacuum filtration(VF)and electrophoretic deposition(EPD)as energy-efficient nanofiltration(NF)membranes to remove dyes from *** the nanosheets with wrinkled structure can provide additional water transport channels,thereby increasing the water permeance,in the premise of a high rejection(>97.0%)for the dye brilliant blue G(BBG)(1.60 nm×1.90 nm),the water permeance of the membrane assembled by the wrinkled nanosheets(~1170 nm)is about 4 times that of the membrane assembled by the flat nanosheets(~530 nm),reaching 16.39 L·m^(−2)·h^(−1)·bar^(−1).Additionally,the use of the relatively flat nanosheets and the membrane preparation method of electrophoretic deposition is more conducive to stack nanosheets orderly and reduce ***,the water permeance of the membrane prepared by EPD(~1170 nm)with flat nanosheets is about twice that of the membrane prepared by VF(~530 nm),achieving 9.40 L·m^(−2)·h^(−1)·bar^(−1)with similar rejection(>97.0%)of dye evans blue(EB)(3.10 nm×1.20 nm).Furthermore,these membranes still exhibit good separation performance at high pressure of 0.6 *** with diverse structures and various membrane fabrication processes provide new directions for the separation performance optimization of 2D MOF materials for water purification.

关键词： two-dimensional material membrane metal-organic framework(MOF) nanofiltration nanosheet morphology electrophoretic deposition

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Separation of chitin from shrimp shells enabled by transition metal salt aqueous solution and ionic liquid

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Chinese Journal of Chemical engineering 2023年第1期53卷 133-141页

作者： Mi Feng Bin He Xinyan Chen Junli Xu Xingmei Lu Cai Jia Jian Sun Key Laboratory of Molecular Medicine and Biotherapy Ministry of Industry and Information TechnologySchool of Life SciencesBeijing Institute of TechnologyBeijing 100081China Key Laboratory of Medical Molecule Science and Pharmaceutics Engineering Ministry of Industry and Information TechnologyAdvanced Research Institute of Multidisciplinary ScienceBeijing Institute of TechnologyBeijing 100081China CAS Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex SystemsState Key Laboratory of Biochemical EngineeringBeijing Key Laboratory of Ionic Liquids Clean ProcessInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemical and Engineering University of Chinese Academy of SciencesBeijing 100049China Innovation Academy for Green Manufacture Chinese Academy of SciencesBeijing 100190China

Chitin is a widely used important industrial polymer mainly from shrimp shells, but its commercial preparation is under the great challenge of serious pollution due to the requirement of HCl and Na ***, we demonstrated that high purity chitin can be obtained from waste shrimp shells(WSSs) by cascade separation with transition metal salt aqueous solution and ionic liquid(IL). Firstly, calcium carbonate of WSSs was effectively removed in the metal salt aqueous solution driven by the ion exchange interaction. Subsequently, 1-butyl-3-methylimidazolium chloride([Bmim]Cl) had bifunctional abilities to remove residual protein and introduced metal salts simultaneously by hydrogen bonding and coordination interactions. The key experimental factors affecting the separation process were systematically studied, including the type of metal salts, temperature, and [Bmim]Cl loading. After sequential treatment with a 20%(mass) Ni SO4aqueous solution at 130 ℃ and [Bmim]Cl at 150 ℃, the purity of a-chitin can be up to 96.5%(mass) that meets commercial requirements. The use of metal salts with higher coordination ability makes the preparation of chitin no longer depend on the commonly acid-base reaction, which is conducive to the preservation of chitin structure.

关键词： Chitin Ionic liquids Transition metal salts Separation Sustainability

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Polarization-induced photocurrent switching effect in heterojunction photodiodes

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Nano Research 2023年第4期16卷 5503-5510页

作者： Dingbo Chen Yu-Chang Chen Guang Zeng Yu-Chun Li Xiao-Xi Li Dong Li Chao Shen Nan Chi Boon S.Ooi David Wei Zhang Hong-Liang Lu State Key Laboratory of ASIC and System Shanghai Institute of Intelligent Electronics&SystemsSchool of MicroelectronicsFudan UniversityShanghai 200433China Key Laboratory for Information Science of Electromagnetic Waves Department of Communication Science and EngineeringFudan UniversityShanghai 200433China Photonics Laboratory Division of ComputerElectricaland Mathematical Sciences and EngineeringKing Abdullah University of Science and Technology(KAUST)Thuwal 23955-6900Kingdom of Saudi Arabia

The unipolar photocurrent in conventional photodiodes(PDs)based on photovoltaic effect limits the output modes and potential versatility of these devices in *** photodiodes with photocurrent switching are emerging as a promising solution for obtaining photoelectric devices with unique and attractive functions,such as optical logic ***,we design an all-solid-state chip-scale ultraviolet(UV)PD based on a hybrid GaN heterojunction with engineered bipolar polarized electric *** introducing the polarization-induced photocurrent switching effect,the photocurrent direction can be switched in response to the wavelength of incident light at 0 V *** particular,the photocurrent direction exhibits negative when the irradiation wavelength is less than 315 nm,but positive when the wavelength is longer than 315 *** device shows a responsivity of up to−6.7 mA/W at 300 nm and 5.3 mA/W at 340 nm,*** particular,three special logic gates in response to different dual UV light inputs are demonstrated via a single bipolar PD,which may be beneficial for future multifunctional UV photonic integrated devices and systems.

关键词： GaN heterostructure ultraviolet(UV)photodiodes bipolar photocurrent optical logic device

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Differentially Private and Heterogeneity-Robust Federated Learning With Theoretical Guarantee

IEEE Transactions on Artificial Intelligence

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IEEE Transactions on Artificial Intelligence 2024年第12期5卷 6369-6384页

作者： Wang, Xiuhua Wang, Shuai Li, Yiwei Fan, Fengrui Li, Shikang Lin, Xiaodong Huazhong University of Science and Technology Hubei Key Laboratory of Distributed System Security Hubei Engineering Research Center on Big Data Security School of Cyber Science and Engineering Wuhan430074 China University of Electronic Science and Technology of China National Key Laboratory of Wireless Communications Chengdu611731 China Xiamen University of Technology Fujian Key Laboratory of Communication Network and Information Processing Xiamen361024 China University of Guelph School of Computer Science GuelphONN1G 2W1 Canada

Federated learning (FL) is a popular distributed paradigm where enormous clients collaboratively train a machine learning (ML) model under the orchestration of a central server without knowing the clients' private raw data. The development of effective FL algorithms faces multiple practical challenges including data heterogeneity and clients' privacy protection. Despite that numerous attempts have been made to deal with data heterogeneity or rigorous privacy protection, none have effectively tackled both issues simultaneously. In this article, we propose a differentially private and heterogeneity-robust FL algorithm, named DP-FedCVR to mitigate the data heterogeneity by following the client-variance-reduction strategy. Besides, it adopts a sophisticated differential privacy (DP) mechanism where the privacy-amplified strategy is applied, to achieve a rigorous privacy protection guarantee. We show that the proposed DP-FedCVR algorithm maintains its heterogeneity-robustness though DP noises are incorporated, while achieving a sublinear convergence rate for a nonconvex FL problem. Numerical experiments based on image classification tasks are presented to demonstrate that DP-FedCVR provides superior performance over the benchmark algorithms in the presence of data heterogeneity and various DP privacy budgets. © 2020 IEEE.

关键词： Federated learning

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Enhanced piezoelectricity and lager strain in Bi0.5Li0.5HfO3 doped sodium potassium niobate-based ceramics with high Curie temperatures

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Ceramics International 2025年第15期51卷 20992-20998页

作者： Li, Yuxuan Peng, Zhanhui Chai, Qizhen Wang, Yuanhao Nie, Xinru Wei, Lingling Liang, Pengfei Wu, Di Chao, Xiaolian Yang, Zupei Key Laboratory for Macromolecular Science of Shaanxi Province Shaanxi Key Laboratory for Advanced Energy Devices Shaanxi Engineering Laboratory for Advanced Energy Technology School of Materials Science and Engineering Shaanxi Normal University Shaanxi Xi'an710062 China Electronic Materials Research Laboratory Key Laboratory of the Ministry of Education School of Electronic Science and Engineering Faculty of Electronic and Information Engineering Xi'an Jiaotong University Xi'an710049 China School of Physics and Information Technology Shaanxi Normal University Shaanxi Xi'an710062 China School of Chemistry and Chemical Engineering Shaanxi Normal University Shaanxi Xi'an710062 China

High-temperature electronic ceramics are indispensable in applications such as the automotive sector, aerospace, oil exploration and other fields. Potassium sodium niobate-based (KNN-based) ceramics have emerged as critical materials for the development of environmentally friendly high-temperature sensors, filters, and other electronic devices. However, achieving a combination of superior piezoelectric properties and a high Curie temperature in KNN-based ceramics remains a significant challenge. In this study, we employed a strategy of constructing an orthorhombic-tetragonal (O-T) phase boundary with the objective of enhancing the piezoelectric properties of KNN-based ceramics and introduced Li+ to optimize the Curie temperature. In (1-x)K0.48Na0.52NbO3-xBi0.5Li0.5HfO3 ceramics, we realized high piezoelectric constant ∼ 340 pC/N, large strain (∼0.21 %) and elevated Curie temperature (Tc ∼ 354 °C) simultaneously. These findings not only identify a promising candidate for high-temperature sensors and filters but also provide valuable insights for advancing the design of high Curie temperature and lead-free piezoelectric ceramics based on KNN systems. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Piezoelectricity

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Cascade equilibrium stage relaxation method by introducing equilibrium efficiency parameter

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Chinese Journal of Chemical engineering 2024年第2期66卷 145-156页

作者： Xuepu Cao Shengkun Jia Xing Qian Yiqing Luo Xigang Yuan College of Chemical and Pharmaceutical Hebei University of Science&TechnologyShijiazhuang 050018China School of Chemical Engineering and Technology State Key Laboratory of Chemical EngineeringTianjin UniversityTianjin 300072China College of Information Science and Technology Beijing University of Chemical TechnologyBeijing 100029China

Optimizing multistage processes,such as distillation or absorption,is a complex mixed-integer nonlinear programming(MINLP)*** integer into continuous variables and solving the easier nonlinear programming(NLP)problem is an optimization idea for the multistage *** this article,we propose a relaxation method based on the efficiency *** the efficiency parameter is 1or 0,the proposed model is equivalent to the complete existence or inexistence of the equilibrium *** non-integer efficiency represents partial existence.A multi-component absorption case shows a natural penalty for non-integer efficiency,which can assist the efficiency parameter converging to 0 or ***,its penalty is weaker than the existing relaxation models,such as the bypass efficiency *** a simple distillation case,we show that this property can weaken the nonconvexity of the optimization problem and increase the probability of obtaining better optimization results.

关键词： Mathematical modeling Absorption Distillation Optimization

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