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A tree-growing graphic model for asymmetrical phantom networks in polymeric gels undergoing dynamic mechanochemical coupling

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science China(Technological sciences) 2024年第2期67卷 558-567页

作者： SHI WeiLin ZHOU Jian LU HaiBao ELMARAKBI Ahmed FU Yong-Qing National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150080China College of Mechanical and Vehicle Engineering Hunan UniversityChangsha 410082China Faculty of Engineering and Environment University of NorthumbriaNewcastle upon Tyne NEI 8STUK

Network structures of various polymers have significant effects on their mechanical properties;therefore,numerous studies have investigated the constitutive relationship between symmetrical network structures and their rubber elasticity in ***,few studies have focused on asymmetrical network structures in polymers that undergo bond exchange reactions,selfassembly,or mechanochemical coupling—all of which are induced by transition probabilities of chemical bonding *** this study,an extended constraint junction and phantom network model is formulated using the tree-growing theory to establish a constitutive relationship between asymmetrical network structures and their rubber elasticity in polymers.A free-energy equation is further developed to explore working principles of configurational transitions on the dynamic rubber elasticity of symmetrical and asymmetrical network *** constitutive relationship between dynamic rubber elasticity and symmetrical and asymmetrical network structures has also been proposed for the gels undergoing mechanochemical and hydromechanical ***,the effectiveness of this newly proposed tree-growing model has been verified by comparing with the classical affine network model,finite element analysis,and the experimental results of gels reported in literature.

关键词： gel polymer network rubber elasticity asymmetric

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Polymorphic cerium-based Prussian blue derivatives with in situ growing CNT/Co heterojunctions for enhanced microwave absorption via polarization and magnetization

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Nano Research 2024年第3期17卷 2050-2060页

作者： Jixi Zhou Xinmeng Huang Di Lan Yuhang Cheng Fengyi Xue Chenyu Jia Guanglei Wu Zirui Jia Institute of Materials for Energy and Environment State Key Laboratory of Bio-fibers and Eco-textilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China School of Materials Science and Engineering Hubei University of Automotive TechnologyShiyan 442002China College of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266071China

In this paper,the structure evolution of cerium cobaltohexanoate(Ce[Co(CN)6],Ce-Co Prussian blue analog(PBA))has been realized by solvent catalysis at room *** hexagonal bipyramidal microcrystals of Ce-Co PBA can be gradually transformed into dendrites by different proportions of ethanol(EtOH)and *** the same time,the porous dendrites CeO_(2)/Co@carbon nanotub(CNT)with oxygen-rich vacancies(OVs)can be obtained by annealing Ce-Co PBA at 700℃.The microstructure study shows that carbon nanotubes will be catalyzed after annealing at high temperature,and the cobalt metal particles encapsulated in carbon nanotubes will be anchored in the matrix,regulating the impedance matching and multi-polarization suppression of the material,and its unique structure,vacancies,and strong interface effect make the material exhibit excellent electromagnetic wave(EMW)absorption *** the matching thickness is 2.5 mm,the minimum reflection loss(RLmin)of the composite is-51.68 dB,and the effective absorption bandwidth(RL<-10 dB)is 7.76 *** results show that the prepared CeO_(2)/Co@CNT composite has excellent EMW absorption *** is expected to be a candidate material for EMW absorption.

关键词： Ce-Co Prussian blue analog(PBA) carbon nanotubes(CNTs) CeO_(2)/Co@CNT solvent catalysis electromagnetic wave absorption

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KCl acts as a flux to assist the growth of sub-millimeter-scale metallic 2D non-layered molybdenum dioxide

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Rare Metals 2025年第1期44卷 404-416页

作者： Li-Ying Deng Qing Zhang Wang-Yang Li Xiao-Yuan Ye Yi-Fan Zhao Shen-Zhong Chen Yu-Lan Wang Xing-Hui Wang Hui-Peng Chen Zhi-Yang Yu Qun Yan Shu-Ying Cheng Tai-Liang Guo Wen-Ping Hu Feng Ding Jie Sun National and Local United Engineering Laboratory of Flat Panel Display Technology College of Physics and Information EngineeringFuzhou UniversityFuzhou350100China Fujian Key Laboratory of Agricultural Information Sensing Technology College of Mechanical and Electrical EngineeringFujian Agriculture and Forestry UniversityFuzhou350002China Key Laboratory of Organic Integrated Circuit Department of ChemistrySchool of ScienceMinistry of Education and Tianjin Key Laboratory of Molecular Optoelectronic SciencesTianjin UniversityTianjin300072China Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) Tianjin300072China College of Physics and Information Engineering Institute of Micro-Nano Devices and Solar CellsFuzhou UniversityFuzhou350108China State Key Laboratory of Photocatalysis on Energy and Environment College of ChemistryFuzhou UniversityFuzhou350116China Faculty of Materials Science and Engineering/Institute of Technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen518000China

Two-dimensional(2D)metal oxides(2DMOs),such as MoO_(2),have made impressive strides in recent years,and their applicability in a number of fields such as electronic devices,optoelectronic devices and lasers has been ***,2DMOs present challenges in their synthesis using conventional methods due to their non-van der Waals *** report that KCl acts as a flux to prepare large-area 2DMOs with sub-millimeter *** systematically investigate the effects of temperature,homogeneous time and cooling rate on the products in the flux method,demonstrating that in this reaction a saturated homogenous solution is obtained upon the melting of the salt and ***,the cooling rate was adjusted to regulate the thickness of the target crystals,leading to the precipitation of 2D non-layered material from the supersaturated solution;by applying this method,the highly crystalline non-layered 2D MoO_(2)flakes with so far the largest lateral size of up to sub-millimeter scale(~464μm)were *** studies have revealed that the 2D MoO_(2)features metallic properties,with an excellent sheet resistance as low as 99Ω·square^(-1 )at room temperature,and exhibits a property of charge density wave in the measurement of resistivity as a function of temperature.

关键词： 2D non-layered materials Metallic Metal oxide Thickness modulation Flux method

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Degradation properties of fulvic acid and its microbially driven mechanism from a partial nitritation bioreactor through multi-spectral and bioinformatic analysis

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Journal of environmental sciences 2024年第1期135卷 318-331页

作者： Quanhao Dou Li Zhang Tingjun Dong Zixuan Song Xuepeng Fan Yongzhen Peng Xiayan Wang Jiachun Yang National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery EngineeringBeijing University of TechnologyBeijing 100124China Department of Chemistry and Biology Center of Excellence for Environmental Safety and Biological EffectsBeijing Key Laboratory for Green Catalysis and SeparationBeijing University of TechnologyBeijing 100124China Environmental Protection Development Group Co. Ltd.Shandong 250101China

This study employed multispectral techniques to evaluate fulvic acid(FA)compositional characteristic and elucidate its biodegradation mechanisms during partial nitritation(PN)*** showed that FA removal efficiency(FRE)decreased from 90.22 to 23.11%when FA concentrations in the reactor were increased from 0 to 162.30 mg/L,and that molecular size,degree of aromatization and humification of the effluent FA macromolecules all increased after *** population analysis indicated that the proliferation of the Comamonas,OLB12 and Thauera exhibit high FA utilization capacity in lower concentrations(<50.59 mg/L),promoting the degradation and removal of macromolecular *** addition,the sustained increase in external FA may decrease the abundance of above functional microorganisms,resulting in a rapid drop in ***,from the genetic perspective,the elevated FA levels restricted carbohydrate(ko00620,ko00010 and ko00020)and nitrogen(HAO,AMO,NIR and NOR)metabolism-related pathways,thereby impeding FA removal and total nitrogen loss associated with N_(2)O emissions.

关键词： Partial nitritation Fulvic acid 3DEEM-PARAFAC UV/Vis Microbially driven mechanism

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Rational construction of heterointerfaces in biomass sugarcane-derived carbon for superior electromagnetic wave absorption

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International Journal of Minerals,Metallurgy and Materials 2024年第12期31卷 2749-2759页

作者： Shijie Zhang Di Lan Jiajun Zheng Ailing Feng Yaxing Pei Shichang Cai Suxuan Du Xingliang Chen Guanglei Wu Zirui Jia Key Laboratory of Clean Dyeing and Finishing Technology of Zhejiang Province Shaoxing Key Laboratory of High Performance Fibers&ProductsShaoxing UniversityShaoxing 312000China School of Materials Science and Engineering Hubei University of Automotive TechnologyShiyan 442002China School of Material Science and Engineering Henan University of TechnologyZhengzhou 450001China Institute of Physics&Optoelectronics Technology Baoji University of Arts and SciencesBaoji 721016China Zhengzhou Research Institute for Abrasives and Grinding Zhengzhou 450002China Institute of Materials for Energy and Environment State Key Laboratory of Bio-fibers and Eco-textilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China

The pervasive adoption of 5th generation mobile communication technology propels electromagnetic wave(EW)absorbents to achieve high-level *** heterointerface construction is crucial to the improvement of absorption ***,a series of ultralight composites with rational heterointerfaces(Co/ZnO@N-doped C/layer-stacked C,MSC)is fabricated by calcination with ration-al construction of sugarcane and CoZn-zeolitic imidazolate framework(ZIF).The components and structures of as-prepared composites were investigated,and their electromagnetic parameters could be adjusted by the content of *** composites possess excellent EW absorption performance,especially *** optimal minimum reflection loss and effective absorption band of MSC-3 can reach−42 dB and 7.28 GHz at the thickness of only 1.6 mm with 20wt%filler *** excellent performance is attributed to the syner-gistic effect of dielectric loss stemming from the multiple heterointerfaces and magnetic loss induced by magnetic single *** sugar-cane-derived layer-stacked carbon has formed consecutive conductive networks and has further dissipated the electromagnetic energy through multiple reflection and conduction ***,the simulated radar cross section(RCS)technology manifests that MSC-3 possesses outstanding EW attenuation capacity under realistic far-field *** study provides a strategy for building efficient ab-sorbents based on biomass.

关键词： sugarcane-derived carbon heterointerfaces bimetallic metal-organic frameworks EW absorption radar cross section

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Electrical stress and acid orange 7 synergistically clear the blockage of electron flow in the methanogenesis of low-strength wastewater

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environmental science and Ecotechnology 2024年第4期20卷 291-299页

作者： Ze-Chong Guo Min-Hua Cui Chun-Xue Yang Hong-Liang Dai Tong-Yi Yang Lin-Zhi Zhai Yong Chen Wen-Zong Liu Ai-Jie Wang School of Environmental and Chemical Engineering Jiangsu University of Science and TechnologyZhenjiang212100China State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin150090China Jiangsu Key Laboratory of Anaerobic Biotechnology Jiangnan UniversityWuxi214122China School of Civil and Environmental Engineering Harbin Institute of TechnologyShenzhen518055China School of Geography and Tourism Harbin UniversityHarbin150001China School of Environmental Science and Engineering Huazhong University of Science and TechnologyWuhan430074China

Energy recovery from low-strength wastewater through anaerobic methanogenesis is constrained by limited substrate *** development of efficient methanogenic communities is critical but *** we develop a strategy to acclimate methanogenic communities using conductive carrier(CC),electrical stress(ES),and Acid Orange 7(AO7)in a modified *** synergistic integration of CC,ES,and AO7 precipitated a remarkable 72-fold surge in methane production rate compared to the *** increase was attributed to an altered methanogenic community function,independent of the continuous presence of AO7 and ***7 acted as an external electron acceptor,accelerating acetogenesis from fermentation intermediates,restructuring the bacterial community,and enriching electroactive bacteria(EAB).Meanwhile,CC and ES orchestrated the assembly of the archaeal community and promoted electrotrophic methanogens,enhancing acetotrophic methanogenesis electron flow via a mechanism distinct from direct electrochemical *** collective application of CC,ES,and AO7 effectively mitigated electron flow impediments in low-strength wastewater methanogenesis,achieving an additional 34%electron recovery from the *** study proposes a new method of amending anaerobic digestion systems with conductive materials to advance wastewater treatment,sustainability,and energy self-sufficiency.

关键词： Methanogenesis Conductive carrier Electrical stress Acid orange 7 Electron transfer

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A review on electrocatalytic CO_(2) conversion via C-C and C-N coupling

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Carbon Energy 2024年第2期6卷 167-194页

作者： Zhuangzhi Zhang Sijun Li Zheng Zhang Zhou Chen Hua Wang Xianguang Meng Wenquan Cui Xiwei Qi Jiacheng Wang Hebei Provincial Laboratory of Inorganic Nonmetallic Materials College of Materials Science and EngineeringNorth China University of Science and TechnologyTangshanChina Key Laboratory of Luminescence Analysis and Molecular Sensing Ministry of EducationCollege of Chemistry and Chemical EngineeringSouthwest UniversityChongqingChina State Key Laboratory of New Textile Materials and Advanced Processing Technologies Hubei Key Laboratory of Biomass Fibers and Eco-Dyeing and FinishingCollege of Chemistry and Chemical EngineeringWuhan Textile UniversityWuhanChina College of Materials Xiamen UniversityXiamenChina Hebei Iron and Steel Laboratory TangshanChina Hebei Key Laboratory for Environment Photocatalytic and Electrocatalytic Materials College of Chemical EngineeringNorth China University of Science and TechnologyTangshanChina College of Metallurgy and Energy North China University of Science and TechnologyTangshanChina State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghaiChina Institute of Electrochemistry School of Materials Science and EngineeringTaizhou UniversityTaizhouChina

Electrochemical C-C and C-N coupling reactions with the conversion of abundant and inexpensive small molecules,such as CO_(2) and nitrogencontaining species,are considered a promising route for increasing the value of CO_(2) reduction *** development of high-performance catalysts is the key to the both electrocatalytic *** this review,we present a systematic summary of the reaction systems for electrocatalytic CO_(2) reduction,along with the coupling mechanisms of C-C and C-N bonds over outstanding electrocatalytic materials recently *** key intermediate species and reaction pathways related to the coupling as well as the catalyst-structure relationship will be also discussed,aiming to provide insights and guidance for designing efficient CO_(2) reduction systems.

关键词： C-C coupling C-N coupling CO_(2) conversion electrocatalysis urea synthesis

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The preparation, microstructure, and performance of MoAlB-Si ceramic sintered from combustion-synthesized powder

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Ceramics International 2025年第16期51卷 21800-21809页

作者： Yu, Wanjun Ding, Qizhang Li, Xiangming Zhang, Enliang Han, Wenbo Zheng, Yongting Qi, Yushi School of Environment and Materials Engineering Yantai University Yantai264005 China School of Materials Science and Engineering Harbin Institute of Technology Weihai264209 China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments and Center for Composite Materials and Structures Harbin Institute of Technology Harbin150080 China

To streamline the preparation process and improve the performance of the MoAlB phase, the technical potential of an ultra-fast combustion synthesis followed by hot pressing to prepare the MoAlB–Si ceramic was investigated. During the combustion process, the Si atoms occupied the Al positions, which forms a Mo(Al,Si)B solid solution phase. Si doping resulted in the effective grain refinement of the hot-pressed MoAlB-Si ceramic. The grain-refined and solid-solution-strengthened MoAlB-Si ceramic exhibits excellent mechanical properties with a compressive strength of 2.63 GPa, flexural strength of 650 MPa, fracture toughness of 7.26 MPa m1/2, and Vickers hardness of 13.32 GPa. At elevated temperatures, a newly formed oxidation-derived dense and continuous layer on the surface prevents the inward diffusion of oxygen and the volatilisation of oxidation products, indicating good oxidation resistance of the MoAlB-Si ceramic. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Compressive strength

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Integrated navigation algorithm based on Vision-Inertial extended Kalman filter for low-cost Unmanned Aerial Vehicle

Integrated navigation algorithm based on Vision-Inertial ext...

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2023 International Conference on Computer, Artificial Intelligence, and Control engineering, CAICE 2023

作者： Wu, Helong Sun, Lijun Hu, Yang Yang, Jianfeng China Electronic Product Reliability and Environment Testing Research Institute Guangdong Provincial Key Laboratory of Electronic Information Products Reliability Technology Guangdong Provincial Engineering Technology Research Center of UAV Reliability and Safety Guangzhou China

ISBN: (纸本)9781510665040

In order to solve the problem of low attitude estimation accuracy of low-cost UAV without GNSS (Global Navigation Satellite System) signal, the integrated navigation algorithm was improved. Binocular vision sensor is introduced as the observation sensor, and the position and attitude angle of the image information collected by binocular camera were estimated by the SLAM theory, the position and attitude angle were entered into the EKF algorithm, and the Vision Inertial EKF(VI-EKF) algorithm is established. It realizes the high-precision navigation of low-cost UAV without GNSS signal. The biases of gyroscope and accelerometer are calculated by the relative motion increment between the two key frames of binocular camera and IMU pre-integration data, and these two biases were taken as observations to update IMU bias in the process of EKF algorithm. In this paper, the effectiveness of IMU pre-integration algorithm is verified firstly, and then the VI-EKF navigation algorithm is compared with the pure visual SLAM algorithm through dataset simulation. The simulation results show that the VI-EKF algorithm proposed in this paper has a good performance in the environment without GNSS signal. © 2023 SPIE.

关键词： Unmanned aerial vehicles (UAV)

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Reproductive toxicity of enrofloxacin in Caenorhabditis elegans involves oxidative stress-induced cell apoptosis

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Journal of environmental sciences 2023年第5期127卷 726-737页

作者： Jiahao Huang Lizi Liao Guowei Wang Zhongkun Du Zhengxing Wu Key Laboratory of Molecular Biophysics Ministry of EducationCollege of Life Science and TechnologyHuazhong University of Science and TechnologyWuhan 430074China School of Environmental Ecology and Biological Engineering Wuhan Institute of TechnologyWuhan 430205China Key Laboratory of Green Chemical Engineering Process of Ministry of Education Wuhan 430205China College of Resources and Environment Shandong Agricultural UniversityTaian 271018China

Fluoroquinolone antibiotics(FQs)that persist and bioaccumulate in the environment have aroused people’s great ***,we studied the adverse effects of FQs in soil animals of Caenorhabditis elegans via food-chronically *** result shows *** exposed to FQs exhibited reproductive toxicity with small-brood size and low-egg *** study the underlying mechanism,we conduct a deep investigation of enrofloxacin(ENR),one of the most frequently detected FQs,on nematodes which is one of commonly used animal indicator of soil *** concentration-effect curves simulated by the Hill model showed that the half effect concentrations(EC50)of ENR were(494.3±272.9)μmol/kg and(107.4±30.9)μmol/kg for the brood size and the hatchability,*** gene expression between the control and the ENR-exposure group enriched with the oxidative stress and cell apoptosis *** results together with the enzyme activity in oxidative stress and the cell corpses suggested that ENR-induced reproductive toxicity was related to germ cell apoptosis under oxidative *** risk quotients of some soil and livestock samples were calculated based on the threshold value of EC10 for the egg hatchability(2.65μmol/kg).The results indicated that there was possible reproductive toxicity on the nematodes in certain agricultural soils for the *** study suggested that chronic exposure to FQs at certain levels in environment would induce reproductive toxicity to the nematodes and might reduce the soil sustainability,alarming the environment risks of antibiotics abuse.

关键词： environmental toxicity Nematodes Chronic exposure Oxidative stress response Germ cell apoptosis

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