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Carbon Nanofiber/Polyaniline Composite Aerogel with Excellent Electromagnetic Interference Shielding,Low Thermal Conductivity,and Extremely Low Heat Release

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Nano-Micro Letters 2025年第4期17卷 77-95页

作者： Mingyi Chen Jian Zhu Kai Zhang Hongkang Zhou Yufei Gao Jie Fan Rouxi Chen Hsing-Lin Wang School of Textile Science and Engineering Tiangong UniversityTianjin 300387People’s Republic of China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055People’s Republic of China School of Innovation and Entrepreneurship Southern University of Science and TechnologyShenzhen 518055People’s Republic of China Guangdong Provincial Key Laboratory of Energy Materials for Electric Power Southern University of Science and TechnologyShenzhen 518055People’s Republic of China Ministry of Education Key Laboratory of Advanced Textile Composite Materials Tiangong UniversityTianjin 300387People’s Republic of China

The rapid development of communication technology and high-frequency electronic devices has created a need for more advanced electromagnetic interference(EMI)shielding *** response to this demand,a study has been conducted to develop multifunctional carbon nanofibers(CNFs)/polyaniline(PANI)aerogels with excellent electromagnetic interference shielding,flame retardancy,and thermal insulation *** process involved freeze-drying of electrospun CNFs and PANI nanoparticles followed by in situ growth PANI to coat the CNFs,creating the core-shell structured CNFs/PANI composite fiber and its hybrid aerogels(CP-3@PANI).The interaction between PANI and aniline(ANI)provides attachment sites,allowing additional ANI adsorption into the aerogel for in situ *** results in PANI uniformly covering the surface of the CNFs,creating a core-shell composite fiber with a flexible CNF core and PANI *** process enhances the utilization rate of the ANI monomer and increases the PANI content loaded onto the ***,effective connections are established between the CNFs,forming a stable,conductive three-dimensional network *** prepared CP-3@PANI aerogels exhibit excellent EMI shielding efficiency(SE)of 85.4 dB and specific EMI SE(SE d^(-1))of 791.2 dB cm^(3)g^(-1)in the *** to the synergistic flame-retardant effect of CNFs,PANI,and the dopant(phytic acid),the CP-3@PANI aerogels demonstrate outstanding flame-retardant and thermal insulation properties,with a peak heat release rate(PHRR)as low as 7.8 W g^(-1)and a total heat release of only 0.58 kJ g^(-1).This study provides an effective strategy for preparing multifunctional integrated EMI shielding materials.

关键词： CNFs/PANI hybrid aerogels EMI shielding Flame retardancy Thermal insulation

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MXene derivative Ta_(4)C_(3)-Ta_(2)O_(5) heterostructure as bi-functional barrier for Li-S batteries

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Journal of Materials science & technology 2023年第20期151卷 89-98页

作者： Qi Liang Sizhe Wang Xiaohua Jia Jin Yang Yong Li Dan Shao Lei Feng Jiaxuan Liao Haojie Song School of Materials Science and Engineering Shaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials Shaanxi University of Science&TechnologyXi’an 710021China Yangtze Delta Region Institute(Quzhou) University of Electronic Science and Technology of ChinaQuzhou 313001China

The shuttle effect of polysulfides during the charging and discharging of lithium-sulfur(Li-S)batteries and the growth of Li dendrites are crucial obstacles to hinder the commercialization of Li-S *** engineering is an effective strategy to accelerate catalytic conversion and suppress the dissolution of ***,we report a Ta_(4)C_(3)-Ta_(2)O_(5) heterostructure composite as a bi-functional modified separator that not only achieves effective protection for lithium metal but also accelerates the polysulfides redox kinetics *** heterostructure possesses efficient chemical anchoring and abundant active sites to immobilize polysulfides by synergistic effect,which endows a stable long cycling performance for Li-S *** corresponds to an initial high capacity of 801.9 mAh g^(–1) at 1 C with a decay rate of 0.086%for 500 *** to its high Young’s modulus(up to 384 GPa),Ta_(4)C_(3) contributes to forming a protective layer on the Li metal surface to inhibit the growth of Li ***,the symmetrical cell has a stable overpotential for 700 cycles at 20 mA cm^(–2)/20 mAh cm^(–2).So,this“one stone two birds”design affords a novel perspective for high-energy Li-S battery storage system design and Li metal protection.

关键词： MXene Ta_(4)C_(3) Ta_(2)O_(5) Lithium-sulfur batteries Li metal protection

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Tropical cyclone genesis over the western north Pacific in La Ni?a decay summers: Comparison between 2018 and 2021

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science China Earth sciences 2024年第10期67卷 3098-3109页

作者： Yunyun LIU Zhensong GONG China Meteorological Administration Key Laboratory for Climate Prediction Studies National Climate CentreBeijing 100081China Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science&TechnologyNanjing 210044China

As the primary interannual signal of variability in the tropical ocean-atmosphere interaction, the El Ni?o-Southern Oscillation has a considerable impact on tropical cyclone(TC) activity over the western North Pacific(WNP). Both 2018 and2021 were La Ni?a decay years, but TC activity over the WNP during the two summers(June–August) showed notable differences. In 2018, summer TC activity was unusually high with a total of 18 TCs, and the region of TC genesis was mainly in the central and eastern WNP. In contrast, only 9 TCs were generated in summer 2021, and the region of TC genesis was primarily in the western WNP. By comparing the characteristics of the large-scale environmental conditions over the regions of TC genesis, the thermal factors of the tropical oceans, and the activity of the Madden-Julian Oscillation(MJO), this study revealed the possible causes for the marked differences in TC genesis over the WNP during the two summers, which both had a similar background of La Ni?a decay. The Indian Ocean Basin Mode(IOBM) transitioned of a cold anomaly in the winter of 2017/2018and persisted until summer 2018. At the same time, the Pacific Meridional Mode(PMM) maintained a positive phase, leading to eastward and northward displacement of the Western Pacific Subtropical High in summer, and eastward extension of the tropical monsoon trough, which presented conditions conducive to TC genesis over the Northwest Pacific. Moreover, the days when the MJO stagnated in phases 5 and 6 in the summer of 2018 increased by approximately 150% relative to climatological state,providing dynamic conditions favorable for TC formation. In 2021, the IOBM quickly turned to a warm anomaly in March and persisted until summer, whereas the PMM became a negative phase in January and remained so until summer. At the same time,the MJO stagnated in phases 2 and 3 for up to 47 days, with the center of convection located over the western Maritime Continent, producing conditions unconducive to TC ge

关键词： Tropical cyclone La Nina events Indian Ocean Basin Mode Pacific Meridional Mode Madden-Julian Oscillation Western Pacific Subtropical High Monsoon trough

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Typhoon-Induced Ocean Waves and Stokes Drift:A Case Study of Typhoon Mangkhut(2018)

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China Ocean Engineering 2024年第4期38卷 711-724页

作者： WU Zhi-yuan GAO Kai CHEN Jie ZHANG Hao-jian DENG Bin JIANG Chang-bo LIU Yi-zhuang LYU Zhao YAN Ren School of Hydraulic and Environmental Engineering Changsha University of Science&TechnologyChangsha 410114China Key Laboratory of Water-Sediment Sciences and Water Disaster Prevention of Hunan Province Changsha 410114China State Key Laboratory of Hydrology-Water Resources and Hydraulic Engineering Hohai UniversityNanjing 210024China State Key Laboratory of Coastal and Offshore Engineering Dalian University of TechnologyDalian 116024China School of Civil Engineering Hunan University of TechnologyZhuzhou 412007China

Ocean waves and Stokes drift are generated by *** study investigated the characteristics of ocean waves and wave-induced Stokes drift and their effects during Typhoon Mangkhut using European Centre for MediumRange Weather Forecasts(ECMWF)ERA5 datasets and observational *** results revealed that the typhoon generated intense cyclones and huge typhoon waves with a maximum wind speed of 45 m/s,a minimum pressure of955 h Pa,and a maximum significant wave height of 12 *** Stokes drift caused by typhoon waves exceeded 0.6m/s,the Stokes depth scale exceeded 18 m,and the maximum Stokes transport reached 6 m^(2)/*** spatial distribution of 10-m wind speed,typhoon wave height,Stokes drift,Stokes depth,and Stokes transport during the typhoon was highly correlated with the typhoon *** distribution along the typhoon track showed significant zonal asymmetry,with greater intensity on the right side of the typhoon track than on the left *** findings provide important insights into the impact of typhoons on ocean waves and Stokes drift,thus improving our understanding of the interactions between typhoons and the ocean *** study also investigated the contribution of Stokes transport to the total net transport during typhoons using Ekman-Stokes Numbers as a comparative *** results indicated that the ratio of Stokes transport to the total net transport reached up to 50%within the typhoon radius,while it was approximately 30%outside the *** Stokes transport induced by typhoon waves led to divergence in the transport direction,which resulted in upwelling of the lower ocean as a compensation ***,Stokes transport played a crucial role in the vertical mixing of the ocean during *** findings suggested that Stokes transport should be paid more attention to,particularly in high latitude ocean regions,where strong winds can amplify its effects.

关键词： Stokes drift typhoon waves Ekman-Stokes transport vertical mixing Typhoon Mangkhut

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Epitaxy growth of pure phase CeFeO_(3) thin films with high magneto-optical performance and strong vertical magnetic anisotropy

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Journal of Rare Earths 2023年第12期41卷 2018-2024,I0007页

作者： Nanxi Lin Fangliang Sheng Xin Chen Xiaolin Hu Naifeng Zhuang College of Chemistry Fuzhou UniversityFuzhou350108China Key Laboratory of Non-destructive Testing Technology Fujian Polytechnic Normal UniversityFuqing350300China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou350108China

The magneto-optical effects of rare earth ferrite can be greatly improved by doping Ce^(3+)***_(3)with high Ce^(3+)concentration has excellent magneto-optical properties in *** due to its perovskite structure it is more suitable to be deposited on the substrates of optical devices compared with the commercial garnet *** this paper,the pure phase Ce_(x)Fe_(2-x)O_(3)films were successfully obtained on the quartz glass and <100>-oriented SrTiO3crystal substrates by radio frequency magnetron *** effects of substrate and Ce:Fe ratio on the epitaxial orientation,magnetism and magnetooptical performance of films were systematically *** the Ce1.0Fe1.0O3/STO film,its MCD ellipticity(ψF) intensity can reach up to 4750(°)/cm in the visible band and 14090(°)/cm in near ultraviolet *** it also shows a strong vertical magnetic anisotropy,which makes it maintain a good thermal stability when the device size is *** mean that the Ce_(1.0)Fe_(1.0)O_(3)/STO film has a promising application in integrated optical communication devices.

关键词： Magneto-optical effect Thin film Magnetic anisotropy Magnetic circular dichroism Cerium Rare earths

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Organization of microtubule plus-end dynamics by phase separation in mitosis

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Journal of Molecular Cell Biology 2024年第2期16卷 24-35页

作者： Fengrui Yang Mingrui Ding Xiaoyu Song Fang Chen Tongtong Yang Chunyue Wang Chengcheng Hu Qing Hu Yihan Yao Shihao Du Phil YYao Peng Xia Gregory Adams Jr Chuanhai Fu Shengqi Xiang Dan Liu Zhikai Wang Kai Yuan Xing Liu MOE Key Laboratory for Membraneless Organelles&Cellular Dynamics Hefei National Research Center for Cross-disciplinary SciencesCenter for Advanced Interdisciplinary Science and Biomedicine of IHMDivision of Life Sciences and MedicineUniversity of Science&Technology of ChinaHefei 230027China Anhui Key Laboratory for Cellular Dynamics and Chemical Biology University of Science&Technology of ChinaHefei 230027China Keck Center for Organoids Plasticity Morehouse School of MedicineAtlantaGA 30310USA Hunan Key Laboratory of Molecular Precision Medicine Central South UniversityChangsha 410083China

In eukaryotes,microtubule polymers are essential for cellular plasticity and fate ***-binding(EB)proteins serve as scaffolds for orchestrating microtubule polymer dynamics and are essential for cellular dynamics and chromosome segregation in ***,we show that EB1 forms molecular condensates with TIP150 and MCAK through liquid–liquid phase separation to compartmentalize the kinetochore–microtubule plus-end machinery,ensuring accurate kinetochore–microtubule interactions during chromosome segregation in *** of EB1–TIP150 polymer formation by a competing peptide prevents phase separation of the EB1-mediated complex and chromosome alignment at the metaphase equator in both cultured cells and Drosophila ***220 of EB1 is dynamically acetylated by p300/CBP-associated factor in early mitosis,and persistent acetylation at Lys220 attenuates phase separation of the EB1-mediated complex,dissolves droplets in vitro,and harnesses accurate chromosome *** data suggest a novel framework for understanding the organization and regulation of eukaryotic spindle for accurate chromosome segregation in mitosis.

关键词： phase separation mitosis microtubule dynamics EB1 acetylation

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1D p-type molecular-based coordination polymer semiconductor with ultrahigh mobility

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science Bulletin 2024年第17期69卷 2705-2711页

作者： Chenhui Yu Xinxu Zhu Kefeng Li Guan-E Wang Gang Xu State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China University of Chinese Academy of Sciences Beijing 100049China

One-dimensional(1D)semiconductor nanostructures exhibit exceptional performance in mitigating short-channel effects and ensuring low power ***,the scarcity of high-mobility ptype 1D materials impedes further ***-based materials offer high designability in structure and properties,making them a promising candidate for 1D p-type semiconductor materials.A molecular-based 1D p-type material was developed under the guidance of coordination ***-HT(HT is the abbreviation of p-hydroxy thiophenol)combines the merits of highly orbital overlap between Cu and S,fully covered surface modification with phenol functional groups,and unique cuprophilic(Cu-Cu)*** such,Cu-HT has a remarkable hole mobility of 27.2 cm2V-1s-1,which is one of the highest reported values for 1D molecular-based materials to date and even surpass those of commonly used amorphous silicon as well as the majority of 1D inorganic *** achievement underscores the significant potential of coordination polymers in optimizing carrier transport and represents a major advancement in the synthesis of high-performance,1D p-type semiconductor materials.?2024 science China *** by Elsevier *** science China *** rights are reserved.

关键词： Molecular-basedmaterials Hole mobility Coordinationpolymer Field-effecttransistors

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Polyisoprene Bearing Dual Functionalized Mini-blocky Chain-ends Prepared from Neodymium-mediated Coordinative Chain Transfer Polymerizations

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Chinese Journal of Polymer science 2023年第5期41卷 720-727,I0008页

作者： Wei-Xin Wang Wen-Peng Zhao Jing Dong Hua-Qiang Zhang Feng Wang Heng Liu Xue-Quan Zhang Key Laboratory of Rubber-Plastics Ministry of EducationShandong Provincial Key Laboratory of Rubber-PlasticsQingdao University of Science&TechnologyQingdao 266042China Petrochemical Research Institute PetroChinaBeijing 102206China School of Chemical Engineering Changchun University of TechnologyChangchun 130012China

Through neodymium-mediated coordinative chain transfer copolymerizaiton(CCTcoP),polyisoprenes bearing dual hydroxylated mini-blocky chain-ends were prepared via a three-step *** studies revealed that,the polymerization demonstrated typical features of CCTcoP across the whole polymerization process,i.e.,quasi-living polymerization characteristic,tunable molecular weights,narrow molecular weight distributions,and atom *** to previously reported CCTP homopolymerization systems,the presence of oxygen-containing IpOAl polar comonomer slowed down chain transfer rates obviously,rendering slightly higher molecular weights of the resultant PIps and smaller Np(number of polymer chains per Nd atom)***,to mimic the structure of natural rubber,the hydroxyl end groups can be facilely modified into phosphonate,amide,and UPy,whose structures were further confirmed by NMR *** these functionalities could greatly improve the hydrophilic properties of the polymers,as revealed from the significantly reduced static water contact angles.

关键词： Functional polyisoprene Neodymium Coordinative chain transfer polymerization Synthetic rubber

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High-brightness near-infrared luminescent bioprobes based on lanthanide-doped Na3CrF6 nanoparticles

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science China Materials 2024年第12期67卷 4113-4114页

作者： Yun Xing Shiqi Yu Datao Tu Xueyuan Chen State Key Laboratory of Structural Chemistry Fujian Key Laboratory of Nanomaterialsand CAS Key Laboratory of Design and Assembly of Functional NanostructuresFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China University of Chinese Academy of Sciences Beijing 100049China

Over the past decade,near-infrared(NIR)luminescent materials have emerged as a frontier in photonics and material science,finding diverse applications in bioimaging,encryption,and photodetection[1].Particularly,NIR nanoprobes are widely utilized in life science and clinical medicine because of their high spatial resolution,deep tissue penetration,low optical absorption and scattering,and minimal autofluorescence[2,3].

关键词： nanoparticles frontier utilized

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Mechanical responses and acoustic emission behaviors of coal under compressive differential cyclic loading(DCL):a numerical study via 3D heterogeneous particle model

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International Journal of Coal science & technology 2023年第3期10卷 136-154页

作者： Zhengyang Song Yunfeng Wu Yong Zhang Yi Yang Zhen Yang State Key Laboratory of Water Resource Protection and Utilization in Coal Mining BeijingChina Department of Civil Engineering University of Science&Technology BejingBeijing 100083China State Key Laboratory of Mining Response and Disaster Prevention and Control in Deep Coal Mines Anhui University of Science and TechnologyHuainan 232001China

The stability of coal walls(pillars)can be seriously undermined by diverse in-situ dynamic *** on a 3D par-ticle model,this work strives to numerically replicate the major mechanical responses and acoustic emission(AE)behaviors of coal samples under multi-stage compressive cyclic loading with different loading and unloading rates,which is termed differential cyclic loading(DCL).A Weibull-distribution-based model with heterogeneous bond strengths is constructed by both considering the stress-strain relations and AE *** previously loaded samples were respectively grouped to indicate two DCL regimes,the damage mechanisms for the two groups are explicitly characterized via the time-stress-dependent variation of bond size multiplier,and it is found the two regimes correlate with distinct damage patterns,which involves the competition between stiffness hardening and *** numerical b-value is calculated based on the mag-nitudes of AE energy,the results show that both stress level and bond radius multiplier can impact the numerical *** proposed numerical model succeeds in replicating the stress-strain relations of lab data as well as the elastic-after effect in DCL *** effect of damping on energy dissipation and phase shift in numerical model is summarized.

关键词： Differential cyclic loading(DCL) Particle model Acoustic emission(AE) Discrete element method(DEM)Damage mechanism

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