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Fe doping 1T phase MoS_(2)with enhanced zinc-ion storage ability and durability for high-performance aqueous zinc-ion batteries

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Rare Metals 2025年第1期44卷 253-263页

作者： Jing-Yi Liu Rong-Jie Zhe Zhan-Hong Peng Yi-Hui Song Lin-Xuan Yang Chen Qing Jun-Ling Guo Jin-Ping Liu Yunnan Key Laboratory of Opto-Electronic Information Technology College of Physics and Electronic Information TechnologyYunnan Normal UniversityKunming 650000China Country State Center for International Cooperation on Designer Low-Carbon and Environmental Materials School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China School of Chemistry Chemical Engineering and Life ScienceState Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070China

As a promising cathode material for aqueous zinc-ion batteries,1T-MoS_(2)has been extensively investigated because of its facile two-dimensional ion-diffusion channels and high electrical ***,the limited number of available Zn storage sites,i.e.,limited capacity,hinders its application because the inserted Zn^(2+),which form strong electrostatic interactions with 1T-MoS_(2),preventing subsequent Zn^(2+)***,the approach of enlarging the interlayer distance to reduce electrostatic interactions has been commonly used to enhance the capacity and reduce Zn^(2+)migration ***,an enlarged interlayer spacing can weaken the van der Waals force between 1T-MoS_(2)monolayers,easily disrupting the structural ***,to address this issue,an effective strategy based on Fe doping is proposed for 1T-MoS_(2)(Fe-1T-MoS_(2)).The theoretical calculations reveal that Fe doping can simultaneously moderate the rate of decrease in the adsorption energy after gradually increasing the number of stored atoms,and enhance the electron delocalization on metal-O ***,the experiment results show that Fe doping can simultaneously activate more Zn storage sites,thus enhancing the capacity,and stabilize the structural stability for improved cycling ***,Fe-1T-MoS_(2)exhibits a larger capacity(189 mAh·g^(-1)at 0.1 A·g^(-1))and superior cycling stability(78%capacity retention after 400 cycles at 2 A·g^(-1))than pure 1T-MoS_(2).This work may open up a new avenue for constructing high-performance MoS_(2)-based cathodes.

关键词： Aqueous zinc-ion battery 1T-MoS_(2) Fe doping More Zn storage sites Enhanced structural stability

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Adaptive Human Movement Compensation Control of Supernumerary Robotic Limb for Overhead Support Task With Non-Zero-Sum Differential Game Theory

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IEEE Transactions on Automation science and engineering 2025年 22卷 14159-14170页

作者： Zhang, Jianxi Zeng, Hong Liu, Jia Chen, Dapeng Song, Aiguo Southeast University State Key Laboratory of Digital Medical Engineering Jiangsu Key Laboratory of Robot Sensing and Control School of Instrument Science and Engineering Nanjing210096 China Nanjing University of Information Science and Technology Cicaeet Nanjing210044 China

The supernumerary robotic limb (SRL) mounted on the shoulder has been demonstrated to be able to serve as a third arm to assist human in overhead support task. However, the mechanical connection between the wearer and the SRL means that human operator's movement will continually disturb the SRL and may lead to instability. Moreover, there may be physical conflicts between SRL and human operator due to their different intentions, which may potentially increase the load on human operator. Therefore, it's necessary to control SRL to ensure stable supporting and transparent interaction. Here, we propose an adaptive controller for human movement compensation. Firstly, we model the human-SRL coordinative behavior based on non-zero-sum differential game theory aiming to enhance the support stability and reduce the operator's load, which is a framework capable of dynamically regulating the control strategies between two interacting agents. We then implement an adaptive control strategy that adjusts the SRL's input optimally responsive to the human operator's input in the sense of Nash equilibrium to meet predefined control objectives. From experimental results during overhead support task, the proposed controller reduces the peak reaction force from 15.59 N to 4.50 N compared to the state-of-the-art controller that disregards human input while ensuring the stability of support, thereby providing advantage for human-SRL coordination in overhead support task. Note to Practitioners - To ensure optimal overhead assistance, the stability of the support and the safety of the human operator are of paramount importance. Therefore, this study investigates how to provide stable support and transparent interaction through movement compensation. Previous compensation methods lacked the understanding for the wearer and the optimal adjustment for the control of SRL. Consequently, this paper proposes a non-zero-sum differential game to model the desired behaviors between human operator an

关键词： Adaptive control systems

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Turbulent drag reduction by sector-shaped counter-flow dielectric barrier discharge plasma actuator

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Chinese Physics B 2025年第2期34卷 362-370页

作者： Borui Zheng Shaojie Qi Minghao Yu Jianbo Zhang Linwu Wang Dongliang Bian School of Automation and Information Engineering Xi’an University of TechnologyXi’an 710048China School of Mechanical and Precision Instrument Engineering Xi’an University of TechnologyXi’an 710048China Science and Technology on Plasma Dynamics Laboratory Air Force Engineering UniversityXi’an 710038China Shaanxi Key Laboratory of Complex System Control and Intelligent Information Processing Xi’an 710048China Shaanxi University Key Laboratory of Photonic Power Devices and Discharge Regulation Xi’an 710048China

The primary objective in aircraft transportation is to minimize turbulent drag, thereby conserving energy and reducing emissions. We propose a sector-shaped counter-flow dielectric barrier discharge plasma actuator, which leverages jet synthesis for drag reduction. A drag control experiment was conducted in a low-speed wind tunnel with a controlled flow velocity of 9.6 m/s(Re = 1.445 × 10^(4)). This study investigated the effects of varying pulse frequencies and actuation voltages on the turbulent boundary layer. Using a hot-wire measurement system, we analyzed the pulsating and time-averaged velocity distributions within the boundary layer to evaluate the streamwise turbulent drag reduction. The results show that the local TDR decreases as the pulse frequency increases, reaching a maximum reduction of approximately 20.97% at a pulse frequency of 50 Hz. In addition, as the actuation voltage increases, the friction coefficient decreases, increasing the drag reduction rate. The maximum drag reduction of approximately 33.34% is achieved at an actuation voltage of 10 kV.

关键词： plasma flow control turbulent boundary layer turbulent drag reduction

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Seeking a Sense of Meaning and Companionship in Life: Informal Learning on Douyin Among Chinese Older Adults

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Proceedings of the ACM on Human-Computer Interaction 2025年第2期9卷 1-24页

作者： Qian, Zhigu Fu, Jiaojiao Zhou, Yangfan School of Computer Science Fudan University Shanghai Key Laboratory of Intelligent Information Processing China School of Information Science and Engineering East China University of Science and Technology China

This study examines how Chinese older adults leverage Douyin, a short video platform, for informal learning purposes, analyzing their usage patterns, motivations, and encountered challenges. Although Douyin was not explicitly designed with educational features, it has emerged as a significant informal learning platform for this demographic. Through a qualitative investigation comprising participant observations and semi-structured interviews with 17 participants, we reveal the distinctive learning experience that Douyin facilitates. The platform’s unique combination of short-form videos, live streaming capabilities, and interactive community features creates an engaging learning environment that particularly resonates with older adults. Our findings demonstrate that participants derive substantial social-emotional benefits beyond knowledge acquisition, including strengthened social connections, enhanced companionship, and a reinforced sense of purpose through their Douyin engagement. These social-emotional aspects emerge as crucial factors driving older adults’ selection of Douyin as their preferred learning platform. By providing comprehensive insights into older adults’ engagement with digital platforms for lifelong learning, this research offers valuable implications for HCI, particularly in understanding how technology can be optimized to support the learning needs of older populations. © 2025 Association for Computing Machinery. All rights reserved.

关键词： Social aspects

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Non-uniform electron density estimation based on electromagnetic wave attenuation in plasma

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Chinese Physics B 2025年第1期34卷 381-386页

作者： Zhaoying Wang Lixin Guo Maixia Fu Shaoshuai Guo Yinsheng Li Key Laboratory of Grain Information Processing and Control(Henan University of Technology) Ministry of EducationZhengzhou 450001China College of Information Science and Engineering Henan University of TechnologyZhengzhou 450001China School of Physics Xidian UniversityXi’an 710071China

The surface of a high-speed vehicle reentering the atmosphere is surrounded by plasma *** to the influence of the inhomogeneous flow field around the vehicle,understanding the electromagnetic properties of the plasma sheath can be *** the electron density of the plasma sheath is crucial for understanding and achieving plasma stealth of *** this work,the relationship between electromagnetic wave attenuation and electron density is deduced *** attenuation distribution along the propagation path is found to be proportional to the integral of the plasma electron *** result is used to predict the electron density ***,the average electron density is obtained using a back-propagation neural network ***,the spatial distribution of the electron density can be determined from the average electron density and the normalized derivative of attenuation with respect to the propagation *** to traditional probe measurement methods,the proposed approach not only improves efficiency but also preserves the integrity of the plasma environment.

关键词： attenuation electromagnetic propagation plasma electron density

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A brief review of preparation and applications of monolithic aerogels in atmospheric environmental purification

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Journal of Environmental sciences 2025年第3期149卷 209-220页

作者： Linfeng Nie Shuangde Li Mengjie Cao Ning Han Yunfa Chen State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Key Laboratory of Science&Technology on Particle Materials Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Monolithic aerogels are promising candidates for use in atmospheric environmental purification due to their structural advantages,such as fine building block size together with high specific surface area,abundant pore structure,***,monolithic aerogels possess a unique monolithic macrostructure that sets them apart from aerogel powders and nanoparticles in practical environmental clean-up *** review delves into the available synthesis strategies and atmospheric environmental applications of monolithic aerogels,covering types of monolithic aerogels including SiO_(2),graphene,metal oxides and their combinations,along with their preparation *** particular,recent developments for VOC adsorption,CO_(2)capture,catalytic oxidation of VOCs and catalytic reduction of CO_(2)are ***,challenges and future opportunities for monolithic aerogels in the atmospheric environmental purification field are *** reviewprovides valuable insights for designing and utilizing monolithic aerogel-based functional materials.

关键词： Monolithic aerogel Environmental purification Catalysis Adsorption

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Cooperative output regulation of heterogeneous directed multi-agent systems:a fully distributed model-free reinforcement learning framework

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science China(information sciences) 2025年第2期68卷 170-185页

作者： Xiongtao SHI Yanjie LI Chenglong DU Huiping LI Chaoyang CHEN Weihua GUI Guangdong Key Laboratory of Intelligent Morphing Mechanisms and Adaptive Robotics School of Mechanical Engineering and AutomationHarbin Institute of Technology (Shenzhen) School of Automation Central South University School of Marine Science and Technology Northwestern Polytechnical University School of Information and Electrical Engineering Hunan University of Science and Technology

In this paper, the cooperative output regulation(COR) problem of a class of unknown heterogeneous multi-agent systems(MASs) with directed graphs is studied via a model-free reinforcement learning(RL) based fully distributed eventtriggered control(ETC) strategy. First, we consider the scenario that the exosystem is accessible globally to all agents, an internal model-based augmented algebraic Riccati equation(AARE) is constructed, and its solution is learned by the proposed model-free RL algorithm via online input-output data. Further, for the scenario that the exosystem is accessible only to its adjacent followers, the distributed observers are designed for each agent to get the state of the exosystem, and an internal modelbased fully distributed adaptive ETC protocol is then synthesized to construct the corresponding AARE, and the feedback gain matrix is learned in a model-free fashion. The model-free RL-based control protocol proposed in this paper can not only remove the prior knowledge of agents' dynamics, but also release the dependence on global information by the adaptive event-triggered mechanism(ETM) and the new graph-based Lyapunov function. Finally, simulation results are illustrated to show the feasibility and effectiveness of the proposed control scheme.

关键词： model-free reinforcement learning unknown heterogeneous multi-agent systems fully distributed event-triggered control directed graph

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Smart fiber-optic masks: real-time respiratory monitoring and health analysis

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science China(information sciences) 2025年第4期68卷 216-227页

作者： Qi YU Ya-Nan ZHANG Jiaqi ZHANG Shuang YANG Lingxiao JIANG Xuegang LI College of Information Science and Engineering Northeastern University State Key Laboratory of Synthetical Automation for Process Industries Northeastern University Hebei Key Laboratory of Micro-Nano Precision Optical Sensing and Measurement Technology Affiliated Hospital of North Sichuan Medical College

In this study, we design a smart mask based on an ultrathin retractable flexible fiber optic sensor with high sensitivity(0.56 V/m-1), ultra-light mass（0.24 g）, and excellent tensile properties. The sensor was integrated with a medical mask to recognize multiple breathing patterns（standard, fast, slow, shallow, deep, breath-holding）, coughing, and speaking,as well as to study gender characteristics and physiological differences in the respiratory system. By comparing the nasal-oral respiratory waveforms and frequencies, guidance for respiratory correction was provided. In addition, affixing flexible fiber optic sensors to the outside of the mask reduces the risk of cross-infection and significantly reduces temperature and humidity disturbances. Studies have shown that nine sensor locations placed on the outside of the mask responded significantly to respiratory waveforms. For personalized health management, the system is also equipped with a communication module,web and mobile apps to support data downloads, real-time monitoring, and exception alerts.

关键词： smart mask respiratory monitoring fiber optic sensor health management anti-interference

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Emergency Communications in Post-Disaster Scenarios: IoT-Enhanced Airship and Buffer Support

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IEEE Internet of Things Journal 2025年第9期12卷 11457-11468页

作者： He, Yixin Huang, Fanghui Wang, Dawei Chen, Bin Zhang, Ruonan Jiaxing University College of Information Science and Engineering Provincial Key Laboratory of Multimodal Perceiving and Intelligent Systems Jiaxing314001 China Jiaxing Key Laboratory of Smart Transportations Jiaxing314001 China Jiaxing University College of Information Science and Engineering Jiaxing314001 China Northwestern Polytechnical University School of Electronics and Information Xi’an710072 China

Ensuring reliable and secure emergency communications in post-disaster scenarios is challenging, particularly when mobile communication infrastructures are damaged. In response to challenges in post-disaster emergency communications (PDEComs), this article proposes a cooperative relaying system (CRS) enhanced with Internet of Things (IoT) technology. The system features an airship equipped with buffers that serves as an aerial relay, designed to improve data transmission performance and communication security. To achieve this, it incorporates physical layer security techniques. Additionally, we introduce a hybrid mechanism that combines nonorthogonal multiple access (NOMA) and orthogonal multiple access (OMA), facilitating flexible resource allocation in IoT-enhanced CRSs. To fully leverage the advantages of the proposed airship-and-buffer aided CRS, we formulate a weighted secure sum rate (WSSR) maximization problem, jointly considering the power control, mode selection, and information security. Initially, we address the formulated WSSR maximization problem using Lyapunov optimization. Subsequently, the primal problem is divided into four cases, from which optimal power control and mode selection policies can be derived. This process is constrained by the stability of buffer queues and privacy transmission requirements. Finally, the simulation results show that the proposed scheme outperforms state-of-the-art schemes in terms of the WSSR. By adopting the airship and the hybrid NOMA/OMA mechanism, the WSSR can be increased by 29.9% and 96.4%, respectively. Moreover, we explore the impact of network parameters (e.g., the distance between the eavesdropper and airship, and decoding thresholds) on information security. © 2014 IEEE.

关键词： Mobile telecommunication systems

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Structure-performance relationship between denitration performance and catalytic interface morphologies of MnCeO_(x)/P84 catalytic filters

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Journal of Rare Earths 2025年第3期43卷 516-525,I0004页

作者： Bo Yang Yujie Lei Maosen Ni Liuying Wang Qiong Huang Mindong Chen Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology(CICAEET) Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution ControlSchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing210044China

MnCeO_(x)/P84 catalytic filters with spherical,flower-like,cubic and rod-like catalytic interfaces were synthesized respectively,and their catalytic activities in the NH_(3)-SCR reaction were *** MnCeO_(x)/P84 catalytic filter with spherical catalytic interfaces(recorded as S-MnCeO_(x)/P84)exhibits the best catalytic denitration *** NO_(x)removal efficiency of S-MnCeO_(x)/P84 reaches the highest value of 98.6%at 160℃when the catalyst loading is 100 g/m^(2).At the same time,S-MnCeO_(x)/P84 exhibits good SO_(2)resistance and stability,achieving a NO_(x)removal rate of 83%at 190℃with 30 ppm SO_(2).The characterization results illustrate that the MnCeO_x active component in S-MnCeO_(x)/P84 is present in weak crystalline states,tightly wrapped around the surface of the filter fiber,and uniformly dispersed,and the mesopore is the main pore structure of the S-MnCeO_(x)/P84,which can provide a channel for the catalytic reaction to *** the same time,transmission electron microscopy(TEM)characterization shows that y-MnO_(2)is the main form of MnO_(2)in the S-MnCeO_(x)/*** analysis of H_(2)temperature programmed reduction(H_(2)-TPR).NH_(3)temperature programmed desorption(NH_(3)-TPD)and in-situ diffuse reflectance infrared spectra(DRIFTS)show that S-MnCeO_(x)/P84 has good redox ability at 100-200℃and has abundant Lewis acid sites and Bronsteds acid sites,which provides an important guarantee for its superior low-temperature NH_(3)-SCR denitration performance.

关键词： Catalytic filter Nitrogen oxides(NO_x) Denitration Catalytic interface Rare earths

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