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Ultrafast nanomanufacturing via high-temperature shock of La_(0.6)Sr_(0.4)CoO_(3)catalysts for overall water splitting

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Journal of Materials science & technology 2024年第24期191卷 1-7页

作者： Xiaoya Cui Wenyu Li Yanchang Liu Yumei Zhu Yanan Chen Cairong Gong Gang Xue School of Materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin Key Laboratory of Composite and Functional MaterialsTianjin UniversityTianjin 300072China School of Materials Science and Engineering Institute of New EnergyTianjin UniversityTianjin 300072China Key Laboratory of Special Functional Materials for Ecological Environment and Information Ministry of EducationHebei University of TechnologyTianjin 300132China

Electrochemical water splitting,as an effective sustainable and eco-friendly energy conversion strategy,can produce high-purity hydrogen(H_(2))and oxygen(O_(2))via hydrogen evolution reaction(HER)and oxygen evolution reaction(OER),respectively,altering the nonrenewable fossil ***,La_(0.6)Sr_(0.4)CoO_(3)perovskite oxide nanoparticles with an orthorhombic phase were synthesized within 2 min in a one-step reaction,using a rapid and efficient high-temperature shock(HTS)***,the as-prepared La_(0.6)Sr_(0.4)CoO_(3)with orthorhombic phase(HTS-2)exhibited better OER and HER performance than the hexagonal phase counterpart prepared using the traditional muffle furnace calcination *** electrocatalytic performance enhancement of orthorhombic La_(0.6)Sr_(0.4)CoO_(3)can be attributed to the novel orthorhombic structure,such as confined strontium segregation,a higher percentage of highly oxidative oxygen species,and more active sites on the *** facile and rapid synthesis technique shows great potential for the rational design and crystal phase engineering of nanocatalysts.

关键词： Perovskite oxides High-temperature shock Water splitting High Gibbs free energy Phase engineering

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Fabrication of bamboo-inspired continuous carbon fiber-reinforced SiC composites via dual-material thermally assisted extrusion-based 3D printing

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材料科学技术（英文版） 2025年第5期208卷 92-103页

作者： Sai Li Haitian Zhang Zhongliang Lu Fusheng Cao Ziyao Wang Yan Liu Xiaohui Zhu Shuai Ning Kai Miao Shaoyu Qiu Dichen Li State Key Laboratory for Manufacturing Systems Engineering School of Mechanical EngineeringXi'an Jiaotong UniversityXi'an 710049China State Key Laboratory for Manufacturing Systems Engineering School of Mechanical EngineeringXi'an Jiaotong UniversityXi'an 710049China School of Intelligent Manufacturing Modern Industry Xinjiang UniversityUrumqi 830046China Science and Technology on Reactor Fuel and Materials Laboratory Nuclear Power Institute of ChinaChengdu 610213China

Ceramic matrix composites(CMCs)structural components encounter the dual challenges of severe mechanical conditions and complex electromagnetic environments due to the increasing demand for stealth technology in aerospace *** address various functional requirements,this study integrates a biomimetic strategy inspired by gradient bamboo vascular bundles with a novel dual-material 3D print-ing *** distinct bamboo-inspired structural configurations Cf/SiC composites are designed and manufactured,and the effects of these different structural configurations on the CVI process are *** method is utilized to characterize the relationship between interface bonding strength and mechanical *** results reveal that the maximum flexural strength and fracture toughness reach 108.6±5.2 MPa and 16.45±1.52 MPa m1/2,respectively,attributed to the enhanced crack propagation resistance and path caused by the weak fiber-matrix ***,the bio-inspired configuration enhances the dielectric loss and conductivity loss,exhibiting a minimum reflection loss of-24.3 dB with the effective absorption band of 3.89 *** work introduces an innovative biomimetic strategy and 3D printing method for continuous fiber-reinforced ceramic composites,expanding the ap-plication of 3D printing technology in the field of CMCs.

关键词： 3D printing Cf/SiC composites Mechanical properties Electromagnetic wave absorption

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Phase-tailored assembly and encoding of dissipative soliton molecules

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Light(science & Applications) 2023年第6期12卷 1061-1070页

作者： Yusong Liu Siyun Huang Zilong Li Haoguang Liu Yixiang Sun Ran Xia Lisong Yan Yiyang Luo Huanhuan Liu Gang Xu Qizhen Sun Xiahui Tang Perry Ping Shum School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhanChina Key Laboratory of Optoelectronic Technology and Systems(Ministry of Education) Chongqing UniversityChongqingChina School of Engineering and Materials Science Queen Mary University of LondonLondonUK Department of Electronic and Electrical Engineering Southern University of Science and TechnologyShenzhenChina

Self-assembly of particle-like dissipative solitons,in the presence of mutual interactions,emphasizes the vibrant concept of soliton molecules in varieties of laser *** manipulation of the molecular patterns,held by the degrees of freedom of internal motions,still remains challenging to explore more efficient and subtle tailoring approaches for the increasing ***,we report a new phase-tailored quaternary encoding format based on the controllable internal assembly of dissipative soliton *** manipulation of the energy exchange of soliton-molecular elements stimulates the deterministic harnessing of the assemblies of internal ***-assembled soliton molecules are tailored into four phase-defined regimes,thus constituting the phase-tailored quaternary encoding *** phase-tailored streams are endowed with great robustness and are resistant to significant timing *** these results experimentally demonstrate the programmable phase tailoring and exemplify the application of the phase-tailored quaternary encoding,prospectively promoting high-capacity all-optical storage.

关键词： soliton dissipative quaternary

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Adaptive Graph Embedding With Consistency and Specificity for Domain Adaptation

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IEEE/CAA Journal of Automatica Sinica 2023年第11期10卷 2094-2107页

作者： Shaohua Teng Zefeng Zheng Naiqi Wu Luyao Teng Wei Zhang School of Computer Science and Technology Guangdong University of TechnologyGuangzhou 510006China Institute of Systems Engineering and Collaborative Laboratory for Intelligent Science and Systems Macao University of Science and TechnologyMacao 999078China School of Information Engineering Guangzhou Panyu PolytechicGuangzhou 511483China Faculty of Information Technology Monash University20 Exhibition Walk ClaytonVIC 3800Australia IEEE

Domain adaptation(DA) aims to find a subspace,where the discrepancies between the source and target domains are reduced. Based on this subspace, the classifier trained by the labeled source samples can classify unlabeled target samples *** approaches leverage Graph Embedding Learning to explore such a subspace. Unfortunately, due to 1) the interaction of the consistency and specificity between samples, and 2) the joint impact of the degenerated features and incorrect labels in the samples, the existing approaches might assign unsuitable similarity, which restricts their performance. In this paper, we propose an approach called adaptive graph embedding with consistency and specificity(AGE-CS) to cope with these issues. AGE-CS consists of two methods, i.e., graph embedding with consistency and specificity(GECS), and adaptive graph embedding(AGE).GECS jointly learns the similarity of samples under the geometric distance and semantic similarity metrics, while AGE adaptively adjusts the relative importance between the geometric distance and semantic similarity during the iterations. By AGE-CS,the neighborhood samples with the same label are rewarded,while the neighborhood samples with different labels are punished. As a result, compact structures are preserved, and advanced performance is achieved. Extensive experiments on five benchmark datasets demonstrate that the proposed method performs better than other Graph Embedding methods.

关键词： Adaptive adjustment consistency and specificity domain adaptation graph embedding geometrical and semantic metrics

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Femtosecond laser-induced periodic surface structures on hard and brittle materials

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science China(Technological sciences) 2024年第1期67卷 19-36页

作者： ZHAO GuoXu WANG Gong LI YunFei WANG Lei LIAN YuDong YU Yu ZHAO Hui WANG YuLei LU ZhiWei Center for Advanced Laser Technology Hebei University of TechnologyTianjin 300401China Hebei Key Laboratory of Advanced Laser Technology and Equipment Tianjin 300401China State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China School of Information and Electrical Engineering Hebei University of EngineeringHandan 056038China

Hard and brittle materials have high hardness,excellent optical stability,chemical stability,and high thermal ***,they have huge application potential in various fields,such as optical components,substrate materials,and quantum information,especially under harsh conditions,such as high temperatures and high *** laser direct writing technology has greatly promoted the development of femtosecond laser-induced periodic surface structure(Fs-LIPSS or LIPSS by a femtosecond laser)applications of hard and brittle materials due to its high precision,controllability,and three-dimensional processing *** far,LIPSSs have been widely used in material surface treatment,optoelectronic devices,and ***,a consensus has not been reached regarding the formation mechanism of LIPSSs on hard and brittle *** this paper,three widely accepted LIPSS formation mechanisms are introduced,and the characteristics and applications of LIPSSs on diamonds,silicon,silicon carbide,and fused silica surfaces in recent years are *** addition,the application prospects and challenges of LIPSSs on hard and brittle materials by a femtosecond laser are discussed.

关键词： laser-induced periodic surface structures hard and brittle materials femtosecond laser

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The synergistic effect of Lewis acidic etching V_(4)C_(3)(MXene)@CuSe_(2)/CoSe_(2) as an advanced cathode material for aluminum batteries

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Journal of Materials science & technology 2024年第10期177卷 205-213页

作者： Yi Wang Hanqing Gu Yong Lu Wenming Zhang Zhanyu Li Hebei Key Laboratory of Optic-Electronic Information and Materials National&Local Joint Engineering Laboratory of New Energy Photoelectric DevicesCollege of Physics Science and TechnologyHebei UniversityBaoding 071002China

Herein,we focused on the development of the V_(4)C_(3) MXene composite bimetallic selenide heterostruc-ture(V_(4)C_(3)@CuSe_(2)/CoSe_(2))as a cathode material for aluminum *** heterostructure was pre-pared through a Lewis melt salt etching and selenization *** capitalizing on the synergistic effect between the bimetallic selenide and V_(4)C_(3) MXene,V_(4)C_(3)@CuSe_(2)/CoSe_(2) exhibited rapid charge transfer and demonstrated superior discharge specific capacity compared to V_(4)C_(3) composite monometallic ***,the incorporation of V_(4)C_(3) improved the material's stability during charging/*** initial discharge specific capacity of V_(4)C_(3)@CuSe_(2)/CoSe_(2) reached an impressive 809 mAh g^(-1) at 1 Ag^(-1).Even after nearly 3000 cycles,it retained a substantial capacity of 169.1 mAh g^(-1).Ex-situ XPS analysis confirmed the reversible valence transitions of Cu,Co,and Se elements as the main energy storage reac-tions taking place in the cathode *** functional theory analysis provided further insights,revealing that the strong metallic behavior of the heterostructure stemmed from the charge rearrange-ment facilitated by the bimetallic selenide structure and the optimization of the energy level ***,the presence of the bimetallic selenide structure significantly improved the adsorption ef-ficiency of[AlCl4]^(-).Overall,this research contributes to the advancement of rechargeable aluminum ion batteries and presents a promising avenue for future developments in composite metal selenide struc-tures and MXene-based materials.

关键词： Rechargeable aluminum batteries V_(4)C_(3) MXene Bimetallic selenides Heterostructure Electrochemical performance

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Knowledge Transfer Learning via Dual Density Sampling for Resource-Limited Domain Adaptation

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IEEE/CAA Journal of Automatica Sinica 2023年第12期10卷 2269-2291页

作者： Zefeng Zheng Luyao Teng Wei Zhang Naiqi Wu Shaohua Teng the School of Computer Science and Technology Guangdong University of TechnologyGuangzhou 510006China the School of Information Engineering Guangzhou Panyu PolytechicGuangzhou 511483China the Faculty of Information Technology Monash University20 Exhibition Walk ClaytonVIC 3800Australia IEEE the Institute of Systems Engineering and Collaborative Laboratory for Intelligent Science and Systems Macao University of Science and TechnologyMacao 999078China

Most existing domain adaptation(DA) methods aim to explore favorable performance under complicated environments by ***,there are three unsolved problems that limit their efficiencies:ⅰ) they adopt global sampling but neglect to exploit global and local sampling simultaneously;ⅱ)they either transfer knowledge from a global perspective or a local perspective,while overlooking transmission of confident knowledge from both perspectives;and ⅲ) they apply repeated sampling during iteration,which takes a lot of *** address these problems,knowledge transfer learning via dual density sampling(KTL-DDS) is proposed in this study,which consists of three parts:ⅰ) Dual density sampling(DDS) that jointly leverages two sampling methods associated with different views,i.e.,global density sampling that extracts representative samples with the most common features and local density sampling that selects representative samples with critical boundary information;ⅱ)Consistent maximum mean discrepancy(CMMD) that reduces intra-and cross-domain risks and guarantees high consistency of knowledge by shortening the distances of every two subsets among the four subsets collected by DDS;and ⅲ) Knowledge dissemination(KD) that transmits confident and consistent knowledge from the representative target samples with global and local properties to the whole target domain by preserving the neighboring relationships of the target *** analyses show that DDS avoids repeated sampling during the *** the above three actions,confident knowledge with both global and local properties is transferred,and the memory and running time are greatly *** addition,a general framework named dual density sampling approximation(DDSA) is extended,which can be easily applied to other DA *** experiments on five datasets in clean,label corruption(LC),feature missing(FM),and LC&FM environments demonstrate the encouraging performance of KTL-DDS.

关键词： Cross-domain risk dual density sampling intra-domain risk maximum mean discrepancy knowledge transfer learning resource-limited domain adaptation

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Cold sintered BaTiO_(3)–poly(ether imide)nanocomposites with superior comprehensive performances

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Journal of Advanced Ceramics 2024年第9期13卷 1453-1460页

作者： Xinyi Li Li Li Mingming Si Xiaoqian Tai Hong Wang Jing Guo State Key Laboratory for Mechanical Behavior of Materials&School of Materials Science and Engineering Xi’an Jiaotong UniversityXi’an 710049China Guangdong Provisional Key Laboratory of Functional Oxide Materials and Devices Southern University of Science and TechnologyShenzhen 518055China Department of Materials Science and Engineering&Shenzhen Engineering Research Center for Novel Electronic Information Materials and Devices Southern University of Science and TechnologyShenzhen 518055China

With the rapid development of the electronics industry,the demand for dielectric materials with high permittivities,low losses,and excellent electrical breakdown strengths prepared via low-temperature fabrication techniques is ***,we propose a one-step cold sintering process route to improve the comprehensive performance of BaTiO_(3)−based ceramics by integrating polyetherimide(PEI).Dense BaTiO_(3)–PEI nanocomposites can be prepared via a cold sintering process at 250℃ using Ba(OH)_(2)∙8H_(2)O and H_(2)TiO_(3) as the transient liquid *** grain growth of BaTiO_(3) is inhibited,and thin PEI layers less than 10 nm in size are located at the grain *** dissolution‒precipitation process triggered by the transient liquid phase and viscous flow assisted by PEI dominates the cold sintering mechanism of the(1−x)BaTiO_(3)–xPEI *** dielectric properties are stable over a broad temperature range up to 200℃.Compared with BaTiO_(3),80%BaTiO_(3)–20%PEI has superior performance,with a relative permittivity of 163 and a low dielectric loss of 0.014,and the electrical breakdown strength is increased by 80.65%compared with BaTiO_(3).Overall,the cold sintering process provides a potential way to develop dielectric nanocomposites with excellent comprehensive performance.

关键词： cold sintering process(CSP) dielectrics BaTiO_(3) ceramic-polymer composites

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Enhancing fairness of trading environment:discovering overlapping spammer groups with dynamic co‑review graph optimization

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Cybersecurity 2025年第2期8卷 242-269页

作者： Chaoqun Wang Ning Li Shujuan Ji Xianwen Fang Zhen Wang Shandong Provincial Key Laboratory of Wisdom Mine Information Technology Shandong University of Science&TechnologyQingdao 266590ShandongChina Anhui Province Engineering Laboratory for Big Data Analysis and Early Warning Technology of Coal Mine Safety Anhui University of Science and TechnologyHuainanChina

Within the thriving e-commerce landscape,some unscrupulous merchants hire spammer groups to post misleading reviews or ratings,aiming to manipulate public perception and disrupt fair market *** phenomenon has prompted a heightened research focus on spammer groups *** the e-commerce domain,current spammer group detection algorithms can be classified into three categories,i.e.,Frequent Item Mining-based,graph-based,and burst-based ***,existing graph-based algorithms have limitations in that they did not adequately consider the redundant relationships within co-review graphs and neglected to detect overlapping members within spammer *** address these issues,we introduce an overlapping spammer group detection algorithm based on deep reinforcement learning named ***,the algorithm filters out highly suspicious products and gets the set of reviewers who have reviewed these ***,taking these reviewers as nodes and their co-reviewing relationships as edges,we construct a homogeneous co-reviewing ***,to efficiently identify and handle the redundant relationships that are accidentally formed between ordinary users and spammer group members,we propose the Auto-Sim algorithm,which is a specifically tailored algorithm for dynamic optimization of the co-reviewing graph,allowing for adjustments to the reviewers’relationship network within the ***,candidate spammer groups are discovered by using the Ego-Splitting overlapping clustering algorithm,allowing overlapping members to exist in these ***,these groups are refined and ranked to derive the final list of spammer *** results based on real-life datasets show that our proposed DRL-OSG algorithm performs better than the baseline algorithms in Precision.

关键词： Spammer groups Homogeneous network Redundant relationships Overlapping members Deep reinforcement learning Ego-splitting algorithm

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Rapid Reconnaissance of Fixed Targets on the ground by Multiple UAVs

Rapid Reconnaissance of Fixed Targets on the ground by Multi...

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2024 International Conference on Remote Sensing, Mapping, and Image Processing, RSMIP 2024

作者： Yao, Kaiqi Liu, Bin Zhu, Xianqiang National University of Defense Technology Science and Technology on Information Systems Engineering Laboratory Changsha China

ISBN: (纸本)9781510680012

UAV reconnaissance has many advantages, such as high reliability, strong flexibility and wide coverage. When using unmanned aerial vehicles to scout targets, it is often necessary to quickly scout many fixed targets. If it is obviously unreasonable to send one unmanned aerial vehicle for each target, it is also unreasonable to send one unmanned aerial vehicle to scout all targets. At the same time, we should also consider the actual needs, such as our own safety and the number of airport reconnaissance drones. Considering many factors, a fast reconnaissance model of multi-UAV fixed targets on the ground is established, and the minimum number of UAV sorties needed for reconnaissance of all targets is obtained by combining branch and bound method and modified combined optimization algorithm. The modified Dijkstra algorithm is used to determine the appropriate delivery point, which can meet the actual requirements of rapid reconnaissance in the battlefield, considering the factors such as air defense firepower range and transportation conditions. Finally, the feasibility of the model is verified by using simulation data, and the benefits and possible improvements of the model are analyzed. © 2024 SPIE.

关键词： Branch and bound method

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